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RESEARCH PAPER · ACS Sustainable Chemistry & Engineering · 2022

Cyanamide as a Highly Efficient Organocatalyst for the Glycolysis Recycling of PET

Zishuai Wang, Yu Jin, Yaoqiang Wang, Zequn Tang, Shaojie Wang, Gang Xiao, Haijia Su

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Cyanamide as a Highly Efficient Organocatalyst for the Glycolysis Recycling of PETOriginalEfficient glycolysis of recycling poly(ethylene terephthalate) via combination of organocatalyst and metal salt46Recent Advances in the Chemobiological Upcycling of Polyethylene Terephthalate (PET) into Value-Added Chemicals47Recycling of polyethylene terephthalate (PET Or PETE) plastics – An alternative to obtain value added products: A review80Biodegradation of poly(ethylene terephthalate): Mechanistic insights, advances, and future innovative strategies122Co-Al-CO 3 layered double hydroxide: an efficient and regenerable catalyst for glycolysis of polyethylene terephthalate24Chemical recycling of multi-materials from glycol-modified poly(ethylene terephthalate)25Designed for Circularity: Chemically Recyclable and Enzymatically Degradable Biorenewable Schiff Base Polyester-Imines24Mechanistic Insights of Cosolvent Efficient Enhancement of PET Methanol Alcohololysis58Controlling PET oligomers vs monomers via microwave-induced heating and swelling49Comparsion of Catalyst Effectiveness in Different Chemical Depolymerization Methods of Poly(ethylene terephthalate)43Circularizing PET-G Multimaterials: Life Cycle Assessment and Techno-Economic Analysis24Ligand-Aided Glycolysis of PET Using Functionalized Silica-Supported Fe 2 O 3 Nanoparticles27Synergistic catalysis of ionic liquids and metal salts for facile PET glycolysis44Computational design of highly efficient thermostable MHET hydrolases and dual enzyme system for PET recycling74Synthesis of bis(2-ethylhexyl) terephthalate from waste poly(ethylene terephthalate) catalyzed by tin catalysts9The controllable and efficient synthesis of two-dimensional metal–organic framework nanosheets for heterogeneous catalysis9Monomer recycling of polyethylene terephthalate, polycarbonate and polyethers: Scalable processes to achieve high carbon circularity62Catalytic recycling of PET waste bottles into a value-added amide monomer using a heterogeneous niobium pentoxide nanocatalyst12Efficient glycolysis of used PET bottles into a high-quality valuable monomer using a shape-engineered MnO x nanocatalyst27From trash to cash: current strategies for bio-upcycling of recaptured monomeric building blocks from poly(ethylene terephthalate) (PET) waste57Highly Efficient Kilogram-Scale Mechanochemical Catalytic Depolymerization of Pet Polyester Waste into Reusable Monomers0Recycle waste PET yarn on site by feeding waste yarn as grinded powder to improve product quality, increase energy efficiency and reduce environmental impact1Recycling and depolymerisation of poly(ethylene terephthalate): a review43Upcycling of waste polyesters for the development of a circular economy36Using waste to treat waste: efficient alcoholysis of PET waste with a shrimp shell derived catalyst using the response surface method4Hydrogenation of waste PET degraded bis(2-hydroxyethyl)cyclohexane- 1,4-dicarboxylate to 1,4-cyclohexanedimethanol over Cu-based catalysts15Recycling and high-value utilization of polyethylene terephthalate wastes: A review90Depolymerization within a Circular Plastics System387Polyethylene terephthalate (PET) recycling: A review355Polymeric Carbon Nitride Nanosheets as a Metal‐Free Heterogeneous Catalyst for Highly Efficient Methanolysis of Polycarbonates14Theoretical insights into chemical recycling of polyethylene terephthalate (PET)108Textile production by additive manufacturing and textile waste recycling: a review71Integrating glycolysis and enzymatic catalyst to convert waste poly(ethylene terephthalate) into terephthalic acid7Optimization of Ti-PA efficiently catalytic the alcoholysis of waste PET using response surface methodology7The Recyclable Dual-Functional Zeolite Nanocrystals Promoting the High Efficiency Glycolysis of PET15Recent advances in the chemical recycling of polyesters44Green Catalytic Ionic Liquids Containing Organophosphorus for Efficient Glycolysis of Waste PET Bottle Flakes14A review on sustainable PET recycling: Strategies and trends55Sustainable and Renewable Microcross-Linked Polyurethane Pressure-Sensitive Adhesive from Waste Polyethylene Terephthalate10Rapid and Metal-Free Green Synthesis of Coumarins Catalyzed by Humic Acid2Converting Waste Polyethylene Terephthalate to High Value Monomers by Synergistic Catalysts14Highly efficient kilogram-scale mechanochemical catalytic depolymerization of PET polyester waste into reusable monomers23Circular Economy and Chemical Conversion for Polyester Wastes23Low-temperature chemical upcycling of poly(ethylene terephthalate) waste to recyclable polyurethane thermosets using biomass-derived materials18Depolymerization of waste poly(ethylene terephthalate) into bis(2-hydroxyethyl) terephthalate: Catalytic glycolysis mechanism and kinetics14Using waste to treat waste: Catalysts from spent alkaline batteries for glycolysis of PET waste13Magnetically recyclable CoFe2O4 nanocatalysts for efficient glycolysis of polyethylene terephthalate12Modular chem‐bio upcycling of waste poly(ethylene terephthalate) to glycolic acid and 2,4‐pyridine dicarboxylic acid15Development of Glycolysis Catalysts for PET Wastes Including Polyester Textiles32A sustainable framework for advancing circular practices for polyethylene terephthalate textiles: optimized recycling of depolymerization byproducts and LCA validation8Circular plastic economy for sustainable development: current advances and future perspectives49Insights into 1-ethyl 3-methyl imidazolium dicyanamide-catalysed glycolysis of polyethylene terephthalate1Magnetically recoverable cobalt oxide nanoparticle catalyst for PET glycolysis2Morphology-tuned MnO x /TiO 2 nanocatalysts for recycling PET plastic waste using biomass-derived ethylene glycol15Solvent-promoted catalyst-free aminolytic upcycling of waste polyethylene terephthalate under low-temperature conditions11Glycolysis of poly (ethylene terephthalate) using DBU-based ionic liquid catalysts9Recyclable Zinc Cyanamide Dual-Site Catalyst Enables Efficient PET Glycolysis11Enhancing sustainability in PET glycolysis by closed-loop recycling12Recent Advances and Applications of NMR Techniques in Plastic Characterizations19Efficient synergistic enhancing degradation of waste poly(ethylene terephthalate) by combination of DBU with zinc 2-ethylhexanoate3Upcycling of Waste Plastics into Value-Added Chemicals6From waste to wealth: Glycolysis of PET for high-value resource utilization24Metal Synergistic Dual Activation Enables Efficient Transesterification by Multinuclear Titanium Catalyst: Recycling and Upcycling of Polyester Waste25Metal Synergistic Dual Activation Enables Efficient Transesterification by Multinuclear Titanium Catalyst: Recycling and Upcycling of Polyester Waste7Biochar-based catalytic upgrading of plastic waste into liquid fuels towards sustainability34Chemical recycling of waste polyester plastics1γ-Valerolactone-Enabled Mild Methanolysis of Waste Polyethylene Terephthalate for Efficient Chemical Recycling6Computational study of poly(ethylene terephthalate) glycolysis catalyzed by cyanamide0Strategies for Electrochemical Recycling of Plastic Polyethylene Terephthalate‐Derived Ethylene Glycol Into High‐Value Chemicals59Integrated Chemical Upcycling of Poly(ethylene terephthalate) Waste to Multiple Value-Added Products Catalyzed by Ni2P Supported on SiO2: From Trash-to-Treasure14A Spectroscopic and Theoretical Calculation Study on Mechanistic Insights into Glycolysis of Polyethylene Terephthalate Catalyzed by 1, 5-Diazabicyclo [4.3.0]-5-nonene2Constructing frustrated Lewis pairs on defect-engineered biphasic catalysts for polyester depolymerization12Highly Efficient, Co-solvent Assisted Glycolytic Depolymerization of Waste Polyethylene Terephthalate (PET) into Bis(2-hydroxyethyl) Terephthalate (BHET) Monomer12Chemo-catalytic recycling of PET waste: Progress and prospects for circular economy and valorization6Efficient chemical recycling of mixed plastics by intramolecular glycolysis13Towards the next development of vitrimers: Recent key topics for the practical application and understanding of the fundamental physics46Depolymerization of polyesters catalyzed by binuclear metal complexes0Regeneration of polyester from waste polyester-spandex textiles by ethylene glycolysis0Catalyst of a Mytilus galloprovincialis shell substrate: optimization of alcoholysis conditions for the catalytic depolymerization of waste polyester films0Closed-loop recycling of polyesters through glycolysis using catalytic deep eutectic solvents and the influence of glycol types on reaction kinetics4Highly efficient glycolic acid electrosynthesis from waste ethylene glycol on layered mesoporous Pd 2 Ni alloy0Unveiling the Molecular-level Mechanism of Water-Induced Deactivation in TBD-Catalyzed PET Glycolysis0Tunable ether-functionalized protic ionic liquid for efficient glycolysis of polyethylene terephthalate5Advances in Polyester Waste Recycling Technology: Focused on the PET System and Prospects for PETG Challenges2A Sustainable Circular Route for PET LDH Nanocomposites: Catalyst-Driven Polymerization and Depolymerization for a BHET-to-BHET Cycle2Toward Green Manufacturing of Low-Cost, Robust Unsaturated Polyester Resin from Waste PET Glycolysis Products0Optimizing toward Discovery: AI-Driven Exploration of Lewis Acid–Base Catalysts for PET Glycolysis16Frustrated Lewis Pairs‐Engineered Boron‐Doped Carbon Nitride: An Efficient Metal‐Free Catalyst for the Depolymerization of Polyethylene Terephthalate3Efficient Glycolysis of Waste PET at Room Temperature Enabled by a Bifunctional Catalyst System and Co-solvent5Synergistic Barium–Oxygen Vacancy Catalysis Engineered with MWW Zeolites for Efficient PET Glycolytic Depolymerization10Process intensification and techno-economic analysis of ethylene glycol recovery from PET glycolysis: a comparative evaluation of distillation configurations0Efficient Recycling of Polyethylene Terephthalate by Ultrasmall ZnFe 2 O 4 Nanoparticles1Recent advances in the glycolysis of poly(ethylene terephthalate)1Mechanistic Insights on Fe(II)‐Catalyzed Depolymerization of Poly(Ethylene Terephthalate) by Transesterification0Chemical Recycling as a Tool for Enabling a Second Life for Polyesters0Low‐temperature transesterification strategy for universal upcycling of waste polyesters into high‐value esters1Sustainable production of allylic monomers for dental applications using post-industrial PET as raw material0Boosting cascade PET glycolysis by exposing coordinatively unsaturated Zn sites within open nanopores for efficient BHET recovery0Activation barriers in the glycolysis of PET as catalyzed by tertiary amines: Density functional calculations and predictions from interpretable machine learning0Structure Designed Methylpiperidine Ionic Liquids for Efficient and Recyclable PET Glycolysis0Mechanistic insights into zinc acetate dihydrate–catalyzed depolymerization of recycled PET for polyol production: a combined experimental and DFT study0Cooperative Dual-Site Hydrogen-Bonding Organocatalysis for Efficient Metal-Free PET Glycolysis0

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  3. Recycling of polyethylene terephthalate (PET Or PETE) plastics – An alternative to obtain value added products: A review

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  50. A sustainable framework for advancing circular practices for polyethylene terephthalate textiles: optimized recycling of depolymerization byproducts and LCA validation

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