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RESEARCH PAPER · Chemical Reviews · 2021

Recent Progress and Future Prospects on All-Organic Polymer Dielectrics for Energy Storage Capacitors

Qi‐Kun Feng, Shao‐Long Zhong, Jia‐Yao Pei, Yu Hua Zhao, Dongli Zhang, Di‐Fan Liu, Yongxin Zhang, Zhi‐Min Dang

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Recent Progress and Future Prospects on All-Organic Polymer Dielectrics for Energy Storage CapacitorsOriginalAll-Organic Sandwich-Structured Bopp/Pvdf/Bopp Dielectric Films with Significantly Improved Energy Density and Charge-Discharge Efficiency51Design of Thin-Layer Porous Nickel Cobalt Sulfide for High-Performance Asymmetric Supercapacitors83Double gradient composite dielectric with high energy density and efficiency42Largely enhanced energy density of BOPP–OBT@CPP–BOPP sandwich-structured dielectric composites35Preparation and application of dielectric polymers with high permittivity and low energy loss: A mini review113Ultrahigh Energy Density in Continuously Gradient‐Structured All‐Organic Dielectric Polymer Films145Improved breakdown strength and energy storage performances of PEI-based nanocomposite with core-shell structured PI@BaTiO3 nanofillers47Multiscale Characterization of the Influence of the Organic–Inorganic Interface on the Dielectric Breakdown of Nanocomposites32Improved Energy Density and Energy Efficiency of Poly(vinylidene difluoride) Nanocomposite Dielectrics Using 0.93Na 0.5 Bi 0.5 TiO 3 -0.07BaTiO 3 Nanofibers41Outstanding discharge energy density and efficiency of the bilayer nanocomposite films with BaTiO3-dispersed PVDF polymer and polyetherimide layer75Achieving high insulating strength and energy storage properties of all-organic dielectric composites by surface morphology modification41Significantly improved high-temperature charge-discharge efficiency of all-organic polyimide composites by suppressing space charges116Ultra-sensitive flexible piezoelectric energy harvesters inspired by pine branches for detection41Insulating materials for realising carbon neutrality: Opportunities, remaining issues and challenges226Suppressing the Loss of Polymer‐Based Dielectrics for High Power Energy Storage182All-polymeric multilayer para/ferroelectric dielectric films utilizing a gradient structure toward concurrent high discharge efficiency and energy density39Polyimide/BaTiO3/NiNWs composites with enhanced dielectric properties25Dielectric and energy storage properties of all-organic sandwich-structured films used for high-temperature film capacitors56Rational design of all-organic flexible high-temperature polymer dielectrics74Ceramic‐Polymer Nanocomposites Design for Energy Storage Capacitor Applications26All-Organic Polymer Dielectric Materials for Advanced Dielectric Capacitors: Theory, Property, Modified Design and Future Prospects76Scalable Ultrathin All‐Organic Polymer Dielectric Films for High‐Temperature Capacitive Energy Storage220Self-Healing Polymers for Electronics and Energy Devices289Enhanced Quasilinear Dielectric Behavior of Polyvinylidene Fluoride via Confined Crystallization and Aligned Dipole Polarization35Constructing bidirectional-matched interface between polymer and 2D nanosheets for enhancing energy storage performance of the composites87Preparation of a novel cross‐linked polyetherimide with enhanced breakdown strength and high‐temperature energy storage performance43Superior High‐Temperature Energy Density in Molecular Semiconductor/Polymer All‐Organic Composites274Recent advances in composite films of lead-free ferroelectric ceramics and poly (vinylidene fluoride) (PVDF) for energy storage capacitor: a review28High energy density and superior charge/discharge efficiency polymer dielectrics enabled by rationally designed dipolar polarization27High-temperature energy storage polyimide dielectric materials: polymer multiple-structure design136A mini-review on the dielectric properties of cellulose and nanocellulose-based materials as electronic components147Achieving Synergistic Improvement in Dielectric and Energy Storage Properties of All‐Organic Poly(Methyl Methacrylate)‐Based Copolymers Via Establishing Charge Traps49Enhanced High-Temperature Capacitive Performance of a Bilayer-Structured Composite Film Employing a Charge Blocking Layer50Depressing relaxation and conduction loss of polar polymer materials by inserting bulky charge traps for superior energy storage performance in high-pulse energy storage capacitor applications56Modulating piezoelectricity and mechanical strength via three-dimensional gradient structure for piezoelectric composites32Recent advances in the utilization of covalent organic frameworks (COFs) as electrode materials for supercapacitors142Excellent energy storage performance in polymer composites with insulating and polarized two-dimensional fillers36Recent progress of W18O49 nanowires for energy conversion and storage59Contributing Factors of Dielectric Properties for Polymer Matrix Composites116Ultrahigh Energy Storage Density in Poly(vinylidene fluoride)‐Based Composite Dielectrics via Constructing the Electric Potential Well59Evolution Characteristics of DC Breakdown for Biaxially Oriented Polypropylene Films29Hydrogen Bonding of Aramid Boosts High-Temperature Capacitive Properties of Polyetherimide Blends52Theoretical connection from the dielectric constant of films to the capacitance of capacitors under high temperature30Massively Parallel Aligned Poly(vinylidene fluoride) Nanofibrils in All-Organic Dielectric Polymer Composite Films for Electric Energy Storage33High-temperature polymer dielectrics with superior capacitive energy storage performance72Realizing high energy density in BiFeO3-based ceramics capacitors via bandgap engineering and polarization optimization42High‐Energy‐Density All‐Organic Dielectric Film via a Continuous Preparation Processing42Single‐Crystalline BaZr0.2Ti0.8O3 Membranes Enabled High Energy Density in PEI‐Based Composites for High‐Temperature Electrostatic Capacitors61Scalable Polyimide‐Organosilicate Hybrid Films for High‐Temperature Capacitive Energy Storage254Effect of charge transport on electrical degradation in polypropylene/organic molecular semiconductor composites for HVDC cable insulation58Polyvinyl chloride-based dielectric elastomer with high permittivity and low viscoelasticity for actuation and sensing112Fabrication of Advanced Cellulosic Triboelectric Materials via Dielectric Modulation162Quantum Size Effect to Induce Colossal High‐Temperature Energy Storage Density and Efficiency in Polymer/Inorganic Cluster Composites1472D‐Nanofiller‐Based Polymer Nanocomposites for Capacitive Energy Storage Applications69Computational Simulation for Breakdown and Energy Storage Performances with Optimization in Polymer Dielectrics86Inorganic–Organic Hybrid Dielectrics for Energy Conversion: Mechanism, Strategy, and Applications107Toward Excellent Energy Storage Performance via Well-Aligned and Isolated Interfaces in Multicomponent Polypropylene-Based All-Organic Polymer Dielectric Films25Polyimides Physically Crosslinked by Aromatic Molecules Exhibit Ultrahigh Energy Density at 200 °C137Flexible all-organic nanocomposite films interlayered with in situ synthesized covalent organic frameworks for electrostatic energy storage35A Bilayer High-Temperature Dielectric Film with Superior Breakdown Strength and Energy Storage Density73Carboxylated Poly (p‐Phenylene Terephthalamide) Reinforced Polyetherimide for High‐Temperature Dielectric Energy Storage52Enhanced Dielectric Properties of All-Cellulose Composite Film via Modulating Hydroxymethyl Conformation and Hydrogen Bonding Network39Dynamic Covalent Adaptable Polyimide Hybrid Dielectric Films with Superior Recyclability86All organic polymer dielectrics for high‐temperature energy storage from the classification of heat‐resistant insulation grades27Functionalization of nanocellulose using atom transfer radical polymerization and applications: a review33Effects of Electromagnetic Field on Partial Discharge Behavior in BOPP Film Capacitors26Polymer dielectrics for capacitive energy storage: From theories, materials to industrial capacitors180Smart and Multifunctional Materials Based on Electroactive Poly(vinylidene fluoride): Recent Advances and Opportunities in Sensors, Actuators, Energy, Environmental, and Biomedical Applications497Mobile energy storage technologies for boosting carbon neutrality81Improved high-temperature energy storage of polyetherimide by energy level structure regulation28A new strategy to improve the dielectric properties of cellulose nanocrystals (CNCs): Surface modification of small molecules30High-temperature polymer dielectric films with excellent energy storage performance utilizing inorganic outerlayers49Manipulating fluorine induced bulky dipoles and their strong interaction to achieve high efficiency electric energy storage performance in polymer dielectrics37Recent progress in polymer dielectric energy storage: From film fabrication and modification to capacitor performance and application252Highly Flexible Dielectric Films from Solution Processable Covalent Organic Frameworks**35Polymer dielectrics for high-temperature energy storage: Constructing carrier traps241Progress in percolative composites with negative permittivity for applications in electromagnetic interference shielding and capacitors82Improved Capacitive Energy Storage at High Temperature via Constructing Physical Cross‐Link and Electron–Hole Pairs Based on P‐Type Semiconductive Polymer Filler141Constructing asymmetric gradient structures to enhance the energy storage performance of PEI-based composite dielectrics64Novel relaxor ferroelectric BTWO nanofillers for improving the energy storage performance of polymer-based dielectric composites25Enhanced energy storage characteristics of the epoxy film with rigid phenyl-flexible etherified methylene chains52Unifying and Suppressing Conduction Losses of Polymer Dielectrics for Superior High‐Temperature Capacitive Energy Storage107Mechanism Study of Molecular Trap in All‐Organic Polystyrene‐Based Dielectric Composite37Scalable High‐Permittivity Polyimide Copolymer with Ultrahigh High‐Temperature Capacitive Performance Enabled by Molecular Engineering117Boosting the maximized output energy density of triboelectric nanogenerators27Electrostatic interaction bridges the charge transport kinetics and high-temperature capacitive energy storage performance of polymer dielectrics64Gradient core–shell structure enabling high energy storage performances in PVDF-based copolymers27PEI-based all-organic composite films with simultaneous excellent energy storage density and high efficiency31Surface ion-activated polymer composite dielectrics for superior high-temperature capacitive energy storage123Polymer nanocomposite dielectrics for capacitive energy storage423Harnessing HfO 2 Nanoparticles for Wearable Tumor Monitoring and Sonodynamic Therapy in Advancing Cancer Care37Interfacial Engineering Using Covalent Organic Frameworks in Polymer Composites for High‐Temperature Electrostatic Energy Storage93Dilute Nanocomposites: Tuning Polymer Chain Local Nanostructures to Enhance Dielectric Responses60Polyimide composites crosslinked by aromatic molecules for high-temperature capacitive energy storage52Enhancing high-temperature energy storage performance of poly(arylene ether nitrile) hybrids synergistically via phthalonitrile modified boron nitride and carbon nanotube40Atomic‐Level Matching Metal‐Ion Organic Hybrid Interface to Enhance Energy Storage of Polymer‐Based Composite Dielectrics73Ultrahigh energy density in dielectric nanocomposites by modulating nanofiller orientation and polymer crystallization behavior43Versatile Landscape of Low- k Polyimide: Theories, Synthesis, Synergistic Properties, and Industrial Integration150Generative learning facilitated discovery of high-entropy ceramic dielectrics for capacitive energy storage57Synergistic Enhancement of Dielectric Polymers Through Fluorine Incorporation for Improved Energy Storage, Reduced Loss, and Enhanced Processability45Synergistically depressed dielectric loss and elevated breakdown strength in core@double-shell structured Cu@CuO@MgO/PVDF nanocomposites59Advances in electroactive biomaterials: Through the lens of electrical stimulation promoting bone regeneration strategy68Ultrahigh Dielectric Energy Density and Efficiency in PEI‐Based Gradient Layered Polymer Nanocomposite86Polymeric insulating materials characteristics for high-voltage applications101Interface engineering of polymer composite films for high-temperature capacitive energy storage55Review of Energy Storage Capacitor Technology112Development and characterization of PVA-based nanocomposites with graphene and natural quartz nanoparticles for energy storage applications39Flexible High‐Temperature Polymer Dielectrics Induced by Ultraviolet Radiation for High Efficient Energy Storage59Outstanding comprehensive energy storage performances in multiscale synergistic regulation-engineered (Bi0.5Na0.5)TiO3-based multilayer ceramics25Ultrahigh Energy Density Achieved at High Efficiency in Dielectric Capacitors by Regulating α‐Phase Crystallization in Polypropylene Films with Fluorinated Groups41Scalable polyolefin-based all-organic dielectrics with superior high-temperature capacitive energy storage performance64Design of functional and sustainable polymers assisted by artificial intelligence229Surface modification engineering on polymer materials toward multilevel insulation properties and subsequent dielectric energy storage55Enhanced high-temperature energy storage performances in polymer dielectrics by synergistically optimizing band-gap and polarization of dipolar glass85Flexible Graphene Field-Effect Transistors and Their Application in Flexible Biomedical Sensing108Alicyclic Polyimide With Multiple Breakdown Self‐Healing Based on Gas‐Condensation Phase Validation for High Temperature Capacitive Energy Storage148A Broad‐High Temperature Ceramic Capacitor with Local Polymorphic Heterogeneous Structures30Enhanced high-temperature energy storage performance in all-organic dielectric films through synergistic crosslinking of chemical and physical interaction40Advancing high-temperature electrostatic energy storage via linker engineering of metal–organic frameworks in polymer nanocomposites47Superior Capacitive Energy Storage Enabled by Molecularly Interpenetrating Interfaces in Layered Polymers25Machine learning-accelerated discovery of heat-resistant polysulfates for electrostatic energy storage94Scalable Hybrid Films of Polyimide‐Animated Quantum Dots for High‐Temperature Capacitive Energy Storage Utilizing Quantum Confinement Effect129In-plane aligned doping pattern in electrospun PEI/MBene nanocomposites for high-temperature capacitive energy storage25Nature-inspired synergistic strategy: carrier regulation in breakdown self-healing all-organic polymer dielectrics for enhanced high-temperature energy storage40Scalable all-organic polymer dielectrics for high-temperature film capacitors with construction of deep-trap level and cross-linking network29Scalable assembly of micron boron nitride into high-temperature-resistant insulating papers with superior thermal conductivity60Ultrahigh energy storage density and efficiency in facile dual-layered PVDF/PEI-based nanocomposites via an electrical/thermal synergistic effect26The Effects of Chain Conformation and Nanostructure on the Dielectric Properties of Polymers36Machine Learning Approaches in Polymer Science: Progress and Fundamental for a New Paradigm86Metal-organic cage crosslinked nanocomposites with enhanced high-temperature capacitive energy storage performance60Linear Dielectric Polymers with Ferroelectric‐Like Crystals for High‐Temperature Capacitive Energy Storage40High‐Temperature Polymer Composite Dielectrics: Energy Storage Performance, Large‐Scale Preparation, and Device Design105Rationally designed high-temperature polymer dielectrics for capacitive energy storage: An experimental and computational alliance31Ordering‐Structured Antiferroelectric Composite Ceramics for Energy Storage Applications44Film capacitor materials for electric vehicle applications: Status quo and future prospects73Significantly Enhancing the Energy‐Storage Properties of Polypropylene Films by Physically Manipulating Their Permittivity and Crystalline Behavior with Polar Organic Molecules28Benzene ring structural design strategy toward well-balanced thermal and electrical properties in epoxy dielectric polymers27Enhanced high-temperature capacitive energy storage in polyetherimide dielectrics through dense crosslinked network structures33Enhanced energy storage performance of nano-submicron structural dielectric films by suppressed ferroelectric phase aggregation48Interfacial dielectric enhancement in MXene/PVDF nanocomposites via hydrogen bond-induced dipole modulation27Continuous self-assembled BNNS layer on/within polymer film significantly enhances high-temperature capacitive energy storage26The Large‐Scale Manufacturing of Polymer Dielectric Capacitors: Advancements and Challenges41Regulating Carrier Transport Behavior for Capacitive Energy Storage of Polymer Dielectrics in Harsh Environments50Optimizing the Charge Transfer Complex Structure of Polyimides with Fluorinated Side Biphenyl for Superior High‐Temperature Capacitive Performance41Recent trends in all-organic polymer dielectrics for high-temperature electrostatic energy storage capacitors64Superior Energy Storage Performance Induced by Cross‐Scale Electric Field Modulation Utilizing Hybrid Hierarchical Micro–Nano Fillers in PEI‐based Composites25A Review on Multifunctional Polymer–MXene Hybrid Materials for Electronic Applications31Excellent high-temperature dielectric energy storage performance in bilayer nanocomposites with high-entropy ferroelectric oxide fillers40Materials informatics: A review of AI and machine learning tools, platforms, data repositories, and applications to architectured porous materials41Multiscale microstructure design for high-performance dielectric energy storage materials28

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