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RESEARCH PAPER · Journal of the American Chemical Society · 2021

Alkyl–Aryl Cation Mixing in Chiral 2D Perovskites

Liang Yu Yan, Manoj K. Jana, Peter C. Sercel, David B. Mitzi, Wei You

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Alkyl–Aryl Cation Mixing in Chiral 2D PerovskitesOriginalSpin-polarized excitons and charge carriers in chiral metal halide semiconductors23Two-dimensional BA 2 PbBr 4 -based wafer for X-rays imaging application15Advances in single crystals and thin films of chiral hybrid metal halides38cis/trans-Isomeric Cation Tuning Photoluminescence and Photodetection in 2D Perovskites21Structural Origin of Enhanced Circularly Polarized Luminescence in Hybrid Manganese Bromides113Structural Origin of Enhanced Circularly Polarized Luminescence in Hybrid Manganese Bromides16Core–Shell Three-Dimensional Perovskite Nanocrystals with Chiral-Induced Spin Selectivity for Room-Temperature Spin Light-Emitting Diodes183Strong Induced Circular Dichroism in a Hybrid Lead‐Halide Semiconductor Using Chiral Amino Acids for Crystallite Surface Functionalization26Tailoring the Distinctive Chiral‐Polar Perovskites with Alternating Cations in the Interlayer Space for Self‐Driven Circularly Polarized Light Detection65Leveraging Hierarchical Chirality in Perovskite(‐Inspired) Halides for Transformative Device Applications41Ordered Mixed-Spacer 2D Bromide Perovskites and the Dual Role of 1,2,4-Triazolium Cation38Direct Detection of Near-Infrared Circularly Polarized Light via Precisely Designed Chiral Perovskite Heterostructures37Ligand Coverage and Exciton Delocalization Control Chiral Imprinting in Perovskite Nanoplatelets18Tailoring the Time-Averaged Structure for Polarization-Sensitive Chiral Perovskites43Chain-to-Layer Dimensionality Engineering of Chiral Hybrid Perovskites to Realize Passive Highly Circular-Polarization-Sensitive Photodetection124Strong two-photon absorption induced by energy funneling in chiral quasi-2D perovskites6Structural Descriptors to Correlate Pb Ion Displacement and Broadband Emission in 2D Halide Perovskites121Multilayered Alternating‐Cations‐Intercalation Chiral Hybrid Perovskites with High Circular Polarization Sensitivity28Spin Selectivity in Chiral Hybrid Cobalt Halide Films with Ultrasmooth Surface27Spacer Cation Alloying Enables Markedly Improved Chiroptical Properties of Two‐Dimensional Chiral Hybrid Perovskite Nanosheets37Alternating chiral and achiral spacers for constructing two-dimensional chiral hybrid perovskites toward circular-polarization-sensitive photodetection22Circularly polarized luminescence enlargement from crystals to oriented films of enantiopure 2D hybrid perovskites13Second harmonic generation from symmetry breaking stimulated by mixed organic cations in zero-dimensional hybrid metal halides7Simultaneously achieving room-temperature circularly polarized luminescence and high stability in chiral perovskite nanocrystals via block copolymer micellar nanoreactors20Two-dimensional lead-free silver-bismuth double perovskite nanobelts with intrinsic chirality via co-antisolvent modulation strategy4Pressure‐Tuned Multicolor Emission of 2D Lead Halide Perovskites with Ultrahigh Color Purity64Pressure‐Tuned Multicolor Emission of 2D Lead Halide Perovskites with Ultrahigh Color Purity5Toward Efficient Two‐Photon Circularly Polarized Light Detection through Cooperative Strategies in Chiral Quasi‐2D Perovskites65Synthesis of five-layered chiral perovskite nanowires and enacting chiroptical activity regulation15One‐Dimensional Chiral Copper Iodide Chain‐Like Structure Cu 4 I 4 ( R / S ‐3‐quinuclidinol) 3 with Near‐Unity Photoluminescence Quantum Yield and Efficient Circularly Polarized Luminescence47Optical properties of two-dimensional perovskites9Discovering New Type of Lead‐Free Cluster‐Based Hybrid Double Perovskite Derivatives with Chiral Optical Activities and Low X‐Ray Detection Limit43Mixed-cation chiral perovskites displaying warm-white circularly polarized luminescence24Unique Chiro-optical Properties of the Weakly-2D (R-/S-MBA)2CuBr4 Hybrid Material31Insight into efficient photoluminescence regulation mechanism by lattice distortion and Mn2+ doping in organic-inorganic hybrid perovskites1Ligand‐Assisted Self‐Assembly of 3D Perovskite Nanocrystals into Chiral Inorganic Quasi‐2D Perovskites ( n = 3) with Ligand‐Ratio‐Dependent Chirality Inversion23Mono‐ and Bi‐Dentate Chiral Ligands Lead to Efficient Circularly Polarized Luminescence in 0D and 3D Semiconducting Copper(I) Iodides37Controlling Phase Transitions in Two-Dimensional Perovskites through Organic Cation Alloying37Mixed perovskites (2D/3D)-based solar cells: a review on crystallization and surface modification for enhanced efficiency and stability57Non-covalent interactions involving π effect between organic cations in low-dimensional organic/inorganic hybrid perovskites20Unprecedented Chiral Three‐dimensional Hybrid Organic‐Inorganic Perovskitoids36Unprecedented Chiral Three‐dimensional Hybrid Organic‐Inorganic Perovskitoids0Integrating Achiral and Chiral Organic Ligands in Zero‐Dimensional Hybrid Metal Halides to Boost Circularly Polarized Luminescence81Integrating Achiral and Chiral Organic Ligands in Zero‐Dimensional Hybrid Metal Halides to Boost Circularly Polarized Luminescence8Formamidine Engineering the Lattice Distortion of Chiral Halide Perovskites for Efficient Blue Circularly Polarized Emission28Chiral Cation Doping for Modulating Structural Symmetry of 2D Perovskites62Spatially Correlated Chirality in Chiral Two-Dimensional Perovskites Revealed by Second-Harmonic-Generation Circular Dichroism Microscopy56Real-Time Monitoring of Progressive Crystal Phase Transformations and Associated Multi-Phase Optical Exciton Dynamics in Mixed (2D/3D) Inorganic–Organic Hybrid Semiconductors3Chiral‐Achiral Cations Intercalation Induced Lead‐Free Chiral‐Polar Hybrid Perovskites Enable Self‐Powered X‐Ray and Ultraviolet–Visible–Near‐Infrared Photo Detection33In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation11In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation68Rational design of enantiomeric lead-free double perovskites by achiral-chiral cation intercalation28Chiral 2D and quasi-2D hybrid organic inorganic perovskites: from fundamentals to applications51Chirality-driven amplification of sensitive polarized light detection in alternating cation-intercalated perovskites0Constructing Multilayered Alternating Cations Intercalation Hybrid Perovskites with Short Interlayer Distance Using Aromatic Cations as Spacers0Precise design of chiral-polar hybrid perovskites toward efficient self-powered full-stokes photodetection14Tuning the circularly polarized phosphorescence of platinum( ii ) complexes through a chiral cation strategy7Variable energy transfer in one-dimensional chiral Mn/Cd-based halides and strong stereo-selective fluorescence for chiral recognition5Highly Circularly Polarized Light‐Sensitive Chiral One‐Dimensional Perovskites Enabled by Antisolvent Engineering26Giant Apparent Optical Circular Dichroism in Thin Films of Bismuth‐Based Hybrid Organic–Inorganic Metal Halide Semiconductor Through Preferred Orientation16Phase Transitions and Dynamics in Mixed Three- and Low-Dimensional Lead Halide Perovskites134Perovskite-Supramolecular Co-Assembly for Chiral Optoelectronics15Structure-Guided Approaches for Enhanced Spin-Splitting in Chiral Perovskite42Directed Assembly of Ordered Mixed‐Spacer Quasi‐2D Halide Perovskites through Homomeric Chains of Intermolecular Bonds7Efficient Quasi-2D Perovskite Spin Light-Emitting Diodes Based on Chiral-Induced Spin Selectivity47Self-Powered Circularly Polarized Light Detection Enabled by Chiral Two-Dimensional Perovskites with Mixed Chiral–Achiral Organic Cations42Structural Diversity in 2-(2-Aminoethyl)pyridine-Based Lead Iodide Hybrids1Anomalous Correlation between Thermal Conductivity and Elastic Modulus in Two-Dimensional Hybrid Metal Halide Perovskites15The Mn2+‐Doped Chiral 2D Perovskite with Strong Orange Fluorescent and Enhanced Circularly Polarized Luminescence5Recent progress on chiral perovskites as chiroptical active layers for next-generation LEDs25Homochiral and Heterochiral Cation Mixing in 2D Perovskites for Enhanced Structural Asymmetry and Spin Splitting11Mixed Organic Cation in Chiral Two-Dimensional Organic–Inorganic Hybrid Metal Halides─An Ab Initio Study of Nonlinear Optical (NLO) Properties10Enhanced Stability of Spin-Dependent Chiral 2D Perovskite Embedded PV-Biased Anode via Cross-Linking Strategy13Polar Alternating Cations Intercalated Hybrid Perovskite with Iodine‐Substituted Spacers Toward Efficient Passive X‐Ray Detection21Strain-Amplified Exciton Chirality in Organic-Inorganic Hybrid Materials9Mixed‐Ligand Chiral Quasi‐2D Perovskites for Standard and Deep Blue CP‐LEDs27Boosted Chirality Transfer in 2D Perovskites through Structural Isomer‐Driven Halogen–Halogen Interaction33Giant chiral amplification of chiral 2D perovskites via dynamic crystal reconstruction52Efficient Room-Temperature Phosphorescence in 2D Perovskite via Mixed Organic Cation Incorporation6Enhancing Circular Dichroism in Chiral Perovskites via Dual Spacer Cation Engineering for Circularly Polarized Light Detection14Unveiling Chirality Transfer between Chiral Centers and Metal Halides in Chiral Organic–Inorganic Hybrid Metal Halides25Enhancing Chiroptoelectronic Activity in Chiral 2D Perovskites via Chiral–Achiral Cation Mixing11Chiral 0D hybrid lead-bromide perovskites with strong nonlinear chiroptical properties16Regulating Second‐Harmonic Generation in 2D Chiral Perovskites Through Achiral Organic Spacer Cation Alloying Strategy15Structural Reconfiguration via Alternating Cation Intercalation of Chiral Hybrid Perovskites for Efficient Self-Driven X-ray Detection11Chiral-Polar Alternating Cation Intercalation-Type Perovskite Enables Sensitive Self-Driven X-ray Detection with an Ultralow Detection Limit32D/3D Heterostructured Perovskites for Highly Selective Room-Temperature Blue Spin-Polarized Light-Emitting Diodes01.5D Chiral Perovskites Mediated by Hydrogen‐Bonding Network with Remarkable Spin‐Polarized Property21.5D Chiral Perovskites Mediated by Hydrogen‐Bonding Network with Remarkable Spin‐Polarized Property18Dramatical enhancement of circular dichroism in chiral hybrid perovskites via carboxylic hydrogen bond engineering6Chirality-Induced Spin Selectivity in Hybrid Organic-Inorganic Perovskite Semiconductors36Temperature-responsive opto-electrical characteristics combined with reversible thermochromism in copper chloride hybrid perovskite for smart window applications4Ordered Cationic Mixing in a 1D Organic–Inorganic Hybrid2Ordered assembly of templated chiral/achiral organic cations toward efficient circularly polarized emission in hybrid antimony chlorides11Two-photon excited spin excitonic properties in two-dimensional chiral perovskite films1Inverted Chiroptical Properties of Hybrid Metal Halides Through Reversible Chiral Induction Driven by External and Internal Chirality Transfer18Inverted Chiroptical Properties of Hybrid Metal Halides Through Reversible Chiral Induction Driven by External and Internal Chirality Transfer2Regulating Circularly Polarized Luminescence in Zero-Dimensional Chiral Hybrid Metal Halides28High Circularly Polarized Luminescence Dissymmetry Factor and Efficient Chiral Second Harmonic Generation in Chiral Hybrid Lead‐Bromide Perovskites13Realization of Tunable X-ray Detection in 2D Chiral-Polar Hybrid Perovskites0Anomalous Photovoltaic Effect in a Chiral Alternating‐Cation Intercalation‐Type Perovskite for Efficient Self‐Driven X‐Ray Detection4Impact of Halide Substitution in the Inorganic Framework on the Optical Activity of Chiral Metal-Halide Perovskites4Achiral Cation-Induced Chirality Tuning in Cycloalkyl Chiral Cation-Based Quasi-1D and 2D Perovskites6Controlling Energy Flow in Perovskite Heterostructures Through Dimensionality and Phase Engineering7Origins of Structural and Electronic Chirality in the 2D Hybrid Perovskites8Challenges, Solutions, and Opportunities in Chiral Perovskites: From Synthesis Strategies to Technological Advancements4Engineering the Electronic Structure and Optoelectronic Properties of Chiral Metal Halides through Cation Design0Dimensional Engineering in Hybrid Transition Metal Halide Materials through the Introduction of Chiral Organic Cations5Chiroptical Amplification Beyond Enantiopurity in Chiral Films4Self‐Powered Circularly Polarized Photodetectors Based on Chiral (R/S‐MBA) 2 PbI 4 Perovskite7Chiral Metal Halides toward Circularly Polarized Photodetectors13Chiral Hybrid Organic–Inorganic Metal Halides: Preparation, Luminescent Properties, and Applications2Structural Engineering for Chirality-Induced Spin Control in Metal–Halide Perovskites10Chirality amplification in semiconductors for advanced optoelectronics23Engineering Efficient Circularly Polarized Luminescence in Copper(I) Iodides through Supramolecular Chirality Control13Bifunctional Spacer Cation Enables High-Efficiency Chiral Red Quasi-2D Perovskite Light-Emitting Diodes via Defect Passivation and Chirality Enhancement12Internally and externally induced chiral hybrid metal halide materials for advanced chiroptoelectronic applications23Alternating cations intercalation-type chiral-polar hybrid perovskites for efficient self-powered polarization detection0Chirality Transfer in Metal Halide Semiconductors16Integrated Photon Ellipticity Recognition with Chiral Nanomaterials1Boosting Intrinsic Chirality of One‐dimensional Perovskite Single Crystals via Extended Cation Conjugation4Reducing the symmetry of organic cations and reconfiguring hydrogen bond networks to construct polar lead-free hybrid perovskite1Phase-Transition-Enabled Switching of Chiroptical Properties in 2D Hybrid Perovskites1Chiral Metal Halide Perovskites for Spin‐Polarized Light‐Emitting Diodes9Overcoming the chiroptical activity-photoelectricity trade-off via the construction of multilayered Cs-based chiral-polar perovskite1Mixed Coordination and Pronounced Distortion Enabling Strong Nonlinear Optics in Chiral Lead Halides0Control of Symmetry and Photophysical Properties of Hybrid Antimony Chlorides via Mixed Organic Cations0Mixing of Spacer Cations in 2D Halide Perovskites0Dual‐Color Tunable Circularly Polarized Luminescence With Anti‐Thermal‐Quenching Enabled by Asymmetric Hydrogen‐Bonding Networks in Hybrid Manganese Halides32D/3D perovskite heterostructures for highly selective room-temperature blue spin-polarized light-emitting diodes0Ultranarrow‐Spaced Polar Green Aromatic Dion–Jacobson Hybrid Perovskite Enables Highly Sensitive and Stable Self‐Powered X‐Ray Detection2Highly stable polymer-based spin light-emitting diode based on chiral perovskite enabled by annealing engineering0Chiral cations intercalation induced lead-free chiral-polar hybrid perovskites for long-term stable and high-temperature self-powered X-ray detection0Rashba-Related Spin-Selective Effect in 2D Chiral Perovskites with Achiral Organic Cation Spacers0Tailoring chiral perovskite nanocrystals for spin light-emitting diodes0Recent Advances of Quasi‐Two‐Dimensional Perovskite Solar Cells0Low-Dimensional Perovskites and Metal Halides across Structures and Functions: Connectivity, Dimensionality, and Emerging Principles1

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  46. Chiral Cation Doping for Modulating Structural Symmetry of 2D Perovskites

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  47. Spatially Correlated Chirality in Chiral Two-Dimensional Perovskites Revealed by Second-Harmonic-Generation Circular Dichroism Microscopy

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  48. Real-Time Monitoring of Progressive Crystal Phase Transformations and Associated Multi-Phase Optical Exciton Dynamics in Mixed (2D/3D) Inorganic–Organic Hybrid Semiconductors

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  49. Chiral‐Achiral Cations Intercalation Induced Lead‐Free Chiral‐Polar Hybrid Perovskites Enable Self‐Powered X‐Ray and Ultraviolet–Visible–Near‐Infrared Photo Detection

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  50. In Situ Chiral Template Approach to Synthesize Homochiral Lead Iodides for Second‐Harmonic Generation

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