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RESEARCH PAPER · Angewandte Chemie International Edition · 2022

Subsurface Engineering Induced Fermi Level De‐pinning in Metal Oxide Semiconductors for Photoelectrochemical Water Splitting

Jun Wang, Ganghai Ni, Wanru Liao, Kang Liu, Jiawei Chen, Fangyang Liu, Zongliang Zhang, Ming Jia, Jie Li, Junwei Fu, Evangelina Pensa, Liangxing Jiang, Zhenfeng Bian, Emiliano Cortés, Min Liu

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Subsurface Engineering Induced Fermi Level De‐pinning in Metal Oxide Semiconductors for Photoelectrochemical Water SplittingOriginalSustainable catalytic strategies for the transformation of plastic wastes into valued products53Interface-Engineered Ni-Coated CdTe Heterojunction Photocathode for Enhanced Photoelectrochemical Hydrogen Evolution35Nearly 100% selective and visible-light-driven methane conversion to formaldehyde via. single-atom Cu and Wδ+154Optimizing Hot Electron Harvesting at Planar Metal–Semiconductor Interfaces with Titanium Oxynitride Thin Films15Surface Oxygen Species in Metal Oxide Photoanodes for Solar Energy Conversion10Recent Progress on Semiconductor Heterogeneous Photocatalysts in Clean Energy Production and Environmental Remediation248Tuning the surface states by in-situ Zr/Hf co-doping and MoO3 hole transport layer modification for boosting photoelectrochemical performance of hematite photoanode43The Positive Versus Negative Effects of Defect Engineering for Solar Water Splitting: A Review72ZnO quantum dots decorated TiO2 nanorod p-n heterojunction for efficient photoelectrocatalysis17Photo-induced enhanced Raman spectroscopy as a probe for photocatalytic surfaces6Suppressing Defects‐Induced Non‐Radiative Recombination for Activating the Near‐Infrared Photoactivity of Red Polymeric Carbon Nitride75Superhydrophilic CoFe Dispersion of Hydrogel Electrocatalysts for Quasi-Solid-State Photoelectrochemical Water Splitting63BiOI/AgI/Ag plasmonic heterostructure for efficient photoelectrochemical water splitting1Highly efficient visible-light-driven CdS-loaded ZnO-GaN nanowire photoanode fabricated on Si for H2 evolution16pH controlled synthesis and photoelectrochemical kinetics of bismuth molybdate (Bi2MoO6) nanoplates as photoanodes for solar-driven water splitting9Recent advances on three-dimensional ordered macroporous metal oxide-based photoelectrodes for photoelectrochemical water splitting20Bimetallic Ni–Co-ZIF derived (Ni, Co)Se2/BiVO4 heterojunction photoelectrodes with oxygen vacancy for enhancing PEC performance21Low Onset‐Potential Z‐Scheme Ta 3 N 5 ‐based Photoanode with Enhanced Light Harvesting and Charge Transport21Molecular interactions of photosystem I and ZIF-8 in bio-nanohybrid materials1Recent advanced strategies for bimetallenes toward electrocatalytic energy conversion reactions97Treasure-bowl style bifunctional site in cerium–tungsten hetero-clusters for superior solar-driven hydrogen production5Morphology-oriented urchin-like TiO2 nanostructures for enhanced photoelectrochemical water splitting1Visible self-luminous indium-based metal–organic framework for electrochemiluminescence detection of Hg2+30Unveiling the Significance of Diverse Valence State Second Dopants on Hf-Doped Fe2O3 Photoanodes for Enhanced Photoelectrochemical Water Splitting12Coupling hole-transporting polyaniline layer with a cobalt phthalocyanine cocatalyst to boost photoelectrochemical water oxidation of bismuth vanadate photoanodes4Particle‐Based Photoelectrodes for PEC Water Splitting: Concepts and Perspectives109TiO2 Thin Film Growth Research to Improve Photoelectrochemical Water Splitting Efficiency1Unveiling the promotion of dual-metal-atom Ir-Fe pair sites on charge transfer for photoelectrochemical water splitting56Rapid Surface Reconstruction of In 2 S 3 Photoanode via Flame Treatment for Enhanced Photoelectrochemical Performance29Amorphous FeSnO x Nanosheets with Hierarchical Vacancies for Room‐Temperature Sodium‐Sulfur Batteries41Amorphous FeSnOx Nanosheets with Hierarchical Vacancies for Room‐Temperature Sodium‐Sulfur Batteries2Modulating built-in electric field via Bi-VO4-Fe interfacial bridges to enhance charge separation for efficient photoelectrochemical water splitting129Au-Cu dual-single-atom sites on Bi2WO6 with oxygen vacancy for CO2 photoreduction towards multicarbon products58Photoinduced defective MIL-100-NH2 as SERS substrate with charge-transfer resonances for direct, sensitive and simultaneous detection of small-molecule biothiols11Fermi level pinning in metal oxides: influence on photocatalysis and photoelectrochemistry4Engineering Charge Separation in α-Ga 2 O 3 Nanorod Arrays for Photoelectrochemical UV Detection12Fabrication of Sb2S3@In2Se3 heterojunction photocathodes with [hk1] dominant orientation towards photoelectrochemical water splitting17Construction of core-shell W18O49@ZnIn2S4 hollow hierarchical structure for boosted photothermal-assisted photocatalytic H2 production9Uv-activated Ni ions as electron donors for in-situ generation of tunable oxygen vacancies on the surface of Bi2O2CO3 with improving photocatalytic activity for sulfadiazine degradation10Enhancement of BiVO4 photoanode surface oxygen evolution kinetics via Ni-Fe-ZIF derived bimetallic NiFeOx co-catalyst for water oxidation27Toward Efficient Utilization of Photogenerated Charge Carriers in Photoelectrochemical Systems: Engineering Strategies from the Atomic Level to Configuration109In-situ construction of bulk and surface defects to activate the near-infrared photocatalytic activity of poly(heptazine imide)20Anchoring group regulation in semiconductor/molecular complex hybrid photoelectrode for photoelectrochemical water splitting24Controllable sulfur vacancy engineering and lean-liquid system for enhanced solar-driven hydrogen evolution on metal sulfide photocatalysts3Transfer dynamics of photo-generated carriers in catalysis194Metal vacancies in semiconductor oxides enhance hole mobility for efficient photoelectrochemical water splitting154Review on the synthesis, construction and photocatalytic applications of double-ligand MOFs33Engineering strategies to minimize bubble-induced optical losses in photoelectrochemical water splitting14Revealing the new role of surface states in interfacial charge transfer at zinc ferrite photoanodes for efficient photoelectrochemical water splitting19Efficient Photogenerated Carrier‐Assisted COads Removal via Schottky Barrier of PdSn/WO3 for Formic Acid Oxidation Reaction6Electrodeposited BiVO4-based photoanodes for an energy-efficient photo-assisted CO2-to-formate conversion17Engineering high-performance BiVO4 homo- and heterojunction Photoanodes for solar-driven Photoelectrochemical water splitting applications36Recent Advances in Resistive Gas Sensors: Fundamentals, Material and Device Design, and Intelligent Applications53A Quasi Solid-State Hydrogel/InGaN Nanorod Heterostructure-Enabled Amphibious Sensor for Stable and Cross-Medium Optical Sensing and Monitoring14Oxygen Vacancy Engineering of Metal Oxide Materials for Photoelectrochemical Water Splitting22Introducing boron-doped carbon dots as a promising noble metal-free co-catalyst on g-C3N4 with enhanced band bending for photoelectrochemical water splitting7Band Structure Engineering of BiVO 4 by Copper and Sulfur Codoping for Efficient Photoelectrochemical Water Oxidation2Bioinspired Reconfigurable Vision Sensor Based on InGaN Semiconductor/Hydrogel Heterostructure for Dynamic‐Static Fusion Perception22Cobalt Hydroxide‐Organic Frameworks Powering Improved Charge Transfer and Oxygen Evolution Kinetics in Photoelectrochemical Water Splitting1Enhancing Performance of Photoanodes With a Dual‐Redox Mediator for Photoelectrocatalytic Water Splitting7A thermodynamic landscape for photocatalytic CO 2 reduction on g-C 3 N 4 : linking Fermi-level position to selectivity and activity0C as a bridge and Bi as a photothermal converter to trigger visible-light catalytic CO 2 reduction over BiOBr by in situ solid-state reduction1Design of multifunctional p-type TiO 2 /nitrogen-functionalized carbon dot hybrids for enhanced photo- and electrocatalysis1From photocorrosion to photoactivity: sulfite-gated self-etching of BiVO 4 into a black Bi–O phase1Synergy of Single-Atom Platinum and Oxygen Vacancy Engineering Boosts Photoelectrochemical Water Oxidation of ZnFe 2 O 4 Photoanodes with Surface State Reconstruction10Defect engineering and graphene quantum dot functionalization synergistically modulate charge transfer and photocurrent stability in TiO2 photoanodes1Loading-Controlled Photoactivity in TiO2@BiVO4 Heterostructures1In Situ Photoelectrochemical Chelation Programs Defect‐Resilient Coordination Microenvironments for Enhanced Water Oxidation6Cationic substitution-induced charge dynamics in Bi2MoxW1−xO6 for efficient solar driven photoelectrochemical water splitting1Breaking π Electron Network in Carbon Planes Enables Electron‐Localized NiN 4 Moieties for Efficient Electrochemical CO 2 Reduction0Defect‐Induced Band Bending Mitigation Enables Cathodic Response in Cu Single Atom Doped Faceted TiO 2 Thin Film Photoelectrodes0Defect- and Geometry-Controlled Fermi-Level Dynamics in TiO 20Arc-Synthesized FeTiO 3 : when Interfacial Charge Transfer Kinetics Controls PEC Water Oxidation0Ru–O Hybridization Strengthens Spatial Charge Separation for Enhanced Photoelectrochemical Water Oxidation0Two‐Dimensional CuTCNQ Built From Supercritical CO 2 ‐Induced Conformational Transform for Charge Transfer and Electron Modulation0

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