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RESEARCH PAPER · Journal of the American Chemical Society · 2023

Expandable Li Percolation Network: The Effects of Site Distortion in Cation-Disordered Rock-Salt Cathode Material

Yujian Sun, Sichen Jiao, Junyang Wang, Yuanpeng Zhang, Jue Liu, Xuelong Wang, Le Kang, Xiqian Yu, Hong Li, Liquan Chen, Xuejie Huang

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Expandable Li Percolation Network: The Effects of Site Distortion in Cation-Disordered Rock-Salt Cathode MaterialOriginalImproved Cycling Stability of Ni-Rich Ncm Cathode Material by In-Situ Introduced Tm-B-O Amorphous Surface Structure0Structure, Lithium-Ion Conductivity Coupled with Second-Order Jahn–Teller Effect, and Electrochemical Stability of Sr-Based Perovskite-Type Solid Electrolytes6The Mechanism of Fluorine Doping for the Enhanced Lithium Storage Behavior in Cation‐Disordered Cathode Oxide32Nickel-Doped Titanium Oxide with Layered Rock-Salt Structure for Advanced Li-Storage Materials9Lithium-rich sulfide Li 2 Ti 1− x Si x S 3 cathode materials optimized through Si-doping for high-capacity all-solid-state lithium-ion batteries10Structural regulation-induced Li-electron disentanglement for stabilized oxygen redox of Li-excess disordered rock-salt cathode materials14Improved Cycling Stability of Ni-Rich Cathode Material by In Situ Introduced TM-B-O Amorphous Surface Structure6High Li-Ion Conductivity in Pyrochlore-Type Solid Electrolyte Li 2– x La (1+ x )/3 M 2 O 6 F (M = Nb, Ta)35Unraveling the functioning mechanism of fluorine-doping in Mn-based layered oxide cathodes toward enhanced sodium-ion storage performance72Manipulating disorder within cathodes of alkali-ion batteries72The mystic role of high-entropy designs in rechargeable metal-ion batteries: A review52Interplay between Intermediate Anionic and Cationic Species and the Reflection to Voltage Hysteresis of Oxygen-Redox Battery Electrodes: A Holistic Picture17Structural Evolution in Disordered Rock Salt Cathodes49Unlocking fast Li-ion transport in micrometer-sized Mn-based cation-disordered rocksalt cathodes24Synergistic enhancement of ion/electron transport by ultrafine nanoparticles and graphene in Li2FeTiO4/C/G nanofibers for symmetric Li-ion batteries10Electrochemical Switching of Electromagnetism by Hierarchical Disorder Tailored Atomic Scale Polarization17Screening Na-Excess Cation-Disordered Rocksalt Cathodes with High Performance9Cation order and disorder in cathode materials for Li-ion batteries7In situ coupling of crosslinked CNTs and Li-excess disordered rock salt vanadium oxide nanowires for high-performance Li storage2A comprehensive understanding on the anionic redox chemistry of high-voltage cathode materials for high-energy-density lithium-ion batteries115Breaking structural symmetry to facilitate fast reaction kinetics1Elucidating lithium-ion diffusion kinetics in cation-disordered rocksalt cathodes18Exploring a new synthesis route to lithium-excess disordered rock salt (DRX) cathode materials12Optimized amounts of excess Li in cation-disordered rocksalt cathodes assisted by carbon nanotubes8Promoting cationic redox and stabilizing lattice oxygen in an Fe-based DRX cathode by the synergy of initial Li deficiency and 3D hierarchical porous architecture2Optimizing Disordered Rock Salt Cathodes by Solid‐State Synthesis and Design of Experiments for Enhanced Battery Performance11Assessing Dimensionality in Electrides4Rocksalt-structured LiBi1-Sb S2 solid solution for all-solid-state batteries2Sn‐Mediated Local Atomic Ordering Enhances Reversible Anionic Redox Activity in Cation‐Disordered Li1.3Mn0.4Nb0.3O2 Cathodes3Disordered Rocksalts as High‐Energy and Earth‐Abundant Li‐Ion Cathodes43Tuning Cation (Dis)Order in Cr‐Based Li‐Excess Oxide Cathode Materials to Improve Li+ Transport Properties9Effect of Ball Milling on the Atomic Configuration of Li1.3Nb0.3Fe0.4O2 with a Disordered Rocksalt Structure0Solvent Determines the Formation Pathway in Sol–Gel Synthesized Disordered Rock Salt Material for Lithium Ion Battery Application4Exceptional layered cathode stability at 4.8 V via supersaturated high-valence cation design45Local structural distortion and energy gradient enhance lithium ionic conductivity in high-entropy oxide8Reducing Structural Distortion by Tailoring Orbital Interactions in High‐Voltage Polyanionic Cathodes7Impact of the d 0 transition metal on local structural transformations in disordered rock salt cathodes7Disordered Rock-Salt Oxide Cathode for Next-Generation Energy Storage0Elucidating ionic–electronic transport in cation-disordered rocksalt cathodes0Revealing the hidden structural complexity of high-capacity oxide cathodes through advanced characterizations1Applications of neutron scattering in solid oxide fuel cells1Preparation and characterization of lithium-rich high-entropy disordered rock-salt cathodes for lithium-ion batteries2Data-driven design of high-energy-density disordered rock-salt cathode via a physically informed graph neural network1Heavy Lanthanide‐Induced Epitaxial Rock‐Salt Shells Enable Chemo‐Mechanically Robust Sodium‐Ion Cathodes0Artificial Intelligence‐Assisted Design of High‐Entropy Oxide Catalysts0Disordered Rock-Salt Structures in Next-Generation Lithium–Ion Batteries: An Outlook from Cation Disorder to Electrochemical Design0Dynamically Stable Networks for Ion Transport in Lithium Transition-Metal Phosphates0Chemically bonded single phase ternary anode materials for alkali metal ion batteries: Intrinsic mechanisms and design perspectives0Interplay of Lattice Distortion and Cation Disorder Governs Li-Ion Transport in Cation-Disordered Rocksalt Cathodes1Neutron Total Scattering and Pair Distribution Function Analysis for Local Structure Determination of Inorganic Materials0Lattice Distortion Regulates Na-Ion Percolation in High-Entropy Cation-Disordered Rocksalt Cathodes0Stereochemical origin of potential hysteresis in lithium metal batteries with lithium-rich cation-disordered rocksalt positive electrodes0

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