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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2021

Ligand Exchange Strategy to Achieve Chiral Perovskite Nanocrystals with a High Photoluminescence Quantum Yield and Regulation of the Chiroptical Property

Shuang Jiang, Yuxin Song, Huimin Kang, Bin Li, Kunlong Yang, Guoxiang Xing, Ying Yu, Siyi Li, Peisheng Zhao, Tianyong Zhang

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Ligand Exchange Strategy to Achieve Chiral Perovskite Nanocrystals with a High Photoluminescence Quantum Yield and Regulation of the Chiroptical PropertyOriginalConstruction and Catalysis Advances of Inorganic Chiral Nanostructures2Spin-polarized excitons and charge carriers in chiral metal halide semiconductors23Leveraging Hierarchical Chirality in Perovskite(‐Inspired) Halides for Transformative Device Applications41Tiny spots to light the future: advances in synthesis, properties, and application of perovskite nanocrystals in solar cells10Size-dependent chiro-optical properties of CsPbBr 3 nanoparticles20Anionic ligand-induced chirality in perovskite nanoplatelets16Metal halide perovskites: promising materials toward next-generation circularly polarized luminescence35Simultaneously achieving room-temperature circularly polarized luminescence and high stability in chiral perovskite nanocrystals via block copolymer micellar nanoreactors20Ligand Chemistry of Inorganic Lead Halide Perovskite Nanocrystals388Chirality–Racemization Strategy Toward Copper (I) Iodide Hybrid Single‐Crystalline Scintillators for X‐Ray Detection and Imaging Applications45Research progress in optical activities and nonlinear optics of chiral perovskites1Chiral Perovskite Nanoplatelets with Tunable Circularly Polarized Luminescence in the Strong Confinement Regime41Visible Light-Driven Luminescence Evolution of CsPbBr3 Quantum Dots via Surface Reconstruction5Efficient Red-Emissive Circularly Polarized Electroluminescence Enabled by Quasi-2D Perovskite with Chiral Spacer Cation92Metal Halide Perovskite Nanocrystals for Near-Infrared Circularly Polarized Luminescence with High Photoluminescence Quantum Yield via Chiral Ligand Exchange32Toward Chiral Lasing from All‐Solution‐Processed Flexible Perovskite‐Nanocrystal–Liquid‐Crystal Membranes68Chiral Ligand‐Induced Inversion and Tuning of Excitonic Optical Activity in Intrinsically Chiral CsPbBr3 Perovskite Nanoplatelets32Chiral Lead Halide Perovskite Nanocrystals: Construction Strategies and Photophysical Properties11Defect-Induced Circularly Polarized Luminescence of Chiral Perovskite Films7All-inorganic lead halide perovskites for photocatalysis: a review56Chiral defect-induced blue photoluminescence and circularly polarized luminescence of zero-dimensional Cs 4 PbBr 6 perovskite nanocrystals4Factors influencing the chiral imprinting in perovskite nanoparticles2Electron-donating functional groups strengthen ligand-induced chiral imprinting on CsPbBr3 quantum dots22Impact of Chiral Spinterfaces on Magneto-Photoluminescence Effects for Chiral Lead Halide Perovskites6Chiral Multidentate Ligand Facilitating Perovskite Nanocrystals with Circularly Polarized Luminescence and Chiral Assembly27Aqueous-phase dual-functional chiral perovskites for hydrogen sulfide (H2S) detection and antibacterial applications in Escherichia coli23Structure-Guided Approaches for Enhanced Spin-Splitting in Chiral Perovskite42Blue Circularly Polarized Luminescence from Quantum-Confined CsPbBr 3 Nanocrystals with a Different Degree of Shape Anisotropy15The Mn2+‐Doped Chiral 2D Perovskite with Strong Orange Fluorescent and Enhanced Circularly Polarized Luminescence5Recent progress on chiral perovskites as chiroptical active layers for next-generation LEDs25Ultrasmall 2D Sn‐Doped MAPbBr 3 Nanoplatelets Enable Bright Pure‐Blue Emission9Chirality of CsPbBr 3 Nanocrystals with Varying Dimensions in the Presence of Chiral Molecules20Strong circularly polarized photoluminescence from mixed halide perovskite nanocrystals induced by anion-assisted chirality imprinting7Room‐Temperature Liquid Crystalline Tetraphenylethylene‐Surfactant Complex with Chiral Supramolecular Structure and Tunable Circularly Polarized Luminescence6Exploring Nanoscale Perovskite Materials for Next-Generation Photodetectors: A Comprehensive Review and Future Directions80Processable Circularly Polarized Luminescence for the Synthesis of Chiral Plasmonic Nanoparticles8Inducing Efficient and Multiwavelength Circularly Polarized Emission From Perovskite Nanocrystals Using Chiral Metasurfaces29Mechanisms for translating chiral enantiomers separation research into macroscopic visualization16Chiral metal-containing semiconductor nanocrystals: Construction, optical activity, and application5A pair of chiral organic–inorganic hybrid tin compounds showing reversible phase transition and enhanced SHG properties3Technical Routes to Achieve High Circular Polarized Luminescence in Chiral Perovskites: A Mini‐Review8Recent Advances in Emerging Polarization‐Sensitive Materials: From Linear/Circular Polarization Detection to Neuromorphic Device Applications60Multi-stimuli circular dichroism responses, UV-enhanced emission in solution and circularly polarized luminescence of a pair of chiral cuprous complexes1Synthesis and Chiroptical Properties of Chiral Lead Halide Molecular Clusters3Chiral naphthalimide ligand-induced perovskites for chirality recognition based on enhanced fluorescence response2Charge Transfer-Driven Modulation of Induced Chirality in Hybrid Perovskite Nanocrystals3Chirality‐Induced Spin Selectivity of Photo‐Generated Electrons in Hybrid Organic–Inorganic Perovskites for Photocatalytic Hydrogen Evolution10Constructing Lead Halide Perovskite Nanocrystal Surfaces10Chiral Engineering: Molecular Recognition to Macroscopic Assembly Dynamics11Polar Solvent‐Assisted Chiral Ligand and Cation Exchange for Bright, Strongly Circularly Polarized Emission in CsPbBr 3 Perovskite Nanoplatelets4Chiral Hybrid Organic–Inorganic Metal Halides: Preparation, Luminescent Properties, and Applications2The Combination of Chiral Assembly and Chiral Template Effects Boosts Circularly Polarized Luminescence of Perovskite Nanocrystals5The Combination of Chiral Assembly and Chiral Template Effects Boosts Circularly Polarized Luminescence of Perovskite Nanocrystals2Recent advances in stable halide perovskite nanocrystals for optoelectronic devices, biological imaging, and X-ray detection12Chiral nanoengineering and biosensors: from construction to selective recognition, and emerging detection applications0Internally and externally induced chiral hybrid metal halide materials for advanced chiroptoelectronic applications23Unraveling Chiral Exciton g ex -Factor through Magneto-Optical Methods for Pure Blue Chiral Perovskite Nanocrystal Emitters5Scale-up synthesis of perovskite nanocrystal/cellulose chiral ink toward patterned and circularly polarized luminescence1Chiral Amine CsPbBr 3 Nanocrystals: Ligand Exchange Strategy‐Induced Circularly Polarized Luminescence and Chirality Modulation3Anti-interference ability of spiking neuron-astrocyte networks in working memory0Chiral perovskites: From chirality mechanisms to photovoltaics2Tailoring chiral perovskite nanocrystals for spin light-emitting diodes0Chiral‐Ligand‐Directed Synthesis of Circularly Polarized Luminescent Perovskite Nanowires0ZIF-8-Confined and APTES-Passivated CsPbBr3 Quantum Dots for Fluorescence Detection of Enrofloxacin Residues in Foods0Defect‐Induced Circularly Polarized Luminescence of Zero‐Dimensional Cs 4 PbBr 6 Perovskite Nanocrystals With Ligand‐Ratio Dependent CPL Inversion0

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  3. Leveraging Hierarchical Chirality in Perovskite(‐Inspired) Halides for Transformative Device Applications

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  4. Tiny spots to light the future: advances in synthesis, properties, and application of perovskite nanocrystals in solar cells

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  5. Size-dependent chiro-optical properties of CsPbBr 3 nanoparticles

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  6. Anionic ligand-induced chirality in perovskite nanoplatelets

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  7. Metal halide perovskites: promising materials toward next-generation circularly polarized luminescence

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  8. Simultaneously achieving room-temperature circularly polarized luminescence and high stability in chiral perovskite nanocrystals via block copolymer micellar nanoreactors

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  9. Ligand Chemistry of Inorganic Lead Halide Perovskite Nanocrystals

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  10. Chirality–Racemization Strategy Toward Copper (I) Iodide Hybrid Single‐Crystalline Scintillators for X‐Ray Detection and Imaging Applications

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  11. Research progress in optical activities and nonlinear optics of chiral perovskites

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  12. Chiral Perovskite Nanoplatelets with Tunable Circularly Polarized Luminescence in the Strong Confinement Regime

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  13. Visible Light-Driven Luminescence Evolution of CsPbBr3 Quantum Dots via Surface Reconstruction

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  14. Efficient Red-Emissive Circularly Polarized Electroluminescence Enabled by Quasi-2D Perovskite with Chiral Spacer Cation

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  15. Metal Halide Perovskite Nanocrystals for Near-Infrared Circularly Polarized Luminescence with High Photoluminescence Quantum Yield via Chiral Ligand Exchange

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  16. Toward Chiral Lasing from All‐Solution‐Processed Flexible Perovskite‐Nanocrystal–Liquid‐Crystal Membranes

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  17. Chiral Ligand‐Induced Inversion and Tuning of Excitonic Optical Activity in Intrinsically Chiral CsPbBr3 Perovskite Nanoplatelets

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  18. Chiral Lead Halide Perovskite Nanocrystals: Construction Strategies and Photophysical Properties

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  19. Defect-Induced Circularly Polarized Luminescence of Chiral Perovskite Films

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  20. All-inorganic lead halide perovskites for photocatalysis: a review

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  21. Chiral defect-induced blue photoluminescence and circularly polarized luminescence of zero-dimensional Cs 4 PbBr 6 perovskite nanocrystals

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  23. Electron-donating functional groups strengthen ligand-induced chiral imprinting on CsPbBr3 quantum dots

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