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RESEARCH ARTICLE · Science · 2021

Semiconductor quantum dots: Technological progress and future challenges

Francisco Pelayo García de Arquer, Dmitri V. Talapin, Victor I. Klimov, Yasuhiko Arakawa, M. Bayer, Edward Hartley Sargent

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Semiconductor quantum dots: Technological progress and future challengesOriginalSurface Chemistry Engineering of Perovskite Quantum Dots: Strategies, Applications, and Perspectives394How Exciton–Phonon Coupling Impacts Photoluminescence in Halide Perovskite Nanoplatelets59Advances and Challenges of Fluorescent Nanomaterials for Synthesis and Biomedical Applications113Luminescence Enhancement, Encapsulation, and Patterning of Quantum Dots Toward Display Applications74Colloidal Inorganic Ligand-Capped Nanocrystals: Fundamentals, Status, and Insights into Advanced Functional Nanodevices137AgBiS 2 as a photoabsorber for eco-friendly solar cells: a review71Narrow‐bandwidth emissive carbon dots: A rising star in the fluorescent material family126All-solid-state SARS-CoV-2 protein biosensor employing colloidal quantum dots-modified electrode68Preparation of flower-like Co3O4 QDs/Bi2WO6 p-n heterojunction photocatalyst and its degradation mechanism of efficient visible-light-driven photocatalytic tetracycline antibiotics91Modulation of BiOBr-based photocatalysts for energy and environmental application: A critical review57Beyond a Linker: The Role of Photochemistry of Crosslinkers in the Direct Optical Patterning of Colloidal Nanocrystals101Nanomaterials‐assisted metabolic analysis toward in vitro diagnostics66Colloidal Quantum Dot Light Emitting Diodes at Telecom Wavelength with 18% Quantum Efficiency and Over 1 MHz Bandwidth57Solution-processed green and blue quantum-dot light-emitting diodes with eliminated charge leakage536Recent Progress in the Development of MOF-Based Photocatalysts for the Photoreduction of Cr(VI)122Blue LED‐Pumped Broadband Short‐Wave Infrared Emitter Based on LiMgPO4:Cr3+,Ni2+ Phosphor97Elucidating the Role of Antisolvents on the Surface Chemistry and Optoelectronic Properties of CsPbBrxI3-x Perovskite Nanocrystals111Mid-Infrared Intraband Photodetector via High Carrier Mobility HgSe Colloidal Quantum Dots61The Rise of Colloidal Lead Halide Perovskite Quantum Dot Solar Cells56Aminophosphate precursors for the synthesis of near‐unity emitting InP quantum dots and their application in liver cancer diagnosis55Cadmium Chalcogenide (CdS, CdSe, CdTe) Quantum Dots for Solar‐to‐Fuel Conversion79Hue Recognition Competitive Fluorescent Lateral Flow Immunoassay for Aflatoxin M 1 Detection with Improved Visual and Quantitative Performance62Industry outlook of perovskite quantum dots for display applications203Structure of a subnanometer-sized semiconductor Cd14Se13 cluster69Inkjet-printed blue InP/ZnS/ZnS quantum dot light-emitting diodes75Quantum Dots Compete at the Acme of MXene Family for the Optimal Catalysis89Finite confinement potentials, core and shell size effects on excitonic and electron-atom properties in cylindrical core/shell/shell quantum dots57Lattice distortion inducing exciton splitting and coherent quantum beating in CsPbI3 perovskite quantum dots108Encapsulation of Dual‐Passivated Perovskite Quantum Dots for Bio‐Imaging59Information‐Storage Expansion Enabled by a Resilient Aggregation‐Induced‐Emission‐Active Nanocomposite Hydrogel71Electrochemiluminescence biosensing and bioimaging with nanomaterials as emitters82Photocatalytic hydrogen peroxide evolution: What is the most effective strategy?315Negative Photoconductivity: Bizarre Physics in Semiconductors111Post-2000 nonlinear optical materials and measurements: data tables and best practices76Recent Progress of Bismuth Effect on All‐Inorganic Lead‐Free Metal Halide Derivatives: Crystals Structure, Luminescence Properties, and Applications70Room-Temperature Semiconductor Gas Sensors: Challenges and Opportunities258Zn‐Doped P‐Type InAs Nanocrystal Quantum Dots54Wide Band Gap Devices and Their Application in Power Electronics136Perovskite quantum dots: Synthesis, applications, prospects, and challenges54Development of Group III–V Colloidal Quantum Dots for Optoelectronic Applications69Recent Advances in Synthesis and Application of Metal Oxide Nanostructures in Chemical Sensors and Biosensors55Room-temperature coherent optical manipulation of hole spins in solution-grown perovskite quantum dots75Colloidal Quantum Dots: Synthesis, Composition, Structure, and Emerging Optoelectronic Applications118High-operating-temperature mid-infrared photodetectors via quantum dot gradient homojunction130Microreactor-based micro/nanomaterials: fabrication, advances, and outlook62Synthesis and hybridization of CuInS 2 nanocrystals for emerging applications81A reactivity-controlled epitaxial growth strategy for synthesizing large nanocrystals92High‐Efficiency Perovskite Quantum Dot Photovoltaic with Homogeneous Structure and Energy Landscape61Synthesis, Surface Chemistry, and Fluorescent Properties of InP Quantum Dots101Aggregation-Induced Emission-Active Nanostructures: Beyond Biomedical Applications111Emerging Trends of Carbon‐Based Quantum Dots: Nanoarchitectonics and Applications305Copper indium sulfide quantum dots in photocatalysis1333D Laser Nanoprinting of Functional Materials64Semiconducting Quantum Dots for Energy Conversion and Storage134Carbon Dots Based Photoinduced Reactions: Advances and Perspective184Quantitative Determination of Charge Accumulation and Recombination in Operational Quantum Dots Light Emitting Diodes via Time-Resolved Electroluminescence Spectroscopy61Closed-loop optimization of nanoparticle synthesis enabled by robotics and machine learning72Direct Photo-Patterning of Efficient and Stable Quantum Dot Light-Emitting Diodes via Light-Triggered, Carbocation-Enabled Ligand Stripping72Epitaxial CsPbBr3/CdS Janus Nanocrystal Heterostructures for Efficient Charge Separation57Breaking the Size Limitation of Directly‐Synthesized PbS Quantum Dot Inks Toward Efficient Short‐wavelength Infrared Optoelectronic Applications79Robust integration of polymerizable perovskite quantum dots with responsive polymers enables 4D-printed self-deployable information display126Flexible Quantum Dot Light‐Emitting Device for Emerging Multifunctional and Smart Applications125Tunable Efficient White Emission in Holmium Doped Double Perovskites Cs 2 KInCl 6 via Antimony Sensitization73Graphene-Related Nanomaterials for Biomedical Applications52Anisotropic Heavy-Metal-Free Semiconductor Nanocrystals: Synthesis, Properties, and Applications78Carbon Dots for Electroluminescent Light‐Emitting Diodes: Recent Progress and Future Prospects121Biomass-based carbon quantum dots for polycrystalline silicon solar cells with enhanced photovoltaic performance52Intense Circularly Polarized Fluorescence and Room-Temperature Phosphorescence in Carbon Dots/Chiral Helical Polymer Composite Films119Thermal tolerance of perovskite quantum dots dependent on A-site cation and surface ligand96Luminescent quantum dots: Synthesis, optical properties, bioimaging and toxicity230Development and challenges of indium phosphide-based quantum-dot light-emitting diodes58Dual-mode biosensor platform based on synergistic effects of dual-functional hybrid nanomaterials64Atomic and Electronic Reconstruction in Defective 0D Molybdenum Carbide Heterostructure for Regulating Lower‐Frequency Microwaves90Nonlocal interaction enhanced biexciton emission in large CsPbBr3 nanocrystals55Enabling metallic behaviour in two-dimensional superlattice of semiconductor colloidal quantum dots56Quantum dots: an overview of synthesis, properties, and applications246Perovskite Scintillators for Improved X‐ray Detection and Imaging188Exploring the multifunctional roles of quantum dots for unlocking the future of biology and medicine64Design Rules for Obtaining Narrow Luminescence from Semiconductors Made in Solution87Progress in Bioinspired Photodetectors Design for Visual Information Processing54Toxicity Mechanisms of Copper Nanoparticles and Copper Surfaces on Bacterial Cells and Viruses186Color Revolution: Prospects and Challenges of Quantum‐Dot Light‐Emitting Diode Display Technologies108Quantum Junction Solar Cells: Development and Prospects56Molecular‐Additive‐Assisted Tellurium Homogenization in ZnSeTe Quantum Dots67Carbon Dot Based Multicolor Electroluminescent LEDs with Nearly 100% Exciton Utilization Efficiency74Recent advances in surface regulation and engineering strategies of photoelectrodes toward enhanced photoelectrochemical water splitting86A Review on Quantum Dot‐Based Color Conversion Layers for Mini/Micro‐LED Displays: Packaging, Light Management, and Pixelation104Advances and significances of nanoparticles in semiconductor applications – A review260Flexible and broadband colloidal quantum dots photodiode array for pixel-level X-ray to near-infrared image fusion102Low‐Dimensional‐Materials‐Based Photodetectors for Next‐Generation Polarized Detection and Imaging155Toward the Controlled Synthesis of Lead Halide Perovskite Nanocrystals68Halide‐Driven Synthetic Control of InSb Colloidal Quantum Dots Enables Short‐Wave Infrared Photodetectors59Progress on quantum dot photocatalysts for biomass valorization73Multivariate chemical analysis: From sensors to sensor arrays56A Comprehensive Review and Analysis of Nanosensors for Structural Health Monitoring in Bridge Maintenance: Innovations, Challenges, and Future Perspectives66InP colloidal quantum dots for visible and near-infrared photonics164Artificial photosynthetic cells with biotic–abiotic hybrid energy modules for customized CO2 conversion66A High-Nuclearity Copper Sulfide Nanocluster [S-Cu 50 ] Featuring a Double-Shell Structure Configuration with Cu(II)/Cu(I) Valences68A Review of Top‐Down Strategies for the Production of Quantum‐Sized Materials60Electron‐Induced Degradation in Blue Quantum‐Dot Light‐Emitting Diodes77Colloidal PbS Quantum Dot Photodiode Imager with Suppressed Dark Current52Highly ordered inkjet-printed quantum-dot thin films enable efficient and stable QLEDs with EQE exceeding 23%67Advancements in semiconductor quantum dots: expanding frontiers in optoelectronics, analytical sensing, biomedicine, and catalysis138Atomic surface achieved through a novel cross-scale model from macroscale to nanoscale77Engineering functionalization and properties of graphene quantum dots (GQDs) with controllable synthesis for energy and display applications82Fluorescent chemosensors facilitate the visualization of plant health and their living environment in sustainable agriculture93Photophysics of fluorescent nanoparticles based on organic dyes – challenges and design principles56Carbon quantum dots in bioimaging and biomedicines210Ratiometric fluorescence sensing NADH using AIE-dots transducers at the point of care77Single-photon superradiance in individual caesium lead halide quantum dots139Microencapsulation for Pharmaceutical Applications: A Review84Tempospatially Confined Catalytic Membranes for Advanced Water Remediation91Size-dependent lanthanide energy transfer amplifies upconversion luminescence quantum yields176Narrow‐Band Green‐Emitting Hybrid Organic–Inorganic Eu (II)‐Iodides for Next‐Generation Micro‐LED Displays84Perovskite Quantum Dots for the Next‐Generation Displays: Progress and Prospect169Photophysical properties of materials for high-speed photodetection119Probing charge transfer of NiCo2O4/g-C3N4 photocatalyst for hydrogen production59Short‐Wave Infrared Colloidal QD Photodetector with Nanosecond Response Times Enabled by Ultrathin Absorber Layers75Narrowband room temperature phosphorescence of closed-loop molecules through the multiple resonance effect56Nanocrystal Assemblies: Current Advances and Open Problems124Recent Progress of Quantum Dots Light‐Emitting Diodes: Materials, Device Structures, and Display Applications160Novel full-scale model verified by atomic surface and developed composite microfiber and slurry polishing system67Plasmonic Near‐Infrared‐Response S‐Scheme ZnO/CuInS2 Photocatalyst for H2O2 Production Coupled with Glycerin Oxidation232Heavy‐Metal‐Free Colloidal Quantum Dots: Progress and Opportunities in Solar Technologies63Coherent phenomena and dynamics of lead halide perovskite nanocrystals for quantum information technologies72Carbon Dots: A Review with Focus on Sustainability118Two‐Photon Mediated Cancer Therapy: A Comprehensive Review on Two‐Photon Photodynamic Therapy and Two‐Photon‐Activated Therapeutic Delivery Systems55Ions‐induced Assembly of Perovskite Nanocomposites for Highly Efficient Light‐Emitting Diodes with EQE Exceeding 30%91Direct Photopatterning of Colloidal Quantum Dots with Electronically Optimized Diazirine Cross-Linkers64Reductive pathways in molten inorganic salts enable colloidal synthesis of III-V semiconductor nanocrystals52Emerging 2D MXene quantum dots for catalytic conversion of CO252In Situ Fabricated Perovskite Quantum Dots: From Materials to Applications69Efficient green InP-based QD-LED by controlling electron injection and leakage182Surface chemistry-engineered perovskite quantum dot photovoltaics97Quantum dot nanomaterials: Empowering advances in optoelectronic devices87Remote epitaxial crystalline perovskites for ultrahigh-resolution micro-LED displays53Carbon quantum dots: Classification-structure-property-application relationship for biomedical and environment remediation69Ultrathin Ti-Deficient TiO 2 Nanosheets with Pt Single Atoms Enable Efficient Photocatalytic Nitrate Reduction to Ammonia66Efficient and stable near-infrared InAs quantum dot light-emitting diodes53Advancing Ecofriendly Indium Phosphide Quantum Dots: Comprehensive Strategies toward Color-Pure Luminescence for Wide Color Gamut Displays52Overcoming efficiency and cost barriers for large-area quantum dot photovoltaics through stable ink engineering56Perovskite Solar Cells and Light Emitting Diodes: Materials Chemistry, Device Physics and Relationship72Designing Physical Unclonable Functions From Optically Active Materials58Colloidal quantum dots for optoelectronics69Materials Engineering for Light‐Activated Gas Sensors: Insights, Advances, and Future Perspectives56Prospects of Nanoscience with Nanocrystals: 2025 Edition59Future trends of display technology: micro-LEDs toward transparent, free-form, and near-eye displays63Triple-color emission ratiometric fluorescence in biochemical sensing analysis; principles, probe fabrication and applications62Toward Next-Generation Semiartificial Photosynthesis: Multidisciplinary Engineering of Biohybrid Systems60S-Scheme Shapes Heterojunction Photocatalysis131

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