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RESEARCH PAPER · Angewandte Chemie · 2017

Tailored Engineering of an Unusual (C 4 H 9 NH 3 ) 2 (CH 3 NH 3 ) 2 Pb 3 Br 10 Two‐Dimensional Multilayered Perovskite Ferroelectric for a High‐Performance Photodetector

Lina Li, Zhihua Sun, Peng Wang, Weida Hu, Sasa Wang, Chengmin Ji, Maochun Hong, Junhua Luo

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Tailored Engineering of an Unusual (C 4 H 9 NH 3 ) 2 (CH 3 NH 3 ) 2 Pb 3 Br 10 Two‐Dimensional Multilayered Perovskite Ferroelectric for a High‐Performance PhotodetectorOriginal(2-Methylpiperidine)PbI 3 : an ABX 3 -type organic–inorganic hybrid chain compound and its semiconducting nanowires with photoconductive properties25Controllable Synthesis of Two-Dimensional Ruddlesden–Popper-Type Perovskite Heterostructures65Broadband white-light emission with a high color rendering index in a two-dimensional organic–inorganic hybrid perovskite94Extra thermo- and water-stable one-dimensional organic–inorganic hybrid perovskite [ N -methyldabconium]PbI 3 showing switchable dielectric behaviour, conductivity and bright yellow-green emission58Highly efficient white-light emission in a polar two-dimensional hybrid perovskite115Molecular engineering of perovskite photodetectors: recent advances in materials and devices37White-light emission in a chiral one-dimensional organic–inorganic hybrid perovskite195Hybrid Dion–Jacobson 2D Lead Iodide Perovskites980Guanidinium-Formamidinium Lead Iodide: A Layered Perovskite-Related Compound with Red Luminescence at Room Temperature153Boosting Visible Light Absorption of Metal-Oxide-Based Phototransistors via Heterogeneous In–Ga–Zn–O and CH3NH3PbI3 Films60Alloying n‐Butylamine into CsPbBr3 To Give a Two‐Dimensional Bilayered Perovskite Ferroelectric Material189Alloying n‐Butylamine into CsPbBr3 To Give a Two‐Dimensional Bilayered Perovskite Ferroelectric Material31Towards a Spectrally Customized Photoresponse from an Organic–Inorganic Hybrid Ferroelectric22Towards a Spectrally Customized Photoresponse from an Organic–Inorganic Hybrid Ferroelectric3Low-temperature processed inorganic perovskites for flexible detectors with a broadband photoresponse85Two‐Step Structure Phase Transition, Dielectric Anomalies, and Thermochromic Luminescence Behavior in a Direct Band Gap 2D Corrugated Layer Lead Chloride Hybrid of [(CH3)4 N ]4Pb3Cl1022(C6H13NH3)2(NH2CHNH2)Pb2I7: A Two‐dimensional Bilayer Inorganic–Organic Hybrid Perovskite Showing Photodetecting Behavior24An above-room-temperature phosphonium-based molecular ferroelectric perovskite, [(CH3)4P]CdCl3, with Sb3+-doped luminescence61An Unprecedented Biaxial Trilayered Hybrid Perovskite Ferroelectric with Directionally Tunable Photovoltaic Effects204High‐Temperature Reversible Phase‐Transition Behavior, Switchable Dielectric and Second Harmonic Generation Response of Two Homochiral Crown Ether Clathrates11Exploring Lead‐Free Hybrid Double Perovskite Crystals of (BA) 2 CsAgBiBr 7 with Large Mobility‐Lifetime Product toward X‐Ray Detection225Exploring Lead‐Free Hybrid Double Perovskite Crystals of (BA)2CsAgBiBr7 with Large Mobility‐Lifetime Product toward X‐Ray Detection32Designing and Constructing a High‐Temperature Molecular Ferroelectric by Anion and Cation Replacement in a Simple Crown Ether Clathrate19A Three‐Dimensional M3AB‐Type Hybrid Organic–Inorganic Antiperovskite Ferroelectric: [C3H7FN]3[SnCl6]Cl35Dimensional Reduction of Cs2AgBiBr6: A 2D Hybrid Double Perovskite with Strong Polarization Sensitivity102Dimensional Reduction of Cs2AgBiBr6: A 2D Hybrid Double Perovskite with Strong Polarization Sensitivity21Exploiting the Bulk Photovoltaic Effect in a 2D Trilayered Hybrid Ferroelectric for Highly Sensitive Polarized Light Detection180Exploiting the Bulk Photovoltaic Effect in a 2D Trilayered Hybrid Ferroelectric for Highly Sensitive Polarized Light Detection21Multilayered 2D Cesium‐Based Hybrid Perovskite with Strong Polarization Sensitivity: Dimensional Reduction of CsPbBr325Halide Double Perovskite Ferroelectrics104Halide Double Perovskite Ferroelectrics31Room‐Temperature Ferroelectric Material Composed of a Two‐Dimensional Metal Halide Double Perovskite for X‐ray Detection186Room‐Temperature Ferroelectric Material Composed of a Two‐Dimensional Metal Halide Double Perovskite for X‐ray Detection37Solution‐Grown Large‐Sized Single‐Crystalline 2D/3D Perovskite Heterostructure for Self‐Powered Photodetection56Ferroelectricity‐Driven Self‐Powered Ultraviolet Photodetection with Strong Polarization Sensitivity in a Two‐Dimensional Halide Hybrid Perovskite45Ferroelectricity‐Driven Self‐Powered Ultraviolet Photodetection with Strong Polarization Sensitivity in a Two‐Dimensional Halide Hybrid Perovskite1643D‐to‐2D Dimensional Reduction for Exploiting a Multilayered Perovskite Ferroelectric toward Polarized‐Light Detection in the Solar‐Blind Ultraviolet Region823D‐to‐2D Dimensional Reduction for Exploiting a Multilayered Perovskite Ferroelectric toward Polarized‐Light Detection in the Solar‐Blind Ultraviolet Region17Recent advances in hybrid perovskite nanogenerators36Acquiring High‐ T C Layered Metal Halide Ferroelectrics via Cage‐Confined Ethylamine Rotators76Acquiring High‐TC Layered Metal Halide Ferroelectrics via Cage‐Confined Ethylamine Rotators10Perovskite‐Related 2D Compounds in the System 5‐Amino Valerian Acid Cation/MA/Pb/X (X = Cl, Br) – Synthesis, Crystal Structures, and Optical Properties16Solution and Solid‐Phase Growth of Bulk Halide Perovskite Single Crystals10Bromine-Substitution-Induced High-Tc Two-Dimensional Bilayered Perovskite Photoferroelectric93Recent Progress on Electrical and Optical Manipulations of Perovskite Photodetectors315Effective Piezo‐Phototronic Enhancement of Flexible Photodetectors Based on 2D Hybrid Perovskite Ferroelectric Single‐Crystalline Thin‐Films115Monolayer‐to‐Multilayer Dimensionality Reconstruction in a Hybrid Perovskite for Exploring the Bulk Photovoltaic Effect Enables Passive X‐ray Detection15Great Amplification of Circular Polarization Sensitivity via Heterostructure Engineering of a Chiral Two-Dimensional Hybrid Perovskite Crystal with a Three-Dimensional MAPbI3 Crystal73Monolayer‐to‐Multilayer Dimensionality Reconstruction in a Hybrid Perovskite for Exploring the Bulk Photovoltaic Effect Enables Passive X‐ray Detection99Two Dimensional Perovskites/Transition Metal Dichalcogenides Heterostructures: Puzzles and Challenges8Anisotropy in a 2D Perovskite Ferroelectric Drives Self‐Powered Polarization‐Sensitive Photoresponse for Ultraviolet Solar‐Blind Polarized‐Light Detection73Anisotropy in a 2D Perovskite Ferroelectric Drives Self‐Powered Polarization‐Sensitive Photoresponse for Ultraviolet Solar‐Blind Polarized‐Light Detection8Unprecedented Ferroelectricity and Ferromagnetism in a Cr 2+ ‐Based Two‐Dimensional Hybrid Perovskite9Unprecedented Ferroelectricity and Ferromagnetism in a Cr 2+ ‐Based Two‐Dimensional Hybrid Perovskite83Ferroelasticity Mediated Energy Conversion in Strained Perovskite Films14Cs2XI2Cl2 (X = Pb, Sn) All‐Inorganic Layered Ruddlesden–Popper Mixed Halide Perovskite Single Junction and Tandem Solar Cells: Ultra‐High Carrier Mobility and Excellent Power Conversion Efficiency10Modulating the Schottky barriers of metal–2D perovskite junctions through molecular engineering of spacer ligands4Recent progress in layered metal halide perovskites for solar cells, photodetectors, and field-effect transistors53The rise of quasi-2D Dion–Jacobson perovskites for photovoltaics21Ultrafast relaxation of lattice distortion in two-dimensional perovskites69Ferroelectric field effect transistors for electronics and optoelectronics114Ferroelectricity in Hybrid Perovskites44Photonic van der Waals integration from 2D materials to 3D nanomembranes215High-performance photodetectors based on two-dimensional perovskite crystals with alternating interlayer cations14Synergy of 3D and 2D Perovskites for Durable, Efficient Solar Cells and Beyond249Tunable Interlayer Delocalization of Excitons in Layered Organic–Inorganic Halide Perovskites182D Hybrid Perovskites Employing an Organic Cation Paired with a Neutral Molecule21Ferroelectricity and Thermochromism in a 2D Dion‐Jacobson Organic–Inorganic Hybrid Perovskite7Developments in perovskite photodetectors: performance optimization and dimensional diversity20Electronic Structure, Optical Transitions, and Transport Properties of Thiocyanate-Substituted α-FAPbI 3 Perovskite Analogues4A comprehensive review on dark current in perovskite photodetectors: Origin, drawbacks, and reducing strategies422D Molecular Ferroelectric with Large Out‐of‐plane Polarization for In‐Memory Computing18A Chiral B−N Adduct as a New Frontier in Ferroelectrics and Piezoelectric Energy Harvesting1A Chiral B−N Adduct as a New Frontier in Ferroelectrics and Piezoelectric Energy Harvesting32High responsivity VIS-NIR photodetector based on (PEA)2PbI4/P3HT heterojunction3Tuning Electronic and Structural Properties of Lead‐Free Metal Halide Perovskites: A Comparative Study of 2D Ruddlesden‐Popper and 3D Compositions10Organic and inorganic sublattice coupling in two-dimensional lead halide perovskites32Tadpole-Like Polar Molecule Encapsulated in a Two-in-One Supramolecular Cage: Molecular Motion, Phase Transition and Ferroelectricity21Development of a self-powered mixed halide perovskite-based planar near-ultraviolet photodetector by leveraging the pyro-phototronic effect8Anomalous Behavior in Dark–Bright Splitting Impacts the Biexciton Binding Energy in (BA)2(MA)n−1PbnBr3n+1 (n = 1–3)62D and quasi-2D hybrid halide perovskite single crystals: From fundamentals to functionalized photodetectors15Structural Reconfiguration via Alternating Cation Intercalation of Chiral Hybrid Perovskites for Efficient Self-Driven X-ray Detection11Out-of-Plane Polarization in a 2D Ruddlesden–Popper Hybrid Lead Halide Perovskite Ferroelectric Semiconductor7Mechanochemical synthesis of 2D n -butylammonium-based layered mixed-halide lead perovskites02D Halide Perovskite Single Crystals Constructed by Aromatic Diammonium for High Sensitivity and Low Detection Limit X‐Ray Detectors0

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  2. Controllable Synthesis of Two-Dimensional Ruddlesden–Popper-Type Perovskite Heterostructures

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  3. Broadband white-light emission with a high color rendering index in a two-dimensional organic–inorganic hybrid perovskite

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  4. Extra thermo- and water-stable one-dimensional organic–inorganic hybrid perovskite [ N -methyldabconium]PbI 3 showing switchable dielectric behaviour, conductivity and bright yellow-green emission

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  12. Alloying n‐Butylamine into CsPbBr3 To Give a Two‐Dimensional Bilayered Perovskite Ferroelectric Material

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  15. Low-temperature processed inorganic perovskites for flexible detectors with a broadband photoresponse

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  16. Two‐Step Structure Phase Transition, Dielectric Anomalies, and Thermochromic Luminescence Behavior in a Direct Band Gap 2D Corrugated Layer Lead Chloride Hybrid of [(CH3)4 N ]4Pb3Cl10

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  17. (C6H13NH3)2(NH2CHNH2)Pb2I7: A Two‐dimensional Bilayer Inorganic–Organic Hybrid Perovskite Showing Photodetecting Behavior

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  18. An above-room-temperature phosphonium-based molecular ferroelectric perovskite, [(CH3)4P]CdCl3, with Sb3+-doped luminescence

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  19. An Unprecedented Biaxial Trilayered Hybrid Perovskite Ferroelectric with Directionally Tunable Photovoltaic Effects

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  21. Exploring Lead‐Free Hybrid Double Perovskite Crystals of (BA) 2 CsAgBiBr 7 with Large Mobility‐Lifetime Product toward X‐Ray Detection

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  29. Multilayered 2D Cesium‐Based Hybrid Perovskite with Strong Polarization Sensitivity: Dimensional Reduction of CsPbBr3

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  40. Acquiring High‐ T C Layered Metal Halide Ferroelectrics via Cage‐Confined Ethylamine Rotators

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  47. Monolayer‐to‐Multilayer Dimensionality Reconstruction in a Hybrid Perovskite for Exploring the Bulk Photovoltaic Effect Enables Passive X‐ray Detection

    Angewandte Chemie · 2021-07-18

    Chengmin Ji, Yezhan Li, Xitao Liu, Yaxing Wang, Tingting Zhu, Qin Chen, Lina Li, Shuao Wang, Junhua Luo

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  48. Great Amplification of Circular Polarization Sensitivity via Heterostructure Engineering of a Chiral Two-Dimensional Hybrid Perovskite Crystal with a Three-Dimensional MAPbI3 Crystal

    ACS Central Science · 2021-07-19

    Xinyuan Zhang, Xitao Liu, Lina Li, Chengmin Ji, Yunpeng Yao, Junhua Luo

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  49. Monolayer‐to‐Multilayer Dimensionality Reconstruction in a Hybrid Perovskite for Exploring the Bulk Photovoltaic Effect Enables Passive X‐ray Detection

    Angewandte Chemie International Edition · 2021-07-19

    Chengmin Ji, Yezhan Li, Xitao Liu, Yaxing Wang, Tingting Zhu, Qin Chen, Lina Li, Shuao Wang, Junhua Luo

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  50. Two Dimensional Perovskites/Transition Metal Dichalcogenides Heterostructures: Puzzles and Challenges

    Israel Journal of Chemistry · 2021-12-29

    Michał Baranowski, Alessandro Surrente, Paulina Płochocka

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