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RESEARCH PAPER · Environmental Science & Technology · 2023

Ferrate(VI)/Periodate System: Synergistic and Rapid Oxidation of Micropollutants via Periodate/Iodate-Modulated Fe(IV)/Fe(V) Intermediates

Lijun Niu, Lin Jiang, Wenzheng Chen, Qian Zhang, Xin Yu, Mingbao Feng

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Ferrate(VI)/Periodate System: Synergistic and Rapid Oxidation of Micropollutants via Periodate/Iodate-Modulated Fe(IV)/Fe(V) IntermediatesOriginalSelective Abatement of Organic Contaminants by Trace Complexed Mn(Ii)-Catalyzed Periodate Via High-Valent Manganese-Oxo Species0Boosted persulfate activation by hierarchically porous carbonaceous materials: Pivotal role of pore structure and electron-accepting capacity32Ru(III)-Periodate for High Performance and Selective Degradation of Aqueous Organic Pollutants: Important Role of Ru(V) and Ru(IV)97Selective abatement of electron-rich organic contaminants by trace complexed Mn(II)-catalyzed periodate via high-valent manganese–oxo species24Solar/periodate inhibits ARGs transformation by degradation of DNA without damaging cell membrane11Promoted micropollutant degradation and structural evolution of natural organic matter by a novel S(IV)-based water treatment strategy9Iron(III)-(1,10-Phenanthroline) Complex Can Enhance Ferrate(VI) and Ferrate(V) Oxidation of Organic Contaminants via Mediating Electron Transfer48Ru(III)/Periodate System: Rapid Microbial Inactivation and Micropollutant Abatement in Seconds4Redox property of coordinated iron ion enables activation of O2 via in-situ generated H2O2 and additionally added H2O2 in EDTA-chelated Fenton reaction114Degradation of ciprofloxacin using magnetite nanoparticle-activated periodate: Kinetic, mechanistic and toxicity evaluation69pH-Driven Efficacy of the Ferrate(VI)–Peracetic Acid System in Swift Sulfonamide Antibiotic Degradation: A Deep Dive into Active Species Evolution and Mechanistic Insights95Simple and rapid photometry for measuring low dosage of periodate with bromide ion-catalyzed oxidation of ABTS4Activation of periodate by ABTS as an electron shuttle for degradation of aqueous organic pollutants and enhancement effect of phosphate16Iodate(V) activated ferrate(VI) for enhanced oxidation of micropollutants from water and sediment media12The synergistic effect of oxidant-peroxide coupling systems for water and wastewater treatments29Water decontamination by reactive high-valent iron species14From nano- to macroarchitectures: designing and constructing MOF-derived porous materials for persulfate-based advanced oxidation processes28Trace Benzoquinone Inducing Periodate for Tetracyclines Selective Degradation: Role of Unstable Intermediate0Simultaneous generation of free radicals, Fe(IV) and Fe(V) by ferrate activation: A review67Iron-based materials for activation of periodate in water and wastewater treatment processes: The important role of Fe species42Fe(IV)/Fe(V)-mediated polyferric sulfate/periodate system: A novel coagulant/oxidant strategy in promoting micropollutant abatement17Tetracycline removal using NaIO4 activated by MnSO4: Design and optimization via response surface methodology1Direct generation of high-valent iron-oxo species to eliminate oxytetracycline at circumneutral pH via paper mill sludge ash activating peroxymonosulfate13How Should We Activate Ferrate(VI)? Fe(IV) and Fe(V) Tell Different Stories about Fluoroquinolone Transformation and Toxicity Changes35Ferrate(VI)/percarbonate for the oxidation of micropollutants: Interactive activation and release of low-concentration hydrogen peroxide for efficient electron utilization22How Do Metal Oxides Mislead Spin-Trapping Electron Paramagnetic Resonance Analysis?100Unexpectedly enhanced degradation of acetaminophen by sulfoxides probe in Fe(II)-activated persulfate oxidation: The mechanism and the selectivity11MoO2 co-catalytic Fe3+/periodate for tetracycline degradation: Key role of Fe/Mo cycling and high-valent iron (Fe(IV)) generation40Solar-light-activated periodate for degradation and detoxification of highly toxic 6PPD-quinone at environmental levels125Nickel–manganese sulfide on nickel foam toward highly efficient and stable potassium periodate activation for organic pollutant degradation16Revisiting the role of H2O2 in periodate electro-activation system: The non-dependence in Bisphenol A (BPA) removal20Enhanced diclofenac abatement by ferrate in the presence of montmorillonite: Trapping in-situ formed Fe(III)3Buffer-free ozone-ferrate(VI) systems for enhanced oxidation of electron-deficient contaminants: Synergistic enhancement effects, systematic toxicity assessment, and practical applications40Insights on the degradation mechanism of neotame using UV/periodate: Roles of reactive species, kinetics, and pathways29Elimination of representative antibiotic-resistant bacteria, antibiotic resistance genes and ciprofloxacin from water via photoactivation of periodate using FeS224Natural pyrite and ascorbic acid co-enhance periodate activation for inactivation of antibiotic resistant bacteria and inhibition of resistance genes transmission: A green disinfection process dominated by singlet oxygen23Insights into the non-radical elimination mechanism of DOPO in trace TEMPO+ enhanced UVB/Periodate process5Trace benzoquinone inducing periodate for tetracyclines selective degradation: Role of the unstable intermediate5Revisiting iodide species transformation in peracetic acid oxidation: unexpected role of radicals in micropollutants decontamination and iodate formation95Regulating the dominant reactive oxygen species from Fe(IV)-oxo to 1O2 by deprotonation of Fe(IV)-oxo in electro-Fe(II)/periodate system18Periodate activation via metals and metal-based complexes: progress in degradation properties and mechanisms13Nanolaminated MAB phase Mn2AlB2: An emerging ternary transition metal boride to efficiently activate periodate for antibiotic degradation8Deciphering the Novel Picolinate-Mn(II)/peroxymonosulfate System for Sustainable Fenton-like Oxidation: Dominance of the Picolinate-Mn(IV)-peroxymonosulfate Complex23Degradation of aqueous organic pollutants by dual oxidant advanced oxidation processes: A comprehensive review20CO2(OH)2CO3 and Fe doped Co2(OH)2CO3 prepared as efficient and stable catalysts for activation of PMS: Two systems comparison and key role of high-valent metal-oxo species in mechanism revealing17Percarbonate-periodate system: A novel and efficient “oxidant-oxidant” strategy for selective oxidation of micropollutants in water3Regulating the generation of singlet oxygen (1O2) in Advanced oxidation processes by catalyst design for water treatment56Simultaneous removal of antibiotics and recovery of phosphate in urine by ferrate(VI)-peracetic acid: The critical role of iron species5Effective periodate activation by the ball-milled bimetallic zero-valent iron/manganese oxides catalyst for sulfamethoxazole degradation10Efficient Degradation of Metronidazole by In Situ High-Valent Iron-Oxo Species in Nanoclustered Iron–Carbon Particles9Synergistic degradation of polycyclic aromatic hydrocarbons using ferrate(VI) and periodate: Efficiency and mechanisms6Innovative spherical Fe-Mn layered double hydroxides (LDH) for the degradation of sulfisoxazole through activated periodate: Efficacy and mechanistic insights7Enhancing degradation of micropollutants and utilization of ferrate by oxygen-vacancy-activated ferrate species on CeO216Insight on the optimized electronic structure of carbon nitride on ultrafast water treatment via photocatalytic activation of ferrate3A New Idea of Water Treatment Based on Hydroxyl Radicals, When Periodate Encounters Paa0Atrazine degradation by aqueous ferrate( vi ) activated with sulfite vs. thiosulfate: performance, products, and pathways3Carboxymethyl-Β-Cyclodextrin Enhanced Persulfate/Fe2+ System for Organic Contaminant Removal in Groundwater: Performance, Influencing Factors, and Mechanisms0Kinetics, contributions, and pathways of the degradation of artificial sweeteners by primary and secondary radicals during UV/persulfate14Efficient degradation of SCP by Co2(OH)2CO3/CuCo2S4-enhanced electron transfer-activated PMS: Dual role of Cu active site17Applications of periodate activation for emerging contaminants treatment in water: Activation methods, reaction parameters and mechanism24Covalently bonded aluminum-iron modified activated carbon moderately activated ferrate(VI) through enhanced interaction path: pH-driven efficacy on active species evolution and synergic mechanistic9Heterogeneous Peroxymonosulfate-Based Advanced Oxidation Mechanisms: New Wine in Old Bottles?204Dynamic in-situ reconstruction of active site circulators for photo-Fenton-like reactions57Breaking Oxygen Dependency: Enhanced Micropollutant Degradation during Periodate-Based Catalysis under Deoxygenated Conditions2Ultra-efficient degradation of isoquinoline from shale gas wastewater with the diethylamine-ferrate(VI) system: The key role of Fe(IV)/Fe(V) active species7Overlooking the effect of alcohol quenchers can mislead mechanistic understanding in ferrate-based advanced oxidation processes6Enhancing ferrate(VI) oxidation by ferrous iron for pretreating shale gas produced water and mitigating ultrafiltration membrane fouling2Visible light regulates the activation pathway of periodate on Bi/Mo dual sites for efficient micropollutant degradation: The overlooked roles of metastable complex8Overlooked Role of Iodate in Micropollutant Degradation by UV/Periodate: Kinetic Modeling and Mechanism26Innovative catalytic approaches in fabricating bimetallic heterostructures for remediation of antibiotic-polluted water: Mechanistic insights and application prospects1Low ultraviolet dose with high efficiency: Synergistic coupling of far-UVC and ferrate(VI) for ultrafast and selective degradation of micropollutants14Piezoelectric-driven hydrogen peroxide production and in-situ utilization for organic wastewater decontamination and synchronous disinfection: Efficacy, mechanisms and comprehensive assessments17Enhanced selective oxidation capacity and utilization efficiency of Fe(VI) initiated by HBT for contaminant oxidation: Identification of HBT radicals and function2Photoinduced electron transfer-driven dual-ligand MOF fluorescence sensor for highly selective and sensitive detection of periodate in complex water samples10Boosting Low-Dose Ferrate(VI) Activation by Layered FeOCl for the Efficient Removal of Antibiotic-Resistant Bacteria and Antibiotic Resistance Genes via Enhancing Fe(IV)/Fe(V) Generation14Nitrilotriacetic acid-assisted activation of periodate by Fe(III) for organic pollutant degradation: the critical roles of high-valent iron species formation and coordination inhibition by phenolic contaminants10Development of a novel and highly efficient catalyst-free mediated “oxidant-oxidant” process for enhanced decontamination of water contaminants7Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification20Comparative study on degradation of PVC microplastics under four processes: mechanism, pathway and toxicological assessment6Efficient synergistic removal of antibiotics and Cr(VI) in water by Co-Metallene/WS2: Interfacial microenvironment and dynamic strengthening mechanism7Secondary amine-activated ferrate(VI) for isoquinoline degradation: Relationship between molecular structure and reactive performance1Insight into oxytetracycline abatement via periodate driven with ferrous sulfide: parameter optimization, mechanism exploration, improvement strategies, and application performance0Role of multivalent iron in enhancing sodium percarbonate oxidation for alleviating membrane distillation fouling caused by shale gas produced water8Ferrate meets carbon nanotubes: Unraveling the catalytic pathways for enhanced oxidation efficiency of polycyclic aromatic hydrocarbons0Radical-free ultra-rapid disinfection: Application of the periodate/Mn(II) system in eliminating antibiotic-resistant bacteria and genes and degrading emerging contaminants2High-Valent Iron Species (Fe(IV)/Fe(V)) for Selective Oxidation of Emerging Contaminants: Mechanisms, Applications, and Future Directions46Mechanistic Unveiling of Radical and Nonradical Pathways in Periodate Activation for Water Treatment: Generation Mechanism, Oxidative Behaviors, and Functional Merits21Porous amorphous manganese oxide micro-nanostructures boosted electron transfer between periodate and organic contaminants: The significance of surface reactive oxygen species0Revisiting periodate photoactivation by solar light: Organic contaminant-specific and wavelength-dependent mechanism4Carbonate Radical Anion (CO 3 •– ) in Carbonated Water: Generation and Importance in Environmental Processes19Enhanced removal of cytotoxicity from wastewater by silica gel-activated ferrate (VI)0Interfacial engineering of hematite trigger periodate activation reaction for sustainable sulfisoxazole removal: Mechanism insight and environmental significance enhancement12Fe(IV)/Fe(V)-mediated oxidation processes in water and wastewater treatment: Recent progress and current challenges8Pitfalls in Probing Singlet Oxygen by Electron Paramagnetic Resonance Spectroscopy in Engineered Environmental Systems19Sunlight-driven synergistic activation of ferrate and periodate for ultrafast degradation of emerging contaminants: Unveiling DOM-enabled Fe(II) recycling in real complex aquatic matrices3Electron Beam Irradiation-Assisted Synthesis of MIL-88A(Fe) Toward Efficient Periodate Activation for Tetracycline Degradation1Nonradical hydrogen peroxide activation for water treatment: mechanisms, regulation strategies, and polymerization-driven processes0Performance and mechanisms of iodide removal from water by potassium ferrate (K2FeO4)0Ultralow Dose Protoporphyrin IX-Mediated Ferrate(VI) System for Rapid Degradation of Phenolic Pollutants: Key Roles of Fe(V/IV/III) Complexes5Bridging molecular mechanisms and engineering practice: CeO2 mediated Fe(VI) activation on for deep thallium removal from complex industrial wastewater4Carbon nanotube-engineered electron transfer pathways in NiFe-LDH for enhanced photocatalytic ferrate activation1Acidic ozone-ferric sulfate system for leaching of chalcopyrite: A self-sustained synergistic mechanism by regulating iron species distribution2Hydrated metal charge density as a universal descriptor explaining mechanistic variations in periodate activation toward pollutant degradation4Polarity reversal enabled copper cycling in an electro-Fenton-based combined system for suppressed Cu(II) release and enhanced BPA degradation0Dual-functional carboxymethyl-β-cyclodextrin for enhanced peroxydisulfate/Fe2+ removal of tetrachloroethylene in simulated groundwater0Nitrogen-doped sludge biochar for periodate activation: Synergistic radical/non-radical pathways for rapid sulfadiazine degradation0Facile synthesis of Fe-BDC/2-MI heterojunction from waste PET for efficient visible-light-driven periodate activation toward organic pollutant degradation1Mechanochemical biochar enables electron-transfer-mediated ferrate(VI) activation for enhanced micropollutant degradation2Electrocatalytic activation of peracetic acid with plasma-etched carbon nanotubes for moderate iodide oxidation followed by in-situ adsorption0Unveiling the transformation patterns and mechanisms of organic micropollutants and wastewater effluent organic matter during UV222-based oxidation systems0Mechanistic insights into activation of periodate by sludge biogas residue biochar loaded with manganese for efficient sulfadiazine degradation in aqueous solutions1Valorizing aquatic plant biomass into carbonaceous sorbents for sustainable water treatment: A review and meta-analysis1Orbital-tailored MnO2-CNT hybrids for interfacial electron transfer-dominated periodate activation toward selective IO3• generation in complex water remediation9Far-UVC (222 nm) activation of periodate for rapid degradation of imidacloprid: Kinetics, degradation mechanisms, and toxicity evaluation0Halogen-doped δ-MnO2 for direct degradation of micropollutants: Role of surface Mn(III) and mechanistic insights0Spatial confinement of FeCu nanoalloys in N-doped graphitic carbon nanotubes enables accelerated periodate activation for water decontamination1Fe-Cu‑sodium alginate microspheres activate periodate for ultrafast disinfection: Dual mechanisms toward ARB inactivation and regrowth inhibition0EGCG-Enhanced Ferrous-Activated Peroxydisulfate Processes for Shigella flexneri Biofilm Inactivation: Efficacy, Underlying Mechanisms, and Practical Implications0Accelerated micropollutant degradation by Mn(VII) in the presence of periodate: The critical role of hydrogen-bond-bridged electron transfer0Sulfur Surface-Modified Mesoporous Manganese Ferrite for Electron Transfer Driven Periodate Activation and Tetracycline Degradation0Unveiling radical and non-radical species in ferrate-based advanced oxidation processes for wastewater treatment: Generation, mechanisms, and identification0Tuning the reactive species in oxidant activation by single-atom catalysts: Mechanisms, manipulations, and perspectives0Singlet oxygen-mediated pollutant degradation in the UV-powered EDTA-Fe(II) system: Insights into electron transfer and reactive oxygen species generation pathways0Fabrication of blue fluorescent carbon dots derived from Garcinia indica fruit peel for the detection of periodate ion in wastewater samples0Role of Fe(IV) and Fe(V) in micropollutant abatement by visible-light-activated ferrate(VI) via ligand-to-metal charge transfer0Harnessing Coordination Chemistry for Selective and Efficient Water Decontamination in Metal-Based Homogeneous Oxidation Systems0

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  1. Selective Abatement of Organic Contaminants by Trace Complexed Mn(Ii)-Catalyzed Periodate Via High-Valent Manganese-Oxo Species

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  4. Selective abatement of electron-rich organic contaminants by trace complexed Mn(II)-catalyzed periodate via high-valent manganese–oxo species

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  5. Solar/periodate inhibits ARGs transformation by degradation of DNA without damaging cell membrane

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  6. Promoted micropollutant degradation and structural evolution of natural organic matter by a novel S(IV)-based water treatment strategy

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  7. Iron(III)-(1,10-Phenanthroline) Complex Can Enhance Ferrate(VI) and Ferrate(V) Oxidation of Organic Contaminants via Mediating Electron Transfer

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  8. Ru(III)/Periodate System: Rapid Microbial Inactivation and Micropollutant Abatement in Seconds

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  10. Degradation of ciprofloxacin using magnetite nanoparticle-activated periodate: Kinetic, mechanistic and toxicity evaluation

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  11. pH-Driven Efficacy of the Ferrate(VI)–Peracetic Acid System in Swift Sulfonamide Antibiotic Degradation: A Deep Dive into Active Species Evolution and Mechanistic Insights

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  12. Simple and rapid photometry for measuring low dosage of periodate with bromide ion-catalyzed oxidation of ABTS

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  13. Activation of periodate by ABTS as an electron shuttle for degradation of aqueous organic pollutants and enhancement effect of phosphate

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  14. Iodate(V) activated ferrate(VI) for enhanced oxidation of micropollutants from water and sediment media

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  16. Water decontamination by reactive high-valent iron species

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  18. Trace Benzoquinone Inducing Periodate for Tetracyclines Selective Degradation: Role of Unstable Intermediate

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  19. Simultaneous generation of free radicals, Fe(IV) and Fe(V) by ferrate activation: A review

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  31. Revisiting the role of H2O2 in periodate electro-activation system: The non-dependence in Bisphenol A (BPA) removal

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  32. Enhanced diclofenac abatement by ferrate in the presence of montmorillonite: Trapping in-situ formed Fe(III)

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  33. Buffer-free ozone-ferrate(VI) systems for enhanced oxidation of electron-deficient contaminants: Synergistic enhancement effects, systematic toxicity assessment, and practical applications

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  34. Insights on the degradation mechanism of neotame using UV/periodate: Roles of reactive species, kinetics, and pathways

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  35. Elimination of representative antibiotic-resistant bacteria, antibiotic resistance genes and ciprofloxacin from water via photoactivation of periodate using FeS2

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  36. Natural pyrite and ascorbic acid co-enhance periodate activation for inactivation of antibiotic resistant bacteria and inhibition of resistance genes transmission: A green disinfection process dominated by singlet oxygen

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  37. Insights into the non-radical elimination mechanism of DOPO in trace TEMPO+ enhanced UVB/Periodate process

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  38. Trace benzoquinone inducing periodate for tetracyclines selective degradation: Role of the unstable intermediate

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  39. Revisiting iodide species transformation in peracetic acid oxidation: unexpected role of radicals in micropollutants decontamination and iodate formation

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  41. Periodate activation via metals and metal-based complexes: progress in degradation properties and mechanisms

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  42. Nanolaminated MAB phase Mn2AlB2: An emerging ternary transition metal boride to efficiently activate periodate for antibiotic degradation

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