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RESEARCH PAPER · Cell Reports Physical Science · 2021

Lead-free B-site bimetallic perovskite photocatalyst for efficient benzylic C–H bond activation

Ming Shi, Hongpeng Zhou, Wenming Tian, Bin Yang, Songqiu Yang, Keli Han, Rengui Li, Can Li

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Lead-free B-site bimetallic perovskite photocatalyst for efficient benzylic C–H bond activationOriginalIn Situ Growth of Lead-Free Perovskite Cs2agbibr6 on a Flexible Ultrathin Carbon Nitride Sheet for Highly Efficient Photocatalytic Benzylic C(Sp3)−H Bond Activation41Recent advances and perspectives for solar-driven water splitting using particulate photocatalysts871Tuning Exciton Recombination Pathways in Inorganic Bismuth-Based Perovskite for Broadband Emission48Determining the Reaction Mechanisms of Photo‐Thermo Synergetic Processes by Kinetic Investigations2Surface active oxygen engineering of photoanodes to boost photoelectrochemical water and alcohol oxidation coupled with hydrogen production112Recent Advancements in Halide and Oxide Double Perovskites as Heterogeneous Photocatalysts for Solar-Driven Photocatalytic Water Splitting and CO2 Reduction2Bismuth-Based Halide Perovskites for Photocatalytic H2 Evolution Application32Cold- and hot-casting to regulate the morphology and charge carrier dynamics of CsBi 3 I 10 towards efficient and stable thin-film solar cells3Crystal structure engineering of metal halide perovskites for photocatalytic organic synthesis45Incorporation of functional polymers into metal halide perovskite thin-films: from interactions in solution to crystallization11Recent developments in lead-free bismuth-based halide perovskite nanomaterials for heterogeneous photocatalysis under visible light49Photovoltaic Materials as Heterogeneous Photocatalysts: A Golden Opportunity for Sustainable Organic Syntheses11Benzyl Alcohol Photo-oxidation Based on Molecular Electronic Transitions in Metal Halide Perovskites19Sb-Substituted Cs2AgBiBr6/g-C3N4 Composite for Photocatalytic C(sp3)–H Bond Activation in Toluene38Resistive switching and artificial synaptic performances of memristor based on low-dimensional bismuth halide perovskites39Transfer matrix method-based efficiency enhancement of lead-free Cs3Sb2Br9 perovskite solar cell26Tuning the Optoelectronic Property of All‐Inorganic Lead‐Free Perovskite via Finely Microstructural Modulation for Photovoltaics21The Dark Side of Lead-Free Metal Halide Nanocrystals: Substituent-Modulated Photocatalytic Activity in Benzyl Bromide Reduction25Mixed Halide Formation in Lead‐Free Antimony‐Based Halide Perovskite for Boosted CO2 Photoreduction: Beyond Band Gap Tuning45Structural Modification Strategies, Interfacial Charge‐Carrier Dynamics, and Solar Energy Conversion Applications of Organic–Inorganic Halide Perovskite Photocatalysts33Cs2SnCl6: To Emit or to Catalyze? Te4+ Ion Calls the Shots35Amplifying photoreduction efficacy of Bi-Sb bimetallic nanocrystals: Manipulating carrier dynamics to boost CO2-to-CO conversion23Lead-free Dion-Jacobson layered double perovskite as a photocatalyst for toluene oxidation17Lead-free metal halide perovskites as the rising star in photocatalysis: The past, present, and prospective49Cs3Bi2Br9/g-C3N4 Direct Z-Scheme Heterojunction for Enhanced Photocatalytic Reduction of CO2 to CO57New visible-light-driven Bi2MoO6/Cs3Sb2Br9 heterostructure for selective photocatalytic oxidation of toluene to benzaldehyde38Rational Atom Substitution to Obtain Efficient, Lead‐Free Photocatalytic Perovskites Assisted by Machine Learning and DFT Calculations37Rational Atom Substitution to Obtain Efficient, Lead‐Free Photocatalytic Perovskites Assisted by Machine Learning and DFT Calculations5Synthesis of small size lead-free Cs 3 Bi 2 x Sb 2−2 x Br 9 solid-solutions using a spatially confined growth method for efficient photocatalytic CO 2 reduction11Photocatalysis Based on Metal Halide Perovskites for Organic Chemical Transformations24Moisture-induced ionovoltaic electricity generation using lead free 2-dimensional Cs 3 SbBiBr 9 perovskite4Polymeric Metal Halides with Bright Luminescence and Versatile Processability6Polymeric Metal Halides with Bright Luminescence and Versatile Processability22Dynamically Cyclic Fe 2+ /Fe 3+ Active Sites as Electron and Proton-Feeding Centers Boosting CO 2 Photoreduction Powered by Benzyl Alcohol Oxidation17Selective oxidative coupling of amines through light‐activated bismuth halide perovskites14Solar‐Driven Selective Oxidation Over Bismuth‐Based Semiconductors: From Prolific Catalysts to Diverse Reactions63Modulating Adsorption–Redox Sites and Charge Separation of Cs3Bi2Br9–x@AgBr Core–Shell Heterostructure for Selective Toluene Photooxidation69Perovskite Paradigm Shift: A Green Revolution with Lead-Free Alternatives in Photocatalytic CO 2 Reduction52Spin-Phonon Coupling in Iron-Doped Ultrathin Bismuth Halide Perovskite Derivatives7Machine‐Learning‐Assisted Discovery of Mechanosynthesized Lead‐Free Metal Halide Perovskites for the Oxidative Photocatalytic Cleavage of Alkenes22Lead‐Free Perovskite‐Based Photocatalysts for Solar‐Driven Chemistry Technologies4Bimetallic B-Site Halide Perovskites for Enhanced Photocatalytic CO2 Reduction22A review of chalcogenide-based perovskites as the next novel materials: Solar cell and optoelectronic applications, catalysis and future perspectives111Efficient hole extraction to reactive oxidation sites over a Co3O4/Cs3Sb2Br9 p-n heterojunction for enhanced benzylic C(sp3)-H bond oxidation28Single‐Atom Catalysts with p‐Block Metals Surpass Transition‐Metal Counterparts in the Photocatalytic H2O2 Production26Single‐Atom Catalysts with p‐Block Metals Surpass Transition‐Metal Counterparts in the Photocatalytic H2O2 Production6Targeted Electron‐Hole Separation to Decoupled Redox‐Active Sites Over a PEA2PbBr4/CeO2 P‐N Heterojunction for Enhanced Photocatalytic Oxidation10A closer look at the interface of Cs3Bi2Br9 lead free perovskite in photocatalytic process8Organic Transformation Mediated by Lead-Free Perovskites and Related Materials0Surface and Defect Engineering Coupling of Charge Shuttle and Redox Site in Cs3Bi2Br9/g-C3N4 for Efficient Photocatalytic C(sp3)–H Bond Activation17Advances in perovskite nanomaterials: Synthesis and catalytic applications in energy and environmental remediation17Lead-Free Metal Halide Double Perovskite-Photoelectrocatalyzed Activation of C(sp3)-H Bonds and Alkylation of Alkenes and Azo Compounds10Oxygen vacancy in lead‐free perovskite Cs 2 AgBiBr 6 /WO 3‐ X for enhanced photocatalytic C(sp 3 )‐H bond oxidation8Interfacial Bi–O Bridge Elevated Bi p -Band Center Boosting Photocatalytic C( sp 3 )–H Bonds Oxidation40Design and performance analysis of Cs 2 Ag ( Sb y Bi 1 ‐ y ) Br 6 perovskite solar cells: Insights from SCAPS-1D device simulations13Chiral Two-Dimensional Cu–Pb Bromides: Circularly Polarized Luminescence and Pressure-Enhanced Optical Properties7Bandgap tuning through controlled Bi/Sb substitution in Cs2AgBi1-xSbxBr6 enhances overall solar cell performance8Photocatalysts for a Sustainable Future: Innovations and Applications0Ce 3+ -Doped Cs 3 Bi 2 Br 9 for Photocatalytic Selective Oxidation of Alcohols to Aldehydes/Ketones3Facet‐Engineering in Cs 3 Bi 2 Br 9 Vacancy‐Ordered Perovskite With Built‐In Anisotropic Charge Separation for Selective Photocatalytic Toluene Oxidation1Simultaneously Enhancing Activity and Stability of Perovskite by Grafting Dodecylphosphonic Acid for Selective Photooxidation of C(sp 3 )–H0Decoupling Thermodynamic Dilemma in the Crystallization of Cs3BiSbBr9 Bimetallic Perovskites for Photocatalytic HBr Splitting0Coupling Electronic Structure Modulation with Self-Trapped Exciton Dynamics in Dual-Doped Cs3Bi2Br9 for Efficient Photocatalytic Hydrogen Evolution0

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  1. In Situ Growth of Lead-Free Perovskite Cs2agbibr6 on a Flexible Ultrathin Carbon Nitride Sheet for Highly Efficient Photocatalytic Benzylic C(Sp3)−H Bond Activation

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  2. Recent advances and perspectives for solar-driven water splitting using particulate photocatalysts

    Chemical Society Reviews · 2022-01-01

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  3. Tuning Exciton Recombination Pathways in Inorganic Bismuth-Based Perovskite for Broadband Emission

    Energy Material Advances · 2022-01-01

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  4. Determining the Reaction Mechanisms of Photo‐Thermo Synergetic Processes by Kinetic Investigations

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  5. Surface active oxygen engineering of photoanodes to boost photoelectrochemical water and alcohol oxidation coupled with hydrogen production

    Applied Catalysis B: Environmental · 2022-11-07

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  6. Recent Advancements in Halide and Oxide Double Perovskites as Heterogeneous Photocatalysts for Solar-Driven Photocatalytic Water Splitting and CO2 Reduction

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  7. Bismuth-Based Halide Perovskites for Photocatalytic H2 Evolution Application

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  8. Cold- and hot-casting to regulate the morphology and charge carrier dynamics of CsBi 3 I 10 towards efficient and stable thin-film solar cells

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  9. Crystal structure engineering of metal halide perovskites for photocatalytic organic synthesis

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  10. Incorporation of functional polymers into metal halide perovskite thin-films: from interactions in solution to crystallization

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  11. Recent developments in lead-free bismuth-based halide perovskite nanomaterials for heterogeneous photocatalysis under visible light

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  12. Photovoltaic Materials as Heterogeneous Photocatalysts: A Golden Opportunity for Sustainable Organic Syntheses

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  13. Benzyl Alcohol Photo-oxidation Based on Molecular Electronic Transitions in Metal Halide Perovskites

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  14. Sb-Substituted Cs2AgBiBr6/g-C3N4 Composite for Photocatalytic C(sp3)–H Bond Activation in Toluene

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  15. Resistive switching and artificial synaptic performances of memristor based on low-dimensional bismuth halide perovskites

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  16. Transfer matrix method-based efficiency enhancement of lead-free Cs3Sb2Br9 perovskite solar cell

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  17. Tuning the Optoelectronic Property of All‐Inorganic Lead‐Free Perovskite via Finely Microstructural Modulation for Photovoltaics

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  18. The Dark Side of Lead-Free Metal Halide Nanocrystals: Substituent-Modulated Photocatalytic Activity in Benzyl Bromide Reduction

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  19. Mixed Halide Formation in Lead‐Free Antimony‐Based Halide Perovskite for Boosted CO2 Photoreduction: Beyond Band Gap Tuning

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  20. Structural Modification Strategies, Interfacial Charge‐Carrier Dynamics, and Solar Energy Conversion Applications of Organic–Inorganic Halide Perovskite Photocatalysts

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  21. Cs2SnCl6: To Emit or to Catalyze? Te4+ Ion Calls the Shots

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  22. Amplifying photoreduction efficacy of Bi-Sb bimetallic nanocrystals: Manipulating carrier dynamics to boost CO2-to-CO conversion

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  23. Lead-free Dion-Jacobson layered double perovskite as a photocatalyst for toluene oxidation

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  24. Lead-free metal halide perovskites as the rising star in photocatalysis: The past, present, and prospective

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  25. Cs3Bi2Br9/g-C3N4 Direct Z-Scheme Heterojunction for Enhanced Photocatalytic Reduction of CO2 to CO

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  26. New visible-light-driven Bi2MoO6/Cs3Sb2Br9 heterostructure for selective photocatalytic oxidation of toluene to benzaldehyde

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  27. Rational Atom Substitution to Obtain Efficient, Lead‐Free Photocatalytic Perovskites Assisted by Machine Learning and DFT Calculations

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  29. Synthesis of small size lead-free Cs 3 Bi 2 x Sb 2−2 x Br 9 solid-solutions using a spatially confined growth method for efficient photocatalytic CO 2 reduction

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  30. Photocatalysis Based on Metal Halide Perovskites for Organic Chemical Transformations

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  31. Moisture-induced ionovoltaic electricity generation using lead free 2-dimensional Cs 3 SbBiBr 9 perovskite

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  32. Polymeric Metal Halides with Bright Luminescence and Versatile Processability

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  34. Dynamically Cyclic Fe 2+ /Fe 3+ Active Sites as Electron and Proton-Feeding Centers Boosting CO 2 Photoreduction Powered by Benzyl Alcohol Oxidation

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  35. Selective oxidative coupling of amines through light‐activated bismuth halide perovskites

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  44. Efficient hole extraction to reactive oxidation sites over a Co3O4/Cs3Sb2Br9 p-n heterojunction for enhanced benzylic C(sp3)-H bond oxidation

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  48. A closer look at the interface of Cs3Bi2Br9 lead free perovskite in photocatalytic process

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  49. Organic Transformation Mediated by Lead-Free Perovskites and Related Materials

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  50. Surface and Defect Engineering Coupling of Charge Shuttle and Redox Site in Cs3Bi2Br9/g-C3N4 for Efficient Photocatalytic C(sp3)–H Bond Activation

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