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RESEARCH PAPER · Angewandte Chemie International Edition · 2022

A‐Site Diamine Cation Anchoring Enables Efficient Charge Transfer and Suppressed Ion Migration in Bi‐Based Hybrid Perovskite Single Crystals

Xin Yang, Yuhua Huang, Xu‐Dong Wang, Wenguang Li, Dai‐Bin Kuang

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A‐Site Diamine Cation Anchoring Enables Efficient Charge Transfer and Suppressed Ion Migration in Bi‐Based Hybrid Perovskite Single CrystalsOriginalLow‐Temperature Melt Processing Monolithic Integration of Organic Manganese (II) Bromide Wafers with Pixelated Substrate for High Sensitivity X‐Ray Imaging57One-dimensional lead-free perovskite single crystals with high X-ray response grown by liquid phase diffusion29Rational Design of Non-Centrosymmetric Hybrid Halide Perovskites109Combining π-Conjugation and Cation−π Interaction for Water-Stable and Photoconductive One-Dimensional Hybrid Lead Bromide28Managing Interfacial Hot‐Carrier Cooling and Extraction Kinetics for Inverted Ma‐Free Perovskite Solar Cells Over 23% Efficiency via Dion–Jacobson 2D Capping Layer50Structure stabilized with robust molecular cation N(CH3)4+ in high efficiency perovskite solar cells2Barium(II)-based semiconductive coordination polymers for high-performance direct X-ray detection and imaging: Reducing the exciton binding energy via enhancing π-π interactions27Incorporating an Aromatic Diammonium To Assemble Bilayered Dion–Jacobson Perovskite Crystals for Weak Light Detection6Ultrasound‐Assisted Crystallization Enables Large‐Area Perovskite Quasi‐Monocrystalline Film for High‐Sensitive X‐ray Detection and Imaging90Manganese‐Halide Single‐Crystal Scintillator Toward High‐Performance X‐Ray Detection and Imaging: Influences of Halogen and Thickness78Realizing 23.9% Flexible Perovskite Solar Cells via Alleviating the Residual Strain Induced by Delayed Heat Transfer113Chiral Substitution on Spaced Cations Lead to Improved Properties and Reversible Phase Transition, Broadband Emission in Parent Compound (3APr)PbBr45Amplifying photoreduction efficacy of Bi-Sb bimetallic nanocrystals: Manipulating carrier dynamics to boost CO2-to-CO conversion23Novel High-Tc, Broadband-Emission Multifunctional Hybrid Compound: (4,4-DCA)2CdCl4 with Sb Doping Enhances Fluorescence Emission4Dimensional and Optoelectronic Tuning of Lead‐free Perovskite Cs 3 Bi 2 I 9−n Br n Single Crystals for Enhanced Hard X‐ray Detection43Dimensional and Optoelectronic Tuning of Lead‐free Perovskite Cs3Bi2I9−nBrn Single Crystals for Enhanced Hard X‐ray Detection8Chiral‐Achiral Cations Intercalation Induced Lead‐Free Chiral‐Polar Hybrid Perovskites Enable Self‐Powered X‐Ray and Ultraviolet–Visible–Near‐Infrared Photo Detection33Centimeter-sized novel two-dimensional organic lead–tin mixed iodide single crystals for efficient photodetector applications6Band Structure Optimized by Electron‐Acceptor Cations for Sensitive Perovskite Single Crystal Self‐Powered Photodetectors7Antimony Bromide Organic–Inorganic Hybrid Compound with a Long-Chain Diamine Showing Switchable Phase Transition and Second-Harmonic Generation Properties9Enhanced photoelectric performance in Cu–Bi double halide perovskite single crystals4Reversible structural transformation of metastable lead-free organic–inorganic hybrid bismuth halide single crystals8Dense Stacking of Millimeter‐Sized Perovskite Single Crystals for Sensitive and Low‐Bias Hard X‐Ray Detection390‐D and 1‐D Perovskite‐like Hybrid Bismuth(III) Iodides7Non-Centrosymmetric Chiral Structures for Hybrid Bismuth Halides With Stable Self-Driven X-Ray Detection6Unique Optoelectronic Properties and Applications of Lead‐Free Perovskites and Derivatives19Lattice Manipulation with Di‐Tertiary Ammonium Spacer in Bismuth Bromide Perovskite Directs Efficient Charge Transport and Suppressed Ion Migration for Photodetector Applications13Unlocking the Potential of Organic‐Inorganic Hybrid Manganese Halides for Advanced Optoelectronic Applications171Rational Design of A‐Site Cation for High Performance Lead‐Free Perovskite X‐Ray Detectors17Conjugated diamine cation based halide perovskitoid enables robust stability and high photodetector performance22Ion Leakage Current Control for Polycrystalline Metal Halide Perovskite Direct X-ray Detectors92D and quasi-2D hybrid halide perovskite single crystals: From fundamentals to functionalized photodetectors15Suppressed Ion Migration in Tin Halide Perovskites for Stable X‐Ray Detectors with Low Dark Current Drift11Dark Current Suppression in Two‐dimensional Histamine Lead Iodine Perovskite Single Crystal for X‐ray Detection and Imaging6Bromine‐Substituted Cation Anchoring to Suppress Ion Migration in Alternating Cations Intercalation‐Type Perovskite for Stable X‐Ray Detection15Reconfiguration of band-edge states via intermolecular packing in organic semiconductor-incorporated perovskites2High-Performance Lead-Free Cs3Bi2IxBr9–x Perovskite X-ray Detector Based on Anionic Engineering6Screening High-Performance Hybrid Halides Scintillators: A Comprehensive Analysis and Prediction Model7Light Management in 2D Perovskite Toward High-Performance Optoelectronic Applications17Manipulating perovskite structural asymmetry for high-performing self-powered full-stokes polarimetry32Multifunctional 0D Manganese‐Based Organic–Inorganic Hybrid Halide for Ultraviolets and X‐Ray Detection252‐Bromonaphthalene‐Induced Defect Passivation to Suppress Ion Migration in CsPbBr 3 Wafer for X‐Ray Detector with Bias‐Resistant Stability17Vacuum‐Assisted Blade Coating MAPbI 3 Homojunction Thick Film for Highly Sensitive X‐Ray Detectors10Molecular Ordering in Low‐Dimensional Hybrid Perovskites for Improved X‐Ray Detection20Molecular Ordering in Low‐Dimensional Hybrid Perovskites for Improved X‐Ray Detection2Pb:Sn Ratio-Driven Polytypism and Band Modulation in Photoresponsive Hexagonal Perovskitoids10Boosting Photovoltaic Respond Through Molecular Engineering in Organic Manganese (II) Bromide for High‐Sensitivity X‑Ray Detection3Scalable Fabrication and Integration Strategies for Metal Halide Perovskite Direct X‐Ray Detectors10Record-High Photoluminescence Efficiency and Excellent Scintillation in Two-Dimensional Diamine Hybrid Copper(I) Halides11Defect passivation and crystallization modulation in methylammonium-free wide-bandgap perovskites for all-perovskite tandem solar cells69An aromatic diamine-constructed lead-free polar perovskite towards stable self-driven X-ray detection4Zero‐Dimensional Indium‐Based Multiaxial Ferroelectric for X‐Ray Detection1A high-performance photodetector enabled by melamine cation-based lead-free perovskitoid single crystals0Multilayered Alternating Cations Intercalation Perovskite Single Crystals with Strong π–π Interactions Unlock nW-Level Weak-Light Detection and Imaging0Zero‐Dimensional Bismuth Halide Perovskite with Direct Bandgap for Ultra‐Low Voltage Photodetection5Eco‐Friendly Preparation of High‐Quality Lead‐Free Halide Ferroelectric Solid‐Solution Toward High‐Performance X‐ray Detection5Photosensitive Halide Semiconductors Enabled by Electron Reservoirs From Extended Viologens0Insights Into Ferroelectric Phase Transition Mechanism for One‐Dimensional Halide Perovskites to Attain Record‐Performance Self‐Powered X‐Ray Detection4Dimensional Engineering in 4AMPBiX 5 Metal Halides: From 0D to 1D for Enhanced X‐Ray Detection Performance1One-Dimensional Hybrid Lead Halide Crystals with Molecular Pb–N Coordination for High-Performance Radiation Detection0Highly Stable Lead‐Free Perovskite Single Crystals With Abundant Intermolecular Interactions for Efficient X‐Ray Detection0

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  4. Combining π-Conjugation and Cation−π Interaction for Water-Stable and Photoconductive One-Dimensional Hybrid Lead Bromide

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  5. Managing Interfacial Hot‐Carrier Cooling and Extraction Kinetics for Inverted Ma‐Free Perovskite Solar Cells Over 23% Efficiency via Dion–Jacobson 2D Capping Layer

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  8. Incorporating an Aromatic Diammonium To Assemble Bilayered Dion–Jacobson Perovskite Crystals for Weak Light Detection

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  9. Ultrasound‐Assisted Crystallization Enables Large‐Area Perovskite Quasi‐Monocrystalline Film for High‐Sensitive X‐ray Detection and Imaging

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