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RESEARCH PAPER · Journal of the American Chemical Society · 2022

Anodic Shock-Triggered Exsolution of Metal Nanoparticles from Perovskite Oxide

Weiwei Fan, Baoming Wang, Rui Gao, Georgios Dimitrakopoulos, Jiayue Wang, Xianghui Xiao, Lu Ma, Kai Wu, Bilge Yildiz, Ju Li

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Anodic Shock-Triggered Exsolution of Metal Nanoparticles from Perovskite OxideOriginalRapid Plasma Exsolution from an A‐site Deficient Perovskite Oxide at Room Temperature57Metal exsolution engineering on perovskites for electrocatalysis: a perspective35Ion irradiation to control size, composition and dispersion of metal nanoparticle exsolution25Nanoparticle exsolution via electrochemical switching in perovskite fibers for solid oxide fuel cell electrodes34Rapidly tuning the electrocatalytic activity of perovskite oxides by plasma treatment5Fast Surface Oxygen Release Kinetics Accelerate Nanoparticle Exsolution in Perovskite Oxides81In situ electrochemical reconstruction of Sr2Fe1.45Ir0.05Mo0.5O6-δ perovskite cathode for CO2 electrolysis in solid oxide electrolysis cells62Exsolved materials for CO2 reduction in high-temperature electrolysis cells32Iron-triggered exsolution of FeNi alloy nanoparticles via topotactic cation exchange on Pr0.7Sr0.3Cr0.9Ni0.1O3−δ perovskite for CO2 electrolysis7Electronic Activation during Nanoparticle Exsolution for Enhanced Activity at Elevated Temperature19Quantifying Electrochemical Driving Force for Exsolution in Perovskite Oxides by Designing Graded Oxygen Chemical Potential29Facile Construction of Nanostructured Cermet Anodes with Strong Metal–Oxide Interaction for Efficient and Durable Solid Oxide Fuel Cells30Nanocarbon assisted green hydrogen production: Development and recent trends65Nano and phase engineering of Fe-Cu alloy exsolved perovskite oxide-based hetero-catalysts for efficient oxygen evolution reaction29Electrochemical exsolution of metal nanoparticles from perovskite oxide upon electrolysis19New trends in nanoparticle exsolution45Dielectric Barrier Plasma Discharge Exsolution of Nanoparticles at Room Temperature and Atmospheric Pressure13The effects of nano-socketed metal particles over perovskite surfaces on the electrochemical synthesis of high-value fuels13Highly efficient perovskite-based fuel electrodes for solid oxide electrochemical cells via in-situ nanoparticle exsolution and electron conduction enhancement19Thermal stability and coalescence dynamics of exsolved metal nanoparticles at charged perovskite surfaces39BaCo0.4Fe0.4Ti0.1Ta0.1O3-δ as an efficient, stable and low-thermal-expansion cathode for solid oxide fuel cells operating at reduced temperatures2Dual exsolution in silver‐functionalized layered and cubic perovskite oxides3In Situ Probing Dynamic Exsolution of Fe0 from Perovskite under Graded Potentials7Visualizing Interface Degradation of Solid Oxide Cell8Electric field–confined synthesis of single atomic TiO x C y electrocatalytic membranes31In‐Situ Exsolved Metal Nanoparticles for Solid Oxide Fuel Cell Anode: Mechanism, Design Strategies and Application9Harmonizing Nanoparticle Exsolution From Ce–Sm Oxide Matrix for Stable Methane Dry Reforming39Harmonizing Nanoparticle Exsolution From Ce–Sm Oxide Matrix for Stable Methane Dry Reforming8Exsolution‐enhanced performance for energy conversion and storage5Selective Regulation of Electron–Ion–Phonon Transport in Thermoelectric Materials toward High Performance and Stability2Greener hydrogen production and storage revolution towards a low-carbon future: an overview of current scenarios and future prospects30Quantifying Interface-Dependent Active Sites Induced by Topotactic Exsolution for CO 2 Electrolysis24Potential reduction-induced fast exsolution of hyperfine nanoparticles afford highly active CO2 reduction reaction11Nanofabrication technologies for low-temperature solid oxide cells: a comprehensive review of techniques, challenges, and future perspectives15A critical review on the design strategies of SFM-based perovskite oxides for high-temperature CO 2 electrolysis in solid oxide electrolysis cells3Cr doping regulates FeNi alloy nanoparticle exsolution on Sr 2 Fe 1.1 Ni 0.2 Cr 0.2 Mo 0.5 O 6− δ cathode to facilitate CO 2 electrolysis1In Situ Exsolved Co‐BaO‐La 2 O 3 Interface from Barium‐Doped Perovskites for Catalyzing Ammonia Decomposition Reaction1Low-Temperature, Rapid Synthesis of Plasma-Exsolved FeNi/NiFe 2 O 4 Composites for Enhanced Oxygen Evolution Reaction2Ultrafast Flame Exsolution of High-Density Metal Nanoparticles on Perovskite Oxides2Prediction of ambient-pressure high-temperature superconductivity in electronically modified transition-metal hydrides0Voltage-Temperature Co-Tuned Exsolution for In Situ and Rapidly Improving Electrochemical Activity of Perovskite Oxide0Electro-chemo-mechanically Driven Ni Exsolution from (Pr,Ce,Ni)O 2−δ : Controlled Nucleation Density and Enhanced Electrode Kinetics0Phase-tunable exsolution approaches to energy-functional nanostructured metal-based hybrid materials: synthesis, application, and perspective3Redox-Driven Ni Exsolution with Embedded Ru-Rich Clusters from LaNi 0.95 Ru 0.05 O 30Nanoengineered Ce2CaMoO6 double perovskites derived oxide decorated on 2D P@g-C3N4 nanohybrid for the sensitive electrochemical sensing of antiscald agent diphenylamine in food and environmental matrices0Decoupling the Roles of B‐Site Cation Defects and Oxygen Vacancies in Exsolved Perovskites for Robust CO 2 Electrolysis in Solid‐State Cells0Exsolution in oxide lattices: from fundamentals to catalytic applications0

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  2. Metal exsolution engineering on perovskites for electrocatalysis: a perspective

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  3. Ion irradiation to control size, composition and dispersion of metal nanoparticle exsolution

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  4. Nanoparticle exsolution via electrochemical switching in perovskite fibers for solid oxide fuel cell electrodes

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  5. Rapidly tuning the electrocatalytic activity of perovskite oxides by plasma treatment

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  6. Fast Surface Oxygen Release Kinetics Accelerate Nanoparticle Exsolution in Perovskite Oxides

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  7. In situ electrochemical reconstruction of Sr2Fe1.45Ir0.05Mo0.5O6-δ perovskite cathode for CO2 electrolysis in solid oxide electrolysis cells

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  8. Exsolved materials for CO2 reduction in high-temperature electrolysis cells

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  9. Iron-triggered exsolution of FeNi alloy nanoparticles via topotactic cation exchange on Pr0.7Sr0.3Cr0.9Ni0.1O3−δ perovskite for CO2 electrolysis

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  11. Quantifying Electrochemical Driving Force for Exsolution in Perovskite Oxides by Designing Graded Oxygen Chemical Potential

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  13. Nanocarbon assisted green hydrogen production: Development and recent trends

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  15. Electrochemical exsolution of metal nanoparticles from perovskite oxide upon electrolysis

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  16. New trends in nanoparticle exsolution

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  17. Dielectric Barrier Plasma Discharge Exsolution of Nanoparticles at Room Temperature and Atmospheric Pressure

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  18. The effects of nano-socketed metal particles over perovskite surfaces on the electrochemical synthesis of high-value fuels

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  20. Thermal stability and coalescence dynamics of exsolved metal nanoparticles at charged perovskite surfaces

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