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RESEARCH PAPER · Advanced Energy Materials · 2022

A Roadmap for Transforming Research to Invent the Batteries of the Future Designed within the European Large Scale Research Initiative BATTERY 2030+

Julia Amici, Pietro Asinari, Elixabete Ayerbe, P. Barboux, Pascale Bayle‐Guillemaud, R. Jürgen Behm, Maitane Berecibar, Erik J. Berg, Arghya Bhowmik, Silvia Bodoardo, Ivano E. Castelli, Isidora Cekić-Lasković, Rune Christensen, Simon Clark, Ralf Diehm, Robert Dominko, Maximilian Fichtner, Alejandro A. Franco, Alexis Grimaud, Nicolas Guillet, Maria Hahlin, Sarah Hartmann, Vincent Heiries, Kersti Hermansson, Andreas Heuer, Saibal Jana, Lara Jabbour, Josef Kallo, Arnulf Latz, Henning Lorrmann, Ole Martin Løvvik, Sandrine Lyonnard, Marcel Meeus, Elie E. Paillard, Simon Perraud, Tobias Placke, Christian Punckt, Olivier Raccurt, Janna Ruhland, Edel Sheridan, Helge Sören Stein, Jean‐Marie Tarascon, Victor Trapp, Tejs Vegge, Marcel Weil, Wolfgang Wenzel, Martin Winter, Andreas Wolf, Kristina Edström

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A Roadmap for Transforming Research to Invent the Batteries of the Future Designed within the European Large Scale Research Initiative BATTERY 2030+OriginalAccelerating Battery Characterization Using Neutron and Synchrotron Techniques: Toward a Multi‐Modal and Multi‐Scale Standardized Experimental Workflow62Accelerating the Adoption of Research Data Management Strategies1Composite Mn–Co electrode materials for supercapacitors: why the precursor's morphology matters!5Robotic cell assembly to accelerate battery research46Modeling the Solid Electrolyte Interphase: Machine Learning as a Game Changer?87A renaissance for lithium-sulfur batteries through low-cost, efficient, and sustainable biomass cathodes8From materials discovery to system optimization by integrating combinatorial electrochemistry and data science37Deciphering the Interplay between Binders and Electrolytes on the Performance of Li4Ti5O12 Electrodes for Li-Ion Batteries3Gaussian process sensitivity analysis of a capacityfade model for lithium-ion batteries0Electrochemical Protocols to Assess the Effects of Dissolved Transition Metal in Graphite/LiNiO2 Cells Performance22Advances in Intelligent Regeneration of Cathode Materials for Sustainable Lithium‐Ion Batteries195Failure analysis of high-energy-density lithium‒sulfur pouch cells64A Review and Perspective on Path Dependency in Batteries30Material science as a cornerstone driving battery research41Brokering between tenants for an international materials acceleration platform5UV-cured self-healing gel polymer electrolyte toward safer room temperature lithium metal batteries50Principles of the Battery Data Genome132Accelerating the adoption of research data management strategies16Sensitivity analysis methodology for battery degradation models34Cross-Linked Gel Electrolytes with Self-Healing Functionalities for Smart Lithium Batteries51Simultaneous Strain and Temperature Discrimination in 18650 Li-ion Batteries Using Polarization-Maintaining Fiber Bragg Gratings33Toward a function realization of multi‐scale modeling for lithium‐ion battery based on CHAIN framework19Uncertainty-aware and explainable machine learning for early prediction of battery degradation trajectory37Electro-chemo-mechanical design of polymer matrix in composited LiNi0.8Co0.1Mn0.1O2 cathode endows solid-state batteries with superior performance18Recent Advances in Conduction Mechanisms, Synthesis Methods, and Improvement Strategies for Li 1+ x Al x Ti 2− x (PO 4 ) 3 Solid Electrolyte for All‐Solid‐State Lithium Batteries85Robotised screening and characterisation for accelerated discovery of novel Lithium-ion battery electrolytes: Building a platform and proof of principle studies20First-principles study of ZIF-8 as anode for Na and K ion batteries12An inexpensive electrolyte with double-site hydrogen bonding and a regulated Zn 2+ solvation structure for aqueous Zn-ion batteries capable of high-rate and ultra-long low-temperature operation228Automated electrolyte formulation and coin cell assembly for high-throughput lithium-ion battery research35Cycle-dependent morphology and surface potential of germanium nanowire anode electrodes3Distinct thermal runaway mechanisms of sulfide-based all-solid-state batteries157Ionic conductivity, viscosity, and self-diffusion coefficients of novel imidazole salts for lithium-ion battery electrolytes23The materials experiment knowledge graph25Lithium Batteries and the Solid Electrolyte Interphase (SEI)—Progress and Outlook830Advances in thermal‐related analysis techniques for solid‐state lithium batteries85Unveiling the Effects of Cr Single Atoms with Controllable Configurations on Solid Electrolyte Interphase and Storage Mechanism of Sodium Ions41A particle filter-based virtual sensor for estimating the state of charge and internal temperature of lithium-ion batteries: Implementation in a simulated study case26Customized Optical Fiber Birefringent Sensors to Multipoint and Simultaneous Temperature and Radial Strain Tracking of Lithium‐Ion Batteries15In Situ Plastic-Crystal-Coated Cathode toward High-Performance Na-Ion Batteries138Environmental impact of direct lithium extraction from brines751Self-Healing Polymer Electrolytes for Next-Generation Lithium Batteries73Real-time nondestructive methods for examining battery electrode materials19Transferring state of health estimation neural networks for different battery chemistries and charging protocols using renormalization and transfer learning7Influence of electrode fabrication process on nanocrystalline tin oxide electrochemical behaviour for high voltage SnO2/LNMO full cell Li-ion battery6Dual parameters discrimination comparison between two types of optical fiber sensors during the operation of a Li-ion battery0Multifunctional Additive Ethoxy(pentafluoro)cyclotriphosphazene Enables Safe Carbonate Electrolyte for SiO x ‐Graphite/NMC811 Batteries13BATTERY 2030+ and its Research Roadmap: A Bibliometric Analysis10An Overview on Transport Phenomena within Solid Electrolyte Interphase and Their Impact on the Performance and Durability of Lithium-Ion Batteries27Technical, Safety and Environmental Challenges in the Electrification of Cable Yarding Equipment10Lithium–Ion Battery Data: From Production to Prediction42Binder-Free LiNi0.8Mn0.1Co0.1O2/Multi-Walled Carbon Nanotube Prepared by One-Step Electrophoretic Deposition Method for Efficient Li-Ion-Battery Cathodes7Enhancing ReaxFF for Molecular Dynamics Simulations of Lithium-Ion Batteries: An interactive reparameterization protocol0The Promise of 3D Printed Solid Polymer Electrolytes for Developing Sustainable Batteries: A Techno-Commercial Perspective18Holistic optimization of lithium-ion battery negative electrode formulation using a combination of theory of mixtures, Box-Behnken matrix, multi-variant analysis and desirability functions of Derringer-Suich3Brokering between tenants for an international materials acceleration platform46Multi sensor fusion methods for state of charge estimation of smart lithium-ion batteries41Multi‐Physical Field Simulation: A Powerful Tool for Accelerating Exploration of High‐Energy‐Density Rechargeable Lithium Batteries29Building Smarter Aqueous Batteries23Mitigating the Ion Transport Tortuosity in Composite Cathodes of All-Solid-State Batteries by Wet Milling of the Solid Electrolyte Particles20Unraveling the importance of water ratio in direct lithium-ion battery cathode recycling8Role of copper as current collectors in the reductive reactivity of polymers for anode-free lithium metal batteries - Insights from DFT and AIMD studies13Optimizing Current Collector Interfaces for Efficient “Anode‐Free” Lithium Metal Batteries136Lithium-Ion Battery Manufacturing: Industrial View on Processing Challenges, Possible Solutions and Recent Advances70A composite solid-state electrolyte of high ionic-conductivity garnet-type Li6.5La3Zr1.5Ta0.1Nb0.4O12 filler in PEO matrix12Research on the process of carbon thermal reduction for recovery and resynthesis of LiNi0.6Co0.2Mn0.2O213Thermal safety boundary of lithium-ion battery at different state of charge93Thermo-luminescent optical fibre sensor for Li-ion cell internal temperature monitoring10Advanced Functional Optical Fiber Sensors for Smart Battery Monitoring35Apples to apples: shift from mass ratio to additive molecules per electrode area to optimize Li-ion batteries6Artificial intelligence and machine learning in battery materials and their applications12Autonomous millimeter scale high throughput battery research system12Emerging Battery Technologies to Boost the Clean Energy Transition48Lithium-ion battery cell formation: status and future directions towards a knowledge-based process design193Principles of a Circular Economy for Batteries5Sapiential battery systems: beyond traditional electrochemical energy81The origins of critical deformations in cylindrical silicon based Li-ion batteries38Autonomous millimeter scale high throughput battery research system (Auto-MISCHBARES)0Autonomous millimeter scale high throughput battery research system (Auto-MISCHBARES)1Autonomous millimeter scale high throughput battery research system (Auto-MISCHBARES)0Enhancing ReaxFF for molecular dynamics simulations of lithium-ion batteries: an interactive reparameterization protocol18Effects of electrolyte/cathode ratio on investigation of their thermal behaviors using differential scanning calorimetry8Salt Effects on the Mechanical Properties of Ionic Conductive Polymer: A Molecular Dynamics Study17Insights on advanced g‐C 3 N 4 in energy storage: Applications, challenges, and future80Nonlinear Potentiodynamic Battery Charging Protocols for Fun, Education, and Application4Efficient and Stable Magnesium Plating/Stripping in High-Capacity Novel Mg//Ni0.6Co0.4Se2 Batteries Enabled by Interfacial Chemistry Modulation10Potentials and hotspots of post-lithium-ion batteries: Environmental impacts and supply risks for sodium- and potassium-ion batteries52Integrated Propulsion System Analysis Framework for Designing Advanced Air Mobility Aircraft11Functional Optical Fiber Sensors Detecting Imperceptible Physical/Chemical Changes for Smart Batteries52Towards Greener Recycling: Direct Repair of Cathode Materials in Spent Lithium-Ion Batteries94Review of lithium-ion batteries’ supply-chain in Europe: Material flow analysis and environmental assessment39The Future of Energy Storage in Vietnam: A Fuzzy Multi-Criteria Decision-Making Approach to Metal-Ion Battery Assessments10Toward Carbon Neutral Road Transport: Development Strategies and New R&D Organizational Paradigms27Recent advances in organic cathodes for dual-ion batteries12Deciphering Advanced Sensors for Life and Safety Monitoring of Lithium Batteries53Attention towards chemistry agnostic and explainable battery lifetime prediction24Autonomous battery optimisation by deploying distributed experiments and simulations2Promoted Reaction Reversibility by Dual-Effect 15-Crown-5 Ether Additive for High-Performance Li–O2 Batteries8Designer Anions for Better Rechargeable Lithium Batteries and Beyond50Life cycle assessment of bio-based hard carbon for sodium-ion batteries across different production scales38Tailoring cathode materials: A comprehensive study on LNMO/LFP blending for next generation lithium-ion batteries63All-solid-state lithium–sulfur batteries through a reaction engineering lens120Designing Better Flow Batteries: An Overview on Fifty Years’ Research116Investigating the Temperature Dependency of Trimethyl Aluminum Assisted Atomic Surface Reduction of Li and Mn-Rich NCM1Fluorinated Linkers Enable High‐Voltage Pyrrolidinium‐based Dicationic Ionic Liquid Electrolytes4CALiSol-23: Experimental electrolyte conductivity data for various Li-salts and solvent combinations15Application of silicon nanowires in sensors of temperature, light and humidity10Challenges and opportunities to advance manufacturing research for sustainable battery life cycles11The Integration of Innovative Power Sources and Storage Systems in the Railway Sector: A Brief Perspective Analysis0Investigation on Psyllium Gum as a Bio‐Based Binder for Silicon Anode in Lithium‐Ion Batteries4Design of Environmental Sensor Board for Energy Harvesting: Integration of Conventional and Eco-Friendly Sensors with Power Generation Sources5Nanostructures of metal oxides0A critical analysis of the role of artificial intelligence and machine learning in enhancing nuclear waste management6Estudios operando de los mecanismos fisicoquímicos en nanomateriales de interés para el desarrollo de tecnologías energéticas sostenibles0Critical material and device parameters for building a beyond-500-Wh/kg lithium-sulfur battery14Autonomous Battery Optimization by Deploying Distributed Experiments and Simulations19Smart Cell with Internal Sensors to Limit Lithium Plating During Fast-Charge at Low Temperature0Towards smart and secure batteries: Linking pressure and temperature profiles with electrochemical behavior through hybrid optical fiber sensors22Lead-Acid Battery Electrolyte Density Sensor using Heterocore Optical Fiber2Confinement strategy construction (0D/3D)MoSe2@HrGO hybrid for enhancing reaction kinetics in aqueous zinc-tellurium batteries15Capacity degradation prediction model of LiMn0.6Fe0.4PO4/LiNi0.5Co0.2Mn0.3O2 composite cathode materials for lithium-ion batteries1Revealing how internal sensors in a smart battery impact the local graphite lithiation mechanism44Unveiling multi-component hybrid organic-inorganic SEI formation in gel polymer electrolytes: A computational study15A hierarchical electrochemical-thermal-mechanical coupled model capable of predicting non-uniform behaviors in large-format Li-ion cells20A flexible integrated temperature-pressure sensor for wearable detection of thermal runaway in lithium batteries64A sustainable approach to energy storage in buildings: the first rechargeable geopolymer-based battery6ADEL: an automated drop-cast electrode setup for high-throughput screening of battery materials4Emerging processing guidelines for solid electrolytes in the era of oxide-based solid-state batteries84Internal Strain Characterization of High-Capacity Lithium-Ion Batteries Based on In-Situ Measurements with Array Fiber Grating Sensors0Machine learning-assisted design of cathode materials for lithium–sulfur batteries derived from a metal–organic framework12Non-destructive degradation pattern decoupling for early battery trajectory prediction via physics-informed learning81Smart batteries: materials, monitoring, and artificial intelligence22Structural engineering of MXene frameworks with abundant surface functionalities for enhanced lithium–sulfur battery electrochemistry3Unlocking the Potential of Second-Life Batteries: A Nonlinear Frequency and Machine Learning Approach to Health Prediction0Unveiling capacity limitations of MnO 2 in rechargeable Zn chemistry19Life prediction model and performance degradation of lithium-ion battery under different cut-off voltages2Deciphering the Impacts of Al, Fe, Li Sulfate Impurities on the Synthesis and Performances of LiNi0.6Mn0.2Co0.2O2 Cathode Materials3Lithiophilic copper oxide–polyacrylonitrile composite coating on copper current collector for high-voltage anode-free lithium batteries2Thermal Runaway Mechanism of Composite Cathodes for All‐Solid‐State Batteries42Advancements in specialty batteries: Innovations, challenges, and future directions9Long‐Term Stability Evaluation of Optical Fiber Sensors Immersed in LiPF6 Electrolyte2Deep Learning-Driven Molecular Generation and Electrochemical Property Prediction for Optimal Electrolyte Additive Design8Bioinspired microcapsules toward smart lithium-ion batteries: Concept, mechanism, performance, and criteria6Fluoride‐Ion‐Mediated Fabrication of Cerium‐Incorporated Ternary Layered Double Hydroxide Microflowers for Enhanced Chlorine Storage18A critical review of recent progress on lithium ion batteries: Challenges, applications, and future prospects69State estimation of lithium-ion batteries via physics-machine learning combined methods: A methodological review and future perspectives67Towards digitized electrochemical power source for electric vehicles18In-situ solvent-free preparation of MOF/polymer composite electrolytes with highly dispersed and defected MOF nanoparticles for lithium-metal batteries16Current Status and Future Perspective in Electric Vehicle Battery Stacking: A Review5Sufficient cathode infiltration for stable 500 Wh kg−1 level lithium–sulfur batteries49Investigating the structural change and degradation mechanism of MnO2 for lithium-ion batteries5

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  30. Cycle-dependent morphology and surface potential of germanium nanowire anode electrodes

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  31. Distinct thermal runaway mechanisms of sulfide-based all-solid-state batteries

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  32. Ionic conductivity, viscosity, and self-diffusion coefficients of novel imidazole salts for lithium-ion battery electrolytes

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  33. The materials experiment knowledge graph

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  38. Customized Optical Fiber Birefringent Sensors to Multipoint and Simultaneous Temperature and Radial Strain Tracking of Lithium‐Ion Batteries

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  39. In Situ Plastic-Crystal-Coated Cathode toward High-Performance Na-Ion Batteries

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  40. Environmental impact of direct lithium extraction from brines

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  41. Self-Healing Polymer Electrolytes for Next-Generation Lithium Batteries

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  42. Real-time nondestructive methods for examining battery electrode materials

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  43. Transferring state of health estimation neural networks for different battery chemistries and charging protocols using renormalization and transfer learning

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  44. Influence of electrode fabrication process on nanocrystalline tin oxide electrochemical behaviour for high voltage SnO2/LNMO full cell Li-ion battery

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  45. Dual parameters discrimination comparison between two types of optical fiber sensors during the operation of a Li-ion battery

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