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RESEARCH PAPER · Nature Communications · 2022

Filming movies of attosecond charge migration in single molecules with high harmonic spectroscopy

Lixin He, Siqi Sun, Pengfei Lan, Yanqing He, Bincheng Wang, Pu Perry Wang, Xiaosong Zhu, Liang Li, Wei Cao, Peixiang Lu, C. D. Lin

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Filming movies of attosecond charge migration in single molecules with high harmonic spectroscopyOriginalGeneration of waveform-tunable unipolar pulses in a nonlinear resonant medium30Comparative study of medium length-dependent high-harmonic generation from metal ions9Attosecond spectroscopy for filming the ultrafast movies of atoms, molecules and solids15Development of attosecond pulses and their application to ultrafast dynamics of atoms and molecules4Measurement of molecular alignment with deep learning-based M-XFROG technique [Invited]2Untitled work0气体高次谐波产生中的角动量守恒4Dynamical analysis of attosecond molecular modes7Modeling the sequential dissociative double ionization of O2 by ultrashort intense infrared laser pulses9Attochemistry Regulation of Charge Migration23Iterative projection algorithm for retrieval of angle-resolved single-molecule dipoles from high-harmonic spectra6Attosecond probing and control of charge migration in carbon-chain molecule1Extension of high-order harmonic generation cutoff from laser-ablated tin plasma plumes13Topical Review: Extracting molecular frame photoionization dynamics from experimental data4Comparative study of optical nonlinearities of CO 2 and N 2 O via single-shot spatio-temporally-resolved visualization2Manipulating Attosecond Charge Migration in Molecules by Optical Cavities12Role of excited states in helium-like ions on high-order harmonic generation1High-harmonic-generation spectra of HCN: A time-dependent density-functional-theory study6Attosecond charge migration in heterocyclic five-membered rings6Universality in odd-even harmonic generation and application in terahertz waveform sampling9Area theorem in a ring laser cavity8Time-dependent variational approach to solve multi-dimensional time-dependent Schrödinger equation1High harmonic generation in solids: particle and wave perspectives35Attosecond probing and control of charge migration in carbon-chain molecule32Coherence from multiorbital tunneling ionization of molecules15Role of Inner Molecular Orbitals in High-Harmonic Generation Spectra of Aligned Uracil15Controlling polarization of high-order harmonics generated in the mixed gases with orthogonal two-color laser fields7Nobel de physique : qu’est-ce qu’une attoseconde ?0What is an attosecond? A physical chemist explains the tiny time scale behind Nobel Prize-winning research0From transformations to the notion of time1Strong Laser Field-Driven Coupled Electron–Nuclear Dynamics: Quantum vs Classical Description3Molecular orbital tomography of HOMO and HOMO-1 of the nonlinear molecule H2O: The study on multi-orbital effects15Coherent control of a multilevel resonant medium by subcycle pulses11From transformations to the notion of time1Spatially resolved macroscopic near-threshold harmonics generated from harmoniclike and resonant transitions using an artificial neural network7Jellyfish: A modular code for wave function‐based electron dynamics simulations and visualizations on traditional and quantum compute architectures2Effects of polarization direction, amplitude, and photon energy of linearly polarized laser on high order harmonic generation of C600Robustness of attosecond molecular modes under nuclear dynamics1Probing the electron motion in molecules using forward-scattering photoelectron holography2Introduction of the year 20220High-harmonic spectroscopy of impulsively aligned 1,3-cyclohexadiene: Signatures of attosecond charge migration5单个阿秒脉冲表征技术研究进展1高平均功率高次谐波光源的研究进展（特邀）0Enhancement of High-Order Harmonic Generation in Low-Density Ti Plasma Plumes Induced by Intense Laser Fields4Tracking Charge Migration with Frequency-Matched Strobo-Spectroscopy7Probing vibronic coherence in charge migration in molecules using strong-field sequential double ionization10Electron-wave-packet-deformation–induced attosecond emission time shift in gas high-order harmonic generation3Double-blind decoupling of molecular rotation and high-order harmonic generation with a neural network5High-Harmonic Generation Spectroscopy of Gas-Phase Bromoform9Comparative study of enhancement and suppression of N2+ lasing induced by coherent molecular rotational wave packets of N2 and N2+1SLIMP 2.0: A new version of strong laser interaction model package for atoms and molecules, now with molecular orbital tomography based on high-order harmonic spectra3Effect of molecular alignment and orientation on elliptically polarized high-order harmonic generation10From Transformations to the Notion of Time0Ultrafast Picometer-Resolved Molecular Structure Imaging by Laser-Induced High-Order Harmonics17Efficient Control of Electron Localization and Probability Modulation with Synthesized Two-Color Intense Laser Pulses1Analytically controlling the laser-induced electron phase in sub-cycle motion8Investigating wavelength dependence of near-threshold harmonics with different atoms and laser intensities: from analysis of an expanded quantum trajectory Monte Carlo model2Controlling the generation of elliptically polarized isolated attosecond pulses from mixed gases with a polarization-gating technique13Bloch-Wave Phase Matching of High Harmonic Generation in Solids12Dynamical channel coupling in strong-field ionization of CO 25Elliptically polarized high-order harmonic generation from N 2 -CO mixed gases5Quantum chemistry challenges the continuum : high harmonic generation and photoionization for atoms and molecules0Time-dependent ab initio molecular-orbital decomposition for high-harmonic generation spectroscopy7Research progress on ultrafast electron dynamics in solids0Electron dynamical phase difference and high-order harmonic frequency shift: A Bohmian-trajectory perspective4Control of attosecond-pulse helicity and ellipticity by the ionization-gating technique3Ionization and recombination times of high-order harmonic generation with single-photon ionization1Polarization Control in High Harmonic Generation Using Molecular Structures in Nonaligned Molecules13Strong-field ionization with few-cycle, midinfrared laser pulses inducing a localized ionization followed by long-lasting charge migration in halogenated organic molecules6THz-assisted population inversion in strong-field excitation0Generation of Fourier-limited ultrashort soft X-ray isolated attosecond pulses by two-color chirped lasers without chirp compensation3Phase-space Gaussian quantum ensemble for high-order harmonic generation3High-order harmonic generation in the vanadium monoanion and its hexacarbonyl complex0Revisiting the measurement of a quantum mechanical experiment by an Ehrenfest theorem-based Fourier Transformation0Quantitative comparison of high-order harmonic yields in ring-shaped organic molecules calculated using time-dependent density-functional theory3Optimal control of redshift of high-order harmonic in two-color laser fields0Machine-learning-constructed molecular potential and its application for exploring deep-lying-orbital effects in high-order harmonic generation5Time-dependent hole states in multiconfigurational time-dependent Hartree-Fock approaches: Applications in photoionization of water molecule0The Effect of Core-Hole Shape on Attosecond Valence Electron Dynamics0Molecular Wave Plate for the Control of Ultrashort Pulses Carrying Orbital Angular Momentum2Generation of isolated elliptically polarized sub-100-as pulses from Ne atoms in combined chirped fields0Optical interference effect in strong-field electronic coherence spectroscopy1Quantum path control in high-order harmonic generation via squeezed light3Effects of laser parameters on orbital competition in high-order harmonic generation from a hydrogen cyanide molecule1Complete suppression of the nondipole drift effect in high-order harmonic generation1Correlation-induced phase shifts and time delays in resonance-enhanced high-harmonic generation0Structural and dynamical phase jumps in molecular high harmonic spectroscopy0Time-Dependent Hole States in Multiconfigurational Time-Dependent Hartree-Fock Approaches: A Time-Domain Generalization of Extended Koopmans’ Theorem1Single-frame randomized probe imaging in the EUV using a high-order harmonic source1人工智能在高次谐波模拟与预测中的研究进展（特邀）0阿秒啁啾补偿及无啁啾孤立阿秒脉冲的产生（特邀）0高次谐波时空耦合特性对阿秒时间分辨测量精度的影响（特邀）0Macroscopic aspects of the laser-wavelength-dependent spectral minimum in high-order harmonic generation from aligned CO 2 molecules1Two-dimensional electron dynamics reconstructed by polarization-resolved high harmonic spectroscopy0Enhancement of Vacuum-Ultraviolet Laser Generation through Near-Threshold Harmonics Driven by a Few-Cycle Two-Color Laser Field0Light symmetry, chirality, and their role in nonlinear optics and ultrafast phenomena5Optical Field Control of Ultrafast Dynamics in Complex Systems: Frontiers and Perspectives1Bright XUV pulses with spin-orbital angular momentum control via laser-plasma mirror interaction0Nonadiabatic theory for subcycle ionic dynamics in multielectron tunneling ionization0High-fidelity surrogate modeling of high-harmonic generation using Fourier neural operator with high-frequency weighted loss0Theoretical exploration of photoelectron momentum distribution and ultrafast magnetic-field generation in N 2 molecules by an extreme-ultraviolet laser field0Coulomb-corrected reconstruction of ionization and recombination times in high-order harmonic generation with orthogonally polarized two-color fields0Resonance-enhanced high-harmonic generation and attosecond transient absorption spectroscopy of hydrogen atoms0Quantum Trajectory Separation and Attosecond Mapping in Liquid High-Harmonic Generation1Exciton-induced frequency shift in high-harmonic generation from solids0Toward ultimate attosecond light sources with ultrashort duration and high flux0The decoherence and recoherence of charge migration in ionized 1-iodo-1,3-butadiyne0Moderate-terahertz-induced plateau expansion of high-order harmonic generation to the soft-x-ray region0Entanglement and nonclassicality of harmonic modes in solid-state high-harmonic generation0

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  2. Comparative study of medium length-dependent high-harmonic generation from metal ions

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  3. Attosecond spectroscopy for filming the ultrafast movies of atoms, molecules and solids

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  4. Development of attosecond pulses and their application to ultrafast dynamics of atoms and molecules

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  5. Measurement of molecular alignment with deep learning-based M-XFROG technique [Invited]

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  7. 气体高次谐波产生中的角动量守恒

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  8. Dynamical analysis of attosecond molecular modes

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  9. Modeling the sequential dissociative double ionization of O2 by ultrashort intense infrared laser pulses

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  10. Attochemistry Regulation of Charge Migration

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  11. Iterative projection algorithm for retrieval of angle-resolved single-molecule dipoles from high-harmonic spectra

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  12. Attosecond probing and control of charge migration in carbon-chain molecule

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  14. Topical Review: Extracting molecular frame photoionization dynamics from experimental data

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  15. Comparative study of optical nonlinearities of CO 2 and N 2 O via single-shot spatio-temporally-resolved visualization

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  16. Manipulating Attosecond Charge Migration in Molecules by Optical Cavities

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  17. Role of excited states in helium-like ions on high-order harmonic generation

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  18. High-harmonic-generation spectra of HCN: A time-dependent density-functional-theory study

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  19. Attosecond charge migration in heterocyclic five-membered rings

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  20. Universality in odd-even harmonic generation and application in terahertz waveform sampling

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  21. Area theorem in a ring laser cavity

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  22. Time-dependent variational approach to solve multi-dimensional time-dependent Schrödinger equation

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  24. Attosecond probing and control of charge migration in carbon-chain molecule

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  25. Coherence from multiorbital tunneling ionization of molecules

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  26. Role of Inner Molecular Orbitals in High-Harmonic Generation Spectra of Aligned Uracil

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  29. What is an attosecond? A physical chemist explains the tiny time scale behind Nobel Prize-winning research

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  30. From transformations to the notion of time

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  32. Molecular orbital tomography of HOMO and HOMO-1 of the nonlinear molecule H2O: The study on multi-orbital effects

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  38. Robustness of attosecond molecular modes under nuclear dynamics

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  39. Probing the electron motion in molecules using forward-scattering photoelectron holography

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  41. High-harmonic spectroscopy of impulsively aligned 1,3-cyclohexadiene: Signatures of attosecond charge migration

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  44. Enhancement of High-Order Harmonic Generation in Low-Density Ti Plasma Plumes Induced by Intense Laser Fields

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  45. Tracking Charge Migration with Frequency-Matched Strobo-Spectroscopy

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  46. Probing vibronic coherence in charge migration in molecules using strong-field sequential double ionization

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  49. High-Harmonic Generation Spectroscopy of Gas-Phase Bromoform

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  50. Comparative study of enhancement and suppression of N2+ lasing induced by coherent molecular rotational wave packets of N2 and N2+

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