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RESEARCH PAPER · Angewandte Chemie · 2023

New Oxyhalide Solid Electrolytes with High Lithium Ionic Conductivity >10 mS cm−1for All‐Solid‐State Batteries

Yoshiaki Tanaka, Koki Ueno, Keita Mizuno, Kaori Takeuchi, Tetsuya Asano, Akihiro Sakai

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New Oxyhalide Solid Electrolytes with High Lithium Ionic Conductivity >10 mS cm−1for All‐Solid‐State BatteriesOriginalHopping Rate and Migration Entropy as the Origin of Superionic Conduction within Solid-State Electrolytes62Dynamic Monkey Bar Mechanism of Superionic Li‐ion Transport in LiTaCl67Dynamic Monkey Bar Mechanism of Superionic Li‐ion Transport in LiTaCl636Engineering Strategies to Improve All-Solid-State Battery Performance under Low-Pressure Conditions0Lithium Batteries – Lithium Secondary Batteries – Lithium All-Solid State Battery | Halides and Oxy-Halide Electrolytes0Structure design of a BiOF solid electrolyte with remarkably outstanding fluoride ion diffusion performance induced by Ga doping3Atmospheric-Pressure Operation of All-Solid-State Batteries Enabled by Halide Solid Electrolyte76Superionic Conductivity Invoked by Enhanced Correlation Migration in Lithium Halides Solid Electrolytes84Na M Cl 6 ( M = Nb and Ta): A New Class of Sodium-Conducting Halide-Based Solid Electrolytes60A Universal Self‐Propagating Synthesis of Aluminum‐Based Oxyhalide Solid‐State Electrolytes3A Universal Self‐Propagating Synthesis of Aluminum‐Based Oxyhalide Solid‐State Electrolytes58LaCl3-based sodium halide solid electrolytes with high ionic conductivity for all-solid-state batteries88KTaCl6: High-voltage stable potassium-ion conducting chloride solid electrolyte13Exploring superionic conduction in lithium oxyhalide solid electrolytes considering composition and structural factors31High Fire‐Safety and Multifunctional Eutectogel for Flexible Quasi‐Solid‐State Supercapacitors83The importance of A-site cation chemistry in superionic halide solid electrolytes10Crystal-dependent doping effects over MnO2 for Fenton-like catalysis optimization8Fast Sodium-Ion Conducting Amorphous Oxychloride Embedding Nanoparticles10Superior Li‐Ion Transport in LiNb 0.5 Ta 0.5 Cl 617Oxychloride Polyanion Clustered Solid‐State Electrolytes via Hydrate‐Assisted Synthesis for All‐Solid‐State Batteries56A facile route to plastic inorganic electrolytes for all-solid state batteries based on molecular design43A compactable Na 2.5 PS 3.5 F 0.5 electrolyte for solid-state sodium batteries10Data-driven atomistic modeling of crystalline and glassy solid-state electrolytes6Correlation between the Coherence Length and Ionic Conductivity in LiNbOCl 4 via the Anion Stoichiometry18Beneficial redox activity of halide solid electrolytes empowering high-performance anodes in all-solid-state batteries49Progress and Challenges in Li M OCl 4 and Na M OCl 4 ( M = Nb, Ta) Oxyhalide Solid Electrolytes for Solid‐State Batteries14Minutes‐Scale Ultrafast Synthesis of New Oxyhalides Solid Electrolytes with Interfacial Ionic Conduction for All‐Solid‐State Batteries2A Surface Non‐Destructive Modification Strategy Addressing Moisture and Oxidation Instabilities of Sulfide Solid‐State Electrolytes0A Surface Non‐Destructive Modification Strategy Addressing Moisture and Oxidation Instabilities of Sulfide Solid‐State Electrolytes15Correlated terahertz phonon–ion interactions control ion conduction in a solid electrolyte6Atomic Level Fabrication of Oxychloride Interface for High‐Rate and High‐Voltage Lithium‐Ion Batteries0Microscopic Mechanisms of Superionic Na-ion Conductivity in Crystalline and Amorphous NaMOCl 4 (M = Nb, Ta) Solid Electrolytes10Mechanisms of Alkali Ionic Transport in Amorphous Oxyhalides Solid State Conductors1Comparison of Li3InxY(1−x)Cl6 Solid Electrolytes Synthesized by Mechanochemical and Water-Based Methods for All-Solid-State Batteries0

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  1. Hopping Rate and Migration Entropy as the Origin of Superionic Conduction within Solid-State Electrolytes

    Journal of the American Chemical Society · 2023-05-17

    Xiaona Li, Honggang Liu, Changtai Zhao, Jung Tae Kim, Jiamin Fu, Xiaoge Hao, Weihan Li, Ruying Li, Ning Chen, Duanyun Cao, Zhenwei Wu, Yuefeng Su, Jianwen Liang, Xueliang Andy Sun

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  2. Dynamic Monkey Bar Mechanism of Superionic Li‐ion Transport in LiTaCl6

    Angewandte Chemie · 2023-12-12

    Ming Lei, Bo Li, Hongjun Liu, De‐en Jiang

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  3. Dynamic Monkey Bar Mechanism of Superionic Li‐ion Transport in LiTaCl6

    Angewandte Chemie International Edition · 2023-12-12

    Ming Lei, Bo Li, Hongjun Liu, De‐en Jiang

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  4. Engineering Strategies to Improve All-Solid-State Battery Performance under Low-Pressure Conditions

    Unknown journal · 2023-12-18

    Benjamin Hennequart

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  5. Lithium Batteries – Lithium Secondary Batteries – Lithium All-Solid State Battery | Halides and Oxy-Halide Electrolytes

    Elsevier eBooks · 2023-12-18

    Artur V. Tron, Palanivel Molaiyan, Marcus Jahn, Andrea Paolella

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  6. Structure design of a BiOF solid electrolyte with remarkably outstanding fluoride ion diffusion performance induced by Ga doping

    Journal of Materials Chemistry A · 2024-01-01

    Jiyu Ning, Weijia Meng, Chuang Wang, Huangkai Wang, Chao Jun Wu, Lidong You, Xianyou Wang, Yong Pei, Haibo Wang, Zhenhua Yang

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  7. Atmospheric-Pressure Operation of All-Solid-State Batteries Enabled by Halide Solid Electrolyte

    ACS Energy Letters · 2024-01-12

    Benjamin Hennequart, Maria Platonova, Ronan Chometon, Thomas Marchandier, Alessandro Benedetto, Elisa Quemin, Romain Dugas, Christophe Lethien, Jean‐Marie Tarascon

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  8. Superionic Conductivity Invoked by Enhanced Correlation Migration in Lithium Halides Solid Electrolytes

    ACS Energy Letters · 2024-02-19

    Rui Li, Pushun Lu, Xinmiao Liang, Liwei Liu, Maxim Avdeev, Zhi Bing Deng, Shuai Li, Kaiqi Xu, Jiwen Feng, Rui Si, Fan Bean Wu, Zhizhen Zhang, Yong‐Sheng Hu

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  9. Na M Cl 6 ( M = Nb and Ta): A New Class of Sodium-Conducting Halide-Based Solid Electrolytes

    ACS Materials Letters · 2024-04-01

    Zheng Huang, Suguru Yoshida, Hirofumi Akamatsu, Katsuro Hayashi, Saneyuki Ohno

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  10. A Universal Self‐Propagating Synthesis of Aluminum‐Based Oxyhalide Solid‐State Electrolytes

    Angewandte Chemie · 2024-04-25

    Simeng Zhang, Yang Xu, Han Shui Wu, Tianlu Pang, Nian Zhang, Changtai Zhao, Junyi Yue, Jiamin Fu, Shengjie Xia, Xiangzhen Zhu, Guanzhi Wang, Hui Duan, Biwei Xiao, Tao Mei, Jianwen Liang, Xueliang Andy Sun, Xiaona Li

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  11. A Universal Self‐Propagating Synthesis of Aluminum‐Based Oxyhalide Solid‐State Electrolytes

    Angewandte Chemie International Edition · 2024-04-25

    Simeng Zhang, Yang Xu, Han Shui Wu, Tianlu Pang, Nian Zhang, Changtai Zhao, Junyi Yue, Jiamin Fu, Shengjie Xia, Xiangzhen Zhu, Guanzhi Wang, Hui Duan, Biwei Xiao, Tao Mei, Jianwen Liang, Xueliang Andy Sun, Xiaona Li

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  12. LaCl3-based sodium halide solid electrolytes with high ionic conductivity for all-solid-state batteries

    Nature Communications · 2024-05-21

    Chengyu Fu, Yifan Li, Wenjie Xu, Xuyong Feng, Weijian Gu, Jue Liu, Wenwen Deng, Wei Wang, Milinda Abeykoon, Laisuo Su, Lingyun Zhu, Xiaojun Wu, Hongfa Xiang

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  13. KTaCl6: High-voltage stable potassium-ion conducting chloride solid electrolyte

    Energy storage materials · 2024-07-03

    Changhoon Kim, Juhyoun Park, Hiram Kwak, Jae‐Seung Kim, Seunggoo Jun, Dong‐Hwa Seo, Yoon Seok Jung

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  14. Exploring superionic conduction in lithium oxyhalide solid electrolytes considering composition and structural factors

    npj Computational Materials · 2024-07-14

    Fiaz Hussain, Jinlong Zhu, Yusheng Zhao, Wei Xia

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  15. High Fire‐Safety and Multifunctional Eutectogel for Flexible Quasi‐Solid‐State Supercapacitors

    Advanced Functional Materials · 2024-08-10

    Qingtao Zeng, Xuejun Lai, Hongqiang Li, Zhonghua Chen, Xingrong Zeng, Liqun Zhang

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  16. The importance of A-site cation chemistry in superionic halide solid electrolytes

    Nature Communications · 2024-08-29

    K. H. Barker, Sarah B. McKinney, Raül Artal, Ricardo Jiménez, Nuria Tapia‐Ruiz, Stephen J. Skinner, Ainara Aguadero, Ieuan David Seymour

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  17. Crystal-dependent doping effects over MnO2 for Fenton-like catalysis optimization

    Separation and Purification Technology · 2024-09-19

    Shan‐Li Wang, Zi-Juan Yang, Zheren Hu, Chao Li, Fan Yang, Mingyan Zhang, Deyou Yu, Minghua Wu, Bin Yu

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  18. Fast Sodium-Ion Conducting Amorphous Oxychloride Embedding Nanoparticles

    Chemistry of Materials · 2024-09-24

    Kota Motohashi, Hirofumi Tsukasaki, Shigeo Mori, Atsushi Sakuda, Akitoshi Hayashi

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  19. Superior Li‐Ion Transport in LiNb 0.5 Ta 0.5 Cl 6

    Advanced Functional Materials · 2024-09-24

    Ming Lei, Bo Li, Rongrong Yin, Xiulei Ji, De‐en Jiang

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  20. Oxychloride Polyanion Clustered Solid‐State Electrolytes via Hydrate‐Assisted Synthesis for All‐Solid‐State Batteries

    Advanced Materials · 2024-11-12

    Guanzhi Wang, Simeng Zhang, Han Wu, Matthew Liu Zheng, Changtai Zhao, Jianwen Liang, Liyu Zhou, Junyi Yue, Xiangzhen Zhu, Yang Xu, Nian Zhang, Tianlu Pang, Jiamin Fu, Weihan Li, Yuanguang Xia, Wen Yin, Xueliang Andy Sun, Xiaona Li

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  21. A facile route to plastic inorganic electrolytes for all-solid state batteries based on molecular design

    Energy & Environmental Science · 2024-11-21

    Insang You, Baltej Singh, Mengyang Cui, Gillian R. Goward, Lanting Qian, Zachary Arthur, Graham King, Linda F. Nazar

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  22. A compactable Na 2.5 PS 3.5 F 0.5 electrolyte for solid-state sodium batteries

    Energy & Environmental Science · 2025-01-01

    Xianguang Miao, Yifan Wu, Huirong Jing, Yuchuang Cao, Yichao Wang, Junyeob Moon, Xin Li

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  23. Data-driven atomistic modeling of crystalline and glassy solid-state electrolytes

    Chemical Communications · 2025-01-01

    Rongkang Zhou, Kun Luo, Qi An

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  24. Correlation between the Coherence Length and Ionic Conductivity in LiNbOCl 4 via the Anion Stoichiometry

    Chemistry of Materials · 2025-05-21

    Jon A. Newnham, Jędrzej Kondek, Johannes Hartel, Carolin Rosenbach, Cheng Li, Vasiliki Faka, Lara M. Gronych, Dana Glikman, Fabian Schreiner, Domenik D. Wind, Björn Braunschweig, Michael Ryan Hansen, Wolfgang G. Zeier

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  25. Beneficial redox activity of halide solid electrolytes empowering high-performance anodes in all-solid-state batteries

    Nature Materials · 2025-07-16

    Zhu Qing Cheng, Wen-Xuan Zhao, Qidi Wang, Chenglong Zhao, Anastasia K. Lavrinenko, Alexandros Vasileiadis, Victor Landgraf, Lars Johannes Bannenberg, Yuhang Li, Junwei Liang, Ming Liu, Swapna Ganapathy, Marnix Wagemaker

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  26. Progress and Challenges in Li M OCl 4 and Na M OCl 4 ( M = Nb, Ta) Oxyhalide Solid Electrolytes for Solid‐State Batteries

    Advanced Energy Materials · 2025-09-12

    Jon A. Newnham, Alexander G. Squires, Marvin A. Kraft, David O. Scanlon, Wolfgang G. Zeier

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  27. Minutes‐Scale Ultrafast Synthesis of New Oxyhalides Solid Electrolytes with Interfacial Ionic Conduction for All‐Solid‐State Batteries

    Angewandte Chemie · 2025-11-04

    Yanfeng Zhang, Qiankun Meng, Ao Zeng, Shuaiqin Qiu, Hong Zhang, Enyue Zhao, Xiaoling Xiao

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  28. A Surface Non‐Destructive Modification Strategy Addressing Moisture and Oxidation Instabilities of Sulfide Solid‐State Electrolytes

    Angewandte Chemie · 2025-12-29

    Yicheng Deng, Guo Tang, Gengzhong Lin, Kean Chen, Hui Li, Yuliang Cao, Yongjin Fang, Jiangfeng Qian, He Yang, Xinping Ai

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  29. A Surface Non‐Destructive Modification Strategy Addressing Moisture and Oxidation Instabilities of Sulfide Solid‐State Electrolytes

    Angewandte Chemie International Edition · 2025-12-29

    Yicheng Deng, Guo Tang, Gengzhong Lin, Kean Chen, Hui Li, Yuliang Cao, Yongjin Fang, Jiangfeng Qian, He Yang, Xinping Ai

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  30. Correlated terahertz phonon–ion interactions control ion conduction in a solid electrolyte

    Materials Horizons · 2026-01-01

    Kim H. Pham, Kiarash Gordiz, Natan A. Spear, Amy K. Lin, Jonathan M. Michelsen, Hanzhe Liu, Daniele Vivona, Geoffrey A. Blake, Yang Shao‐Horn, Asegun S. Henry, Kimberly A. See, Scott K. Cushing

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  31. Atomic Level Fabrication of Oxychloride Interface for High‐Rate and High‐Voltage Lithium‐Ion Batteries

    Angewandte Chemie · 2026-01-13

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  32. Microscopic Mechanisms of Superionic Na-ion Conductivity in Crystalline and Amorphous NaMOCl 4 (M = Nb, Ta) Solid Electrolytes

    ACS Energy Letters · 2026-01-31

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  33. Mechanisms of Alkali Ionic Transport in Amorphous Oxyhalides Solid State Conductors

    Advanced Energy Materials · 2026-06-04

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  34. Comparison of Li3InxY(1−x)Cl6 Solid Electrolytes Synthesized by Mechanochemical and Water-Based Methods for All-Solid-State Batteries

    ChemEngineering · 2026-06-18

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