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RESEARCH PAPER · Journal of the American Chemical Society · 2023

Optimal Binding Affinity for Sieving Separation of Propylene from Propane in an Oxyfluoride Anion-Based Metal–Organic Framework

Yi Xie, Yanshu Shi, Eder Moisés Cedeño Morales, Ayoub El Karch, Bin Wang, Hadi D. Arman, Kui Tan, Banglin Chen

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Optimal Binding Affinity for Sieving Separation of Propylene from Propane in an Oxyfluoride Anion-Based Metal–Organic FrameworkOriginalA metal–organic framework based propylene nano-trap with dual functionalities for highly efficient propylene/propane separation13A zirconium-based microporous metal–organic framework for molecular sieving CO 2 separation7Cation exchange in an anionic metal–organic framework enhancing propylene/propane separation7Enhanced CO 2 sorption properties in a polarizable [WO 2 F 4 ] 2− -pillared physisorbent under direct air capture conditions8Metal–organic frameworks for hydrocarbon separation: design, progress, and challenges38Rational design of metal–organic frameworks featuring macrocycle and helical chain motifs for propylene/propane separation2Recent progress in metal–organic frameworks for the separation of gaseous hydrocarbons29Amine-functionalized ultramicroporous metal-organic framework for efficient propylene/propane separation3Polarization enhanced CH4/N2 separation in bromine functionalized ZIF-62 based mixed-matrix membranes20Membrane adsorbers with ultrahigh metal–organic framework loading for high flux selective separations to isomer7Topological Design of Unprecedented Metal‐Organic Frameworks Featuring Multiple Anion Functionalities and Hierarchical Porosity for Benchmark Acetylene Separation103Topological Design of Unprecedented Metal‐Organic Frameworks Featuring Multiple Anion Functionalities and Hierarchical Porosity for Benchmark Acetylene Separation27Porous Metal–Organic Frameworks for Light Hydrocarbon Separation28Fabrication of Pillar‐Cage Fluorinated Anion Pillared Metal–Organic Frameworks via a Pillar Embedding Strategy and Efficient Separation of SO 2 through Multi‐Site Trapping36Fabrication of Pillar‐Cage Fluorinated Anion Pillared Metal–Organic Frameworks via a Pillar Embedding Strategy and Efficient Separation of SO 2 through Multi‐Site Trapping2Separation of Propylene and Propane Using Metal–Organic Frameworks22Delicate Softness in a Temperature-Responsive Porous Crystal for Accelerated Sieving of Propylene/Propane100Specific Propyne Trapping Sites within a Robust MOF for Efficient Propyne/Propadiene Separation with Record Propadiene Productivity36Comparative study of metal–organic frameworks synthesized via imide condensation and coordination assembly3Recent advances on metal–organic frameworks for deep purification of olefins54Robust 5p-4f Heterometallic {Snln 2 }-Organic Frameworks For Efficiently Chemical Fixation of Co 2 Under Mild Conditions0Water-stable metal–organic frameworks (MOFs): rational construction and carbon dioxide capture246Temperature-dependent molecular sieving of fluorinated propane/propylene mixtures by a flexible-robust metal-organic framework73Interaction-selective molecular sieving adsorbent for direct separation of ethylene from senary C2-C4 olefin/paraffin mixture59Fine-tuning the pore environment of isoreticular metal-organic frameworks through installing functional sites for boosting C2H6/C2H4 separation25Fluorinated MOF‐Based Hexafluoropropylene Nanotrap for Highly Efficient Purification of Octafluoropropane Electronic Specialty Gas12Fluorinated MOF‐Based Hexafluoropropylene Nanotrap for Highly Efficient Purification of Octafluoropropane Electronic Specialty Gas67Scalable Synthesis of Robust MOF for Challenging Ethylene Purification and Propylene Recovery with Record Productivity77Scalable Synthesis of Robust MOF for Challenging Ethylene Purification and Propylene Recovery with Record Productivity23State of the art, challenges and prospects in metal–organic frameworks for the separation of binary propylene/propane mixtures70Recent advances in metal–organic frameworks for C3H6- and C3H8-selective separation of C3H6/C3H8 binary natural gas mixtures: A review13Diffusion-rate sieving of propylene and propane mixtures in a cooperatively dynamic porous crystal59Biological metal–organic frameworks for natural gas purification and MTO product separation25Recent Advances of Multidentate Ligand-Based Anion-Pillared MOFs for Enhanced Separation and Purification Processes44A robust metal–organic framework for simultaneous C2H4/C3H6 capture and C2H2/CO2 separation9Immobilization of Lewis Basic Sites into a Quasi‐Molecular‐Sieving Metal–Organic Framework for Enhanced C3H6/C3H8 Separation22Surface sieving carbon skins for propylene and propane separation37Hyper-Cross-Linked Resin Modified by a Micropore Polymer for Gas Adsorption and Separation4Tuning redox activity in metal–organic frameworks: From structure to application62Kinetic sieving separation of a gating macrocyclic crystal for purification of propylene26Wood-structured carbon with reassembled pores showing high propylene adsorption rate for efficient separation of propylene/propane8Robust heterometallic {In2CdO}-Organic framework for efficiently catalyzing CO2 cycloaddition and Knoevenagel condensation22Green and Scalable Preparation of an Isomeric CALF‐20 Adsorbent with Tailored Pore Size for Molecular Sieving of Propylene from Propane26A Pillar[5]arene-Containing Metal–Organic Framework for Rapid and Highly Capable Adsorption of a Mustard Gas Simulant33Synthesis of Cuprous Organic Frameworks with Adjustable Pores as Membrane Materials for C3H6/C3H8 Separation19Defect-engineered indium–organic framework displays the higher CO2 adsorption and more excellent catalytic performance on the cycloaddition of CO2 with epoxides under mild conditions14Isoreticular Metal–Organic Frameworks with Aromatic Pores and Dimethylammonium Cations Enable Separation of Light Hydrocarbons and Xenon/Krypton12RETRACTED: Catalytic engineering of transition metal (TM: Ni, Pd, Pt)-coordinated Ge-doped graphitic carbon nitride (Ge@g-c3n4) nanostructures for petroleum hydrocarbon separation: An outlook from theoretical calculations6High‐Throughput Computational Screening‐Driven Porous Material Discovery for Benchmark Propylene/Propane Separation25Bioinspired recognition in metal-organic frameworks enabling precise sieving separation of fluorinated propylene and propane mixtures42Separation of xylene isomers using metal-organic frameworks: Addressing challenges in the petrochemical industry35Efficient C3H6/C3H8 separation within a bifunctional ultramicroporous metal-organic framework with high purity and record packing density10Hydrogen Bonds Defined Pore Windows Enable Sieving Separation of Propylene from Propane in an Ultramicroporous Metal–Organic Framework12Reviews on propylene/propane separation by using ionic liquids materials0Optimizing Propylene/Propane Sieving Separation through Gate‐Pressure Control within a Flexible Organic Framework23Optimizing Propylene/Propane Sieving Separation through Gate‐Pressure Control within a Flexible Organic Framework10Pore configuration control in hybrid azolate ultra-microporous frameworks for sieving propylene from propane79A new SIFSIX anion pillared cage MOF with crs topological structure for efficient C2H2/CO2 separation19A hybrid azolate framework for record propylene/propane sieving separation2Construction of synergistic binding sites in a robust MOF for excellent C 2 H 4 purification and C 3 H 6 recovery performance20Ionic porous materials: from synthetic strategies to applications in gas separation and catalysis45Precise tuning of pore size distribution in amorphous carbon molecular sieves at the sub-angstrom scale via a synergic mechanism of pore-making and shrinking for separating similar gases9An amino-functionalized ultra-micropore metal–organic framework using for argon/oxygen adsorption separation5Pore Engineering in Metal–Organic Frameworks for Enhanced Hydrocarbon Adsorption and Separation42Tailoring Metal–Organic Frameworks for One‐Step Separation of Alkane/Alkene/Alkyne Mixtures3Lowering Linker Symmetry to Access Zirconium Metal–Organic Frameworks for Inverse Alkane/Alkene Separations19Lowering Linker Symmetry to Access Zirconium Metal–Organic Frameworks for Inverse Alkane/Alkene Separations13One new Co-MOF with F sites in the pores for selective C 2 H 2 adsorption over CO 2 and CH 43Architecting Metal–Organic Frameworks at Molecular Level toward Direct Air Capture103Zinc-Based flexible coordination network for precise butane isomer sieving and low-carbon alkane recovery from oilfield associated gas5Pore engineering in double-wall MOFs through immobilizing functional bonding sites for boosting efficient ethane/ethylene separation6Two-Dimensional Anion-Pillared Metal–Organic Framework for Sieving Separation of Propylene from Propane with Ultrahigh Kinetic Performance5Self‐assembled Metal−Organic Framework Microspheres for Thermodynamic−Kinetic Synergistic Separation of Propylene and Propane†8Adsorption separation of propylene/propane by pressure induced flexible porous MOF7Robust Fluorine-Decorated {Yb4}-Organic Framework for C2H6 Capture and Efficient Catalytic Performance on CO2-Epoxide Cycloaddition33Direct synthesis of low-molecular-weight poly(2,6-dimethyl-1,4-phenylene oxide) (LMW-PPO) by Cu(II)-ionic liquids3Microsize regulation and scalable synthesis of two isoreticular fluorinated MOFs for ethylene purification and MTO products separation23Modulating Adsorption Kinetics in a 3D-Interconnected Nanocavity Framework with Narrow Apertures for Enhanced Propylene Separation20Highly Robust Zr-MOF Platform Featuring Aromatic-Rich Cores for Efficient Paraffin/Olefin Separation2Probing bimodal sub‐nanopores in carbon for ideal fast sieving separation of propylene/propane1Stabilization of Supramolecular Frameworks by Surface-Confined Polymerization for Natural Gas Purification6A Novel Multifunctional Cd-MOF Containing Thiazolo[5,4-d]thiazole and Azo Moieties for Highly Efficient Adsorption of Iodine and Catalytic CO2 Cycloaddition7Simultaneous C 2 H 4 and C 3 H 6 Purification via a MOF with Hierarchical Cages by Unique Combination of Coordination Patterns7Structural engineering of metal-organic frameworks for perfluorinated gas separation28Carbon Dioxide Capture by a Hydrothermally Synthesized Water-Resistant Zinc-Oxalate-Aminotriazolate Framework5Regulating the pore configuration of hybrid azolate ultra-microporous frameworks for efficient sieving propylene from propane0A Distinct Microporous Metal–Organic Framework with Multiple Accessible Adsorption Sites for Separation of C2H2/CO2/CH4 Mixtures10A scalable ultramicroporous metal-organic framework for highly effective propylene/propane separation at elevated temperatures9Inverse Hydrocarbon Recognition via Nitro Group–Programmed Soft Porous Crystal for One-Step C3H6 Purification16Low-Temperature Decarboxylation and Sensitive Detection of Trifluoroacetic Acid on the Interface of Active Amino Nickel Metal Organic Layers4Cost‐Effective Scalable Production of Ultra‐Stable Alkyl MOF Featuring Single‐Molecule C 3 H 6 Trap for Record Capture of Trace C 3 H 6 from C 2 H 43Cost‐Effective Scalable Production of Ultra‐Stable Alkyl MOF Featuring Single‐Molecule C 3 H 6 Trap for Record Capture of Trace C 3 H 6 from C 2 H 423Pore engineering via controlled decomposition of counter cations in an anion-based metal-organic framework1Scalable Synthesis of the Robust Ultramicroporous Metal–Organic Framework for Reinforced C 3 H 6 /C 3 H 8 Separation5The Molecular Sieving of Propylene and Propane on SAPO-35 Molecular Sieve1Temperature-regulated synthesis of carbonate-pillared zinc-triazolate frameworks for precise molecular recognition6Cation-regulated rigid and soft crystalline porous frameworks for CO 2 sieving and C 3 H 6 /C 3 H 8 separation0Integrating hydrogen-bonding nanotraps in a cost-effective metal–organic framework enables highly efficient C 3 F 6 /C 3 F 8 separation0Nitro-Triazole-Functionalized Metal-organic Framework for Improved Water Stability and Trace C3H6 Capture from MTO Products0A stable two-fold interpenetrated Zn(II) metal-organic framework as rapid fluorescence sensor toward 2,6-dichloro-4-nitroaniline in the aqueous solution1Green synthesis of metal–organic frameworks: Toward sustainable fabrication and environmental responsibility4A low-cost and scalable green-produced ultra-stable Al-MOF with leverage effect of surface microenvironment for record C2H4 purification from MTO products15Zn8(CH3COO)8-siloxane cluster-based metal-organic frameworks for inverse propylene/propane separation7Crystal Engineering of Reticular Materials for Gas‐ and Liquid‐Phase Hydrocarbon Separation4Regulation Mechanism of Entropy–Enthalpy Compensation Effect on Charge Trap Energy Levels in Hydrogen-Bonded PP- g -MA/PVDF Composites2Trace Capture Hexafluoropropylene From Octafluoropropane via Complete Molecular Sieving Mechanism in a Highly Robust Metal−Organic Framework8Trace Capture Hexafluoropropylene From Octafluoropropane via Complete Molecular Sieving Mechanism in a Highly Robust Metal−Organic Framework4MOF‐on‐MOF Core–Shell Heterostructure With Synergistic Porous Interface for Highly Efficient Propane/Propylene Separation2Microporous MOF for simultaneous high thermodynamic and kinetic synergistic separation of propylene and propane18Electrostatic Potential Tuning‐Driven Molecular Rotor Rotation in Isostructural Metal‐Organic Frameworks for C 3 H 6 /C 3 H 8 Separation0Electrostatic Potential Tuning‐Driven Molecular Rotor Rotation in Isostructural Metal‐Organic Frameworks for C 3 H 6 /C 3 H 8 Separation3Metal–Organic Framework with Lewis Basic N-Rich Channels for Separating Hydrocarbons from CO 2 -Containing Mixtures0Metal–Organic Frameworks for Hydrocarbon Separations0Hydrogen-bonding guided isoreticular supramolecular frameworks with self-recovery for efficient natural gas purification1Tunable π ‐Basic Platforms in Porous Crystals for Enhanced C 2 H 2 /CO 2 Separation at Elevated Temperature2Adaptive Throat‐Sieving Gate in a Metal Azolate Framework Enabling Synergistic Equilibrium‐Kinetic Separation of Propylene and Propane6Template-to-pore modifier engineering of pure-silica STT zeolite for humid tolerant C3H6/C3H8 separation0Crystal Engineering of Chelating Hybrid Ultramicroporous Materials via Pillar Modulation for Energy‐Efficient Acetylene Separation0Ambient and scalable synthesis of Zn-based MOF in a water–ethanol system for CO2 capture and catalytic valorization0Lone-pair-electron-governed gas-recognizable flexibility in a stable MOF for boosting C3H6/C3H8 separation via aqueous scalable synthesis0Pendant group engineering to tune gate-opening pressures in flexible metal-organic frameworks for C3H6/C3H8 separation0Balancing the Selectivity and Capacity of Propylene via Synergistic Binding in A Nitro-Functionalized Metal–Organic Framework0Dinitrogen‐containing five‐membered heterocyclic porous liquids for selective separation of 1,3‐butadiene0Interconnected Pore Channels with Sieving Windows Deliver Ultrafast Propylene Purification0Multi-objective optimization of multi-stage membrane reactors considering catalyst deactivation for propane dehydrogenation0Ultra-Microporous Anion-Pillared Metal–Organic Framework with Fast Adsorption Kinetics for C3H6/C3H8 Separation0Physics‐constrained artificial intelligence for accelerating experimental discovery of MOFs in gas separation0

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