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RESEARCH PAPER · Chemical Reviews · 2022

Renewed Prospects for Organic Photovoltaics

Guichuan Zhang, Francis R. Lin, Qi Feng, Thomas Heumueller, Andreas Distler, Hans‐Joachim Egelhaaf, Ning Li, Philip C. Y. Chow, Christoph Josef Brabec, Alex K.‐Y. Jen, Hin‐Lap Yip

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Renewed Prospects for Organic PhotovoltaicsOriginalA structurally simple linear conjugated polymer toward practical application of organic solar cells65Wide Band‐Gap Polymer Donors Functionalized with Unconventional Carbamate Side Chains for Polymer Solar Cells44Recent progress in non-fused ring electron acceptors for high performance organic solar cells90A Versatile and Low‐Cost Polymer Donor Based on 4‐Chlorothiazole for Highly Efficient Polymer Solar Cells65Ternary All‐Polymer Solar Cells with Efficiency up to 18.14% Employing a Two‐Step Sequential Deposition92Unsymmetrically Chlorinated Non‐Fused Electron Acceptor Leads to High‐Efficiency and Stable Organic Solar Cells109Non‐Fused Ring Acceptors Achieving over 15.6% Efficiency Organic Solar Cell by Long Exciton Diffusion Length of Alloy‐Like Phase and Vertical Phase Separation Induced by Hole Transport Layer76A 2.20 eV Bandgap Polymer Donor for Efficient Colorful Semitransparent Organic Solar Cells5818.73% efficient and stable inverted organic photovoltaics featuring a hybrid hole-extraction layer503D acceptors with multiple A–D–A architectures for highly efficient organic solar cells146A 19% efficient and stable organic photovoltaic device enabled by a guest nonfullerene acceptor with fibril-like morphology152Aggregation behaviour of pyrene-based luminescent materials, from molecular design and optical properties to application382Machine-learning-guided prediction of photovoltaic performance of non-fullerene organic solar cells using novel molecular and structural descriptors51Refined molecular microstructure and optimized carrier management of multicomponent organic photovoltaics toward 19.3% certified efficiency112Selective halogenation of central and end-units of nonfullerene acceptors enables enhanced molecular packing and photovoltaic performance78Side-chain engineering of nonfullerene small-molecule acceptors for organic solar cells132Stable block copolymer single-material organic solar cells: progress and perspective70Y‐Type Non‐Fullerene Acceptors with Outer Branched Side Chains and Inner Cyclohexane Side Chains for 19.36% Efficiency Polymer Solar Cells199Real‐Time Probing and Unraveling the Morphology Formation of Blade‐Coated Ternary Nonfullerene Organic Photovoltaics with In Situ X‐Ray Scattering60Sequential Deposition of Multicomponent Bulk Heterojunctions Increases Efficiency of Organic Solar Cells187Understanding the Thickness and Light-Intensity Dependent Performance of Green-Solvent Processed Organic Solar Cells54BN‐Bond‐Embedded Triplet Terpolymers with Small Singlet–Triplet Energy Gaps for Suppressing Non‐Radiative Recombination and Improving Blend Morphology in Organic Solar Cells77Prospects and challenges for perovskite-organic tandem solar cells135Compromising Charge Generation and Recombination of Organic Photovoltaics with Mixed Diluent Strategy for Certified 19.4% Efficiency320Interface Engineering for Highly Efficient Organic Solar Cells325Benzo[1,2‐b:4,5‐b′]Difuran‐Based Polymer for Organic Solar Cells with 17.5% Efficiency via Halogenation‐Mediated Aggregation Control62Benzo[d]thiazole Based Wide Bandgap Donor Polymers Enable 19.54% Efficiency Organic Solar Cells Along with Desirable Batch‐to‐Batch Reproducibility and General Applicability197Correlation of Local Isomerization Induced Lateral and Terminal Torsions with Performance and Stability of Organic Photovoltaics92High‐Efficiency All‐Small‐Molecule Organic Solar Cells Based on New Molecule Donors with Conjugated Symmetric/Asymmetric Hybrid Cyclopentyl‐Hexyl Side Chains64Dimer Acceptor Adopting a Flexible Linker for Efficient and Durable Organic Solar Cells141Development and application of blade-coating technique in organic solar cells41High‐Performance Small Molecule Organic Solar Cells Enabled by a Symmetric‐Asymmetric Alloy Acceptor with a Broad Composition Tolerance110Diazabicyclic Electroactive Ionenes for Efficient and Stable Organic Solar Cells77Structurally Complementary Star‐Shaped Unfused Ring Electron Acceptors with Simultaneously Enhanced Device Parameters for Ternary Organic Solar Cells91Precise control of conjugated polymer synthesis from step-growth polymerization to iterative synthesis42Approaching 19% efficiency and stable binary polymer solar cells enabled by a solidification strategy of solvent additive51Improved photovoltaic performance and robustness of all-polymer solar cells enabled by a polyfullerene guest acceptor159Recent progress on efficient perovskite/organic tandem solar cells42Enabling Highly Efficient and Thermal‐Stable Polymer Solar Cells through Semi‐Alloy Acceptors Composed of a Hinge‐Like Dimer: A Versatile Doping Protocol97Batch-Reproducible and Thickness-Insensitive Mesopolymer Zwitterion Interlayers for Organic Solar Cells77High-Performance Intrinsically Stretchable Polymer Solar Cell with Record Efficiency and Stretchability Enabled by Thymine-Functionalized Terpolymer110High‐Performance Organic Solar Cells Containing Pyrido[2,3‐ b ]quinoxaline‐Core‐Based Small‐Molecule Acceptors with Optimized Orbit Overlap Lengths and Molecular Packing119Polymer Semiconductors: Synthesis, Processing, and Applications539Organic Solar Cells with Over 19% Efficiency Enabled by a 2D‐Conjugated Non‐Fullerene Acceptor Featuring Favorable Electronic and Aggregation Structures199Recent research progress of all-polymer solar cells based on PSMA-type polymer acceptors89Recent Progress in π-Conjugated Polymers for Organic Photovoltaics: Solar Cells and Photodetectors158High-efficiency organic solar cells processed from a halogen-free solvent system46Engineering push–pull structural versatility in highly functional carbazole-based hole transporting materials design for efficient perovskites solar devices42High-performance organic solar cell and self-power photodetector with chemically robust, near-infrared acceptor enabled by strengthening interfacial contact and compositional modulation47Impact of Electrostatic Interaction on Non‐radiative Recombination Energy Losses in Organic Solar Cells Based on Asymmetric Acceptors148Dissecting the structure-stability relationship of Y-series electron acceptors for real-world solar cell applications65Achieving Organic Solar Cells with an Efficiency of 18.80% by Reducing Nonradiative Energy Loss and Tuning Active Layer Morphology54Terminally Chlorinated and Thiophene‐linked Acceptor‐Donor‐Acceptor Structured 3D Acceptors with Versatile Processability for High‐efficiency Organic Solar Cells72Thermodynamic Phase Transition of Three‐Dimensional Solid Additives Guiding Molecular Assembly for Efficient Organic Solar Cells89Powering the Future: A Critical Review of Research Progress in Enhancing Stability of High‐Efficiency Organic Solar Cells95Improving the Stability of Organic Solar Cells: From Materials to Devices56What We have Learnt from PM6:Y6181Non‐Halogen Solvent Processed Binary Organic Solar Cells with Efficiency of 19% and Module Efficiency Over 15% Enabled by Asymmetric Alkyl Chain Engineering97Efficient Semitransparent Organic Solar Cells with CRI over 90% Enabled by an Ultralow‐Bandgap A‐DA'D‐A Small Molecule Acceptor49Over 18% Efficiency Ternary Organic Solar Cells with 300 nm Thick Active Layer Enabled by an Oligomeric Acceptor8918.6% Efficiency All‐Polymer Solar Cells Enabled by a Wide Bandgap Polymer Donor Based on Benzo[1,2‐d:4,5‐d′]bisthiazole55Selectively Modulating Componential Morphologies of Bulk Heterojunction Organic Solar Cells42Current State and Future Perspectives of Printable Organic and Perovskite Solar Cells61Optimized Crystal Framework by Asymmetric Core Isomerization in Selenium‐Substituted Acceptor for Efficient Binary Organic Solar Cells86Key molecular perspectives for high stability in organic photovoltaics113Auxiliary sequential deposition enables 19%-efficiency organic solar cells processed from halogen-free solvents211Control of Properties through Hydrogen Bonding Interactions in Conjugated Polymers96Developing Efficient Benzene Additives for 19.43% Efficiency of Organic Solar Cells by Crossbreeding Effect of Fluorination and Bromination45Embrace the darkness: An experimental perspective on organic exciton–polaritons57Nonfullerene Acceptor Featuring Unique Self‐Regulation Effect for Organic Solar Cells with 19 % Efficiency66Simple and Efficient Synthesis of Novel Tetramers with Enhanced Glass Transition Temperature for High‐Performance and Stable Organic Solar Cells54Boron- and Nitrogen-Embedded Polycyclic Arenes as an Emerging Class of Organic Semiconductors84Precise Methylation Yields Acceptor with Hydrogen‐Bonding Network for High‐Efficiency and Thermally Stable Polymer Solar Cells66The Quest for Air Stability in Organic Semiconductors83Unraveling the Structure–Property–Performance Relationships of Fused-Ring Nonfullerene Acceptors: Toward a C-Shaped ortho -Benzodipyrrole-Based Acceptor for Highly Efficient Organic Photovoltaics90Azobenzene-containing polymer for solar thermal energy storage and release: Advances, challenges, and opportunities77Cyano-functionalized pyrazine: an electron-deficient unit as a solid additive enables binary organic solar cells with 19.67% efficiency80Efficient and stable all-small-molecule solar cells enabled by incorporating a designed giant molecule acceptor53Quinoxaline-based nonfullerene acceptors with powerful core-functionalization ability enabling efficient solar energy utilization52Rational design of flexible-linked 3D dimeric acceptors for stable organic solar cells demonstrating 19.2% efficiency61Synergistic control of multilength-scale morphology and vertical phase separation for high-efficiency organic solar cells66Understanding photochemical degradation mechanisms in photoactive layer materials for organic solar cells87A–D–A'–D–A type nonfused ring electron acceptors for efficient organic solar cells via synergistic molecular packing and orientation control42Discovery of Organic Optoelectronic Materials Powered by Oxidative Ar–H/Ar–H Coupling57Volatile Solid‐Assisted Molecular Assembly Enables Eco‐Friendly Processed Organic Photovoltaic Cells with High Efficiency and Photostability42Oligothiophene Additive‐Assisted Morphology Control and Recombination Suppression Enable High‐Performance Organic Solar Cells89Multiarmed Aromatic Ammonium Salts Boost the Efficiency and Stability of Inverted Organic Solar Cells7919.7% efficiency binary organic solar cells achieved by selective core fluorination of nonfullerene electron acceptors332Binary Organic Solar Cells with over 19 % Efficiency and Enhanced Morphology Stability Enabled by Asymmetric Acceptors85Perovskite–organic tandem solar cells236Isomerization of Benzothiadiazole Yields a Promising Polymer Donor and Organic Solar Cells with Efficiency of 19.0%71Tethered Trimeric Small‐molecular Acceptors through Aromatic‐core Engineering for Highly Efficient and Thermally Stable Polymer Solar Cells41Over 19 % Efficiency Organic Solar Cells Enabled by Manipulating the Intermolecular Interactions through Side Chain Fluorine Functionalization107Non‐Fully Conjugated Dimerized Giant Acceptors with Different Alkyl‐Linked Sites for Stable and 19.13 % Efficiency Organic Solar Cells87Unveiling the Strain‐induced Microstructural Evolution and Morphology‐Stretchability Correlations of Intrinsically Stretchable Organic Photovoltaic Films48Recent advances of polyoxometalate-based materials applied for electron-related devices53Self-Assembled Monolayers for Interfacial Engineering in Solution-Processed Thin-Film Electronic Devices: Design, Fabrication, and Applications642Large-area organic photovoltaic modules with 14.5% certified world record efficiency115Non‐halogenated Solvent‐Processed Organic Solar Cells with Approaching 20 % Efficiency and Improved Photostability185Dimerized Acceptors with Conjugate‐Break Linker Enable Highly Efficient and Mechanically Robust Organic Solar Cells59High Open‐Circuit Voltage Organic Solar Cells with 19.2% Efficiency Enabled by Synergistic Side‐Chain Engineering74Engineering 2D Photocatalysts for Solar Hydrogen Peroxide Production215Guest Acceptors with Lower Electrostatic Potential in Ternary Organic Solar Cells for Minimizing Voltage Losses75On the role of asymmetric molecular geometry in high-performance organic solar cells70Increase in the efficiency and stability of large-area flexible organic photovoltaic modules via improved electrical contact160Insight Into Designing High‐Performance Polythiophenes for Reduced Urbach Energy and Nonradiative Recombination in Organic Solar Cells48High Performance As‐Cast Organic Solar Cells Enabled by a Refined Double‐Fibril Network Morphology and Improved Dielectric Constant of Active Layer55Dipole Moments Regulation of Biphosphonic Acid Molecules for Self-assembled Monolayers Boosts the Efficiency of Organic Solar Cells Exceeding 19.7%193Binary Organic Solar Cells with Exceeding 19% Efficiency via the Synergy of Polyfluoride Polymer and Fluorous Solvent44Tailoring Cyano Substitutions on Quinoxaline‐based Small‐Molecule Acceptors Enabling Enhanced Molecular Packing for High‐Performance Organic Solar Cells68Unleashing the green potential: Assessing Hong Kong's building solar PV capacity42Highly sensitive water pollution monitoring using colloid-processed organic photodetectors58The Development of Quinoxaline‐Based Electron Acceptors for High Performance Organic Solar Cells87A polymer acceptor with double-decker configuration enhances molecular packing for high-performance all-polymer solar cells67Modulating the Photophysical Properties of Twisted Donor–Acceptor–Donor π-Conjugated Molecules: Effect of Heteroatoms, Molecular Conformation, and Molecular Topology131peri-Fused polyaromatic molecular contacts for perovskite solar cells326Approaching 20% Efficiency in Ortho‐Xylene Processed Organic Solar Cells by a Benzo[a]phenazine‐Core‐Based 3D Network Acceptor with Large Electronic Coupling and Long Exciton Diffusion Length112Closed-loop transfer enables artificial intelligence to yield chemical knowledge73A Novel Upside‐Down Thermal Annealing Method Toward High‐Quality Active Layers Enables Organic Solar Cells with Efficiency Approaching 20%85Coherence in Chemistry: Foundations and Frontiers53Sustainable Solution Processing Toward High‐Efficiency Organic Solar Cells: A Comprehensive Review of Materials, Strategies, and Applications72Local Structure‐Induced Selective Interactions Enables High‐Performance and Burn‐in‐Free Organic Photovoltaics51Suppressed non-radiative loss and efficient hole transfer at a small highest occupied molecular orbital offset endows binary organic solar cells with 19.73% efficiency and a small efficiency-cost gap43Manipulating crystallization kinetics and vertical phase distribution via a small molecule donor guest for organic photovoltaic cells with 20% efficiency68CF 3 -Functionalized Side Chains in Nonfullerene Acceptors Promote Electrostatic Interactions for Highly Efficient Organic Solar Cells84The Critical Isomerization Effect of Core Bromination on Nonfullerene Acceptors in Achieving High‐Performance Organic Solar Cells with Low Energy Loss4820.0% efficiency of ternary organic solar cells enabled by a novel wide band gap polymer guest donor60Overcoming optical losses in thin metal-based recombination layers for efficient n-i-p perovskite-organic tandem solar cells47π‐Conjugated Polymers for High‐Performance Organic Electrochemical Transistors: Molecular Design Strategies, Applications and Perspectives78Extending Exciton Diffusion Length via an Organic‐Metal Platinum Complex Additive for High‐Performance Thick‐Film Organic Solar Cells65High Mobility Emissive Organic Semiconductors for Optoelectronic Devices65Integration of Motion and Stillness: A Paradigm Shift in Constructing Nearly Planar NIR-II AIEgen with Ultrahigh Molar Absorptivity and Photothermal Effect for Multimodal Phototheranostics76Simultaneous enhancement of efficiency, stability and stretchability in binary polymer solar cells with a three-dimensional aromatic-core tethered tetrameric acceptor42Non-fullerene acceptors with high crystallinity and photoluminescence quantum yield enable >20% efficiency organic solar cells425Manipulating Aggregation Kinetics toward Efficient All‐Printed Organic Solar Cells77Diluted Ternary Heterojunctions to Suppress Charge Recombination for Organic Solar Cells with 21% Efficiency23720.6% Efficiency Organic Solar Cells Enabled by Incorporating a Lower Bandgap Guest Nonfullerene Acceptor Without Open‐Circuit Voltage Loss174Molecular Design of Dimeric Acceptor Enables Binary Organic Solar Cells with 19.78% Efficiency and Enhanced Stability43Amide-Based Cathode Interfacial Layer with Dual-Modification Mechanisms Enables Stable Organic Solar Cells with High Efficiency Achieving 20%88Advancing organic photovoltaic cells for a sustainable future: The role of artificial intelligence (AI) and deep learning (DL) in enhancing performance and innovation48A Structurally Simple Polymer Donor Enables High‐Efficiency Organic Solar Cells with Minimal Energy Losses50Acceptor Crystallinity Engineering Enables >20% Efficiency Binary Organic Solar Cells with 83.0% Fill Factor101Decoding the Role of Molecular Orientation in Conjugated Self‐Assembled Monolayers for High‐Performance Binary Organic Photovoltaics Approaching 20% Efficiency47Organic Solar Cell with Efficiency of 20.49% Enabled by Solid Additive and Non‐Halogenated Solvent83Building-integrated photovoltaics48Fully non-fused electron acceptor solar cells with 18% efficiency via a synergistic peripheral substituent strategy44Binary Oxide Ceramics (TiO2, ZnO, Al2O3, SiO2, CeO2, Fe2O3, and WO3) for Solar Cell Applications: A Comparative and Bibliometric Analysis62Achieving 20.80% Efficiency in Ternary Organic Solar Cells via Suppression of Static and Dynamic Disorder53Scalable polymer for large-area semitransparent organic photovoltaics46Homology‐Guided Zwitterionic Interlayers for 21% Efficiency Non‐Fullerene Organic Solar Cells43

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