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RESEARCH PAPER · Materials Today · 2020

Hydrogel machines

Xinyue Liu, Ji Liu, Shaoting Lin, Xuanhe Zhao

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Hydrogel machinesOriginalNanocomposite hydrogel-based strain and pressure sensors: a review420Stimuli-responsive functional materials for soft robotics255Ultrasensitive and Stretchable Temperature Sensors Based on Thermally Stable and Self-Healing Organohydrogels210Ultrafast gelling using sulfonated lignin-Fe3+ chelates to produce dynamic crosslinked hydrogel/coating with charming stretchable, conductive, self-healing, and ultraviolet-blocking properties248Programmable Reversible Shape Transformation of Hydrogels Based on Transient Structural Anisotropy145Multifunctional soft machines based on stimuli-responsive hydrogels: from freestanding hydrogels to smart integrated systems141Porous self-floating 3D Ag2O/g-C3N4 hydrogel and photocatalytic inactivation of Microcystis aeruginosa under visible light95Analytical Modeling and Design of Generalized Pneu-Net Soft Actuators with Three-Dimensional Deformations96Soft Actuators for Soft Robotic Applications: A Review552Material innovation and mechanics design for substrates and encapsulation of flexible electronics: a review221Functional hydrogel coatings483Recent Progress in Artificial Muscles for Interactive Soft Robotics2893D Printing of Strong and Tough Double Network Granular Hydrogels168Engineering Biofunctional Enzyme‐Mimics for Catalytic Therapeutics and Diagnostics96The new generation of soft and wearable electronics for health monitoring in varying environment: From normal to extreme conditions224HASEL Artificial Muscles for a New Generation of Lifelike Robots—Recent Progress and Future Opportunities248Multifunctional magnetic soft composites: a review3073D Printing of Dual-Physical Cross-linking Hydrogel with Ultrahigh Strength and Toughness1874D Printable Tough and Thermoresponsive Hydrogels133Multiple-Stimuli-Responsive and Cellulose Conductive Ionic Hydrogel for Smart Wearable Devices and Thermal Actuators228Conducting polymers: a comprehensive review on recent advances in synthesis, properties and applications1354Gels as emerging anti-icing materials: a mini review109Recent advances in materials for hemostatic management101Recent progress on hydrogel actuators111Small molecule-based supramolecular-polymer double-network hydrogel electrolytes for ultra-stretchable and waterproof Zn–air batteries working from −50 to 100 °C184Bioinspired 3D Printable, Self-Healable, and Stretchable Hydrogels with Multiple Conductivities for Skin-like Wearable Strain Sensors193Hydrogel: Diversity of Structures and Applications in Food Science209Mussel-inspired nanozyme catalyzed conductive and self-setting hydrogel for adhesive and antibacterial bioelectronics230Advanced applications of chitosan-based hydrogels: From biosensors to intelligent food packaging system217Endoscopy-assisted magnetic navigation of biohybrid soft microrobots with rapid endoluminal delivery and imaging360Fabricating hydrogels to mimic biological tissues of complex shapes and high fatigue resistance159Reconstructable Gradient Structures and Reprogrammable 3D Deformations of Hydrogels with Coumarin Units as the Photolabile Crosslinks160Engineering Hydrogel Adhesion for Biomedical Applications via Chemical Design of the Junction298Adaptive Ionogel Paint from Room‐Temperature Autonomous Polymerization of α‐Thioctic Acid for Stretchable and Healable Electronics241Soft Materials by Design: Unconventional Polymer Networks Give Extreme Properties1161Self-powered locomotion of a hydrogel water strider105Engineering Hydrogel‐Based Biomedical Photonics: Design, Fabrication, and Applications156Soft Wearable Healthcare Materials and Devices160Soft Robotic Manipulators: Designs, Actuation, Stiffness Tuning, and Sensing237Elastomeric Haptic Devices for Virtual and Augmented Reality107Anisotropically Fatigue‐Resistant Hydrogels351Recent advances of organogels: from fabrications and functions to applications128Programmable Mechanically Active Hydrogel‐Based Materials104An Anti‐Freezing, Ambient‐Stable and Highly Stretchable Ionic Skin with Strong Surface Adhesion for Wearable Sensing and Soft Robotics273Fast-Recoverable, Self-Healable, and Adhesive Nanocomposite Hydrogel Consisting of Hybrid Nanoparticles for Ultrasensitive Strain and Pressure Sensing116Cutaneous Ionogel Mechanoreceptors for Soft Machines, Physiological Sensing, and Amputee Prostheses290Stimuli-Responsive Toughening of Hydrogels145Role of chitosan-based hydrogels in pollutants adsorption and freshwater harvesting: A critical review94Stretchable and self-healable hydrogel artificial skin117Trigger‐Detachable Hydrogel Adhesives for Bioelectronic Interfaces160A stretchable and adhesive ionic conductor based on polyacrylic acid and deep eutectic solvents130Self‐Shaping Soft Electronics Based on Patterned Hydrogel with Stencil‐Printed Liquid Metal172Recent advances in atmosphere water harvesting: Design principle, materials, devices, and applications124Graphene Oxide Encapsulating Liquid Metal to Toughen Hydrogel178One stone for three birds: One-step engineering highly elastic and conductive hydrogel electronics with multilayer MXene as initiator, crosslinker and conductive filler simultaneously1153D Printing of Hydrogels for Stretchable Ionotronic Devices148Bifunctional Smart Hydrogel Dressing with Strain Sensitivity and NIR-Responsive Performance122Skin-like hydrogel devices for wearable sensing, soft robotics and beyond230Recent Progress in Materials Chemistry to Advance Flexible Bioelectronics in Medicine132Polymeric Hydrogels—A Promising Platform in Enhancing Water Security for a Sustainable Future112Hydrogel Ionotronics with Ultra‐Low Impedance and High Signal Fidelity across Broad Frequency and Temperature Ranges98Tough, Transparent, 3D‐Printable, and Self‐Healing Poly(ethylene glycol)‐Gel (PEGgel)148Water-resistant and underwater adhesive ion-conducting gel for motion-robust bioelectric monitoring114Bioinspired 2D Isotropically Fatigue‐Resistant Hydrogels174Hofmeister Effect and Electrostatic Interaction Enhanced Ionic Conductive Organohydrogels for Electronic Applications140Tough Hydrogel Bioadhesives for Sutureless Wound Sealing, Hemostasis and Biointerfaces200Transparent stretchable hydrogel sensors: materials, design and applications112Supramolecular Adhesive Hydrogels for Tissue Engineering Applications711Magnetic Soft Materials and Robots873Azo-Crosslinked Double-Network Hydrogels Enabling Highly Efficient Mechanoradical Generation101Highly Conducting and Stretchable Double‐Network Hydrogel for Soft Bioelectronics443New Insights of Scaffolds Based on Hydrogels in Tissue Engineering198Design of untethered soft material micromachine for life-like locomotion99Engineered Living Hydrogels220Paper‐Structure Inspired Multiresponsive Hydrogels with Solvent‐Induced Reversible Information Recording, Self‐Encryption, and Multidecryption113A Structural Gel Composite Enabled Robust Underwater Mechanosensing Strategy with High Sensitivity169High Quantum Yield Nitrogen-Doped Carbon Quantum Dot-Based Fluorescent Probes for Selective Sensing of 2,4,6-Trinitrotoluene132Hydrogel Bioadhesives with Extreme Acid‐Tolerance for Gastric Perforation Repairing141Programmable Morphing Hydrogels for Soft Actuators and Robots: From Structure Designs to Active Functions273Hydrogel-based strong and fast actuators by electroosmotic turgor pressure308Adhesive and Hydrophobic Bilayer Hydrogel Enabled On‐Skin Biosensors for High‐Fidelity Classification of Human Emotion177Highly stretchable, durable, and transient conductive hydrogel for multi-functional sensor and signal transmission applications164High‐Stretchability, Ultralow‐Hysteresis ConductingPolymer Hydrogel Strain Sensors for Soft Machines574Fatigue-free artificial ionic skin toughened by self-healable elastic nanomesh258Elastic, tough and switchable swelling hydrogels with high entanglements and low crosslinks for water remediation100Tough, anti-freezing and conductive ionic hydrogels122Synthesis and Applications of Carboxymethyl Cellulose Hydrogels141Unbreakable Hydrogels with Self‐Recoverable 10 200% Stretchability109Hydrogel‐Based Flexible Electronics796Gradient Adhesive Hydrogel Decorated Superhydrophilic Membranes for Ultra‐Stable Oil/Water Separation155Intrinsically Electron Conductive, Antibacterial, and Anti‐swelling Hydrogels as Implantable Sensors for Bioelectronics122Ultrastrong, highly conductive and capacitive hydrogel electrode for electron-ion transduction105Hydrogel interfaces for merging humans and machines661Impact‐Resistant Hydrogels by Harnessing 2D Hierarchical Structures154Strong and Ultra‐Tough Supramolecular Hydrogel Enabled by Strain‐Induced Microphase Separation143A stretchable and conductive design based on multi-responsive hydrogel for self-sensing actuators137Engineering Electrodes with Robust Conducting Hydrogel Coating for Neural Recording and Modulation140Tough Ionogels: Synthesis, Toughening Mechanisms, and Mechanical Properties─A Perspective161Functional Tough Hydrogels: Design, Processing, and Biomedical Applications151Functional conductive hydrogels: from performance to flexible sensor applications101Naturally sourced hydrogels: emerging fundamental materials for next-generation healthcare sensing392Concurrent stiffening and softening in hydrogels under dehydration150Strong and tough fibrous hydrogels reinforced by multiscale hierarchical structures with multimechanisms279Smart Skin‐Adhesive Patches: From Design to Biomedical Applications94Mechanically Robust and Transparent Organohydrogel‐Based E‐Skin Nanoengineered from Natural Skin171Recent Progress of Conductive Hydrogel Fibers for Flexible Electronics: Fabrications, Applications, and Perspectives233Deep Eutectic Solvents‐Based Ionogels with Ultrafast Gelation and High Adhesion in Harsh Environments178Entanglement in Smart Hydrogels: Fast Response Time, Anti‐Freezing and Anti‐Drying158Production of Polymer Hydrogel Composites and Their Applications268Hydrogen Bonding Enables Polymer Hydrogels with pH‐Induced Reversible Dynamic Responsive Behaviors94Active Materials for Functional Origami169Flexible Electrodes for Brain–Computer Interface System133Photoresponsive hydrogel-based soft robot: A review96Stimuli-bioresponsive hydrogels as new generation materials for implantable, wearable, and disposable biosensors for medical diagnostics: Principles, opportunities, and challenges116Functionalized Hydrogel-Based Wearable Gas and Humidity Sensors234Multi‐Bioinspired Functional Conductive Hydrogel Patches for Wound Healing Management129Mechanically‐Compliant Bioelectronic Interfaces through Fatigue‐Resistant Conducting Polymer Hydrogel Coating148Sustainable electronic textiles towards scalable commercialization173Tailoring the Swelling‐Shrinkable Behavior of Hydrogels for Biomedical Applications548Hydrogel muscles powering reconfigurable micro-metastructures with wide-spectrum programmability133Designing nanohesives for rapid, universal, and robust hydrogel adhesion145Bio-inspired anisotropic hydrogels and their applications in soft actuators and robots120Bioinspired polydopamine hydrogels: Strategies and applications285Multimaterial 3D and 4D Bioprinting of Heterogenous Constructs for Tissue Engineering154Advanced in carbon dot-based hydrogels for antibacterial, detection and adsorption119Fatigue-resistant hydrogel optical fibers enable peripheral nerve optogenetics during locomotion101Multifunctional solar water harvester with high transport selectivity and fouling rejection capacity133Cascade-heterogated biphasic gel iontronics for electronic-to-multi-ionic signal transmission113High-Saline-Enabled Hydrophobic Homogeneous Cross-Linking for Extremely Soft, Tough, and Stretchable Conductive Hydrogels as High-Sensitive Strain Sensors104Self‐Healing Hydrogel Bioelectronics2573D Printed Implantable Hydrogel Bioelectronics for Electrophysiological Monitoring and Electrical Modulation159Hydrogel sensors for biomedical electronics133Chitosan-based hydrogels: From preparation to applications, a review2303D printing of magneto-active smart materials for advanced actuators and soft robotics applications190Design of Fatigue‐Resistant Hydrogels132Hydrogels for bioinspired soft robots154Fully Polymeric Conductive Hydrogels with Low Hysteresis and High Toughness as Multi‐Responsive and Self‐Powered Wearable Sensors169N-type semiconducting hydrogel218Electronic Skin for Health Monitoring Systems: Properties, Functions, and Applications175In Situ Structural Densification of Hydrogel Network and Its Interface with Electrodes for High-Performance Multimodal Artificial Skin106Constructing phase separation in polymer gels: Strategies, functions and applications108Glassy gels toughened by solvent172Mechanical Regulation of Polymer Gels146Lithography-based 3D printing of hydrogels1023D Printing‐Based Hydrogel Dressings for Wound Healing157Preparation schemes and applications of multifunctional PVA composite hydrogels110Noncovalent Aggregation for Diverse Properties in Hydrogels: A Comprehensive Review113PEDOT:PSS-based electronic materials: Preparation, performance tuning, processing, applications, and future prospect128Technology Roadmap of Micro/Nanorobots126Therapeutic Hydrogels: Properties and Biomedical Applications154

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