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RESEARCH PAPER · Angewandte Chemie International Edition · 2022

Intermolecular Energy Gap‐Induced Formation of High‐Valent Cobalt Species in CoOOH Surface Layer on Cobalt Sulfides for Efficient Water Oxidation

Na Yao, Gongwei Wang, Hongnan Jia, Jinlong Yin, Hengjiang Cong, Shengli Chen, Wei Luo

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Intermolecular Energy Gap‐Induced Formation of High‐Valent Cobalt Species in CoOOH Surface Layer on Cobalt Sulfides for Efficient Water OxidationOriginalSuperior bifunctional cobalt/nitrogen-codoped carbon nanosheet arrays on copper foam enable stable energy-saving hydrogen production accompanied with glucose upgrading42The in situ formation of defective CoOOH catalysts from semi-oxidized Co for alkaline oxygen evolution reaction49CeO2 Functionalized Cobalt Layered Double Hydroxide for Efficient Catalytic Oxygen‐Evolving Reaction73Core–Shell Carbon‐Based Bifunctional Electrocatalysts Derived from COF@MOF Hybrid for Advanced Rechargeable Zn–Air Batteries98Modulation of the interfacial charge density on Fe2P–CoP by coupling CeO2 for accelerating alkaline electrocatalytic hydrogen evolution reaction and overall water splitting115The critical role of A, B-site cations and oxygen vacancies on the OER electrocatalytic performances of Bi0.15Sr0.85Co1−Fe O3−δ (0.2 ≤ x ≤ 1) perovskites in alkaline media74Dealloying‐Derived Porous Spinel Oxide for Bifunctional Oxygen Electrocatalysis and Rechargeable Zinc‐Air Batteries: Promotion of Activity Via Hereditary Al‐Doping20Electron modulation by atomic Ir site decoration in porous Co/N co-doped carbon for electrocatalytic hydrogen evolution18Surface reconstruction-derived heterostructures for electrochemical water splitting171Single-atom Fe Embedded CO3S4 for Efficient Electrocatalytic Oxygen Evolution Reaction25Manipulating the morphology and the electronic structures of nickel-cobalt selenides@N-doped carbon for aqueous alkaline batteries9NiMn-based metal-organic framework with optimized eg orbital occupancy as efficient bifunctional electrocatalyst for lithium-oxygen batteries67CoP/Fe‐Co9S8 for Highly Efficient Overall Water Splitting with Surface Reconstruction and Self‐Termination52Hollow NiCoP Nanoprisms Derived from Prussian Blue Analogues as Bifunctional Electrocatalysts for Urea‐Assisted Hydrogen Production in Alkaline Media104Identifying the geometric catalytic active sites of crystalline cobalt oxyhydroxides for oxygen evolution reaction223Effect of Proton Transfer on Electrocatalytic Water Oxidation by Manganese Phosphates56Effect of Proton Transfer on Electrocatalytic Water Oxidation by Manganese Phosphates12Coupling Plant Polyphenol Coordination Assembly with Co(OH)2 to Enhance Electrocatalytic Performance towards Oxygen Evolution Reaction19Reconstructured Electrocatalysts during Oxygen Evolution Reaction under Alkaline Electrolytes22Transformation mechanism of high-valence metal sites for the optimization of Co- and Ni-based OER catalysts in an alkaline environment: recent progress and perspectives45Waste to Treasure: Regeneration of Porous Co-Based Catalysts from Spent LiCoO2 Cathode Materials for an Efficient Oxygen Evolution Reaction34CeO2 nanoparticles-decorated CoP nanocubes for accelerating alkaline electrocatalytic oxygen evolution reaction12Constructing Cation Vacancy Defects on NiFe-LDH Nanosheets for Efficient Oxygen Evolution Reaction26Design of polymetallic sulfide NiS 2 @Co 4 S 3 @FeS as bifunctional catalyst for high efficiency seawater splitting12Enhancing the electrocatalytic activity of metal–organic frameworks in the oxygen evolution reaction by introducing high-valent metal centers38Role of cobalt phthalocyanine on the formation of high-valent cobalt species revealed by in situ Raman spectroscopy95Slow O–H Dissociation in the First-Order Oxygen Evolution Reaction Kinetics on Polycrystalline γ-FeO(OH)26Unsaturated single-atom CoN3 sites for improved fenton-like reaction towards high-valent metal species88Adenosine triphosphate induced transition-metal phosphide nanostructures encapsulated with N, P-codoped carbon toward electrochemical water splitting32In Situ Surface Reconstruction of Catalysts for Enhanced Hydrogen Evolution26Introducing High‐Valence Iridium Single Atoms into Bimetal Phosphides toward High‐Efficiency Oxygen Evolution and Overall Water Splitting67Revealing the Generation of High-Valent Cobalt Species and Chlorine Dioxide in the Co3O4-Activated Chlorite Process: Insight into the Proton Enhancement Effect113Sulphur-dopant induced breaking of the scaling relation on low-valence Ni sites in nickel ferrite nanocones for water oxidation with industrial-level current density107Long-lasting performance of high-flux perovskite membrane for catalytic degradation of organic pollutants48Composition-Tunable Co3–xFexMo3N Electrocatalysts for the Oxygen Evolution Reaction70Spinel-Derived Formation and Amorphization of Bimetallic Oxyhydroxides for Efficient Electrocatalytic Biomass Oxidation18Boosting Hydrogen Oxidation Kinetics by Promoting Interfacial Water Adsorption on d-p Hybridized Ru Catalysts102Asymmetrically Coordinated CoB 1 N 3 Moieties for Selective Generation of High‐Valence Co‐Oxo Species via Coupled Electron–Proton Transfer in Fenton‐like Reactions275Unveiling anion induced surface reconstruction of perovskite oxide for efficient water oxidation70Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design802Remote Synergy between Heterogeneous Single Atoms and Clusters for Enhanced Oxygen Evolution83Promoting Plasmonic Hot Hole Extraction and Photothermal Effect for the Oxygen Evolution Reactions5Modulating the electronic structure of CoS2 by Sn doping boosting urea oxidation for efficient alkaline hydrogen production27Al3+ leaching induced Co4+ on CoFeAl layered double hydroxide for enhanced oxygen evolution reaction20Regulating electronic states of nitride/hydroxide to accelerate kinetics for oxygen evolution at large current density552Atomically dispersed Ru oxide catalyst with lattice oxygen participation for efficient acidic water oxidation390Biphasic Transition Metal Nitride Electrode Promotes Nucleophile Oxidation Reaction for Practicable Hybrid Water Electrocatalysis145Surface Reconstruction of Covellite CuS Nanocrystals for Enhanced OER Catalytic Performance in Alkaline Solution88Oxidative contaminant degradation on bimetallic boride electrocatalysts enhances anodic charge transfer for efficient H2 production3Heterogeneous activation of peroxymonosulfate by flower-like cobalt sulfide enhanced sulfamethoxazole degradation via non-radical pathways21Spatially confined sub-nanometer Pt in RuO2 nanosheet as robust bifunctional oxygen electrocatalyst for stabilizing Li-O2 batteries17Surface-Fe-doped cobalt sulfide as a highly active and stable oxygen evolution reaction catalyst for seawater splitting12Promoting active species generation by sculpting Co3S4/Co(OH)2 nanotubes with rich sulfide/hydroxide interfaces for efficient oxygen evolution reaction4Understanding the Anion Effect of Basic Cobalt Salts for the Electrocatalytic Oxygen Evolution Reaction72Asymmetric gradient orbital interaction of hetero-diatomic active sites for promoting C − C coupling73Enabling high-efficiency ethanol oxidation on NiFe-LDH via deprotonation promotion and absorption inhibition70Highly efficient electrooxidation of 5-hydroxymethylfurfural (HMF) by Cu regulated Co carbonate hydroxides boosting hydrogen evolution reaction27Controlling dynamic reconstruction chemistry for superior oxygen-evolving catalysts128Selective two-electron electrocatalytic conversion of 5-Hydroxymethylfurfural boosting hydrogen production under neutral condition over Co(OH)2-CeO2 catalyst103Structural Design Induced Electronic Optimization in Single‐Phase MoCoP Nanocrystal for Boosting Oxygen Reduction, Oxygen Evolution, and Hydrogen Evolution39Boosting Efficient and Sustainable Alkaline Water Oxidation on a W‐CoOOH‐TT Pair‐Sites Catalyst Synthesized via Topochemical Transformation45The electrocatalytic activity and selectivity of ethylene glycol oxidation into value-added chemicals at iron-group electrodes in alkaline media61Recent Advances in Synergistic Modulation of Transition-Metal-Based Electrocatalysts for Water Oxidation: A Mini Review20Reversely Trapping Isolated Atoms in High Oxidation State for Accelerating the Oxygen Evolution Reaction Kinetics39Reversely Trapping Isolated Atoms in High Oxidation State for Accelerating the Oxygen Evolution Reaction Kinetics4Constructing flexible composite electrodes of low crystalline cobalt (Oxy)hydroxides nanosheet grown on carbon fiber cloth via self-reconstruction for electrochemical nitrate-to-ammonia conversion25Spatiotemporally and Chemically Resolved Imaging of Electrocatalytic Oxygen Evolution on Single Nanoplates of Cobalt-Layered Hydroxide90Interface engineering of NiS/NiCo2S4 heterostructure with charge redistribution for boosting overall water splitting32Superior bifunctional oxygen electrocatalysts based on Co2MnO4 with mixed site occupancy, Mn-rich surfaces and twin defects25Sulfidation of CoCuOx Supported on Nickel Foam to Form a Heterostructure and Oxygen Vacancies for a High-Performance Anion-Exchange Membrane Water Electrolyzer14Metal-organic framework derived NiFe2O4/FeNi3@C composite for efficient electrocatalytic oxygen evolution reaction23High-entropy alloy CuCrFeNiCoP film of Cu-based as high-efficiency electrocatalyst for water splitting56Accordion-like Co-MOF derived heterostructured Co/CoP@PNC as highly efficient electrocatalyst for alkaline hydrogen evolution reaction25NiCo-Based Heterostructure on Nickel Foam for Boosting Urea-Assisted Electrolytic Hydrogen Production11Unveiling the Electrolyte Cations Dependent Kinetics on CoOOH‐Catalyzed Oxygen Evolution Reaction136Unveiling the Electrolyte Cations Dependent Kinetics on CoOOH‐Catalyzed Oxygen Evolution Reaction17Recent advances in electrochemical non-enzymatic glucose sensor for the detection of glucose in tears and saliva: A Review80Ambient γ‐Rays‐Mediated Noble‐Metal Deposition on Defect‐Rich Manganese Oxide for Glycerol‐Assisted H 2 Evolution at Industrial‐Level Current Density74Ambient γ‐Rays‐Mediated Noble‐Metal Deposition on Defect‐Rich Manganese Oxide for Glycerol‐Assisted H2 Evolution at Industrial‐Level Current Density12Multiple synergies on cobalt-based spinel oxide nanowires for electrocatalytic oxygen evolution20New insights into Co3O4-carbon nanotube membrane for enhanced water purification: Regulated peroxymonosulfate activation mechanism via nanoconfinement21A Review of Transition Metal Boride, Carbide, Pnictide, and Chalcogenide Water Oxidation Electrocatalysts295Dual‐Ligand Strategy to Construct Metal Organic Gel Catalyst with the Optimized Electronic Structure for High‐Efficiency Overall Water Splitting and Flexible Metal–Air Battery12Molecular Mechanisms of Oxygen Evolution Reactions for Artificial Photosynthesis13CoOOH: Synthesis and Application in Alkaline Electrochemical Oxygen Evolution Reaction26Copper dopants facilitated generation of high-valent cobalt sites for improved oxygen evolution4Double self-reinforced coordination modulation constructing stable Ni 4+ for water oxidation168Electric field-induced phosphorization to prepare CoP@Biochar composites for efficient bifunctional oxygen electrocatalysis16Electrochemical water splitting enhancement by introducing mesoporous NiCoFe-trimetallic phosphide nanosheets as catalysts for the oxygen evolution reaction17Engineering hierarchical snowflake-like multi-metal selenide catalysts anchored on Ni foam for high-efficiency and stable overall water splitting3Modulating the geometrical sites of cobalt phosphates by autologous pyrolysis for electrocatalytic water oxidation0Thermocatalytic epoxidation by cobalt sulfide inspired by the material's electrocatalytic activity for oxygen evolution reaction11Ultrathin 2D–2D NiFe LDH/MOF heterojunction nanosheets: an efficient oxygen evolution reaction catalyst for water oxidation50Controllable Electronic Transfer Tailoring d ‐band Center via Cobalt–Oxygen‐Bridged Ru/Fe Dual‐sites for Boosted Oxygen Evolution35Synthesis and Electrocatalytic Applications of Layer‐Structured Metal Chalcogenides Composites43Metal cobalt dot-doped carbon structures with specific exposure surfaces for high-performance capacitive deionization7Boosting the Bifunctionality and Durability of Cobalt-Fluoride-Oxide Nanosheets for Alkaline Water Splitting Through Nitrogen-Plasma-Promoted Electronic Regulation and Structural Reconstruction13Electrochemically Induced Ru/CoOOH Synergistic Catalyst as Bifunctional Electrode Materials for Alkaline Overall Water Splitting25Interfacial Chemistry and Catalysis of Inorganic Materials1Utilizing the oxygen-atom trapping effect of Co 3 O 4 with oxygen vacancies to promote chlorite activation for water decontamination225Spin-Magnetic Effect of d-π Conjugation Polymer Enhanced O–H Cleavage in Water Oxidation92In situ electrodeposition synthesis of CoP@NiFe LDH heterostructure as high-performance electrocatalyst for enhanced seawater electrolysis44Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting859Real Active Site Identification of Co/Co 3 O 4 Anchoring Ni-MOF Nanosheets with Fast OER Kinetics for Overall Water Splitting32Operando Spectroscopic Monitoring of Metal Chalcogenides for Overall Water Splitting: New Views of Active Species and Sites9Operando Spectroscopic Monitoring of Metal Chalcogenides for Overall Water Splitting: New Views of Active Species and Sites30Reversing the Interfacial Electric Field in Metal Phosphide Heterojunction by Fe‐Doping for Large‐Current Oxygen Evolution Reaction50High-valent metal-oxo species in catalytic oxidations for environmental remediation and energy conversion74Crystal Structure Regulation of CoSe2 Induced by Fe Dopant for Promoted Surface Reconstitution toward Energetic Oxygen Evolution Reaction9Highly efficient anion exchange membrane water electrolyzers via chromium-doped amorphous electrocatalysts248Bioinspired axial S-coordinated single-atom cobalt catalyst to efficient activate peroxymonosulfate for selective high-valent Co-Oxo species generation70Novel amorphous FeOOH-modified Co9S8 nanosheets with enhanced catalytic activity in oxygen evolution reaction13Modulating charge storage mechanism of cobalt-tungsten nitride electrodes using in situ formed metal-p-n heterojunction for ultrahigh energy density supercapattery18Manipulating reaction pathway of ruthenium oxide with enhanced performance and stability toward acidic water oxidation28Engineering heterostructured and hierarchical CoP/CoFeP nanosheet for effective oxygen evolution reaction in alkaline freshwater and seawater17Lattice Oxygen Activation through Deep Oxidation of Co 4 N by Jahn–Teller–Active Dopants for Improved Electrocatalytic Oxygen Evolution205Lattice Oxygen Activation through Deep Oxidation of Co4N by Jahn–Teller–Active Dopants for Improved Electrocatalytic Oxygen Evolution13Upcycling electroplating sludge into bioengineering-enabled highly stable dual-site Fe-Ni2P@C electrocatalysts for efficient oxygen evolution4Crystal Face‐Dependent Behavior of Single‐Atom Pt: Construct of SA‐FLP Dual Active Sites for Efficient NO2 Detection22Metal vacancies and self-reconstruction of high entropy metal borates to boost the oxygen evolution reaction37Unleashing unprecedented activation of high-valent Ni and Fe charge dynamics in CeF3-NiFe layered double hydroxide heterostructure: Demonstrating oxygen evolution reaction at an extremely high current density16Nickel Nanoplates Enclosed by (111) Facets as Durable Oxygen Evolution Catalysts in Anion Exchange Membrane Water Electrolyzers17Sulfur‐Vacancy Engineering Accelerates Rapid Surface Reconstruction in Ni‐Co Bimetal Sulfide Nanosheet for Urea Oxidation Electrocatalysis28Lattice strain induced rapid structural reconstruction of NiCo hydroxide for efficient water oxidation44Enhanced Long‐Term Performance of Sulfides in Oxygen Evolution Reaction by Sulfate Ion‐Assisted Strategy36Optical in situ deciphering of the surface reconstruction–assistant multielectron transfer event of single Co 3 O 4 nanoparticles5High-efficiency electrochemical nitrate reduction to ammonia via boron-doped hydroxyl oxide cobalt induced electron delocalization16Coupled electrocatalytic hydrogen production61Inducing Intermolecular Oxygen Coupling by Introducing S and FeOOH on Co(OH) 2 Nanoneedle Arrays for Industrial Water Oxidation22Ga-Induced p–d Orbital Hybridization in CoFe LDH for Boosted Oxygen Evolution Electrocatalysis32Simultaneously Improving Energy Storage and Oxygen Evolution Reaction by Causing Regional Defects in MOF-on-MOF Derived Hollow Se-Doped CoP-Fe2P Heterojunctions25Component synergistic effect of Co9S8/FeBOx composite system for efficient oxygen evolution reaction2Optimizing heterointerface of NiCoP–Co/MXene with regulated charge distribution via built‐in electric field for efficient overall water‐splitting51Unraveling the Dynamic Reconstruction of Active Co(IV)‐O Sites on Ultrathin Amorphous Cobalt‐Iron Hydroxide Nanosheets for Efficient Oxygen‐Evolving18Understanding the Role of Spin State in Cobalt Oxyhydroxides for Water Oxidation12Understanding the Role of Spin State in Cobalt Oxyhydroxides for Water Oxidation122Regioselective Doping into Atomically Aligned Core–Shell Structures for Electrocatalytic Reduction of Nitrate to Ammonia79Surface Cladding Engineering via Oxygen Sulfur Distribution for Stable Electrocatalytic Oxygen Production4Surface Cladding Engineering via Oxygen Sulfur Distribution for Stable Electrocatalytic Oxygen Production37Facet Engineering Boosts Interfacial Compatibility of Inorganic‐Polymer Composites8Interfacial geometric strain-polarization tailoring electron communication toward super-efficient HER and OER activity in TMPs@TM-Oxide-Oxyhydroxide4Rational Construction of Heterostructures with n‐Type Anti‐Barrier Layer for Enhanced Electrochemical Energy Storage15In Situ Reconstructing NiFe Oxalate Toward Overall Water Splitting17In Situ Unraveling Surface Reconstruction of Ni‐ C o P Nanowire for Excellent Alkaline Water Electrolysis17Oxygen Plasma Triggered Co−O−Fe Motif in Prussian Blue Analogue for Efficient and Robust Alkaline Water Oxidation5Oxygen Plasma Triggered Co−O−Fe Motif in Prussian Blue Analogue for Efficient and Robust Alkaline Water Oxidation65Selenate oxyanion-intercalated NiFeOOH for stable water oxidation via lattice oxygen oxidation mechanism59Ternary ZnO/Co3O4/CuO heterostructure nanocomposites derived from trimetallic metal-organic frameworks for efficient electrocatalytic water oxidation0High‐Valence Co Stabilized by In‐Situ Growth of ZIF‐67 on NiCo‐LDH for Enhanced Performance in Oxygen Evolution Reaction9An Interstitial Boron Inserted Metastable Hexagonal Rh Nanocrystal for Efficient Hydrogen Oxidation Electrocatalysis15

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  1. Superior bifunctional cobalt/nitrogen-codoped carbon nanosheet arrays on copper foam enable stable energy-saving hydrogen production accompanied with glucose upgrading

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  3. CeO2 Functionalized Cobalt Layered Double Hydroxide for Efficient Catalytic Oxygen‐Evolving Reaction

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  10. Single-atom Fe Embedded CO3S4 for Efficient Electrocatalytic Oxygen Evolution Reaction

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  20. Transformation mechanism of high-valence metal sites for the optimization of Co- and Ni-based OER catalysts in an alkaline environment: recent progress and perspectives

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  32. Revealing the Generation of High-Valent Cobalt Species and Chlorine Dioxide in the Co3O4-Activated Chlorite Process: Insight into the Proton Enhancement Effect

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  33. Sulphur-dopant induced breaking of the scaling relation on low-valence Ni sites in nickel ferrite nanocones for water oxidation with industrial-level current density

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  41. Remote Synergy between Heterogeneous Single Atoms and Clusters for Enhanced Oxygen Evolution

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  43. Modulating the electronic structure of CoS2 by Sn doping boosting urea oxidation for efficient alkaline hydrogen production

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  44. Al3+ leaching induced Co4+ on CoFeAl layered double hydroxide for enhanced oxygen evolution reaction

    International Journal of Hydrogen Energy · 2023-03-31

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  45. Regulating electronic states of nitride/hydroxide to accelerate kinetics for oxygen evolution at large current density

    Nature Communications · 2023-04-04

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  46. Atomically dispersed Ru oxide catalyst with lattice oxygen participation for efficient acidic water oxidation

    Chem · 2023-04-05

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  47. Biphasic Transition Metal Nitride Electrode Promotes Nucleophile Oxidation Reaction for Practicable Hybrid Water Electrocatalysis

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  48. Surface Reconstruction of Covellite CuS Nanocrystals for Enhanced OER Catalytic Performance in Alkaline Solution

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  49. Oxidative contaminant degradation on bimetallic boride electrocatalysts enhances anodic charge transfer for efficient H2 production

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  50. Heterogeneous activation of peroxymonosulfate by flower-like cobalt sulfide enhanced sulfamethoxazole degradation via non-radical pathways

    Applied Surface Science · 2023-06-04

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