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RESEARCH PAPER · Advanced Materials · 2023

PF 6 − Pseudohalides Anion Based Metal‐Free Perovskite Single Crystal for Stable X‐Ray Detector to Attain Record Sensitivity

Zhizai Li, Zhenhua Li, Guoqiang Peng, Chang Shi, Haoxu Wang, San‐Yuan Ding, Qian Wang, Zitong Liu, Zhiwen Jin

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PF 6 − Pseudohalides Anion Based Metal‐Free Perovskite Single Crystal for Stable X‐Ray Detector to Attain Record SensitivityOriginalAn interfacial toughening strategy for high stability 2D/3D perovskite X-ray detectors with a carbon nanotube thin film electrode8Multifunctional pseudohalide-based ionic liquid doping promotes efficient and stable perovskite solar cells11Two-Dimensional Metal Halides for X-Ray Detection Applications101CsPbX3 Based X‐Ray Detectors24Metal‐Free Perovskites for X‐Ray Detection11Crystalline–Amorphous Heterojunction for a Metal Halides Single Crystals X‐Ray Detector with Substantially Increased Sensitivity23Metal-Free Hydrazinium Halide Perovskitoid Single Crystals for X-ray Detection23Superior photovoltaic performance of BF4-doped perovskite rationalized by ab initio nonadiabatic molecular dynamics13Dimensionality Engineering of Organic–Inorganic Halide Perovskites for Next‐Generation X‐Ray Detector41Molecular Design of Layered Hybrid Silver Bismuth Bromine Single Crystal for Ultra‐Stable X‐Ray Detection With Record Sensitivity58First principles study on polarization and piezoelectric properties of group substitution regulated lead-free organic perovskite ferroelectrics0Synergistic role of hydrogen bonding and band degeneracy leads to enhanced X-ray detection in HPIP-(NH 4 ) 0.7 Cs 0.3 Br 3 ·H 2 O perovskites6Low‐Dose and Stable X‐Ray Imaging Enabled by Low‐Dimensional Dion‐Jacobson Perovskites44Surface Passivation toward Multiple Inherent Dangling Bonds in Indium Phosphide Quantum Dots38Pyroelectric Photoconductive Diode for Highly Sensitive and Fast DUV Detection37Molecularly thin, two-dimensional all-organic perovskites50“One‐Click Restart” Recycling of Metal‐Free Perovskite X‐Ray Detectors20Aminoazanium of A-site Cations in Metal-Free Halide Perovskite Single Crystals to Reduce Thermal Expansion for Efficient X-ray Detection11Dimensional Regulation in Metal‐Free Perovskites by Compositional Engineering to Achieve Record Low X‐Ray Detection Limits21Dimensional Regulation in Metal‐Free Perovskites by Compositional Engineering to Achieve Record Low X‐Ray Detection Limits5Mussel-inspired structure based CsPbBr3/Aramid nanofiber composite film for lightweight, flexible and superior X-ray shielding6Hybrid Perovskite Molecular Rotor Ferroelastic Semiconductor Constructed by Supramolecular Assembly15Non-Centrosymmetric Chiral Structures for Hybrid Bismuth Halides With Stable Self-Driven X-Ray Detection6Tailoring Multi‐Phenyl Ring Cation for Stable Scalable Hybrid Bismuth Iodide Amorphous Film: Enabling Record Sensitivity and High‐Performance X‐Ray Array Imaging40Effect of variable metal cation (Mn2+) on the phase stability of FAPbI31Enhanced thermodynamic stability and carrier lifetime in BF 4 -doped wide-band-gap perovskite solar cells25Tailored molecular for ultra-stability and biocompatible pseudohalide metal-free perovskite towards X-ray detectors with record sensitivity20Transparent Perovskite Wafers via Nanocrystals Ordered Coalescence Toward Sensitive and Stable X‐Ray Detection and Imaging28Exploring Aqueous Solution‐Processed Pseudohalide Rare‐Earth Double Perovskite Ferroelectrics toward X‐Ray Detection with High Sensitivity6Exploring Aqueous Solution‐Processed Pseudohalide Rare‐Earth Double Perovskite Ferroelectrics toward X‐Ray Detection with High Sensitivity25Rational Design of A‐Site Cation for High Performance Lead‐Free Perovskite X‐Ray Detectors17High Sensitivity X‐Ray Detectors with Low Degradation Based on Deuterated Halide Perovskite Single Crystals65Revolutionizing X-ray Imaging: A Leap toward Ultra-Low-Dose Detection with a Cascade-Engineered Approach6Pseudohalide Anions Driven Structural Modulation in Distorted Tetrahedral Manganese(II) Hybrids Toward Tunable Green‐Red Emissions43Pseudohalide Anions Driven Structural Modulation in Distorted Tetrahedral Manganese(II) Hybrids Toward Tunable Green‐Red Emissions4A metal-free molecular pyroelectric material with strong pyro-photovoltaic coupling for enhancing self-powered X-ray response1Applications of Perovskite Wearables in Medical Science1Enhanced X-ray detection of one-dimensional DABCO–NH 4 I 3 perovskites via anisotropic carrier transmission study3Single-crystal perovskites for photovoltaic and high-energy detection applications31Surface reconstruction and defect healing of MAPbI 3 perovskite microcrystalline thick films for sensitive and self-powered X-ray detectors13The emergence of metal-free molecular perovskites: challenges and opportunities5Cesium‐Based Molecular Perovskites With Superior Stability for High‐Performance X‐Ray Detection10Against the Wallach's Rule Through Rational Design of Metal‐Free Chiral Perovskites Toward Efficient Red Circularly Polarized Phosphorescence3Against the Wallach's Rule Through Rational Design of Metal‐Free Chiral Perovskites Toward Efficient Red Circularly Polarized Phosphorescence223D Lead‐Free Double Perovskite via Anchoring A‐Site Cation for Ultralow Dose and Stable X‐Ray Detection14Balance of charge carrier mobility-lifetime and resistivity for enhancing X-ray detection sensitivity in Sn: Ga2TeO6 crystal8Suppressing Ion Migration in Heterostructure Single Crystals for Highly Sensitive Ultra‐Stable X‐Ray Detection3Synergistic Rare‐Earth Alloying and Pseudohalide Coordination Constructing Hybrid Metal Pseudohalide with Robust Crystal Fields for Stable X‐Ray Detection with Record Sensitivity3Metal‐Free Perovskites for X‐Ray Detection and Imaging: Progress and Prospects5Polar Isomer‐Driven Cation‐Anion Coupling Enhances Carrier Dynamics and X‐Ray Detectors Sensitivity in 0D Organic‐Inorganic Hybrid Mn Halides5Self‐Powered Ferroelectric Bi‐Based Perovskite X‐Ray Detector for Radiation Monitoring and Intelligent Imaging Recognition7Hydroxylamine Cation as B‐Site with Radius and Dipole Moment Modulation for Metal‐Free Halide Perovskite to Enhance X‐ray Detection Performance3Advancements in Metal Halide Perovskites and their Derivatives for Direct‐Type X‐Ray Detectors8Novel X‐Ray Detector with High Sensitivity and Low Detection Limit Based on Bandgap‐Engineered Chalcogenide Glass2Stereochemically Active Lone‐Pair Electrons Driven High‐Performance and Self‐Powered X‐Ray Detection in Cs 2 TeMo 3 O 12 Crystal1A-site engineering enabled the fabrication of cesium-based molecular perovskites with three-dimensional hexagonal polytype for high-performance X-ray detection0Engineering dimensionality and band-edges with lone-pair cations to achieve superior X-ray detection in metal-free perovskites0Spatial halide exchange reactions for sculpting light in hybrid perovskites0BiO(IO 3 ) with Ultrahigh Effective Atomic Number and Density for Sensitive and Stable Hard X‐Ray Detection0In Situ Ionic Liquid Oligomer Encapsulation Enabled Robust Perovskite Single Crystals toward High-Efficiency X-ray Detection2High‐Mobility 2D Molecular Crystals Enable Field‐Effect X‐Ray Detectors with Record Volumetric Sensitivity4A‐Site Symmetry Engineering in Designing Metal‐Free Perovskites for Ultrahigh Sensitivity X‐Ray Detection0Dimensional Engineering in 4AMPBiX 5 Metal Halides: From 0D to 1D for Enhanced X‐Ray Detection Performance1Halide Perovskite Single Crystals: A Promising Semiconductor Platform for Advanced X-ray Detection4High Resistivity and Low Defect Covalent Organic Frameworks for Highly Stable and Low Dose X‐Ray Detection0High Resistivity and Low Defect Covalent Organic Frameworks for Highly Stable and Low Dose X‐Ray Detection0Dual‐Anchor Molecular Lock in 3D Lead‐Free Perovskite Quenches Ion Migration for Ultra‐Stable, Nanogray‐Sensitive X‐Ray Detection1Improved Carrier Transport and Enhanced Detection Sensitivity Through Zr 4+ Doping in LiYMo 2 O 8 Single Crystals for X-ray Detectors0An Unprecedented PF6–-Based Pseudohalide Metal-Free Perovskite Ferroelastic0Synergistic Effect of Chirality and Symmetry Reduction Enables Metal‐Free Perovskite Single Crystal With Stable Self‐Driven X‐ray Detection0Synergistic Effect of Chirality and Symmetry Reduction Enables Metal‐Free Perovskite Single Crystal With Stable Self‐Driven X‐ray Detection0Uranium-Incorporated Layered Perovskitoids with Heterostructures Exhibit Hole-Dominant Transport0Multidentate Anion [C 6 H 6 NO 6 ] 3− Coordinated Hybrid Bismuth Complex Single Crystal for Stable X‐Ray Detection With High Sensitivity0Multistage Fluorination in a Metal‐Free Perovskite Ferroelectric Enables Multidirectional Self‐Powered X‐Ray Detection0Multistage Fluorination in a Metal‐Free Perovskite Ferroelectric Enables Multidirectional Self‐Powered X‐Ray Detection0Metal‐Free 1D MPAZE‐N 2 H 5 I 3 Perovskite for X‐Ray Detection With Enhanced Stability and Sensitivity0

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