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RESEARCH PAPER · Laser & Photonics Review · 2023

Ab Initio Site‐Selective Occupancy and Luminescence Enhancement in Broadband NIR Emitting Phosphor Mg 7 Ga 2 GeO 12 :Cr 3+

Jinmeng Xiang, Xue Mei Zhou, Xiaoqi Zhao, Ziyang Wu, Changheng Chen, Xianju Zhou, Chongfeng Guo

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Ab Initio Site‐Selective Occupancy and Luminescence Enhancement in Broadband NIR Emitting Phosphor Mg 7 Ga 2 GeO 12 :Cr 3+OriginalAn efficient and thermally stable Cr 3+ -activated Y 2 GdSc 2 Al 2 GaO 12 garnet phosphor for NIR spectroscopy applications14Convolutional neural networks driving thermally enhanced upconversion luminescence for temperature sensing: achieving high accuracy and robustness across a wide temperature range9K 2 LiScF 6 :Cr 3+ /Mn 4+ fluoride phosphor with enhanced broadband emission for NIR pc-LEDs29Near-infrared emission, energy transfer, and mechanisms of Mn 2+ and Cr 3+ Co-doped lead-free Cs 2 AgInCl 6 double perovskites32Near-infrared luminescence and high thermal stability of Rb 2 NaScF 6 :Cr 3+ phosphor for spectroscopy applications14LiGaP2O7:Cr3+, Yb3+ phosphors for broadband NIR LEDs toward multiple applications44Crystal Field Engineering of Pr-Activated Gehlenite with Near Golden Ultraviolet C Emission for 100% Sterilization Efficiency11Thermally stable near-infrared emission from a double perovskite K2LiScF6:Cr3+ phosphor for light-emitting diodes31A highly thermo-stable far-red LiMgAlF6:Cr3+ phosphor for plant-growth lighting17Broadband near-infrared double-perovskite phosphor Sr2ScTaO6:Cr3+, Yb3+ for NIR pc-LED applications46Bandwidth-based flexible optical fiber thermometry based on sharp line emission regulation of Cr3+ ions34Optical Thermometer Based on Efficient Near‐Infrared Dual‐Emission of Cr3+ and Ni2+ in Magnetoplumbite Structure53Multiple lattice sites occupied AlTaO4:Cr3+ phosphor for luminescence ratiometric thermometry and NIR light source31Large-scale irrigation of Cr3+ into different octahedra of zinc aluminate toward continual broadband near-infrared emission7An ultra broadband NIR phosphor LiScSnO4:Cr3+ with emission wavelength peaking at 900 nm for component analysis14Tunable broadband near-infrared photoluminescence of Mg2LaTaO6:Cr3+ phosphors for light-emitting diodes20Broadband emitting Fe 3+ ‐doped double perovskite‐type antimonates phosphors for NIR spectroscopy applications28Sr2(Ga/Al)TaO6:Cr3+ phosphor with tunable near-infrared emitting for light-emitting diodes and optical thermometer32Multi-site occupancy high-efficient Mg2LaTaO6:Cr3+ phosphor for application in broadband NIR pc-LEDs62Cr3+‐Yb3+‐Ni2+ Tri‐Doped NIR Phosphors with Spectral Output Covering NIR‐I and NIR‐II Regions24Crystal structure and luminescence properties of a novel near-infrared phosphor LiAlO2:Fe3+28A near-infrared fluorescence enhancement strategy of amorphous silicon nanoparticles for night vision imaging and visualizing latent fingerprints4A NIR phosphor with ultra-broadband emission enabled by dual energy transfer within two Cr 3+ emitters and Cr 3+ → Yb 3+18Abnormal spectral broadening of ordered-structure near-infrared phosphor La 2 CaHfO 6 :Cr 3+15Achieving high brightness and thermally stable far-red luminescence via ultrathin phosphor–glass composite engineering3Achieving spectrally tunable and thermally stable near-infrared emission in Fe 3+ -activated spinel phosphors via the cation site modulation strategy34Analysis of Shale Structure Detection Data Based on Comparison Between Bridge and Tunnel0Boosting broadband short-wave infrared emission to achieve near-unity quantum efficiency via bridging Cr 3+ –Ni 2+ in spinel solid-solutions towards light-emitting diode applications31Broadband short-wave infrared Mg 4 Nb 2 O 9 :Cr 3+ ,Li + phosphor for nondestructive safety detection and biomedical imaging17Design of Cr 3+ -activated broadband NIR phosphors with tunable and abnormal thermal quenching behavior for NIR pc-LEDs22Enabling efficient near-infrared emission in lead-free double perovskite via a codoping strategy13High thermal stability and quantum efficiency of (Sr,Ba)2Ga2SiO7: Eu2+ phosphors for full-spectrum WLEDs17Multimodal dynamic luminescence of self-activated Na 2 CaGe 2 O 6 phosphor via defect manipulation2Novel high-efficiency near-infrared phosphor CaZrTaGaO 7 :Cr 3+ and its application in night vision and anti-counterfeiting7Simultaneous NIR photoluminescence and mechanoluminescence from Cr 3+ activated MgGa 2 O 4 phosphors with multifunctions for optical sensing26Site-selective occupancy of Cr 3+ enabling tunable emission from near infrared I to II in fluoride LiInF 4 :Cr 3+18Tunable broadband near-infrared luminescence from Cr 3+ -doped gallium oxide-based phosphors for advanced sensing and LED applications12Awakening the Dumb Site to Realize Ultra‐Broadband NIR Phosphor44Thermally Stable NIR Emission from Disordered Ba5La3MgAl3O15:Cr3+ with Peak Wavelength Beyond 900 nm36Emerging Fe 3+ Doped Broad NIR‐Emitting Phosphor Ca 2.5 Hf 2.5 (Ga, Al) 3 O 12 : Fe 3+ for LWUV Pumped NIR LED134Tuning the emission half-peak width of CaMgSi2O6:Cr3+ from 138 nm to 393 nm by controlling the Cr3+ concentration14Pr3+ ions, another alternative near-infrared luminescence emitter though energy transfer from Eu2+ for NIR pc-LEDs18Host Dependency of Boundary between Strong and Weak Crystal Field Strength of Cr3+ Luminescence111Highly‐Efficiency Far‐Red Emission in Cr3+ Activated Ca1.8Mg1.2Al2Ge3O12 toward Plant Precise Lighting30Broadband near infrared emission in Cr3+,Yb3+, Li+ tri-doped In2TeO614Super Broadband Emission Across NIR‐I and NIR‐II Under Blue Light Excitation of Cr 3+ , Ni 2+ Co‐Doped Sr 2 GaTaO 6 Phosphor Achieved by Two‐Site Occupation and Effective Energy Transfer178Dual substitution of host lattice ions to enhance the luminescence properties of Zn2TiO4:Cr3+ phosphor3Two-Site Occupation for Constructing Double Perovskite BaLaMgNbO 6 :Cr 3+ Ultrabroadband NIR Phosphors31Optimization of near-infrared luminescence performance in Cr3+-doped double perovskite Sr2ScTaO6 phosphor by Nb5+ ion substitution16Realize short-wave infrared luminescence in NaScP2O7:Cr3+,Yb3+ phosphor: Spectral and energy transfer16Unlocking Cr3+–Cr3+ Coupling in Spinel: Ultrabroadband Near-Infrared Emission beyond 900 nm with High Efficiency and Thermal Stability112Broadband NIR phosphor Gd3Lu2Ga3O12: Cr3+, Yb3+ with high thermal stability20Crystal Field-Engineered Cr3+-Doped Gd3(MgxGa5–2xGex)O12 Phosphors for Near-Infrared LEDs and X-ray Imaging Applications17Achieving Ultrahigh Thermal Stability in Cr3+-Activated Garnet Phosphors through Electron Migration between Thermally Coupled Levels17Multifunctional Near-Infrared Phosphors Cr 3+ /Ni 2+ Codoped Mg 3 Ga 2 GeO 8 Based on Energy Transfer from Cr 3+ to Ni 2+63Efficient and Tunable Near-Infrared Luminescence in Cubic Phosphate K 2 AlTi(PO 4 ) 3 :Cr 3+ for Spectroscopy Applications44A novel high-efficient NIR emitting phosphor Ca2YAl3Ge2O12:Cr3+ enabled by chemical unit co-substitution19Structure and photoluminescence properties of broadband NIR phosphor SrGeO3:Cr3+8Dual center luminescence properties of LiGaAl4O8:Cr3+ near infrared phosphors for LED applications10Near‐Infrared Mechanoluminescence of Gd 3 Ga 5 O 12 : Cr 3+ , La 3+ for Biological Stress Imaging26Co-training machine learning enables interpretable discovery of near-infrared phosphors with high performance16Tunable Luminescence in LiSc1‐yGayW2O8:Cr3+ Phosphors for LED Applications34Solvothermal phase selection of Cr3+-doped (NH4) ScF(3+) compounds (x = 0, 1, 3), structure, and NIR luminescence0Developing an efficient garnet-type near-infrared phosphor Na 1.5 Gd 1.5 Sc 2 Ge 3 O 12 :Cr 3+ with relatively long-wavelength emission10Long-Wavelength Broadband Near-Infrared ZrTe3O8:Cr3+, Ti4+ Phosphor of High Luminescence Quantum Yield and Excellent Thermal Stability9Ultra-broadband emission from Mg7Ga2GeO12:Ni2+,Cr3+ phosphor spanning the NIR I–III regions for spectroscopy applications10Achieving Flat Ultra‐Broadband NIR Emission in Cr 3+ Doped Garnet‐Type Phosphors Enabled by Structural Regulation Toward Multi‐Functional Spectroscopy Applications51Enhanced thermal stability of broadband NIR phosphors Ca3.3Mg0.7ZrGe3O12:Cr3+ for pc-LEDs8A broadband near-infrared phosphor: Solid-state synthesis, two Cr3+ sites occupation and enhanced thermal stability6Concentration-dependent NIR emission of Cr3+ in a two-site occupancy within K4Ga3Ta(PO4)615Blue light excitable efficient down-conversion photoluminescence of Yb3+ and Er3+ in ultra-wide NIR region via Cr3+-Yb3+-Er3+ energy transfer in KAlP2O7 and multifunctional applications11Mechanistic Insights into Dual NIR Emission from Cr-Doped Sc2O3 via First-Principles Calculations7Achieving tunable ultra-broadband NIR phosphors via antisite defect stabilized heavy Cr3+ doping for NIR spectroscopy application11Unique Spectral Broadening Induced by Exchange Coupling Between Cr 3+ Ions in LiAl 5 O 8 :Cr 3+ Phosphors for Versatile Optical Applications44Efficient and broadband Na4Al3Ta(PO4)6:Cr3+ phosphors for NIR pc-LED application4Insight into Cr3+-activated NIR phosphor with extremely high thermal stability for NIR LEDs13A novel green-emitting Mg0.75Al2.16O4:Mn2+ transparent ceramic phosphor for white light-emitting device3Recent progress of inorganic phosphors in artificial plant cultivation LEDs46Enhancement of luminescence properties of broadband NIR Cr3+-activated phosphate phosphors through cationic substitution11A novel dual-mode broadband near-infrared phosphor Mg 5 Ga 2 Sn 2 O 12 :Cr 3+ ,Ni 2+ designed based on an energy transfer strategy9Broadband photoluminescence toward the NIR II region and stable green ceramic pigments based on a novel NaBaScSi 2 O 7 : x Cr silicate phosphor10Dual center luminescence characteristics and multifunctional applications of Li 2 Ge 7 O 15 :Cr 3+ near-infrared phosphors6Highly Efficient Broadband Nir Emission of Cr3+- Activated Znwo4 Phosphors and Their Application in Phosphor-Converted Leds0Modulating excitation light to alter temperature-dependence of two-photon upconversion luminescence in Yb 3+ /Tm 3+ co-doped LuAG transparent ceramics3Strategies for broadening the emission spectra of Cr 3+ -doped near-infrared emitting phosphors59Super-wide-range tunable emission across NIR-II and NIR-III achieved by B-site cation co-substitution in Ni 2+ -doped double perovskites for NIR light sources71Enhanced near-infrared luminescence and thermal stability in Cr3+-Activated Y2CaAl4SiO12 phosphors: Towards high-performance NIR light sources24A broadband near-infrared emission of Cr3+-doped MgTiO3 phosphor for pc-LED applications10MTiTaO 6 : Cr 3+ ( M = Al 3+ , Ga 3+ , Sc 3+ ) Phosphors with Ultra‐Broadband Excitation Spectra and Enhanced Near‐Infrared Emission for Solar Cells22Broadband near-infrared phosphor SrGe4O9:Cr3+ for NIR-pc-LED applications6Ultrabroadband NIR Phosphor CaMg2Sc2Ge3O12:Cr3+ for Multifunctional Applications63Direct Blue‐LED Pumped Broadband Long‐Wavelength Near‐Infrared Emitter Based on Ni 2+ Mono‐Doped Double Perovskite Materials for Versatile Optical Applications22A novel broadband near-infrared phosphor NaBaScSi2O7: Fe3+ and its application in pc-LED and night vision32Cr3+-doped double-perovskite Sr2(Sc/In)NbO6 phosphors with broadband near-infrared emission5Near-Infrared Phosphor Zn2InGaO5:Cr3+ with a Wide Bandgap Applicable for Light Sources at Low Temperature9High-performance Cr3+-doped Sr2AlNbO6 double perovskite for near-infrared night-vision applications11Simultaneous enhancement of quantum efficiency and thermal stability through double cation substitution (Sr2+→Lu3+, Ge4+→Al3+) in garnet structure for NIR pc-LED3Self-recoverable and tunable ultra-broadband NIR mechanoluminescence in Cr3+-doped gallogermanate material20Broadening and Enhancing the Emission of Phosphor Li2MgTi3O8:Cr3+ by Cation Substitution10A highly efficient and thermo-stable near-infrared-emitting garnet phosphor for plant lighting5Broadband near-infrared long persistent luminescence in Cr3+-Doped CaY2Ga4GeO12 phosphors for advanced light source applications4Ultra-broadband near infrared phosphor with wide spectral range and long peak wavelength achieved by double-site occupation1Li+ and B3+ Co-Doping Induced Near-Infrared Emission Enhancement of Ga1.6Sc0.4O3:Cr3+2Engineering Broadband Emission of Zn 2 Ga 0.5‐y Al y Sb 0.5 O 4 ∶Cr 3+ Phosphors for Near‐Infrared LED Application17Ultra-broadband near-infrared-I and II emission from chromium doped double perovskite for multifunction application4Achieving Single‐Phased Full Visible Spectrum Broadband White Emission in Ag⁺, Bi 3 ⁺, and Sb 3 ⁺ Tri‐Doped Cs₂NaLuCl₆ Double Perovskite Phosphor21Ultra-broadband near-infrared emission and enhanced thermal stability in Lu3Ga3MgSiO12:Cr3+, Yb3+ garnet phosphor via chemical unit co-substitution and energy transfer17Advancements in the study of ion migration and mechanical properties in solid-state electrolytes through first-principles calculations4Development of Eu 2+ ‐Doped UCr 4 C 4 ‐Type Phosphors Toward Advanced Display Applications22Novel Cr3+-activated SrLu2Ga1.5Al2.5SiO12 garnet-type near-infrared phosphor: synthesis, luminescence and applications0Blue-Light-Excited Y2MgTiO6:Ni2+, Cr3+ Phosphors with Ultrabroadband NIR Emission for Multifunctional Applications11Enhanced thermal stability and energy transfer in Mn2+ co-doped MgAl2O4:Cr3+ for potential applications3Broadband NIR emission with excellent thermal stability for SrLaGaO4:Cr3+ phosphor6Interstitial Solid Solution Design Breaks the Property Ceiling: Cr 3+ Doped Near‐Infrared Phosphors with EQE Exceeding 50% and Zero‐Thermal‐Quenching Characteristics19Highly-efficient near-infrared emission from Cr3+ activated LaMgAl11O19 phosphor toward optical thermometer and pc-LED applications8High-efficiency Cr3+-activated broadband near-infrared phosphor GdGa0.5Sb1.5O6: Cr3+ with superior thermal stability for pc-LED8Near-Infrared Phosphors with Significantly Improved Luminescence Intensity and Zero-Thermal-Quenching for Light-Emitting Diodes3Novel garnet phosphor Tb3Ga5O12:Cr3+: High-efficiency near-infrared luminescence for near-infrared light source applications5Comparative Study of Cr 3+ -Activated Garnet Ca 2 YZnMGe 3 O 12 (M = Sc, In) Phosphors: Ultraefficient Near-Infrared Luminescence and Structure–Property Relationships1Developing a Near-Infrared Garnet Phosphor with Near-Unity Internal Quantum Efficiency and Wide-Range Spectral Tunability26Bias-Switchable Dual-Mode Organic Photodetectors for Spectrally Adaptive Vision and Secure Encoding13Multi-ion ordinated novel perovskite-based multifunctional fibers with tailored emission property toward smart wearables2Simultaneous emission and thermal stability enhancement of long-wavelength NIR luminescence of Cr 3+ ions in spinel phosphors via pivot-polyhedron linkage engineering4Site-selective luminescence in Ca-doped Sr2YNbO6:Eu3+ phosphors for high-color-purity red emission13Crystallographically altered (Mg,Sr) 3 (Al,Ga) 2 GeO 8 :Cr 3+ phosphors with tuned emission width from the ultra-sharp red to profound NIR band2Improved near infrared emission of Li 2 MgZrO 4 :Cr 3+ induced by Ga 3+ doping0Recent advances in Cr 3+ -doped near-infrared phosphors: preparation, luminescence, and LED applications5Vacancy-mediated stabilization of Cr 3+ and near-infrared luminescence enhancement in Mg 2 GeO 4 via Zn 2+ incorporation0Enhanced broadband near-infrared emission based on cation substitution in Cr3+ ion doped YGdScSbO7 phosphor0A thermally stable Ni2 + activated near-infrared II light emission with intense zero-phonon line1High‐Efficiency FWHM‐Variable NIR II Phosphor Mg 4 Al 4.5 Ga 2.45 B 1.05 O 16 : Cr 3+ with Excellent Thermal Stability6Unlocking Broadband Near-Infrared Luminescence from Cr 3+ -Activated NaGd 2 Ga 3 Ge 2 O 12 Garnet Induced by Intrinsic Cation Disorder3Cr3+-activated Mg3Y2Ge3O12 near-infrared phosphor for broadband-emitting pc-LED light source targeting spectroscopic applications4Efficient near-infrared luminescence in phosphate Na2AlTi(PO4)3:Cr3+ for light-emitting-diodes applications0Co-Doped La 3+ Achieves Synergistic Regulation of Spectral Broadening and Energy Level Dynamics in Er 3+ :NaSrY(MoO 4 ) 3 Disordered Crystals1Ga 3+ Cation‐Directed Microstructural Engineering of Glass‐Ceramics Unlocks High‐Power NIR LEDs0A Novel Strategy for High Quantum Efficiency Composite Oxide Far-Red Phosphors: Ca14Mg5.94Li0.03In0.03Ga9.95O35:0.05Mn4+0Efficient broadband near-infrared emission of trivalent chromium in spinel enabled by mixed octahedral cation occupation0Ultrabroadband near-infrared emission in Cr3+-doped garnet phosphors via structural engineering: achieving and applications2Broadband NIR emission from Y2CaGa4GeO12:Cr3+ phosphors via co-substitution engineering for bioimaging and night-vision0Co‐Substitution Crystal Lattice Engineering and Flux‐Assisted Synthesis of Cr 3+ ‐Activated High‐Performance Phosphors for Efficient Near‐Infrared Pc‐LEDs and Multi‐Application2Local lattice modulation via Na+ for K+ substitution to enhance luminescence efficiency and thermal stability of Cr3+-doped K3LiMg4(Si2O5)6 NIR phosphors1Achieving Near‐Infrared II Emission Through Energy Transfer From Cr 3+ to Ni 2+ in Gd 3 Ga 5 O 12 Host0Enhanced luminescence and thermal stability of GdMgAl11O19:Mn2+ phosphor via Si4+ doping for transparent displays2Cr3+ doped rigid garnet phosphors@PDMS composite platforms: Anti-thermal quenching and high sensitivity for multifunctional applications0TSSG Growth and Thermal Field Optimization of Er 3+ :NaSrY(Mo 1– x W x O 4 ) 3 Crystals: Structure Evolution and Anion-Substitution-Induced Disorder0Efficient and thermally stable Cr3+-doped pyrochlore NIR phosphors through chemical pressure engineering-induced crystal field strengthening0Photoluminescence properties of Cr3+-doped Sc2Ge2O7: a spectroscopic investigation of site occupation and concentration-dependent behavior0Design and luminescence properties of novel Nb-based garnet phosphor LuCa2Ga4NbO12:Cr3+ for NIR pc-LEDs0

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  35. Simultaneous NIR photoluminescence and mechanoluminescence from Cr 3+ activated MgGa 2 O 4 phosphors with multifunctions for optical sensing

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  36. Site-selective occupancy of Cr 3+ enabling tunable emission from near infrared I to II in fluoride LiInF 4 :Cr 3+

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  37. Tunable broadband near-infrared luminescence from Cr 3+ -doped gallium oxide-based phosphors for advanced sensing and LED applications

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  38. Awakening the Dumb Site to Realize Ultra‐Broadband NIR Phosphor

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  39. Thermally Stable NIR Emission from Disordered Ba5La3MgAl3O15:Cr3+ with Peak Wavelength Beyond 900 nm

    Advanced Optical Materials · 2024-01-15

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  40. Emerging Fe 3+ Doped Broad NIR‐Emitting Phosphor Ca 2.5 Hf 2.5 (Ga, Al) 3 O 12 : Fe 3+ for LWUV Pumped NIR LED

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  41. Tuning the emission half-peak width of CaMgSi2O6:Cr3+ from 138 nm to 393 nm by controlling the Cr3+ concentration

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  42. Pr3+ ions, another alternative near-infrared luminescence emitter though energy transfer from Eu2+ for NIR pc-LEDs

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  43. Host Dependency of Boundary between Strong and Weak Crystal Field Strength of Cr3+ Luminescence

    The Journal of Physical Chemistry Letters · 2024-02-22

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  44. Highly‐Efficiency Far‐Red Emission in Cr3+ Activated Ca1.8Mg1.2Al2Ge3O12 toward Plant Precise Lighting

    Advanced Optical Materials · 2024-02-25

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  45. Broadband near infrared emission in Cr3+,Yb3+, Li+ tri-doped In2TeO6

    Materials Research Bulletin · 2024-03-17

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  46. Super Broadband Emission Across NIR‐I and NIR‐II Under Blue Light Excitation of Cr 3+ , Ni 2+ Co‐Doped Sr 2 GaTaO 6 Phosphor Achieved by Two‐Site Occupation and Effective Energy Transfer

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  47. Dual substitution of host lattice ions to enhance the luminescence properties of Zn2TiO4:Cr3+ phosphor

    Luminescence · 2024-03-28

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  48. Two-Site Occupation for Constructing Double Perovskite BaLaMgNbO 6 :Cr 3+ Ultrabroadband NIR Phosphors

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  49. Optimization of near-infrared luminescence performance in Cr3+-doped double perovskite Sr2ScTaO6 phosphor by Nb5+ ion substitution

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