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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2022

High Entropy Oxide Relaxor Ferroelectrics

Yogesh Sharma, Min‐Cheol Lee, Krishna Chaitanya Pitike, K. K. Mishra, Qiang Zheng, Xiang Gao, Brianna L. Musicó, Alessandro R. Mazza, Ram S. Katiyar, V. Keppens, Matthew Brahlek, Dmitry Yarotski, Rohit P. Prasankumar, Aiping Chen, Valentino R. Cooper, Thomas Zac Ward

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High Entropy Oxide Relaxor FerroelectricsOriginalStructural and Optical Properties of High Entropy (La,Lu,Y,Gd,Ce)AlO3 Perovskite Thin Films47Relaxor ferroelectric behaviour observed in (Ca0.5Sr0.5Ba0.5Pb0.5)Nb2O7 perovskite layered structure ceramics13Design and preparation of lead-free (Bi0.4Na0.2K0.2Ba0.2)TiO3-Sr(Mg1/3Nb2/3)O3 high-entropy relaxor ceramics for dielectric energy storage131What is in a name: Defining “high entropy” oxides170Sub-Ångstrom-scale structural variations in high-entropy oxides10Water uptake and energetics of the formation of barium zirconate based multicomponent oxides8Variance induced decoupling of spin, lattice, and charge ordering in perovskite nickelates21Hole doping in compositionally complex correlated oxide enables tunable exchange biasing12Understanding the Role of Entropy in High Entropy Oxides574High-entropy design for dielectric materials: Status, challenges, and beyond60Improved dielectric, ferroelectric and energy storage properties of (Sr0.55Bi0.3)(Ni1/3Nb2/3)O3 modified NaNbO3 ceramics via phase modulation and relaxation enhancement6Novel high-entropy oxides for energy storage and conversion: From fundamentals to practical applications144High‐entropy oxides: Harnessing crystalline disorder for emergent functionality125Enhanced energy‐storage properties in Zr 4+ ‐modified (Bi 0.4 Ba 0.2 K 0.2 Na 0.2 )TiO 3 high‐entropy ceramics39A review on structure–property relationships in dielectric ceramics using high‐entropy compositional strategies73A reflection on recent efforts in optimization of cooling capacity of electrocaloric thin films15Synthesis of (Bi0.2Ln0.2Sr0.2K0.2Na0.2)TiO3 high-entropy perovskite oxides containing Ln element13High-entropic relaxor ferroelectric perovskites ceramics with A-site modification for energy storage applications29Anisotropic Properties of Epitaxial Ferroelectric Lead-Free 0.5[Ba(Ti0.8Zr0.2)O3]-0.5(Ba0.7Ca0.3)TiO3 Films5High‐performance ferroelectric based materials via high‐entropy strategy: Design, properties, and mechanism96High-Entropy Lead-Free Perovskite Bi0.2K0.2Ba0.2Sr0.2Ca0.2TiO3 Powders and Related Ceramics: Synthesis, Processing, and Electrical Properties13A remarkable high entropy effect on the magnetic behaviour of quadruple perovskites8Enhancement of piezo–photocatalytic activity in perovskite (Bi0·2Na0·2Ba0·2K0·2La0.2)TiO3 oxides via high entropy induced lattice distortion and energy band reconfiguration53Influence of Atmosphere on the Formation of High-Entropy Oxides of the Co-Cu-Fe-Mg-Mn-Ni-O System by Reactive Flash Sintering0Apparent ferrimagnetism in Sr(Fe0.2Mn0.2Co0.2Ti0.2V0.2)O3 high-entropy oxide perovskite thin films9High‐Entropy Perovskite Oxide Photonic Synapses10High entropy ceramics for applications in extreme environments43High-entropy materials for energy and electronic applications448Spin reorientation in Dy-based high-entropy oxide perovskite thin films11High-entropy perovskite oxides for energy materials: A review85Embracing disorder in quantum materials design17Influence of the atmosphere on the formation of high-entropy oxides within the Co–Cu–Fe–Mg–Mn–Ni–O system via reactive flash sintering9The Challenges of Piezoelectric Actuators and Motors Application in a Space Environment18Production of high entropy (FeNiMnCrV)3O4 oxide by mechanical alloying process and electrochemical performance analysis for Li-ion cells3Local structure maturation in high entropy oxide (Mg,Co,Ni,Cu,Zn) 1‐ x (Cr,Mn) x O thin films19Advances in high entropy oxides: synthesis, structure, properties and beyond144Synthesis, characterization, and electrical properties of Nd 3+ ‐doped (Bi 0.4 Na 0.2 K 0.2 Ba 0.2 )TiO 3 high‐entropy ceramics2Preparation and Characterization of a High-Entropy Magnet, (Mg, Mn, Co, Ni, Cu)3TeO64High-Entropy Oxides: Pioneering the Future of Multifunctional Materials112Colossal dielectric constant with high capacitance induced by high entropy in layered bismuth oxychloride containing triple fluorite blocks3Achieving ultra-high energy storage performance in (Bi 0.5 Na 0.5 ) 0.7 Sr 0.3 TiO 3 -based relaxor ferroelectrics15Disorder by design: unveiling local structure and functional insights in high entropy oxides49Exploring the low-temperature electric polarization behavior of spinel CoMn2O43Investigation of the design and performance regulation of (1 − x )Bi 0.5 Na 0.5 TiO 3 – x Bi 0.2 Na 0.2 Ba 0.2 Sr 0.2 Ca 0.2 TiO 3 piezoelectric systems via a high-entropy strategy4Strategic optimization of electrocaloric cooling: from material design to device innovation12High-entropy oxides: Emergent materials for electrochemical energy storage and conversion50Dielectric and electrical energy storage properties of a series of high-entropy tetragonal tungsten bronze ceramics5Piezoelectricity in half-Heusler narrow-bandgap semiconductors32A Multifunctional High‐Entropy Perovskite Ceramics with Enhanced Energy Storage and Photoluminescence Properties2Compositionally Complex Oxide Dielectrics for Microwave Applications: Current Status and Future Trends: A Review0Evidenced piezoelectricity in pulsed laser deposited perovskite tin titanate on silicon substrate1Entropy-driven electromagnetic interference Shielding: Unravelling the mechanism, potential and futuristic prospects of high-entropy materials8High-Entropy Materials: A New Paradigm in the Design of Advanced Batteries66Using high-throughput processing and characterization methods to investigate the role of synthesis conditions on the energy storage properties of a high entropy oxide0Synthesis‐Driven Functionality in High‐Entropy Materials34A-site rare-earth medium-entropy engineering in BaTiO3 ceramics enables local lattice disorder and relaxor-like energy storage0Analytical and Phase-Field Study of Anomalous Electromechanical Behaviors in Na0.5Bi0.5TiO3–xSrTiO30Coexistence of relaxor ferroelectricity and magnetism in hexagonal high-entropy manganite thin films0Ferroelectric high entropy oxides0Introduction to Novel High-Entropy Oxides0Role of liquid water distribution in MgO hydroxylation0Pathways to obtain high-entropy BiFeO3-based thin films modified by rare earth cations2Synthesis and Characteristics of the Microstructure of (6A)TiO3 High-Entropy Titanate Ceramics with a Cubic Perovskite Structure0Analytical and phase-field study of anomalous electromechanical behaviors in Na0.5Bi0.5TiO 3 – x SrTiO 32Versatile Magneto‐Dielectric Response of Epitaxial Thin Films of the High Entropy Oxide Perovskite Nd(Cr 0.2 Mn 0.2 Fe 0.2 Co 0.2 Ni 0.2 )O 30High Entropy–Driven Performance Enhancement in Perovskite Oxides for Energy Conversion and Storage Systems2Beyond Single‐Active Sites: The Emergence of High‐Entropy Perovskites in Energy and Environment Catalysis1Enhanced Energy-Storage Performance of High-Entropy (1 − x )(NaBiBa)0.205(SrCa)0.1925TiO3- x Bi(Zn2/3Ta1/3)O3 Ceramic under Moderate Electric Field0Anomalous Crystallinity and Magnetism in Chemically Disordered Coherent Heterostructures0Engineering relaxor-antiferroelectric crossovers in NaNbO3 via A/B-site doping: Modulating field-induced phase transitions for ultrahigh energy storage performance0Oxygen-Mediated Electronic Reconstruction and Element-Selective Magnetism in Sr-Based High-Entropy Perovskite Oxide Thin Films0Local Atom Clusters Drive Supercritical Relaxor State in Lead‐Free Dielectrics for Giant Energy Storage1Long-range magnetic order and relaxor ferroelectricity in a hexagonal high-entropy ferrite1Defects in medium-and high-entropy materials: a review0

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  1. Structural and Optical Properties of High Entropy (La,Lu,Y,Gd,Ce)AlO3 Perovskite Thin Films

    Advanced Science · 2022-08-26

    Zachary Corey, Ping Lu, Guangran Zhang, Yogesh Sharma, Bethany X. Rutherford, Samyak Dhole, Pinku Roy, ‪Zhehui Wang, Yiquan Wu, Haiyan Wang, Aiping Chen, Quanxi X. Jia

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  2. Relaxor ferroelectric behaviour observed in (Ca0.5Sr0.5Ba0.5Pb0.5)Nb2O7 perovskite layered structure ceramics

    Journal of the European Ceramic Society · 2022-09-26

    Zimeng Hu, Hangfeng Zhang, Michael John Reece, Giuseppe Viola, Haixue Yan

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  3. Design and preparation of lead-free (Bi0.4Na0.2K0.2Ba0.2)TiO3-Sr(Mg1/3Nb2/3)O3 high-entropy relaxor ceramics for dielectric energy storage

    Chemical Engineering Journal · 2022-10-21

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  4. What is in a name: Defining “high entropy” oxides

    APL Materials · 2022-11-01

    Matthew Brahlek, Maria Gazda, Veerle Keppens, Alessandro R. Mazza, Scott J. McCormack, Aleksandra Dorota Mielewczyk-Gryń, Brianna L. Musicó, Katharine Lynn Page, Christina M. Rost, Susan B. Sinnott, Cormac Toher, Thomas Zac Ward, A. Yamamoto

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  5. Sub-Ångstrom-scale structural variations in high-entropy oxides

    Nanoscale · 2023-01-01

    Hanbin Gao, Ning Guo, Yue Gong, Lu Bai, Dongwei Wang, Qiang Zheng

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  6. Water uptake and energetics of the formation of barium zirconate based multicomponent oxides

    Physical Chemistry Chemical Physics · 2023-01-01

    Aleksandra Dorota Mielewczyk-Gryń, Tamilarasan Subramani, Daniel Jaworski, Kristina I. Lilova, Wojciech Skubida, Alexandra Navrotsky, Maria Gazda

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  7. Variance induced decoupling of spin, lattice, and charge ordering in perovskite nickelates

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  8. Hole doping in compositionally complex correlated oxide enables tunable exchange biasing

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  9. Understanding the Role of Entropy in High Entropy Oxides

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  10. High-entropy design for dielectric materials: Status, challenges, and beyond

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    Bingbing Yang, Yiqian Liu, Shun Lan, Lvye Dou, Ce‐Wen Nan, Yuanhua Lin

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  11. Improved dielectric, ferroelectric and energy storage properties of (Sr0.55Bi0.3)(Ni1/3Nb2/3)O3 modified NaNbO3 ceramics via phase modulation and relaxation enhancement

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    Xinrong Zhong, Yuqing Chen, Anze Shui, Chao He

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  12. Novel high-entropy oxides for energy storage and conversion: From fundamentals to practical applications

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  13. High‐entropy oxides: Harnessing crystalline disorder for emergent functionality

    Journal of the American Ceramic Society · 2023-06-09

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  14. Enhanced energy‐storage properties in Zr 4+ ‐modified (Bi 0.4 Ba 0.2 K 0.2 Na 0.2 )TiO 3 high‐entropy ceramics

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    Wenhui Ye, Bo Yan, Jinxu Ma, Qiang He, Linan An, Kepi Chen

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  15. A review on structure–property relationships in dielectric ceramics using high‐entropy compositional strategies

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  16. A reflection on recent efforts in optimization of cooling capacity of electrocaloric thin films

    APL Materials · 2023-09-01

    Yunlong Sun, Sagar E. Shirsath, Siyuan Zhang, Danyang Wang

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  17. Synthesis of (Bi0.2Ln0.2Sr0.2K0.2Na0.2)TiO3 high-entropy perovskite oxides containing Ln element

    Journal of the European Ceramic Society · 2023-09-22

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  18. High-entropic relaxor ferroelectric perovskites ceramics with A-site modification for energy storage applications

    Ceramics International · 2023-09-25

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  19. Anisotropic Properties of Epitaxial Ferroelectric Lead-Free 0.5[Ba(Ti0.8Zr0.2)O3]-0.5(Ba0.7Ca0.3)TiO3 Films

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  20. High‐performance ferroelectric based materials via high‐entropy strategy: Design, properties, and mechanism

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  21. High-Entropy Lead-Free Perovskite Bi0.2K0.2Ba0.2Sr0.2Ca0.2TiO3 Powders and Related Ceramics: Synthesis, Processing, and Electrical Properties

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  22. A remarkable high entropy effect on the magnetic behaviour of quadruple perovskites

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  23. Enhancement of piezo–photocatalytic activity in perovskite (Bi0·2Na0·2Ba0·2K0·2La0.2)TiO3 oxides via high entropy induced lattice distortion and energy band reconfiguration

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  24. Influence of Atmosphere on the Formation of High-Entropy Oxides of the Co-Cu-Fe-Mg-Mn-Ni-O System by Reactive Flash Sintering

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  25. Apparent ferrimagnetism in Sr(Fe0.2Mn0.2Co0.2Ti0.2V0.2)O3 high-entropy oxide perovskite thin films

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  26. High‐Entropy Perovskite Oxide Photonic Synapses

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  27. High entropy ceramics for applications in extreme environments

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  28. High-entropy materials for energy and electronic applications

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  29. Spin reorientation in Dy-based high-entropy oxide perovskite thin films

    Physical review. B./Physical review. B · 2024-04-15

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  30. High-entropy perovskite oxides for energy materials: A review

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  31. Embracing disorder in quantum materials design

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  32. Influence of the atmosphere on the formation of high-entropy oxides within the Co–Cu–Fe–Mg–Mn–Ni–O system via reactive flash sintering

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  33. The Challenges of Piezoelectric Actuators and Motors Application in a Space Environment

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  34. Production of high entropy (FeNiMnCrV)3O4 oxide by mechanical alloying process and electrochemical performance analysis for Li-ion cells

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  35. Local structure maturation in high entropy oxide (Mg,Co,Ni,Cu,Zn) 1‐ x (Cr,Mn) x O thin films

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  36. Advances in high entropy oxides: synthesis, structure, properties and beyond

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  37. Synthesis, characterization, and electrical properties of Nd 3+ ‐doped (Bi 0.4 Na 0.2 K 0.2 Ba 0.2 )TiO 3 high‐entropy ceramics

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  38. Preparation and Characterization of a High-Entropy Magnet, (Mg, Mn, Co, Ni, Cu)3TeO6

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  39. High-Entropy Oxides: Pioneering the Future of Multifunctional Materials

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  40. Colossal dielectric constant with high capacitance induced by high entropy in layered bismuth oxychloride containing triple fluorite blocks

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  41. Achieving ultra-high energy storage performance in (Bi 0.5 Na 0.5 ) 0.7 Sr 0.3 TiO 3 -based relaxor ferroelectrics

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  42. Disorder by design: unveiling local structure and functional insights in high entropy oxides

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  43. Exploring the low-temperature electric polarization behavior of spinel CoMn2O4

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  44. Investigation of the design and performance regulation of (1 − x )Bi 0.5 Na 0.5 TiO 3 – x Bi 0.2 Na 0.2 Ba 0.2 Sr 0.2 Ca 0.2 TiO 3 piezoelectric systems via a high-entropy strategy

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  45. Strategic optimization of electrocaloric cooling: from material design to device innovation

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  46. High-entropy oxides: Emergent materials for electrochemical energy storage and conversion

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  47. Dielectric and electrical energy storage properties of a series of high-entropy tetragonal tungsten bronze ceramics

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  48. Piezoelectricity in half-Heusler narrow-bandgap semiconductors

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  49. A Multifunctional High‐Entropy Perovskite Ceramics with Enhanced Energy Storage and Photoluminescence Properties

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  50. Compositionally Complex Oxide Dielectrics for Microwave Applications: Current Status and Future Trends: A Review

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