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RESEARCH PAPER · Journal of Materials Chemistry A · 2022

Tailoring the selectivity and activity of oxygen reduction by regulating the coordination environments of carbon-supported atomically dispersed metal sites

Pan Zhu, Pengyu Song, Wuyi Feng, Di Zhao, Ting Liu, Jiatao Zhang, Chen Chen

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Tailoring the selectivity and activity of oxygen reduction by regulating the coordination environments of carbon-supported atomically dispersed metal sitesOriginalDefect-stabilized and oxygen-coordinated iron single-atom sites facilitate hydrogen peroxide electrosynthesis28Influence of coordination structure of Fe-585DV/N x C 4− x on the electrocatalytic performance of oxygen reduction reactions4Molecular design and coordination regulation of atomically dispersed bi-functional catalysts for oxygen electrocatalysis17Synergistic enhancement of hydrogen interactions in palladium–silicon–gold metallic glass with multilayered graphene1Challenges and Perspectives of Single-Atom-Based Catalysts for Electrochemical Reactions175Engineering the First Coordination Shell of Single Zn Atoms via Molecular Design Strategy toward High‐Performance Sodium‐Ion Hybrid Capacitors48Selective Oxidation of CH4 to CH3OH by Transition-Metal Single-Atom-Embedded N-Doped Graphene Catalysts with Oxidants N2O and O2: Oxygen Adsorption Energy as an Activity Descriptor7Active sites identification and engineering of M-N-C electrocatalysts toward oxygen reduction reaction50Single-atom catalysts for the photocatalytic and electrocatalytic synthesis of hydrogen peroxide42Enhancing Hydrogen Peroxide Synthesis through Coordination Engineering of Single-Atom Catalysts in the Oxygen Reduction Reaction: A Review3Surface-optimized carbon nanocages with tailorable atomic Fe-N4 sites to boost oxygen reduction in long stable zinc-air battery51Precise Design and Modification Engineering of Single‐Atom Catalytic Materials for Oxygen Reduction23Edge engineering of carbon nitride for enhanced sacrificial agent-free photocatalytic H2O2 evolution17Microenvironment regulation strategies of single-atom catalysts for advanced electrocatalytic CO2 reduction to CO72Atomic-level functionalized carbon-based materials for effective electrosynthesis of hydrogen peroxide: A review31High-efficiency oxygen reduction by late transition metal oxides to produce H 2 O 270Influence of surface terminal groups on the efficiency of two-electron oxygen reduction reaction catalyzed by iron single atoms on Ti 3 C 2 T x (T = Cl, Br, NH) MXene16Sulfur-assisted ammonia treatment of a fibrous carbon matrix to fabricate a high-content pyrrole-type Fe–N–C catalyst for superior oxygen reduction7Electronic structure regulation of the Fe-based single-atom catalysts for oxygen electrocatalysis106Electronegativity Matching of Asymmetrically Coordinated Single‐Atom Catalysts for High‐Performance Lithium–Sulfur Batteries93Highly Efficient Electrosynthesis of Glycine over an Atomically Dispersed Iron Catalyst138Theoretical insights on 3D transition metal anchored poly[5,10,15,20-tetra(4-ethynylphenyl)porphyrin]diyne as highly efficient bifunctional catalyst toward ORR and OER2Nitrogen, sulfur co-coordinated iron single-atom catalysts with the optimized electronic structure for highly efficient oxygen reduction in Zn-air battery and fuel cell16Activity Origin and Catalytic Mechanism of the M–N–C Catalysts for the Oxygen Reduction Reaction43Cathodic Electrosynthesis of H2O2 Using Sustainable Cellulose‐Co‐ZIF Electrocatalyst0In-depth understanding the synergisms of Cu atomic clusters on Cu single atoms for highly effective electrocatalytic oxygen reduction reaction and Zn-Air battery12Atomic‐Level Synergistic Catalysts: Single‐Atom Site Integrated with Atom, Cluster and Nanoparticle14Porous Carbon‐Supported Catalysts for Proton Exchange Membrane Fuel Cells13Modulating the Local Coordination Environment of M‐N x Single‐Atom Site for Enhanced Electrocatalytic Oxygen Reduction78In situ self-grown synthesis of c-MOF@NiO heterostructure anchored to c-MOF/rGA particle electrode: Promoting sustained and efficient degradation of phenol in coking wastewater22Applications of metal oxides in two-electron oxygen reduction reaction electrocatalysis0Rational design of two-electron oxygen-reduction electrocatalysts for H 2 O 2 production and their in situ integration with oxidation reactions in green chemical processes9Sulfonic Acid Group-Reinforced Polyzwitterionic Hydrogel Electrolytes for High-Voltage, Dendrite-Free Zinc-Ion Hybrid Supercapacitors0Bioinspired Molecular Catalyst for Photocatalytic Semihydrogenation of Acetylene with Water as a Proton Source11Atomistic Electrocatalysts for Modulating the Oxygen Reduction Reaction Selectivity in Carbon-Based Materials: Active-Site Engineering, Local Environment, and Magnetism5Regulating Zinc‐Based Compounds with Oxygen Group Elements for Electrosynthesis of Hydrogen Peroxide in Neutral Media3Unveiling the cutting-edge innovations in single atom catalysts: Preparation, mechanism, performance, and applications7Identifying In Situ Activity and Selectivity of Oxygen Reduction Catalysts at the Subparticle Level13Macro-to-micro level modulation of MOF-derived Fe single-atom catalysts with CNT for high-performance Zn–air batteries18Intermediate-spin Fe(III)-N4 sites embedded in FeNi/Fe2P@CNT on nanocarbon architectures as a bifunctional catalyst for advanced zinc-air batteries14Advancing catalyst design for H₂O₂ electrosynthesis via oxygen reduction reaction9Challenges and performance optimization strategies of carbon-based transition metal single-atom catalysts derived from ZIF-8 for oxygen reduction reaction: Active site regulation, 3D structural engineering, and interfacial function design1Optimum hydrogen binding energy at the atomic-level interfaces of Rh atoms/ultrasmall Rh nanoparticles for boosting hydrogen electrocatalysis6Carbon-encapsulated Fe/Fe3C nanoparticles combined with Fe-N4 sites as efficient four electron oxygen reduction catalysts1A cost-effective Fe–Cu–Cr oxide/activated-carbon catalyst for peroxymonosulfate-driven degradation of p -nitrophenol2Green and sustainable Metal–Nitrogen–Carbon (M−N−C) electrocatalysts for oxygen reduction in PEM fuel cells: structure–property relationships and design strategies0Theoretical Insights into Metal-Fe@NC Dual-Atom Catalysts for Oxygen Reduction Reaction3Single-Atom Supports: Versatile Platforms for Regulating Electrocatalysts at the Atomic Level4Tailoring Cu Nanoparticles Motif Into Atomic‐Level Sites for Efficient H 2 O 2 Electrosynthesis0Synergistic Mo doping of Ni3S2 for accelerated high-valent Ni3 + formation and proton-coupled electron transfer in efficient biomass conversion0Sulfonic acid group-reinforced polyionic hydrogel electrolytes for high-voltage, dendrite-free zinc-ion hybrid supercapacitors1Constructing a “switch” for photo-thermal catalytic pathway: Directional regulation of NO reduction product distribution by the coordination mode at the La site over Pd–La/CeO20

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  1. Defect-stabilized and oxygen-coordinated iron single-atom sites facilitate hydrogen peroxide electrosynthesis

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  2. Influence of coordination structure of Fe-585DV/N x C 4− x on the electrocatalytic performance of oxygen reduction reactions

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    Ren Li, Lei Zhang, Yi Wang, Jinbo Bai, Xiaolin Li, Chunmei Zhang

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  3. Molecular design and coordination regulation of atomically dispersed bi-functional catalysts for oxygen electrocatalysis

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  4. Synergistic enhancement of hydrogen interactions in palladium–silicon–gold metallic glass with multilayered graphene

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  5. Challenges and Perspectives of Single-Atom-Based Catalysts for Electrochemical Reactions

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  6. Engineering the First Coordination Shell of Single Zn Atoms via Molecular Design Strategy toward High‐Performance Sodium‐Ion Hybrid Capacitors

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  7. Selective Oxidation of CH4 to CH3OH by Transition-Metal Single-Atom-Embedded N-Doped Graphene Catalysts with Oxidants N2O and O2: Oxygen Adsorption Energy as an Activity Descriptor

    The Journal of Physical Chemistry C · 2023-03-17

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  8. Active sites identification and engineering of M-N-C electrocatalysts toward oxygen reduction reaction

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  9. Single-atom catalysts for the photocatalytic and electrocatalytic synthesis of hydrogen peroxide

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  10. Enhancing Hydrogen Peroxide Synthesis through Coordination Engineering of Single-Atom Catalysts in the Oxygen Reduction Reaction: A Review

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  11. Surface-optimized carbon nanocages with tailorable atomic Fe-N4 sites to boost oxygen reduction in long stable zinc-air battery

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  12. Precise Design and Modification Engineering of Single‐Atom Catalytic Materials for Oxygen Reduction

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  13. Edge engineering of carbon nitride for enhanced sacrificial agent-free photocatalytic H2O2 evolution

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  14. Microenvironment regulation strategies of single-atom catalysts for advanced electrocatalytic CO2 reduction to CO

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  15. Atomic-level functionalized carbon-based materials for effective electrosynthesis of hydrogen peroxide: A review

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  16. High-efficiency oxygen reduction by late transition metal oxides to produce H 2 O 2

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  17. Influence of surface terminal groups on the efficiency of two-electron oxygen reduction reaction catalyzed by iron single atoms on Ti 3 C 2 T x (T = Cl, Br, NH) MXene

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  18. Sulfur-assisted ammonia treatment of a fibrous carbon matrix to fabricate a high-content pyrrole-type Fe–N–C catalyst for superior oxygen reduction

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  19. Electronic structure regulation of the Fe-based single-atom catalysts for oxygen electrocatalysis

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  20. Electronegativity Matching of Asymmetrically Coordinated Single‐Atom Catalysts for High‐Performance Lithium–Sulfur Batteries

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  21. Highly Efficient Electrosynthesis of Glycine over an Atomically Dispersed Iron Catalyst

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  22. Theoretical insights on 3D transition metal anchored poly[5,10,15,20-tetra(4-ethynylphenyl)porphyrin]diyne as highly efficient bifunctional catalyst toward ORR and OER

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  24. Activity Origin and Catalytic Mechanism of the M–N–C Catalysts for the Oxygen Reduction Reaction

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  25. Cathodic Electrosynthesis of H2O2 Using Sustainable Cellulose‐Co‐ZIF Electrocatalyst

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  31. Applications of metal oxides in two-electron oxygen reduction reaction electrocatalysis

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