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RESEARCH PAPER · Advanced Energy Materials · 2021

Cyclohexylammonium‐Based 2D/3D Perovskite Heterojunction with Funnel‐Like Energy Band Alignment for Efficient Solar Cells (23.91%)

Seonghwa Jeong, Seongrok Seo, Hyunwoo Yang, Hyoungmin Park, Sooeun Shin, Hyungju Ahn, Donghwa Lee, Jong Hyeok Park, Nam‐Gyu Park, Hyunjung Shin

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Cyclohexylammonium‐Based 2D/3D Perovskite Heterojunction with Funnel‐Like Energy Band Alignment for Efficient Solar Cells (23.91%)OriginalEfficient and stable mesoscopic perovskite solar cell in high humidity by localized Dion-Jacobson 2D‐3D heterostructures68[PbX 6 ] 4− modulation and organic spacer construction for stable perovskite solar cells66Efficient MA-free perovskite solar cells with balanced carrier transport achieved using 4-trifluorophenylammonium iodide14Hetero-perovskite engineering for stable and efficient perovskite solar cells3Inhibition of PbI 2 -induced defects by doping MABr for high-performance perovskite solar cells18Interfacial engineering from material to solvent: A mechanistic understanding on stabilizing α -formamidinium lead triiodide perovskite photovoltaics36Roles of Long‐Chain Alkylamine Ligands in Triple‐Halide Perovskites for Efficient NiOx‐Based Inverted Perovskite Solar Cells28Strategies to Enhance Light Emission from Two-Dimensional Perovskite Light-Emitting Diodes: Challenges and Future Opportunities152D/3D Heterojunction perovskite light-emitting diodes with tunable ultrapure blue emissions83Efficient and stable pure α-phase FAPbI3 perovskite solar cells with a dual engineering strategy: Additive and dimensional engineering approaches74Dual Optimization of Bulk and Surface via Guanidine Halide for Efficient and Stable 2D/3D Hybrid Perovskite Solar Cells71Light Management through Organic Bulk Heterojunction and Carrier Interfacial Engineering for Perovskite Solar Cells with 23.5% Efficiency33Heterojunction engineering for improving perovskite solar cell performance33D Meniscus‐Guided Evaporative Assembly for Rapid Template‐Free Synthesis of Highly Crystalline Perovskite Nanowire Arrays16Recent Progress on Heterojunction Engineering in Perovskite Solar Cells87Hole-Transporting Vanadium-Containing Oxide (V2O5–x) Interlayers Enhance Stability of α-FAPbI3-Based Perovskite Solar Cells (∼23%)37High‐Performance Flexible All‐Perovskite Tandem Solar Cells with Reduced VOC‐Deficit in Wide‐Bandgap Subcell72High‐Performance Inverted Perovskite Solar Cells Enhanced via Partial Replacement of Dimethyl Sulfoxide with N‐Methyl‐2‐Pyrrolidinone19Two birds with one stone: Simultaneous realization of constructed 3D/2D heterojunction and p-doping of hole transport layer for highly efficient and stable perovskite solar cells33Crystallization and defects regulation of efficient inverted perovskite solar cells via glycine ethyl ester hydrochloride6Effects of Ammonium and Alkali Metal Additives on Anisotropic Photoconductivities and Solar Cell Efficiencies of Two-Dimensional Lead Halide Perovskites4Visualizing field-effects and chemical passivation in efficient 2D/3D heterojunction perovskite solar cells and modules1Ammonium Thiocyanate-Passivated Quasi-Two-Dimensional Dion Jacobson Perovskite Solar Cells for Improved Efficiency and Stability15Conductive Passivator for Efficient Monolithic Perovskite/Silicon Tandem Solar Cell on Commercially Textured Silicon73Regulating microstructure of organic ammonium cations enables interface defect management and stability improvement in 2D/3D perovskite solar cells8Recent review of interfacial engineering for perovskite solar cells: effect of functional groups on the stability and efficiency41Roles that Organic Ammoniums Play on the Surface of the Perovskite Film: A Review18Cetrimonium bromide and potassium thiocyanate assisted post-vapor treatment approach to enhance power conversion efficiency and stability of FAPbI 3 perovskite solar cells15Green N1 Additive Modified Perovskite Precursor Enables Effective Manufacturing of Large-Area Solar Cell Modules with High Efficiency and Stability23Precise modulation strategies of 2D/3D perovskite heterojunctions in efficient and stable solar cells25Recent progress of two-dimensional Ruddlesden–Popper perovskites in solar cells19Research Progress of Cs2AgBiBr6 Perovskite Solar Cell5Simultaneously Realize Defect Passivation and Surface Pre-Sacrifice for Highly Stable 2d/3d Perovskite Solar Cells0Unraveling Its Intrinsic Role of CH3NH3Cl Doping for Efficient Enhancement of Perovskite Solar Cells from Fine Insight by Ultrafast Charge‐Transfer Dynamics18Highly efficient perovskite solar cells by building 2D/3D perovskite heterojuction in situ for interfacial passivation and energy level adjustment51Reexamining the Post‐Treatment Effects on Perovskite Solar Cells: Passivation and Chloride Redistribution24Compositional engineering and surface passivation for carbon-based perovskite solar cells with superior thermal and moisture stability19Surface Passivation of Lead Halide Perovskite Solar Cells by a Bifacial Donor−π–Donor Molecule14Mitigating lattice strain and phase segregation of mixed-halide perovskite films via dual chloride additive strategy toward highly efficient and stable perovskite solar cells17Overview on Different Types of Solar Cells: An Update752D/3D Perovskite: A Step toward Commercialization of Perovskite Solar Cells25Machine-Learning-Assisted Screening of Interface Passivation Materials for Perovskite Solar Cells107Tailoring the Interfacial Termination via Dipole Interlayer for High‐Efficiency Perovskite Solar Cells993,5-dichlorobenzylamine lead high-performance and stable 2D/3D perovskite solar cells4Effective Passivation of Perovskite Solar Cells Involving a Unique Secondary Ammonium Halide Modulator9Efficient Inorganic Vapor‐Assisted Defects Passivation for Perovskite Solar Module62Efficient and Stable Perovskite Solar Cells by Tailoring of Interfaces211Pure Chloride 2D/3D Heterostructure Passivation for Efficient and Stable Perovskite Solar Cells10Molecular Locking with All‐Organic Surface Modifiers Enables Stable and Efficient Slot‐Die‐Coated Methyl‐Ammonium‐Free Perovskite Solar Modules45Two-dimensional materials for boosting the performance of perovskite solar cells: Fundamentals, materials and devices28Kinetic‐Controlled Crystallization of α ‐FAPbI 3 Inducing Preferred Crystallographic Orientation Enhances Photovoltaic Performance49Construction of a 3D/2D heterojunction based on a fluorinated cyclohexylamine 2D Ruddlesden–Popper perovskite for highly efficient and stable perovskite solar cells6Removing residual PbI2 on the perovskite surface for efficient solar cells45Nanocrystal‐Enabled Perovskite Heterojunctions in Photovoltaic Applications and Beyond19Device Physics and Design Principles of Mixed-dimensional Perovskite Solar Cells0Photovoltaic Performance of FAPbI 3 Perovskite Is Hampered by Intrinsic Quantum Confinement30Mixed perovskites (2D/3D)-based solar cells: a review on crystallization and surface modification for enhanced efficiency and stability57Visualizing Interfacial Energy Offset and Defects in Efficient 2D/3D Heterojunction Perovskite Solar Cells and Modules83Epitaxial 2D PbS Nanosheet‐Formamidinium Lead Triiodide Heterostructure Enabling High‐Performance Perovskite Solar Cells34How to GIWAXS: Grazing Incidence Wide Angle X‐Ray Scattering Applied to Metal Halide Perovskite Thin Films230Enhancing Stability of Efficient Perovskite Solar Cells (PCE ≈ 24.5%) by Suppressing PbI2 Inclusion Formation35Probing Band-Alignment at the Interface of 3D/2D Perovskites for Solar Cell Applications8Magnetic Field‐Assisted Interface Embedding Strategy to Construct 2D/3D Composite Structure for Stable Perovskite Solar Cells with Efficiency Over 24%8Transfer-Imprinting-Assisted Growth of 2D/3D Perovskite Heterojunction for Efficient and Stable Flexible Inverted Perovskite Solar Cells37Synergy of 3D and 2D Perovskites for Durable, Efficient Solar Cells and Beyond249Tailoring passivators for highly efficient and stable perovskite solar cells386Modulation of Perovskite Surface Energetics for State‐of‐the‐Art Solar Cells4Regulating Orientational Crystallization and Buried Interface for Efficient Perovskite Solar Cells Enabled by a Multi‐Fluorine‐Containing Higher Fullerene Derivative23Hierarchical Hollow Carbon Particles with Encapsulation of Carbon Nanotubes for High Performance Supercapacitors50Bar Coating Process of Two-Dimensional Lead Iodide Perovskite Solar Cells: Effects of Vertical Orientation, Anisotropic Photoconductivity, and Conversion Time16Post‐Treatment of Metal Halide Perovskites: From Morphology Control, Defect Passivation to Band Alignment and Construction of Heterostructures64Effect of heterojunction order between CaTiO3 and Mn doped SrTiO3 on memristive performance and its mechanism analysis14The role of organic spacers in 2D/3D hybrid perovskite solar cells31Liquid Metal‐Based Perovskite Solar Cells: In Situ Formed Gallium Oxide Interlayer Improves Stability and Efficiency23Surface pre-sacrifice behavior of thiourea-based 2D perovskite s for high-performance perovskite solar cells9Spacer Engineering Enables Fine‐Tuned Thin Film Microstructure and Efficient Charge Transport for Ultrasensitive 2D Perovskite‐Based Heterojunction Phototransistors and Optoelectronic Synapses12Cyclopentylethanamine Hydroiodide for Efficient and Stable 2D/3D Hybrid Perovskite Solar Cells3A resonance spacer cation-based heterostructure enables efficient and stable perovskite solar cells3Chelating Diamine Surface Modifier Enhances Performance and Stability of Lead Halide Perovskite Solar Cells0High performance inverted planar perovskite solar cells enhanced by heteroatomic functionalized hole transport materials32Interface passivation strategies for high-performance perovskite solar cells using two-dimensional perovskites32Large-area all-perovskite-based coplanar photoelectrodes for scaled-up solar hydrogen production32Two-dimensional complex metal halides: influence of restricted dimensionality on functional properties10Device Physics and Design Principles of Mixed‐Dimensional Heterojunction Perovskite Solar Cells11Strongly stable resistive random access memory based on quasi-two-dimensional perovskites6Dimensional Regulation from 1D/3D to 2D/3D of Perovskite Interfaces for Stable Inverted Perovskite Solar Cells130Room Temperature Ionic Liquid Capping Layer for High Efficiency FAPbI3 Perovskite Solar Cells with Long‐Term Stability49Room Temperature Crystallized Phase‐Pure α‐FAPbI 3 Perovskite with In‐Situ Grain‐Boundary Passivation25Functionalized wide-bandgap photoanode via dimensional design using amine fluoride salt to maximize the performance of perovskite solar cells0Factors influencing charge transport at perovskite–charge transport layer interfaces: current strategies, challenges, and perspectives based on first-principles studies7Inhibiting Interfacial Nonradiative Recombination in Inverted Perovskite Solar Cells with a Multifunctional Molecule93Charge Transfer in 2D Halide Perovskites and 2D/3D Heterostructures46Boosted device performance of perovskite solar cells via KI processing additives2Reduction of fabrication time for organic–inorganic hybrid perovskite solar cells in lab-scale4Imidazole derivative spacers functional-group-induced regulation of interfacial recrystallization and defect passivation ability for high-performance perovskite solar cells7Efficient Deep‐Red Perovskite Light‐Emitting Diodes Based on a Vertical 3D/2D Perovskite Heterojunction21High‐throughput study of X‐ray‐induced synthesis of flower‐like CuxO5Nanoscale Graded Nitrogen‐Doping of TiO 2 via Pulsed Laser Deposition for Enhancing Charge Transfer in Perovskite Solar Cells7Co-adsorbed self-assembled monolayer enables high-performance perovskite and organic solar cells242Molecularly Engineered Alicyclic Organic Spacers for 2D/3D Hybrid Tin‐based Perovskite Solar Cells142D Phase Formation on 3D Perovskite: Insights from Molecular Stiffness25Dual‐Passivation Strategy of Bulk and Surface Enables Highly Efficient and Stable Inverted Perovskite Solar Cells4Double-side improved charge extraction via 2D perovskite for efficient inverted perovskite solar cells18Cyclohexylmethylammonium iodide-based bilateral interface engineering for efficient perovskite solar cells with improved stability and negligible hysteresis5Integrated passivation strategy using multifunctional additives for tin–lead mixed perovskite solar cells9Odd-even effects in lead-iodide-based Ruddlesden–Popper 2D perovskites15Deterministic Fabrication of 2D/3D Heterojunction for Efficient and Stable Carbon-Based Hole-Transport-Layer-Free Perovskite Solar Cells4Constructing n/n − Type Perovskite Homojunctions to Achieve High‐Efficiency and Stable Printable Mesoscopic Perovskite Solar Cells9Susceptible organic cations enable stable and efficient perovskite solar cells35Gradient layer arrangement for modulating the buried interface of inverted perovskite solar cells7Spatial Atomic Arrangement of Cyclohexyl‐Based Ligands for Enhanced Interface Passivation in 2D/3D Perovskite Solar Cells7Enhancing the efficiency and stability of carbon‐based perovskite solar cells via 5‐AVAI interface modification4Progress and Challenges of Three-Dimensional/Two-Dimensional Bilayered Perovskite Solar Cells: A Critical Review10Crystallization modulation and interfacial treatment in anti-solvent free process for formamidinium-based perovskite solar cell8Damp-Stable Perovskite/Silicon Tandem Solar Cells with Internal Encapsulating Sulfonium-Based Molecules24Band Engineering at (PEA) 2 (MA) 2 Pb 3 I 10 /CdS Quantum Dot Interfaces: Toward High‐Performance Photodetectors with Optimized Carrier Dynamics03‐(Aminomethyl)piperidinium Spacer‐Induced Dion–Jacobson 2D Perovskite Beneath CsPbI3 for Stable and Efficient Inorganic Perovskite Solar Cells3Advanced Interface Engineering for Perovskite Solar Cells: The Way to Ensure Efficiency and Stability37Mechanically Robust and yet Electrically Conductive C60-SnO2 Electron Transporting Bilayer in Stable Perovskite Solar Cells4Enhancing the Performance of a Tin Halide Perovskite Photodetector through Trifluoromethyl Cation Passivation1FAPbI 3 Powder Synthesis Routes for State‐of‐the‐Art Perovskite Solar Cells: A Review3Micelle‐Induced Nucleation and Surface Chemical Polishing Co‐Strategy for Efficient Tin‐Lead Mixed Perovskite Solar Cells11Co-crystal engineering of a two-dimensional perovskite phase for perovskite solar modules with improved efficiency and stability10Exploring performance limits toward 20.79% efficiency in 2D-layered Ruddlesden–Popper perovskite solar cells2Molecular orientation–steric hindrance tradeoff of cyclohexylammonium passivators for high-performance perovskite solar cells0Nature-Inspired Redox Shuttle with Regenerable Antioxidant for Efficient All-Perovskite Tandem Solar Cells5Dopant-Free Ultra-Thin Spiro-OMeTAD Enables Near 30%-Efficient n–i–p Perovskite/Silicon Tandem Solar Cells4Semiconductive Polarity Control in Halide Perovskites through Defect Chemistry and Interface Engineering7Anion‐Cation Synergistic Passivation for High‐Performance FA‐Cs Halide Perovskite Photodetectors0Experimental and Atomic-Scale Insights into Defects in Ferro- and Non-Ferroelectric Perovskite Solar Cells0

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  1. Efficient and stable mesoscopic perovskite solar cell in high humidity by localized Dion-Jacobson 2D‐3D heterostructures

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  2. [PbX 6 ] 4− modulation and organic spacer construction for stable perovskite solar cells

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  3. Efficient MA-free perovskite solar cells with balanced carrier transport achieved using 4-trifluorophenylammonium iodide

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  5. Inhibition of PbI 2 -induced defects by doping MABr for high-performance perovskite solar cells

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  6. Interfacial engineering from material to solvent: A mechanistic understanding on stabilizing α -formamidinium lead triiodide perovskite photovoltaics

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  7. Roles of Long‐Chain Alkylamine Ligands in Triple‐Halide Perovskites for Efficient NiOx‐Based Inverted Perovskite Solar Cells

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  8. Strategies to Enhance Light Emission from Two-Dimensional Perovskite Light-Emitting Diodes: Challenges and Future Opportunities

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  9. 2D/3D Heterojunction perovskite light-emitting diodes with tunable ultrapure blue emissions

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  10. Efficient and stable pure α-phase FAPbI3 perovskite solar cells with a dual engineering strategy: Additive and dimensional engineering approaches

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  14. 3D Meniscus‐Guided Evaporative Assembly for Rapid Template‐Free Synthesis of Highly Crystalline Perovskite Nanowire Arrays

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  16. Hole-Transporting Vanadium-Containing Oxide (V2O5–x) Interlayers Enhance Stability of α-FAPbI3-Based Perovskite Solar Cells (∼23%)

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  17. High‐Performance Flexible All‐Perovskite Tandem Solar Cells with Reduced VOC‐Deficit in Wide‐Bandgap Subcell

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  18. High‐Performance Inverted Perovskite Solar Cells Enhanced via Partial Replacement of Dimethyl Sulfoxide with N‐Methyl‐2‐Pyrrolidinone

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  19. Two birds with one stone: Simultaneous realization of constructed 3D/2D heterojunction and p-doping of hole transport layer for highly efficient and stable perovskite solar cells

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  20. Crystallization and defects regulation of efficient inverted perovskite solar cells via glycine ethyl ester hydrochloride

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  28. Cetrimonium bromide and potassium thiocyanate assisted post-vapor treatment approach to enhance power conversion efficiency and stability of FAPbI 3 perovskite solar cells

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  30. Precise modulation strategies of 2D/3D perovskite heterojunctions in efficient and stable solar cells

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  31. Recent progress of two-dimensional Ruddlesden–Popper perovskites in solar cells

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  32. Research Progress of Cs2AgBiBr6 Perovskite Solar Cell

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  33. Simultaneously Realize Defect Passivation and Surface Pre-Sacrifice for Highly Stable 2d/3d Perovskite Solar Cells

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  34. Unraveling Its Intrinsic Role of CH3NH3Cl Doping for Efficient Enhancement of Perovskite Solar Cells from Fine Insight by Ultrafast Charge‐Transfer Dynamics

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  36. Reexamining the Post‐Treatment Effects on Perovskite Solar Cells: Passivation and Chloride Redistribution

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  37. Compositional engineering and surface passivation for carbon-based perovskite solar cells with superior thermal and moisture stability

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  39. Mitigating lattice strain and phase segregation of mixed-halide perovskite films via dual chloride additive strategy toward highly efficient and stable perovskite solar cells

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  40. Overview on Different Types of Solar Cells: An Update

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  41. 2D/3D Perovskite: A Step toward Commercialization of Perovskite Solar Cells

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  42. Machine-Learning-Assisted Screening of Interface Passivation Materials for Perovskite Solar Cells

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  43. Tailoring the Interfacial Termination via Dipole Interlayer for High‐Efficiency Perovskite Solar Cells

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