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RESEARCH PAPER · Journal of Catalysis · 2022

Bulk and surface transformations of Ga2O3 nanoparticle catalysts for propane dehydrogenation induced by a H2 treatment

Pedro Castro-Fernández, Deni Mance, Chong Liu, Paula M. Abdala, Elena Willinger, Aurelio A. Rossinelli, Alexander I. Serykh, Evgeny A. Pidko, Christophe Copéret, Alexey Fedorov, Christoph Rüdiger Müller

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Bulk and surface transformations of Ga2O3 nanoparticle catalysts for propane dehydrogenation induced by a H2 treatmentOriginalAtomic-scale changes of silica-supported catalysts with nanocrystalline or amorphous gallia phases: implications of hydrogen pretreatment on their selectivity for propane dehydrogenation14Non‐oxidative Dehydrogenation of Methanol to Formaldehyde over Bulk β‐Ga2O319Fluoride Additive as a Simple Tool to Qualitatively Improve Performance of Nickel-Catalyzed Asymmetric Michael Addition of Malonates to Nitroolefins9Direct Detection of Reactive Gallium-Hydride Species on the Ga2O3 Surface via Solid-State NMR Spectroscopy53Dendritic Mesoporous Silica Nanoparticle Supported PtSn Catalysts for Propane Dehydrogenation14Wound dressing candidate materials based on casted films of cellulose acetate modified with zirconium oxide (ZrO2), and gallium oxide (Ga2O3)13CO2-Assisted Dehydrogenation of Propane to Propene over Zn-BEA Zeolites: Impact of Acid–Base Characteristics on Catalytic Performance22Selective-area growth of β-Ga2O3 nanowire films on nano-patterned Si(111) substrate by metal-organic chemical vapor deposition9Effect of surface modification on the photoluminescent properties of γ-Ga2O3 nanocrystals4Rigorous Oxidation State Assignments for Supported Ga-Containing Catalysts Using Theory-Informed X-ray Absorption Spectroscopy Signatures from Well-Defined Ga(I) and Ga(III) Compounds16Nature of GaOx Shells Grown on Silica by Atomic Layer Deposition19Non-oxidative dehydrogenation of methanol to formaldehyde over supported GaOx-based catalysts15High-temperature vacancy-induced magnetism in nanostructured materials10Synergetic Interaction between Single-Atom Cu and Ga 2 O 3 Enhances CO 2 Hydrogenation to Methanol over CuGaZrO x112Fabrication of β-Ga2O3 Nanotubes via Sacrificial GaSb-Nanowire Templates4Controllable synthesis of gallium-containing MFI zeolite for bifunctionally catalyzing methanol aromatization14Reversible transformation of sub-nanometer Ga-based clusters to isolated [4] Ga (4Si) sites creates active centers for propane dehydrogenation6Oxidative Dehydrogenation of Ethane Over Nanostructured Ga-Ce Bimetallic Oxide Catalysts Using N2o as a Soft Oxidant0Enhanced propane dehydrogenation performance using bimetallic-modified GaPt/SiO2-Al2O3 with ultralow-loading Pt14Liquid Gallium–Zeolite Nanocomposite Catalysts for Propane Dehydrogenation6Uncovering Atomic-scale Dynamics in Solid Catalysts via X-ray-based Methods2The Relation between Nature and Stability of H2‐Dissociating Sites and Propene Selectivity in Silica‐Supported (Ga,Al)2O3 Mixed Oxide Propane Dehydrogenation Catalysts3The new developments of the design and application of novel propane dehydrogenation catalysts0Light alkanes dehydrogenation over silica supported gallium catalysts2Modulation of inter-elemental synergy and oxygen vacancy content of CdZrOx solid solution catalysts by Ga for effective CO2 hydrogenation to methanol13Manipulating Oxygen Vacancies in γ-Ga2O3 Nanocrystals: Correlation between Defect Location, Charge State, and Photophysical Properties8Advanced metal oxide catalysts for propane dehydrogenation: from design strategy to dehydrogenation performance16Zr element promotes gallium oxide-based catalyst activity for direct dehydrogenation of propane2Ga2O3/Al2O3 Catalysts for Propane Dehydrogenation: Effect of H2 Treatment and Cofeeding7Enhancing Catalytic Activity of Gallium Oxide Through Transition Metal Incorporation for Ethane Oxidative Dehydrogenation in the Presence of Carbon Dioxide1Enhancing Photocatalytic Efficiency through Morphology and Bandgap Tuning in Gallium‐Doped Zinc Oxide Nanoparticles2Evolution of [Ga]+ and [GaH2]+ at Propane Dehydrogenation Conditions in MFI Zeolite: A Theoretical Investigation3Ethane Dehydrogenation over Nanostructured Ga‐Ce Bimetallic Oxide Catalysts Using N2O as Oxidant1Hydride Accessibility and Reactivity in the Configurational and Stoichiometric Space of β-Ga2O3 for CO2 Hydrogenation2Uncovering the Pressure-Dependent Mechanism of CO2 Hydrogenation to Methanol on Ga-Promoted Cu/ZrO2 Using Operando Modulation-Excitation DRIFTS53Near-Surface Hydrogen Species Tune the Selectivity of Chemical Reactions on Metal Oxide Surfaces3Unraveling the structure-activity relationship in bare Ga2O3 for propane dehydrogenation: The critical role of crystallite size and phase composition1Structure sensitivity of gallium oxide catalyzed propane dehydrogenation reaction co-fed with hydrogen5Effects of Pt loading on the activity of Pt/γ-Ga 2 O 3 for propane dehydrogenation1Engineering Ga-containing dendritic MFI zeolites as safe-by-design hierarchical and immunomodulatory nanointerfaces0Ga-induced electronic tuning of Ni catalyst surfaces: achieving activity–selectivity balance in propane dehydrogenation0Low dimensionality-engineered Ga 2 O 3 : from structural anisotropy to carrier lifecycle engineering and beyond0Hydroxyl-facilitated efficient propane dehydrogenation over bare Ga2O3 via altering reaction pathway3Crystal Phase-Dependent Ga-H Chemistry and H 2 Roles in Ga 2 O 3 -Catalyzed Propane Dehydrogenation Reaction1Boosting Propane Dehydrogenation on ZnO/Al2O3 via Ni Single Atom-Modified Hydrogen Transfer Kinetics2Recent advances in chemically controlled molecular hydrogen generation for biomedical applications0Surface Oxygen Vacancies as Active Sites for Nonoxidative Propane Dehydrogenation on Metal Oxide Catalysts1

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  1. Atomic-scale changes of silica-supported catalysts with nanocrystalline or amorphous gallia phases: implications of hydrogen pretreatment on their selectivity for propane dehydrogenation

    Catalysis Science & Technology · 2022-01-01

    Pedro Castro-Fernández, Alexander I. Serykh, Alexander V. Yakimov, Igor P. Prosvirin, Andrey V. Bukhtiyarov, Paula M. Abdala, Christophe Copéret, Alexey Fedorov, Christoph Rüdiger Müller

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  2. Non‐oxidative Dehydrogenation of Methanol to Formaldehyde over Bulk β‐Ga2O3

    ChemCatChem · 2022-04-01

    Mariia Merko, G. Wilma Busser, Martin Muhler

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  3. Fluoride Additive as a Simple Tool to Qualitatively Improve Performance of Nickel-Catalyzed Asymmetric Michael Addition of Malonates to Nitroolefins

    The Journal of Organic Chemistry · 2022-09-07

    Oleg I. Afanasyev, Fedor S. Kliuev, Alexey A. Tsygankov, Yulia Vladimirovna Nelyubina, Evgenii I. Gutsul, Valentin V. Novikov, Denis Alexandrovich Chusov

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  4. Direct Detection of Reactive Gallium-Hydride Species on the Ga2O3 Surface via Solid-State NMR Spectroscopy

    Journal of the American Chemical Society · 2022-09-14

    Hongyu Chen, Pan Gao, Zhengmao Liu, Lixin Liang, Qiao Feng Han, Zhili Wang, Kuizhi Chen, Zhenchao Zhao, Meiling Guo, Xuebin Liu, Xiuwen Han, Xinhe Bao, Guangjin Hou

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  5. Dendritic Mesoporous Silica Nanoparticle Supported PtSn Catalysts for Propane Dehydrogenation

    International Journal of Molecular Sciences · 2022-10-22

    Ning Zhang, Yiou Shan, Jiaxin Song, Xiaoqiang Fan, Lian Kong, Xia Xiao, Zean Xie, Zhen Zhao

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  6. Wound dressing candidate materials based on casted films of cellulose acetate modified with zirconium oxide (ZrO2), and gallium oxide (Ga2O3)

    Materials Today Communications · 2022-12-30

    Hind Abdullah Aldossary, Mai M. Khalaf, Mohamed Gouda, Abraham Elmushyakhi, Manal Fawzy Abou Taleb, Hany M. Abd El‐Lateef

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  7. CO2-Assisted Dehydrogenation of Propane to Propene over Zn-BEA Zeolites: Impact of Acid–Base Characteristics on Catalytic Performance

    Catalysts · 2023-03-31

    Svitlana M. Orlyk, Pavlo I. Kyriienko, Andriy Yu. Kapran, Valeriy I. Chedryk, Dmytro Yu. Balakin, Jacek Gurgul, Małgorzata Zimowska, Yannick Millot, Stanisław Dźwigaj

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  8. Selective-area growth of β-Ga2O3 nanowire films on nano-patterned Si(111) substrate by metal-organic chemical vapor deposition

    Ceramics International · 2023-04-07

    Wei Chen, Teng Jiao, Zhaoti Diao, Zhengda Li, Peiran Chen, Xinming Dang, Xinyong Dong, Yuantao Zhang, Baolin Zhang

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  9. Effect of surface modification on the photoluminescent properties of γ-Ga2O3 nanocrystals

    Materials Letters · 2023-04-25

    Qundong Lu, Liqiang Xu, Kun Han, Zhen Huang, Penghui Yin

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  10. Rigorous Oxidation State Assignments for Supported Ga-Containing Catalysts Using Theory-Informed X-ray Absorption Spectroscopy Signatures from Well-Defined Ga(I) and Ga(III) Compounds

    ACS Catalysis · 2023-04-28

    Li Li, Jason A. Chalmers, Simon R. Bare, Susannah L. Scott, Fernando D. Vila

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  11. Nature of GaOx Shells Grown on Silica by Atomic Layer Deposition

    Chemistry of Materials · 2023-08-28

    Zixuan Chen, Nora K. Zimmerli, Muhammad Zubair, Alexander V. Yakimov, Snædís Björgvinsdóttir, Nicholas Alaniva, Elena Willinger, Alexander B. Barnes, Nicholas M. Bedford, Christophe Copéret, Pierre Florian, Paula M. Abdala, Alexey Fedorov, Christoph Rüdiger Müller

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  12. Non-oxidative dehydrogenation of methanol to formaldehyde over supported GaOx-based catalysts

    Journal of Catalysis · 2023-08-28

    Mariia Merko, Sara Delsing, G. Wilma Busser, Martin Muhler

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  13. High-temperature vacancy-induced magnetism in nanostructured materials

    Physical review. B./Physical review. B · 2023-10-09

    Dante Homero Mosca, J. Varalda, César Augusto Dartora

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  14. Synergetic Interaction between Single-Atom Cu and Ga 2 O 3 Enhances CO 2 Hydrogenation to Methanol over CuGaZrO x

    ACS Catalysis · 2023-10-10

    Xiaoyu Han, Tian‐Tian Xiao, Maoshuai Li, Ziwen Hao, Jiyi Chen, Yutong Pan, Xiaohui Zi, Heng Zhang, Shibo Xi, Ming Hui Wai, Sibudjing Kawi, Xinbin Ma

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  15. Fabrication of β-Ga2O3 Nanotubes via Sacrificial GaSb-Nanowire Templates

    Nanomaterials · 2023-10-13

    Lei Shangguan, Longbing He, Shengpan Dong, Yu-Tian Gao, Qian Sun, Jiong-Hao Zhu, Hua Hong, Chao Fu Zhu, Zaixing Yang, Litao Sun

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  16. Controllable synthesis of gallium-containing MFI zeolite for bifunctionally catalyzing methanol aromatization

    Microporous and Mesoporous Materials · 2023-10-27

    Jian Jun Song, Qing Miao, Yunpeng Lv, Zhi‐Peng Wang, Yu Li, Liyan Wang, Mei Dong, Pengfei Wang, Zhangfeng Qin, Weibin Fan

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  17. Reversible transformation of sub-nanometer Ga-based clusters to isolated [4] Ga (4Si) sites creates active centers for propane dehydrogenation

    Catalysis Science & Technology · 2023-11-27

    Zixuan Chen, Alexander I. Serykh, Agnieszka Kierzkowska, David Gajan, Scott R. Docherty, Alexander V. Yakimov, Paula M. Abdala, Christophe Copéret, Pierre Florian, Alexey Fedorov, Christoph Rüdiger Müller

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  18. Oxidative Dehydrogenation of Ethane Over Nanostructured Ga-Ce Bimetallic Oxide Catalysts Using N2o as a Soft Oxidant

    SSRN Electronic Journal · 2024-01-01

    Joaquim Miguel Badalo Branco, Pedro A.L. Martins, Ana Cristina Ferreira, Joana F. Martinho

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  19. Enhanced propane dehydrogenation performance using bimetallic-modified GaPt/SiO2-Al2O3 with ultralow-loading Pt

    Fuel · 2024-04-29

    Jingyi Ma, Hui Yuan, Changcheng Liu, Jieguang Wang, Rongxin Zhang, Aizeng Ma

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  20. Liquid Gallium–Zeolite Nanocomposite Catalysts for Propane Dehydrogenation

    Industrial & Engineering Chemistry Research · 2024-05-09

    Shuo Zhang, Bofeng Zhang, Mingxia Song, Liming Xia, Guozhu Liu

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  21. Uncovering Atomic-scale Dynamics in Solid Catalysts via X-ray-based Methods

    CHIMIA International Journal for Chemistry · 2024-05-29

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  22. The Relation between Nature and Stability of H2‐Dissociating Sites and Propene Selectivity in Silica‐Supported (Ga,Al)2O3 Mixed Oxide Propane Dehydrogenation Catalysts

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    Pedro Castro-Fernández, Alexander I. Serykh, Melis Yarar, Deni Mance, Paula M. Abdala, Christophe Copéret, Alexey Fedorov, Christoph Rüdiger Müller

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  23. The new developments of the design and application of novel propane dehydrogenation catalysts

    Scientia Sinica Chimica · 2024-11-01

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  24. Light alkanes dehydrogenation over silica supported gallium catalysts

    Molecular Catalysis · 2024-11-16

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  25. Modulation of inter-elemental synergy and oxygen vacancy content of CdZrOx solid solution catalysts by Ga for effective CO2 hydrogenation to methanol

    Separation and Purification Technology · 2024-11-28

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  26. Manipulating Oxygen Vacancies in γ-Ga2O3 Nanocrystals: Correlation between Defect Location, Charge State, and Photophysical Properties

    The Journal of Physical Chemistry Letters · 2024-12-12

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  27. Advanced metal oxide catalysts for propane dehydrogenation: from design strategy to dehydrogenation performance

    Nanoscale · 2025-01-01

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  28. Zr element promotes gallium oxide-based catalyst activity for direct dehydrogenation of propane

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  29. Ga2O3/Al2O3 Catalysts for Propane Dehydrogenation: Effect of H2 Treatment and Cofeeding

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    Sebastián Amar Gil, Catherine Especel, Francisco J. Passamonti, Valérie Montouillout, Viviana M. Benítez, Florence Epron

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  30. Enhancing Catalytic Activity of Gallium Oxide Through Transition Metal Incorporation for Ethane Oxidative Dehydrogenation in the Presence of Carbon Dioxide

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  31. Enhancing Photocatalytic Efficiency through Morphology and Bandgap Tuning in Gallium‐Doped Zinc Oxide Nanoparticles

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  32. Evolution of [Ga]+ and [GaH2]+ at Propane Dehydrogenation Conditions in MFI Zeolite: A Theoretical Investigation

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  33. Ethane Dehydrogenation over Nanostructured Ga‐Ce Bimetallic Oxide Catalysts Using N2O as Oxidant

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  34. Hydride Accessibility and Reactivity in the Configurational and Stoichiometric Space of β-Ga2O3 for CO2 Hydrogenation

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  35. Uncovering the Pressure-Dependent Mechanism of CO2 Hydrogenation to Methanol on Ga-Promoted Cu/ZrO2 Using Operando Modulation-Excitation DRIFTS

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  36. Near-Surface Hydrogen Species Tune the Selectivity of Chemical Reactions on Metal Oxide Surfaces

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  37. Unraveling the structure-activity relationship in bare Ga2O3 for propane dehydrogenation: The critical role of crystallite size and phase composition

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  38. Structure sensitivity of gallium oxide catalyzed propane dehydrogenation reaction co-fed with hydrogen

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  39. Effects of Pt loading on the activity of Pt/γ-Ga 2 O 3 for propane dehydrogenation

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  40. Engineering Ga-containing dendritic MFI zeolites as safe-by-design hierarchical and immunomodulatory nanointerfaces

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  41. Ga-induced electronic tuning of Ni catalyst surfaces: achieving activity–selectivity balance in propane dehydrogenation

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  43. Hydroxyl-facilitated efficient propane dehydrogenation over bare Ga2O3 via altering reaction pathway

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  44. Crystal Phase-Dependent Ga-H Chemistry and H 2 Roles in Ga 2 O 3 -Catalyzed Propane Dehydrogenation Reaction

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  47. Surface Oxygen Vacancies as Active Sites for Nonoxidative Propane Dehydrogenation on Metal Oxide Catalysts

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