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RESEARCH PAPER · Chemical Reviews · 2022

Polymer Photoelectrodes for Solar Fuel Production: Progress and Challenges

Madasamy Thangamuthu, Qiushi Ruan, Peter Osei Ohemeng, Bing Luo, Dengwei Jing, Robert Godin, Junwang Tang

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Polymer Photoelectrodes for Solar Fuel Production: Progress and ChallengesOriginalCe-hydroxamate metal–organic frameworks for photocatalytic H 2 generation32Decarbonization of Polluted Air by Solar‐Driven CO2 Conversion into Ethanol Using Polarized Animal Solid Waste as Catalyst2Toward Stable and Efficient Solar Cells with Electropolymerized Films6Electron-Deficient Zn-N6 Configuration Enabling Polymeric Carbon Nitride for Visible-Light Photocatalytic Overall Water Splitting84Transparent Porous Conductive Substrates for Gas‐Phase Photoelectrochemical Hydrogen Production29A Biomass‐Ligand‐Based Ru(III) Complex as a Catalyst for Cycloaddition of CO 2 and Epoxides to Cyclic Carbonates and a Study of the Mechanism15A chemist's guide to photoelectrode development for water splitting – the importance of molecular precursor design53Di-ruthenium complexes of 1,4-diazabutadiene ligands: synthesis, characterization and utilization as catalyst precursors for the oxidative coupling of amines to imines in air8Metalloporphyrin-Based Biomimetic Catalysis: Applications, Modifications and Flexible Microenvironment Influences (A Review)5Methylated precursor leads to carbon nitride (CN x ) with improved interfacial interactions for enhanced photocatalytic performance5Multi-functional photocatalytic systems for solar fuel production10Photocatalytic water oxidation over LaWO 0.6 N 2.4 mesoporous single crystals under visible and near-infrared light illumination4Tilt Angle Optimization of Steam Turbine Blade Model Based on Aluminium: The Multi-Simulation Perspective2Dual Functional Conjugated Acetylenic Polymers: High-Efficacy Modulation for Organic Photoelectrochemical Transistors and Structural Evolution for Bioelectronic Detection55Single‐Site Molecular Ruthenium(II) Water‐Oxidation Catalysts Grafted into a Polymer‐Modified Surface for Improved Stability and Efficiency5Stored photoelectrons in a faradaic junction for decoupled solar hydrogen production in the dark42Tailored BiVO4 Photoanode Hydrophobic Microenvironment Enables Water Oxidative H2O2 Accumulation45The Photocharging Effect and Part Electronic Structure Changes of Organic Semiconductors in Photoelectrochemical Water Splitting3Organic Semiconductor-Based Photoelectrochemical Cells for Efficient Solar-to-Chemical Conversion25Polymer Semiconductors: Synthesis, Processing, and Applications539Tungsten Oxide-Based Z-Scheme for Visible Light-Driven Hydrogen Production from Water Splitting48Oxygen defect rich Bi2S3/SnS2/Bi-self doped Bi2W2O9 multijunction photocatalyst for enhanced degradation of methyl parathion and H2 evolution45The Emergence of High‐Performance Conjugated Polymer/Inorganic Semiconductor Hybrid Photoelectrodes for Solar‐Driven Photoelectrochemical Water Splitting12Artificial Photosynthesis: Current Advancements and Future Prospects68Two‐dimensional conjugated polymer frameworks for solar fuel generation from water65Carbon Nitrides from Supramolecular Crystals: From Single Atoms to Heterojunctions and Advanced Photoelectrodes11Designing of covalent organic framework/2D g-C3N4 heterostructure using a simple method for enhanced photocatalytic hydrogen production84Discovery of a Hybrid System for Photocatalytic CO2 Reduction via Attachment of a Molecular Cobalt-Quaterpyridine Complex to a Crystalline Carbon Nitride21Porous architecture photoelectrode with boosted photoelectrochemical properties for solar fuel production8A Facile Design for Water‐Oxidation Molecular Catalysts Precise Assembling on Photoanodes7Soft Materials for Photoelectrochemical Fuel Production13Enhanced photoelectrochemical water splitting with a donor-acceptor polyimide22Recent advances in photocatalytic water splitting and hydrogen generation (2021–2022)0Metal–organic frameworks (MOFs) for photoelectrocatalytic (PEC) reducing carbon dioxide (CO 2 ) to hydrocarbon fuels25Boosted photoredox capability of visible light-active P-doped C 3 N 4 with efficient harvesting of electron–hole pairs12Efficient single-component nickel catalysts with tetradentate aminopyridine ligands for cycloaddition reactions of CO 2 and epoxides under mild conditions4Metal–insulator–semiconductor photoelectrodes for enhanced photoelectrochemical water splitting76Photocatalytic applications of covalent organic frameworks: synthesis, characterization, and utility33Photoelectrochemical Water Splitting0Synergistic interaction and hybrid association of conducting polymer photocatalysts/photoelectrodes for emerging visible light active photocatalytic applications51A Monodisperse, End‐Capped Ru(bda) Oligomer with Outstanding Performance in Heterogeneous Electrochemical Water Oxidation3Highly planar pseudocapacitive semiconducting polymer electrodes toward symmetric supercapacitors with a wide range of operating potentials33Combined Covalent and Supramolecular Polymerization to Reinforce Perylenebisimide Photosynthetic “Quantasomes”4Artificial Photosynthesis for Regioselective Reduction of NAD(P) + to NAD(P)H Using Water as an Electron and Proton Source28In situ polymerised polyaniline films over multi-walled carbon nanotubes coatings for enhanced photoelectrochemical performance5Metal atom-induced microenvironment regulation in polymeric carbon nitride for photocatalytic hydrogen evolution19Recent Advances in ZnO-Based Photocatalysts for Sustainable Hydrogen Production0Direct formation of copper nanoparticles from atoms at graphitic step edges lowers overpotential and improves selectivity of electrocatalytic CO2 reduction10Síntese e caracterização de filmes de Polipirrol dopados com Tetraquis(4-carboxifenil) porfirina para aplicações fotoelectroquímicas0Bismuth(III) Coordination Linkage with Dimercaptothiadiazole: A p-Type Metallopolymer Photocathode Stable in Protic Electrolytes4Manipulating Photoconduction in Supramolecular Networks for Solar-Driven Nitrate Conversion to Ammonia and Oxygen25Pairing Oxygen Reduction and Water Oxidation for Dual‐Pathway H 2 O 2 Production228Pairing Oxygen Reduction and Water Oxidation for Dual‐Pathway H2O2 Production9Photovoltage Generation at p-Type Semiconducting Polymer/Electrolyte Interfaces4Pitfalls in Photochemical and Photoelectrochemical Reduction of CO2 to Energy Products12Contemporary progress on multifarious coordination polymers for organocatalytic, sensing, and energy-mimetic applications9Kinetic Analysis of Proton-Coupled Electron Transfer at an Electrode-Immobilized Complex5A Halted Photodeposition Technique Controls Co‐Catalyst Loading and Morphology on Organic Semiconductor Nanoparticles for Solar H 2 Production9Interface structure of PN junctions in NiO–WO3–FTO photoelectrode for efficient DSSCs and enhanced photoresponses8Computational Study on the Proton Reduction Potential of Co, Rh, and Ir Molecular Electrocatalysts for the Hydrogen Evolution Reaction3Transient Absorption Microscopy Maps Spatial Heterogeneity and Distinct Chemical Environments in Photocatalytic Carbon Nitride Particles5A Novel Analysis of DC-DC Voltage Conversion Circuit with Modified RBFN Controller for Hydrogen Vehicle Technology1Cobalt complex with a tetradentate aminopyridine ligand: a single-component and efficient catalytic system for the cycloaddition reactions of CO 2 and epoxides4From photocatalysis to photon–phonon co-driven catalysis for methanol reforming to hydrogen and valuable by-products88An efficient strategy to boost photoelectrochemical water oxidation of g-C3N4 films modified with NiO as cocatalyst6Rational Design of Methylated Triazine‐Based Linear Conjugated Polymers for Efficient CO 2 Photoreduction with Water17Length and conjugation-controlled memristive functions of metallopolymer monolayers3Molecular Photoelectrodes with Enhanced Photogenerated Charge Transport for Efficient Solar Hydrogen Evolution32Green Hydrogen Generation by Water Photoelectrolysis: Economic and Environmental Analysis4Enhanced solar water oxidation and unassisted water splitting using graphite-protected bulk heterojunction organic photoactive layers30Delafossite-embedded Z-scheme heterojunction photocathode with abundant heterointerfaces for boosted photoelectrochemical performance7Harnessing Near‐Infrared Light for Enhanced Solar Hydrogen Production from Escherichia coli Interfaced with Biocompatible Low‐Bandgap Conjugated Polymer Nanosheets13Recent Progress in Developing Conjugated Polymer‐Microorganism Biohybrids for Semi‐Artificial Photosynthetic Energy Conversion12Effect of Doping on Photoinduced Charge Carrier Dynamics of Semiconducting Polymer, Poly(benzo(1,2-b:4,5-b′)dithiophene-alt-dione) (PBDB-T), in Photoelectrochemical Cells0Modulating charge transfer dynamics in one-dimensional covalent organic frameworks for boosted photocatalytic H2 generation24Freestanding Polymer Photoelectrodes for Solar Fuel Generation in Photoelectrochemical Cells4Spin-to-charge conversion of chloroplast-functionalized ZnCo2O4 electrode in photoelectrochemical water splitting2A sustainable bias-free photoelectrochemical system for CO2 reduction into formate coupled with aldehyde synthesis0Optimizing PV systems in high-temperature environments: A SWOT-based analysis of cooling technologies11Efficient and Robust Hybrid Molecular Photoanodes for Water Oxidation at Neutral pH Based on Ru Complexes Covalently Bonded to Polymeric Carbon Nitride7Synergistic Design of Cu-Zn Ferrite–g-C3N4 Hybrid Nanocomposite for Solar-Driven Pollutant Degradation and Dye-Sensitized Solar-Cell Applications6Engineering of advanced photoanodes and photocathodes for photoelectrochemical water splitting: Recent advances and prospects8A Global Review of Blue and Green Hydrogen Fuel Production Technologies, Trends and Future Outlook to 205017Nanomaterials for photoelectrochemical energy conversion: Advances and challenges14Artificial Photosynthesis: A Promising Clean Energy Source, Recent Breakthroughs and Challenges0Facile electrophoretic deposition of diverse functional materials for scalable electrode and photoelectrode fabrication0Conjugated Polyelectrolytes with Tunable Ionic Side Chains for Iodide‐Mediated Pt Reduction in Photoelectrochemical H 2 Generation4Impact of Cation Insertion on Semiconducting Polymer Thin Films toward Electrochemical Energy Conversion3Reaction-Oriented Surface Engineering over (Photo)electrodes toward Promoted Artificial Photosynthesis0Advances in photoelectrochemical nitrate reduction for solar ammonia synthesis3Heterogenized homogeneous catalysts for photoelectrochemical carbon dioxide reduction: a path toward ideal hybrid systems2Polycarbazole– NiOOH Interfacial Engineering of BiVO 4 Photoanodes for Efficient and Stable Solar Water Splitting3Linking Photocatalytic Hydrogen Evolution Performance of Carbon Nitrides to Excited State Dynamics via Bulk and Single-Particle Spectroscopic Methods1Cadmium chalcogenides-based polymer materials, synthesis and application for photoelectrochemical (PEC) solar cell: a review0Organic Photoelectrochemical Cells Beyond Performance: Interface and Catalyst Engineering for Durability4Reported synthetic conditions of carbon nitride (CNx) do not directly correlate with photocatalytic activities0Lattice-coupled CdS/CsxWO3 S-scheme heterojunction with complementary UV–vis–NIR absorption for enhanced photocatalytic H2 evolution4A Retina‐Inspired Carbon Dot‐Based and Light‐Suppressed Photochemical Memristor0Bias-free photoelectrochemical co-production of formate from CO2 and biomass-derived plastic precursors2Recent Advances in Photoelectrochemical Synthesis of Value-added Chemicals0Semiartificial CO 2 Fixation Using Metal-Dependent Formate Dehydrogenase1Covalently Integrated Selenoviologen– N ‐Heterocyclic Carbene–Pt Nanoparticles for Visible‐Light‐Driven Hydrogen Evolution0Recent Progress in Photoelectrode Materials for Solar‐Coupled Metal–Air Seawater Batteries0Poly(3,4-Ethylenedioxythiophene)-Centered TiO2 Hybrid Electrodes for HER- and OER-Relevant Photoelectrochemical Responses0Automating Absorbance Spectroelectrochemistry Using Normal Pulse Voltammetry0Solar‐Driven Upcycling of Waste Polyethylene Terephthalate0Photocorrosion, Protection, and Predictive Design in Solar Water Splitting0All-organic semiconductor tandem devices for scalable photoelectrochemical solar H2 production0

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  1. Ce-hydroxamate metal–organic frameworks for photocatalytic H 2 generation

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  2. Decarbonization of Polluted Air by Solar‐Driven CO2 Conversion into Ethanol Using Polarized Animal Solid Waste as Catalyst

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  4. Electron-Deficient Zn-N6 Configuration Enabling Polymeric Carbon Nitride for Visible-Light Photocatalytic Overall Water Splitting

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  5. Transparent Porous Conductive Substrates for Gas‐Phase Photoelectrochemical Hydrogen Production

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