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RESEARCH PAPER · Journal of the American Chemical Society · 2022

Lignin-Supported Heterogeneous Photocatalyst for the Direct Generation of H 2 O 2 from Seawater

Aswin Gopakumar, Peng Rong Ren, Jianhong Chen, Bruno V. M. Rodrigues, H. Y. Vincent Ching, Aleksander Jaworski, Sabine Van Doorslaer, Anna Rokicińska, Piotr Kuśtrowski, Giovanni Barcaro, Susanna Monti, Adam Slabon, Shoubhik Das

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Lignin-Supported Heterogeneous Photocatalyst for the Direct Generation of H 2 O 2 from SeawaterOriginalPhotocatalytic Hydrogen Peroxide Production in Natural Seawater by Agqds(0d)/Bi2o3(3d) Hybrid Structure for In-Situ Bacterial Inactivation8Photosynthesis of Hydrogen Peroxide for In-Situ Bacterial Inactivation in Natural Seawater Based on Agqds/Bi2o3 Photocatalysts0Urushiol derivatives as biomass-based photocatalysts for the transition-metal-free synthesis of 1,2-amino alcohols25Recent advances in bismuth-based photocatalysts: Environment and energy applications185Graphene oxide coupled high-index facets CdZnS with rich sulfur vacancies for synergistic boosting visible-light-catalytic hydrogen evolution in natural seawater: Experimental and DFT study35Electrochemical Depolymerization of Lignin in a Biomass‐based Solvent**41Versatile Gold Telluride Iodide Monolayer as a Potential Photocatalyst for Water Splitting4Nanostructured α‐Fe2O3 Photoelectrodes with Transparent and Conducting Sb‐Doped SnO2 Films Deposited by Atomic Layer Deposition6Carbon dots-modulated covalent triazine frameworks with exceptionally rapid hydrogen peroxide production in water57Critical roles of H2O and O2 in H2O2 photoproduction over biomass derived metal-free catalyst39Electronic Control of Traditional Iron–Carbon Electrodes to Regulate the Oxygen Reduction Route to Scale Up Water Purification33Metal‐Free Photocatalysts for Conversion of H2O into Hydrogen Peroxide33Supported nanostructured photocatalysts: the role of support-photocatalyst interactions45Boosted H2O2 Productivity by Sulfur-Doped Pd/Carbon Catalysts via Direct Synthesis from H2 and O2 at Atmospheric Pressure17Selective functionalization of benzylic C(sp3)–H bonds to synthesize complex molecules104On factors of ions in seawater for CO2 reduction37Regulating the Electronic Structure of Fe3+-Doped BiOClxI1–x Solid Solution by an Amidoxime-Functionalized Fibrous Support for Efficient Photocatalysis37Enhancement of visible-light-driven oxidative amine coupling under aerobic and anaerobic conditions by photocatalyst with spatial separation of photoinduced charge carriers18Catalytic production of hydrogen peroxide and its fuel cells with metalloporphyrins, metallophthalocyanines, and analogs5Solvent effect on the production of spherical lignin nanoparticles61Beyond Photosynthesis: H2O/H2O2/O2 Self-Circulation-Based Biohybrid Photoelectrochemical Cells for Direct and Sustainable Solar-to-Fuel-to-Electric Power Conversion39Photocatalytic generation of H 2 O 2 over a Z-scheme Fe 2 O 3 @C@1T/2H-MoS 2 heterostructured catalyst for high-performance Fenton reaction40Photodegradation of tetracycline antibiotic by ternary recyclable Z-scheme g-C3N4/Fe3O4/Bi2WO6/Bi2S3 photocatalyst with improved charge separation efficiency: Characterization and mechanism studies37A general interfacial-energetics-tuning strategy for enhanced artificial photosynthesis74Organic-inorganic interface chemistry for sustainable materials2Visible-light-induced sulfoxidation using chitosan-supported organic dyes photocatalyst4Biobased polymers from lignocellulosic sources35Extending the π-conjugation system of covalent organic frameworks for more efficient photocatalytic H 2 O 2 production160Gold–nickel phosphide heterostructures for efficient photocatalytic hydrogen peroxide production from real seawater11Highly efficient photocatalytic H 2 O 2 production in microdroplets: accelerated charge separation and transfer at interfaces124Ligand functionalization on Zr-MOFs enables efficient visible-light-driven H 2 O 2 evolution in pure water63MoS 2 nanoflower-decorated lignin nanoparticles for superior lubricant properties13Photocatalysis with atomically thin sheets78Crystal Engineering Enables Cobalt-Based Metal–Organic Frameworks as High-Performance Electrocatalysts for H 2 O 2 Production229Coupling functional anodes with natural air-diffused cathodes enables highly efficient hydrogen peroxide electrosynthesis18Micro-Batch flow reactor for the photoproduction of H2O2 from water/real seawater10Photothermal-enabled single-atom catalysts for high-efficiency hydrogen peroxide photosynthesis from natural seawater167Simultaneous Generation of H2O2 and Formate by Co‐Electrolysis of Water and CO2 over Bifunctional Zn/SnO2 Nanodots43Simultaneous Generation of H2O2 and Formate by Co‐Electrolysis of Water and CO2 over Bifunctional Zn/SnO2 Nanodots3Plasmon Bi in-situ anchored on BiOCl nanosheets assembled microspheres towards optimized photothermal-photocatalytic performance49Iodide-Mediated Etching of Gold Nanostar for the Multicolor Visual Detection of Hydrogen Peroxide5Synergistic Metal‐Nonmetal Active Sites in a Metal‐Organic Cage for Efficient Photocatalytic Synthesis of Hydrogen Peroxide in Pure Water129Synergistic Metal‐Nonmetal Active Sites in a Metal‐Organic Cage for Efficient Photocatalytic Synthesis of Hydrogen Peroxide in Pure Water14Cyano‐Regulated Organic Polymers for Highly Efficient Photocatalytic H 2 O 2 Production in Various Actual Water Bodies61Covalent organic frameworks for direct photosynthesis of hydrogen peroxide from water, air and sunlight391An Atomically Dispersed Mn-Photocatalyst for Generating Hydrogen Peroxide from Seawater via the Water Oxidation Reaction (WOR)231An organic perspective on photocatalytic production of hydrogen peroxide326Thiophene‐Containing Covalent Organic Frameworks for Overall Photocatalytic H 2 O 2 Synthesis in Water and Seawater360Thiophene‐Containing Covalent Organic Frameworks for Overall Photocatalytic H 2 O 2 Synthesis in Water and Seawater16Clean Production of Hydrogen Peroxide: A Heterogeneous Solar‐Driven Redox Process163CoIn dual-atom catalyst for hydrogen peroxide production via oxygen reduction reaction in acid201Preparation of palladium complex supported on magnetic lignin as an effective catalyst for C-N coupling reaction2Sustainable and Continuous Flow Preparation of High-Concentration H 2 O 2 by Visible-Light-Activated Molecular Oxygen Oxidation of Lower Alcohols13Construction of a P, N Co-Doped Nanocarbon-Embedded g-C3N4 Hollow Sphere Nanoreactor for the Efficient Photocatalytic Production of Hydrogen Peroxide39Solar‐driven seawater production H2O2 catalyzed by hydroxyl functionalized crystalline K‐doped g‐C3N4 under ambient conditions10Visible‐Light‐Driven Selective Hydrogenation of Nitrostyrene over Layered Ternary Sulfide Nanostructures8Recoverable Nanocatalyst for Regioselective Triazoles Synthesis: Lignin‐Copper(I) Nanomagnetic Composite3Coordination engineering regulating metal single-atom anchored on n-doped carbon as a bifunctional catalyst for H2O2 production via dual channels24Construction of catalytic ozonation synergistic photo-self-Fenton system and analysis of synergistic catalysis and reaction mechanism activated by modified carbon nitride36Fragmentation engineering on the edge of hydroxy-functional COFs for the enhanced photocatalytic production of H2O2 and direct photo-oxidation of benzene to phenol in aqueous systems35Polymer semiconductors: A unique platform for photocatalytic hydrogen peroxide production81Promoting photo-Fenton reactions by anchoring Fe doped g-C3N4 onto an amidoxime-functionalized fibrous support for organic contaminants removal7Interaction of metal ions in high efficiency seawater hydrogen peroxide production by a carbon-based photocatalyst33Iron oxide-promoted photochemical oxygen reduction to hydrogen peroxide (H 2 O 2 )12Defect-engineered Zr-MOFs with enhanced O 2 adsorption and activation for photocatalytic H 2 O 2 synthesis20Efficient Hydrogen Peroxide Photosynthesis over CdS/COF for Water Disinfection: The S-Scheme Pathway, Oxygen Adsorption, and Reactor Design53Coumarin-based composite material for the latent fingerprint visualization and electrochemical sensing of hydrogen peroxide11Catalyst-free contact-electro-catalytic H 2 O 2 synthesis via simple combination of a poly(tetrafluoroethylene) stir bar and ultrasound26Continuous photocatalytic preparation of hydrogen peroxide with anthraquinone photosensitizers31Cooperative tungsten centers in polymeric carbon nitride for efficient overall photosynthesis of hydrogen peroxide167Highly coordinative molecular cobalt–phthalocyanine electrocatalyst on an oxidized single-walled carbon nanotube for efficient hydrogen peroxide production21Highly selective hydrogen peroxide electrosynthesis on copper phthalocyanine: interface engineering with an azo-polymer6The evolution of photocatalytic H 2 O 2 generation: from pure water to natural systems and beyond154Transition metal chalcogenide nanoparticle embedded metal–organic framework nanosheets for high-performance H 2 O 2 electrosynthesis10Atomically Dispersed Iron Active Sites on Covalent Organic Frameworks for Artificial Photosynthesis of Hydrogen Peroxide77Cutaneous respiration inspired porous seawater electrodes3Photocatalytic hydrogen production from seawater splitting: Current status, challenges, strategies and prospective applications184Visible-Light Photocatalytic H2O2 Production Boosted by Frustrated Lewis Pairs in Defected Polymeric Carbon Nitride Nanosheets129Ligand Functionalization of Metal‐Organic Frameworks for Photocatalytic H2O2 Production15Interface Chemical Bond Enhanced Ions Intercalated Carbon Nitride/CdSe‐Diethylenetriamine S‐Scheme Heterojunction for Photocatalytic H 2 O 2 Synthesis in Pure Water119Photocatalytic hydrogen peroxide production from seawater over graphitic carbon nitride supported titanium dioxide quantum dots11Regulating the H 2 O 2 Photosynthetic Activity of Covalent Organic Frameworks through Linkage Orientation157In-situ study of the hydrogen peroxide photoproduction in seawater on carbon dot-based metal-free catalyst under operation condition39Boosting excitons dissociation in defective-rich graphitic carbon nitride for efficient hydrogen peroxide photosynthesis and on-site environmental governance50Two-phase reaction system for efficient photocatalytic production of hydrogen peroxide69Rational Design of Covalent Organic Frameworks with Redox-Active Catechol Moieties for High-Performance Overall Photosynthesis of Hydrogen Peroxide131Photocatalytic synthesis of high-concentration hydrogen peroxide by efficient photothermal synergy14Dual Channel H2O2 Photosynthesis in Pure Water over S‐Scheme Heterojunction Cs3PMo12/CC Boosted by Proton and Electron Reservoirs2Developing Polymeric Carbon Nitrides for Photocatalytic H2O2 Production27Protonation of an Imine‐linked Covalent Organic Framework for Efficient H 2 O 2 Photosynthesis under Visible Light up to 700 nm24Protonation of an Imine‐linked Covalent Organic Framework for Efficient H 2 O 2 Photosynthesis under Visible Light up to 700 nm183Boosting H2O2 photosynthesis by accumulating photo-electrons on carbonyl active site of polyimide covalent organic frameworks73Metal‐Organic Framework Templated Z‐Scheme ZnIn 2 S 4 /Bi 2 S 3 Hierarchical Heterojunction for Photocatalytic H 2 O 2 Production from Wastewater48Enhancing the crystallinity of covalent organic frameworks to achieve improved photocatalytic hydrogen peroxide production under ambient conditions12Water quality constraints H2O2 production in a dual-fiber photocatalytic reactor13A recyclable ZnIn2S4/PAN photocatalytic nanofiber membrane for boosting visible light hydrogen evolution in seawater without cocatalyst44Innovative lignin photocatalyst system motivated by intramolecular charge dynamics for H2O2 production302D photocatalysts for hydrogen peroxide synthesis47Double-Layered Sillen–Aurivillius Perovskite Oxybromide Sr2Bi3Nb2O11Br as a Fatigue-Free Piezocatalyst with Ultrahigh Hydrogen Evolution Performance12A photocatalytic redox cycle over a polyimide catalyst drives efficient solar-to-H2O2 conversion153Achieving a solar-to-chemical efficiency of 3.6% in ambient conditions by inhibiting interlayer charges transport87Photocatalytic production of H2O2 and its in-situ environmental applications42Photothermal-enabled metal-free polyfuran photocatalysts for efficient solar-to-hydrogen peroxide energy conversion from seawater16Heterostructure engineering of resorcinol-formaldehyde resins and sulfur-vacancy-containing Zn3In2S6 for high-efficiency photocatalytic H2O2 production24Proton‐Enriched Alginate–Graphene Hydrogel Microreactor for Enhanced Hydrogen Peroxide Photosynthesis3Proton‐Enriched Alginate–Graphene Hydrogel Microreactor for Enhanced Hydrogen Peroxide Photosynthesis57Nitrogen‐Site Engineering in Covalent Organic Frameworks for H 2 O 2 Photogeneration via Dual Channels of Indirect Two‐Electron O 2 Reduction36Hierarchical Hybrids Made of Mixed Metal-Based Sillén-Structured CdxBiO2Br @ Graphene Oxide for Efficient Photocatalytic H2O2 Production7Boosting carriers transfer efficiency by 3D vector channels for ameliorating photosynthesis H2O21Recyclable hydrogen peroxide photosynthesis over Z-scheme In2O3/g-C3N4 heterojunction with viable reduction of superoxide radical intermediate14Simultaneous efficient production of hydrogen peroxide, urea and H2 by bifunctional Cu-doped TiO2 electrocatalyst from CO2, N2 and water2Functionalized Modification of Conjugated Porous Polymers for Full Reaction Photosynthesis of H 2 O 265Hydrogen production using vinasse as sacrificial agent and Pt/TiO2 as photocatalyst under UV irradiation0Isolated Ni Atoms for Enhanced Photocatalytic H2O2 Performance with 1.05% Solar-to-Chemical Conversion Efficiency in Pure Water25Al–N 3 Bridge Site Enabling Interlayer Charge Transfer Boosts the Direct Photosynthesis of Hydrogen Peroxide from Water and Air74Pioneering technologies over time to rehabilitate crude oil–contaminated ecosystems: a review4Lignin‐Assisted Photoreactions: Unveiling New Frontiers in Light‐Induced Chemistry10Covalent Organic Frameworks with Constrained Palladium Nanoclusters Lock the Enol‐Keto Tautomerism Enhancing Hydrogen Peroxide Photosynthesis15Selective Oxygen Activation by Integrating Dual Photosensitizers in Conjugated Porous Polymers and Microenvironments Manipulation for High‐Performance Water Purification and H 2 O 2 Production23Polymer gels for solar-driven interfacial evaporation9Compressive interatomic distance stimulates photocatalytic oxygen-oxygen coupling to hydrogen peroxide41Interfacial Engineering of β‐Ketoenamine‐Based COFs/Urea‐Linked Perylene Diimide for Overall Photosynthesis of H2O2 in Seawater21Oxygen Gas Nanovessel Promotes Hydrogen Peroxide Photosynthesis5Photocatalytic Partial Water Oxidation Promoted by a Hydrogen Acceptor‐Hydroxyl Mediator Couple9Mineral-Mediated Epitaxial Growth of CoO Nanoparticles for Efficient Electrochemical H 2 O 2 Activation14Overall solar H2O2 generation in water and real seawater by covalent organic frameworks with kgd topology28Lignin Quaternary Ammonium Phosphotungstate as a Recycle Catalyst for Oxidative Cleavage of Unsaturated Fatty Acids and Soybean Oil5Assembling graphene quantum dots on aminophenol-formaldehyde resin towards efficient artificial photocatalytic hydrogen peroxide synthesis14Enhanced redox kinetics for hydrogen peroxide photosynthesis at high-concentration by encapsulating porphyrin metal–organic frameworks with phenolic resin77Vinasse photoreforming for hydrogen production using Pt/TiO 2 as catalyst under UV irradiation2Construction of spherical WO3/CdS S-scheme heterojunction for photocatalytic H2O2 production in real seawater15Boosting lignin‐based photocatalyst with photocorrosion resistance for efficient H2O2 production via hetero‐interfacial π‐π stacking channels23Photoelectrocatalytic Pathway for the Preparation of Power‐Effective Aviation Fuel Precursors from Lignin34Enhanced Electrocatalytic Hydrogen Peroxide Production via a CuWO4/WO3 Heterojunction with High Selectivity and Stability9Electrocatalytic synthesis of pure H2O2 from crossover oxygen through a porous proton exchange membrane6One‐Pot Synthesis of Fully Conjugated Covalent Organic Frameworks via the Pictet–Spengler Reaction for Boosting H 2 O 2 Photogeneration in Real Seawater53Leveraging Carbon Quantum Dot Spacers as Dual Proton/Electron Boosters to Upgrade TiO 2 @Polydopamine Photocatalysts for pH‐Resilient Conversion of O 2 into H 2 O 214Leveraging Carbon Quantum Dot Spacers as Dual Proton/Electron Boosters to Upgrade TiO 2 @Polydopamine Photocatalysts for pH‐Resilient Conversion of O 2 into H 2 O 223Sulphur-doped carbon electrodes for electrocatalytic production of hydrogen peroxide via oxygen reduction2Boosting hydrogen peroxide electro-generation by adjusting the wetting state of porous Janus electrode during oxygen reduction reaction3Biomass-derived carbon for solar H2O2 production: Current trends and future directions6A photothermal-photocatalytic layered aerogel for harvesting water and hydrogen from seawater23NiB as a Non-noble Metal Cocatalyst Electronic Bridge to Enhance the Photocatalytic Hydrogen Production of Cd3(C3N3S3)222Surface Properties of High-Performing Bi24O31Br10 and its Acid-Driven Conversion to BiOX Photocatalysts (X = Cl, Br)3Shaping the future of solar-driven photocatalysis by reticular framework materials45The bidirectional matter transfer in adsorption-promoted photocatalytic ozonation system derived by triazine nanosheets-heptazine nanotubes homojunction composite biochar11The Redox Cycle of Viologen‐Based Porous Organic Polymers for High‐Performance Hydrogen Peroxide Photosynthesis7Nb2C MXene quantum dots modulate built-in electric field within heterostructures for efficient solar-to-H2O2 conversion from seawater37Zwitterionic covalent organic framework triggering enhanced H2O2 photoproduction via controllable built-in electric field design14Sunlight-driven simultaneous CO2 reduction and water oxidation using indium-organic framework heterostructures102

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  31. Ligand functionalization on Zr-MOFs enables efficient visible-light-driven H 2 O 2 evolution in pure water

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  32. MoS 2 nanoflower-decorated lignin nanoparticles for superior lubricant properties

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  33. Photocatalysis with atomically thin sheets

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  34. Crystal Engineering Enables Cobalt-Based Metal–Organic Frameworks as High-Performance Electrocatalysts for H 2 O 2 Production

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  35. Coupling functional anodes with natural air-diffused cathodes enables highly efficient hydrogen peroxide electrosynthesis

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  36. Micro-Batch flow reactor for the photoproduction of H2O2 from water/real seawater

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  37. Photothermal-enabled single-atom catalysts for high-efficiency hydrogen peroxide photosynthesis from natural seawater

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  38. Simultaneous Generation of H2O2 and Formate by Co‐Electrolysis of Water and CO2 over Bifunctional Zn/SnO2 Nanodots

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  39. Simultaneous Generation of H2O2 and Formate by Co‐Electrolysis of Water and CO2 over Bifunctional Zn/SnO2 Nanodots

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