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RESEARCH PAPER · Advanced Energy Materials · 2021

High‐Entropy Energy Materials in the Age of Big Data: A Critical Guide to Next‐Generation Synthesis and Applications

Qingsong Wang, Leonardo Velasco, Ben Breitung, Volker Presser

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High‐Entropy Energy Materials in the Age of Big Data: A Critical Guide to Next‐Generation Synthesis and ApplicationsOriginalProspects and challenges for autonomous catalyst discovery viewed from an experimental perspective46Shifts in valence states in bimetallic MXenes revealed by electron energy-loss spectroscopy (EELS)19Evaluating quantum alchemy of atoms with thermodynamic cycles: Beyond ground electronic states9Machine learning-enabled framework for the prediction of mechanical properties in new high entropy alloys82Kinetically Accelerated Lithium Storage in High‐Entropy (LiMgCoNiCuZn)O Enabled By Oxygen Vacancies130Laser-aided additive manufacturing of high entropy alloys: Processes, properties, and emerging applications134Materials Data toward Machine Learning: Advances and Challenges62Resolving the Role of Configurational Entropy in Improving Cycling Performance of Multicomponent Hexacyanoferrate Cathodes for Sodium‐Ion Batteries152Surface‐Decorated High‐Entropy Alloy Catalysts with Significantly Boosted Activity and Stability149Review: High-Entropy Materials for Lithium-Ion Battery Electrodes70Mapping Thermoelectric Transport in a Multicomponent Alloy Space15Layered Titanium Niobium Oxides Derived from Solid-Solution Ti–Nb Carbides (MXene) as Anode Materials for Li-Ion Batteries22Thermoelectric properties of a high entropy half-Heusler alloy processed by a fast powder metallurgy route31High-Entropy Perovskite Electrolyte for Protonic Ceramic Fuel Cells Operating below 600 °C119High‐entropy oxide: A future anode contender for lithium‐ion battery120P2-type layered high-entropy oxides as sodium-ion cathode materials94Synthesis and Characterization of High‐Entropy CrMoNbTaVW Thin Films Using High‐Throughput Methods14Effect of synthesis environment on the electrochemical properties of ( FeMnCrCoZn ) 3 O 4 high‐entropy oxides for Li‐ion batteries26High‐Entropy Catalyst—A Novel Platform for Electrochemical Water Splitting190High Entropy Approach to Engineer Strongly Correlated Functionalities in Manganites65A Method for Assessing the Security of Energy Trading Data Based on Big Data and the Pagerank Algorithm0Functional two-dimensional high-entropy materials96Recent Advances in Nanoengineering of Electrode‐Electrolyte Interfaces to Realize High‐Performance Li‐Ion Batteries18The effect of configurational entropy on acoustic emission of P2-type layered oxide cathodes for sodium-ion batteries24High‐Entropy Sulfides as Highly Effective Catalysts for the Oxygen Evolution Reaction69High‐Throughput Exploration of Triple‐Cation Perovskites via All‐in‐One Compositionally‐Graded Films12Strain‐Driven Bidirectional Spin Orientation Control in Epitaxial High Entropy Oxide Films18Shock state distributions in porous tantalum and characterization with multipoint velocimetry5Machine Learning Paves the Way for High Entropy Compounds Exploration: Challenges, Progress, and Outlook78High‐Valence Metal‐Driven Electronic Modulation for Boosting Oxygen Evolution Reaction in High‐Entropy Spinel Oxide166Exploration of Solution-Processed Bi/Sb Solar Cells by Automated Robotic Experiments Equipped with Microwave Conductivity18Machine learning‐based crystal structure prediction for high‐entropy oxide ceramics31High-entropy metal diselenides propels polyselenides immobilization for high performance sodium storage40Acoustic Signal Generation Techniques for Improved Coconut Maturity Classification System0Enhancing lithium storage rate and durability in sphalerite GeP by engineering configurational entropy15Machine learning the screening factor in the soft bond valence approach for rapid crystal structure estimation7Manganese-rich high entropy oxides for lithium-ion batteries:materials design approaches to address voltage fade19Memristor-Based Bayesian Spiking Neural Network for Ibd Diagnosis0More is better: high-entropy electrolyte design in rechargeable batteries196The rise of high-entropy battery materials176Germanium-telluride-based thermoelectrics24Unlocking the Potential of High Entropy Alloys in Electrochemical Water Splitting: A Review122High-entropy materials for energy and electronic applications448Revealing the Potential and Challenges of High‐Entropy Layered Cathodes for Sodium‐Based Energy Storage174Robust high-entropy spinel oxides for peroxymonosulfate activation: Stabilization effect and enhancement mechanism32Crystal‐Phase‐Engineered High‐Entropy Alloy Aerogels for Enhanced Ethylamine Electrosynthesis from Acetonitrile39Machine Learning-Based Prediction of Stability in High-Entropy Nitride Ceramics10Unveiling the potential of (CoFeNiMnCr)3O4 high-entropy oxide synthesized from CoFeNiMnCr high-entropy alloy for efficient oxygen-evolution reaction23Advancements and future prospects of additive manufacturing in high-entropy alloy applications78Elevating energy storage: High-entropy materials take center stage9High entropy oxides for reversible lithium-ion battery: a brief review4Memristor-based Bayesian spiking neural network for IBD diagnosis1Strained single crystal high entropy oxide manganite thin films8Unraveling the origin of the high reversibility in entropy-stabilized rocksalt-type (Mg0.2Co0.2Mn0.2Ni0.2Zn0.2)O anodes for lithium-ion storage17Accelerating the screening of high-entropy Co-Mn-Fe-Ni-Zn-O gradient films for highly stable NTC materials through co-sputtering combinatorial synthesis7A critical review on the high entropy material coatings: criteria for materials selection and coating procedure4The concept of high entropy for rechargeable batteries57Composition Engineering and Crystal Growth of High-Entropy Rare-Earth Monoclinic Aluminates2Structural and functional connections in the technological system of “laser cladding of high-entropy coatings”0Unveiling the Microscopic Origin of Ultrahigh Initial Coulombic Efficiency of High-Entropy Metal–Organic Frameworks for Sodium Storage28High-entropy oxides as energy materials: from complexity to rational design52Advances in high entropy oxides: synthesis, structure, properties and beyond144Machine Learning Accelerated Discovery of Entropy-Stabilized Oxide Catalysts for Catalytic Oxidation58Ultra‐rapid Synthesis of High‐entropy MAX Phases and Their Derivative MXenes for Battery Electrodes18Ultra‐rapid Synthesis of High‐entropy MAX Phases and Their Derivative MXenes for Battery Electrodes6Improving upon rechargeable battery technologies: on the role of high-entropy effects110Synthesis‐Structure‐Property of High‐Entropy Layered Oxide Cathode for Li/Na/K‐Ion Batteries35Understanding of the composition-structure-properties relationships in high-entropy rare earth zirconates10Impact of Synthetic Parameters on Structure and Electrochemistry of High-Entropy Layered Oxide LiNi0.2Co0.2Mn0.2Al0.2Fe0.2O24Advanced high-entropy materials for high-quality energy storage and conversion23Mechanical performance and deformation mechanisms of AlCrFeCuNi high-entropy alloy/graphene nanocomposites10MAX phase coatings: synthesis, protective performance, and functional characteristics63A novel Co-free high-entropy oxide (FeNiCrMnMgAl)3O4 as advanced anode material for lithium-ion batteries17Applications of machine learning in high-entropy alloys: a review of recent advances in design, discovery, and characterization41High entropy alloys: a comprehensive review of synthesis, properties, and characterization for electrochemical energy conversion and storage applications25High-entropy alloys and oxides as catalysts for water-splitting: synthesis, characterization, applications and prospects15High-entropy materials for electrocatalytic oxygen reduction reaction26High-entropy materials: synthesis and energy storage applications7Shaping Tacit Knowledge of Technopreneurs: A Qualitative Survey of ICT SMEs in Malaysia0Finite element analysis, machine learning, and digital twins for soft robots: state-of-arts and perspectives41Rational design of large-scale high-entropy alloy nanosheets anode with excellent lithium storage performance7Designing Nanoporous Non-noble High Entropy Alloys as Efficient Catalysts for the Hydrogen Evolution Reaction18Leveraging Data Augmentation in Improving Machine Learning Algorithms for Coconut Maturity Classification0Improving CO Oxidation Catalysis Over High Entropy Spinels by Increasing Disorder25High‐Entropy Halides for Intercalation Battery Electrode Materials3Advancing NASICON-type materials through high-entropy strategy: Synthesis and applications11The recent progress of high-entropy layered double hydroxides and high-entropy amorphous materials for water electrocatalysis20Controllable Crystalline Phases of Multi‐Cation Oxides2High entropy powering green energy: hydrogen, batteries, electronics, and catalysis23Interpretable machine learning prediction of mechanical properties of AlCoCrFeNi/graphene composites2Clean Energy and Electrocatalysis1AI Design for High Entropy Alloys: Progress, Challenges and Future Prospects16Synthesis‐Driven Functionality in High‐Entropy Materials34Recent advances in the high entropy materials for advanced energy storage with machine learning6A Machine Learning Approach to Determine the Band Gap Energy of High-Entropy Oxides Using UV-Vis Spectroscopy0Toward high entropy material discovery for energy applications using computational and machine learning methods8High Entropy 2D Materials for Electrochemical Water Splitting0High-entropy materials in rechargeable batteries: design principles and structure–performance correlations0High-Entropy Materials Chemistry for Electrochemical Energy Storage34High‐Entropy 2D MXenes: A New Paradigm for Energy Storage7Two-Lever Design Rule for High-Entropy Oxide Oxygen Carriers: Minimize Spin Polarization, Maximize Fe–O–Ni Covalency2Rational Design of Single-Phase High-Entropy Oxides via Large Language Model Data Mining and Explainable Machine Learning1Carbon-Supported High-Entropy Electrocatalyst Design via Large Language Models0Collective Synergistic Effects in High Entropy Perovskite Oxide Electrocatalysts for Enhanced Oxygen Evolution Reaction0High-Entropy Oxides for Energy Storage and Electrocatalysis: Defect Chemistry, Entropy Stabilization, and Structure–Performance Design Rules0Mechanistic Insights Into Entropy Regulation in Sodium/Potassium‐Ion Batteries0Emerging High‐Entropy Alloys for Rechargeable Zinc‐Air Batteries: From Fundamental Concepts to Advanced Electrocatalyst Design0

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  4. Machine learning-enabled framework for the prediction of mechanical properties in new high entropy alloys

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  5. Kinetically Accelerated Lithium Storage in High‐Entropy (LiMgCoNiCuZn)O Enabled By Oxygen Vacancies

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  7. Materials Data toward Machine Learning: Advances and Challenges

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  8. Resolving the Role of Configurational Entropy in Improving Cycling Performance of Multicomponent Hexacyanoferrate Cathodes for Sodium‐Ion Batteries

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  17. Synthesis and Characterization of High‐Entropy CrMoNbTaVW Thin Films Using High‐Throughput Methods

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  18. Effect of synthesis environment on the electrochemical properties of ( FeMnCrCoZn ) 3 O 4 high‐entropy oxides for Li‐ion batteries

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  20. High Entropy Approach to Engineer Strongly Correlated Functionalities in Manganites

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  49. Advancements and future prospects of additive manufacturing in high-entropy alloy applications

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