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RESEARCH PAPER · Journal of Materials Chemistry A · 2021

Impact of Mg and Ti doping in O3 type NaNi 1/2 Mn 1/2 O 2 on reversibility and phase transition during electrochemical Na intercalation

Kei Kubota, Naoya Fujitani, Yusuke Yoda, Kazutoshi Kuroki, Yusuke Tokita, Shinichi Komaba

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Impact of Mg and Ti doping in O3 type NaNi 1/2 Mn 1/2 O 2 on reversibility and phase transition during electrochemical Na intercalationOriginalStructural change induced by electrochemical sodium extraction from layered O′3-NaMnO 235Rational design of Co-free layered cathode material for sodium-ion batteries56A fluorinated O3-type layered cathode for long-life sodium-ion batteries51Phase transitions of Na-ion layered oxide materials and their influence on properties31Transition metal oxides as a cathode for indispensable Na-ion batteries87Mg-doped layered oxide cathode for Na-ion batteries17Multiphase layered transition metal oxide positive electrodes for sodium ion batteries61Boosting the ionic transport and structural stability of Zn-doped O3-type NaNi1/3Mn1/3Fe1/3O2 cathode material for half/full sodium-ion batteries116Using High-Entropy Configuration Strategy to Design Na-Ion Layered Oxide Cathodes with Superior Electrochemical Performance and Thermal Stability492Sodium Layered Oxide Cathode Materials2Review on Cathode Materials for Sodium‐ and Potassium‐Ion Batteries: Structural Design with Electrochemical Properties25Magnesium doping improved characteristics of high voltage cycle of layered cathode of sodium ion battery1Properties of the “Z”‐Phase in Mn‐Rich P2‐Na0.67Ni0.1Mn0.8Fe0.1O2 as Sodium‐Ion‐Battery Cathodes69Solid‐State Synthesis and Characterization of Mg‐Substituted P2‐Na0.70Ni0.45Mn0.55O2 Cathode Materials for Practical Sodium‐Ion Batteries5Heterostructure engineering in electrode materials for sodium-ion batteries: Recent progress and perspectives383Unlocking high-rate O3 layered oxide cathode for Na-ion batteries via ion migration path modulation147O3-Type Na0.95Ni0.40Fe0.15Mn0.3Ti0.15O2 Cathode Materials with Enhanced Storage Stability for High-Energy Na-Ion Batteries114Four‐In‐One Strategy to Boost the Performance of Nax[Ni,Mn]O241Tailoring Electronic Structure to Achieve Maximum Utilization of Transition Metal Redox for High-Entropy Na Layered Oxide Cathodes204Research progresses in O3-type Ni/Fe/Mn based layered cathode materials for sodium ion batteries63Slight Multielement Doping-Induced Structural Order–Disorder Transition for High-Performance Layered Na-Ion Oxide Cathodes19High-voltage stability of O3-type sodium layered cathode enabled by preferred occupation of Na in the OP2 phase78Practical Cathodes for Sodium‐Ion Batteries: Who Will Take The Crown?342Magnesium ion-doped layered oxide cathodes for alkali-metal ion batteries: Recent research progress and outlook64Stabilized O3‐Type Layered Sodium Oxides with Enhanced Rate Performance and Cycling Stability by Dual‐Site Ti4+/K+ Substitution118Effects of elemental doping on phase transitions of manganese-based layered oxides for sodium-ion batteries58Ti/Co co-doped O3-Na(Ni0.3Fe0.2Mn0.5)0.85Ti0.1Co0.05O2 with high rate and durable cathode material for sodium-ion batteries7A highly stable high-energy layered oxide cathode for rechargeable sodium ion batteries27Na[Mn 0.36 Ni 0.44 Ti 0.15 Fe 0.05 ]O 2 predicted via machine learning for high energy Na-ion batteries15Sodium layered oxide cathodes: properties, practicality and prospects363Negative Lattice Expansion in an O3‐Type Transition‐Metal Oxide Cathode for Highly Stable Sodium‐Ion Batteries160Negative Lattice Expansion in an O3‐Type Transition‐Metal Oxide Cathode for Highly Stable Sodium‐Ion Batteries15Effects of Particle Size and Polytype on the Redox Reversibility of the Layered Na0.76Ni0.38Mn0.62O2 Electrode14Fast-charge high-voltage layered cathodes for sodium-ion batteries261O3‐Type Cathodes for Sodium‐Ion Batteries: Recent Advancements and Future Perspectives37Achieving structurally stable O3-type layered oxide cathodes through site-specific cation-anion co-substitution for sodium-ion batteries67Enhanced electrochemical energy storage devices utilizing a one-dimensional (1D) α-MnO2 nanocomposite encased in onion-like carbon20N-doped carbon decorated Na3V2(PO4)3@NC composite derived from melamine as cathode material for high-rate and ultralong-life sodium-ion batteries8Mitigating Sodium Ordering for Enhanced Solid Solution Behavior in Layered NaNiO 2 Cathodes30Mitigating Sodium Ordering for Enhanced Solid Solution Behavior in Layered NaNiO2 Cathodes7Predominant P3-Type Solid–Solution Phase Transition Enables High-Stability O3-Type Na-Ion Cathodes21The critical role of titanium cation for the enhanced Na-ion layer spacing of O3 layered oxide cathode materials10Controlling lithium cobalt oxide phase transition using molten fluoride salt for improved lithium-ion batteries13Improving cycling performance of the NaNiO2 cathode in sodium-ion batteries by titanium substitution20Ribbon-Ordered Superlattice Enables Reversible Anion Redox and Stable High-Voltage Na-Ion Battery Cathodes81Full Exploitation of Charge Compensation of O3‐type Cathode Toward High Energy Sodium‐Ion Batteries by High Entropy Strategy22Van der Waals phase transition investigation toward high-voltage layered cathodes30Layered 3d Transition Metal‐Based Oxides for Sodium‐Ion and Lithium‐Ion Batteries: Differences, Links and Beyond39Effect of Y-doping on high voltage stability of NaNi1/3Fe1/3Mn1/3O2 as a cathode material for sodium-ion batteries25Developments in Sodium-Ion Based Cathode Materials for Energy Storage Applications2Elucidating the Structural Evolution of O3-type NaNi 1/3 Fe 1/3 Mn 1/3 O 2 : A Prototype Cathode for Na-Ion Battery172Local Electron Spin‐State Modulation at Mn Site for Advanced Sodium‐Ion Batteries with Fast‐Kinetic NaNi 0.33 Fe 0.33 Mn 0.33 O 2 Cathode66Understanding Na/vacancy Re-arrangement upon Ion Transport in Sodium Layered Oxide Cathodes10Fast-charging high-entropy O3-type layered cathodes for sodium-ion batteries39Advancements in the Realm of Structural Engineering for Sodium‐Ion Batteries via Elemental Doping: A Focus on P2‐Phase Nickel–Manganese Layered Oxides6Nanostructured sodium vanadate hydrate as a versatile sodium ion cathode material for use in organic media and for aqueous desalination3Optimisation of a P3 phase with superior high voltage reversibility1Substitution of magnesium towards stabilizing low-nickel layered oxides for high voltage and cost-effective sodium-ion batteries11Suppressed P2-Z phase transition and Fe migration in the Na layer of an Fe/Mn-based layered oxide cathode for advanced sodium-ion batteries22Dual‐Pillar Effect in P2‐Type Na 0.67 Ni 0.33 Mn 0.67 O 2 Through Na Site Substitution Achieve Superior Electrochemical and Air/Water Dual‐Stability as Cathode for Sodium‐Ion Batteries75High entropy stabilized O3-type NaNi0.3Fe0.2Mn0.2Ti0.15Sn0.15O2 cathode material for sodium-ion batteries26Melting plus reactive wetting of solid acid enabling stable high-voltage cycling of layered oxide cathodes for sodium-ion batteries15Exploring calcium pillaring of O3-type NaNi0.9Ti0.1O2 cathodes to advance Na-ion battery technology8A Perspective on Pathways Toward Commercial Sodium‐Ion Batteries137Modulating Phase Angle Variations of O3‐Type High‐Entropy Layered Sodium Oxide for Practical Sodium‐Ion Cylindrical Battery37Exploring the limitations and unlocking the potential of sodium-ion battery cathodes10Regulation of P2/O3 layered-oxide cathode by cation potential and dual-site doping provides excellent electrochemical performance16Rational Design of High‐Entropy Cathodes to Optimize Fast Charging Performance in Sodium‐Ion Batteries27A Novel Quantification Method for High Voltage Structural Evolution in Sodium and Lithium Layered Oxides9Pinpointing Chemomechanical Origins of Na Cathode Degradation12Inhibition of phase transition in sodium-ion battery cathode material: From design to validation8Ionic potential for battery materials38Synthesis and Electrochemistry of Stacking Fault‐Free β ‐NaMnO 211A Multi‐Element Composition Modulation Strategy for Designing High‐Capacity and Stable O3‐Type Na‐Layered Oxide21High‐Entropy Engineering of O3‐Type Layered Cathodes for Long‐Cycle Life Sodium‐Ion Batteries1Reversible Phase Transition of an Oxide Cathode in High-Voltage Sodium-Ion Batteries38Lamellar P2-Na0.7CoO2 enables long-cycle life of sodium-ion batteries0The suppression effect of Mg doping on oxygen redox in Mn-based layered oxide cathodes for sodium-ion batteries3A ternary molten salt to synthesize Co/Mg co-doped K0.27MnO2 for a high-performance Na-ion battery cathode3Strain and Kinetics Synergy in Octahedral High‐Entropy Cathodes Enables Ultra‐Durable Sodium‐Ion Batteries5Unique Impacts of Scandium Doping on Electrode Performance of P’2‐ and P2‐type Na 2/3 MnO 213Asymmetric‐Orbital‐Hybridization Induced Electron Redistribution Enabling Stable Sodium Layered Oxides14Understanding of TiO2/Co3O4-modified configuration strategy for stabilizing O3-type NaNi0.4Fe0.2Mn0.4O2 cathodes with enhanced long-term and rate performance7Mg2+ dual-regulation strategy for O3-type sodium-ion battery cathodes: synergistic structural stabilization and dynamic charge compensation4Comprehensive Guide for the Rational Design of High‐Entropy Layered Transition Metal Oxide Cathodes for Sodium‐Ion Batteries19‘Oxygen Bound to Magnesium’ as High Voltage Redox Center Causes Sloping of the Potential Profile in Mg‐Doped Layered Oxides for Na‐Ion Batteries4Mitigating Structural Degradation in O3‐Layered Sodium‐Ion Cathodes: Insights from Mg Doping in NaNi 0.2 Fe 0.4 Mn 0.4 O 214Exploration of High-Entropy Layered Oxides with Ultrahigh Rate Performance for Sodium-Ion Batteries7Identifying cycling current-dependent degradation pathways in high-voltage layered sodium–ion cathodes0Stress accumulation and oxygen activity suppression driven by an anchoring effect and internal electric field in high-voltage O3-type layered cathodes for sodium batteries0The production and electrochemical performance analysis of an O3-NaTi 0.2 Mn 0.2 Fe 0.2 Ni 0.2 Co 0.2 O 2 high-entropy oxide cathode for Na-ion batteries3Unveil the impact of high-entropy agent in cathode material for sodium ion batteries0Combined DFT–experimental, structural and microstructural analysis of Mo-doped NaNiFeMnO2 Layered Oxides3Self‐Regulating Sodium‐Ion Battery Materials: From Phase Reconstruction to Functional Activation11Synergistic inducting P2/O3 mixed phase by thermal diffusion regulation and high-entropy strategy for high performance layered cathode7Enhanced structural stability and ionic conductivity of O3-type NaNi1/3Fe1/3Mn1/3O2 cathode for sodium-ion batteries via Co doping2Strengthening Na−O interaction to stabilize sodium O3-layered cathodes by orbital hybridization regulation4Effect of sodium/vanadium molecular ratio on mixed ionic-electronic conduction and relaxation in sodium vanadophosphate glasses for their use as electrode materials for sodium-ion batteries2Cationic Potential‐Driven Surface Reconstruction Enables Stable High‐Voltage Cylindrical Sodium‐Ion Batteries0Stabilizing O3-type layered oxide cathodes through Zn doping for high-energy sodium-ion batteries1Interlayer–Surface Synergistic Regulation in High‐Entropy O3‐Type Layered Oxides Toward Structurally Robust and Air‐Stable Sodium‐Ion Batteries1Synergistically Engineering Low-Coordination Mn Sites via Cu/Sb Co-Doping toward Low-Strain O3-Type Sodium Oxide Cathodes0Enhanced Performance by Zn-Substitution in Biphasic P2/P3–Na 0.75 Mn 0.68 Ni 0.25 Zn 0.07 O 20Significance of particle morphology: Semi-single-crystalline O3-Type Na[Ni1/3Fe1/3Mn1/3]O2 cathode for practical Na-ion batteries0Chemical Design Principles for Managing the Capacity–Stability Trade‐Off in High‐Voltage Sodium Layered Cathodes0Chemical Design Principles for Managing the Capacity–Stability Trade‐Off in High‐Voltage Sodium Layered Cathodes00.71% Lattice‐Mismatched Intergrowth Achieves 2000‐Cycle Stability in O3‐Type Na‐Layered Oxide Cathodes0Scandium Doping and Coating for Improving O3‐NaNi 1/2 Mn 1/2 O 2 Electrode in Sodium Battery0Recent Advances and Perspectives on Single‐Crystalline Layered Oxide Cathodes for Na‐Ion Batteries0Coupled Evolution of Charged-State Stacking and Redox Partitioning in O3-Type Sodium Cathodes0Insights Into Mg 2+ ‐Driven Lattice Stabilization and Na + Kinetics Regulation in O3‐Type NaMn 0.5 Fe 0.5 O 2 Cathodes for Sodium‐Ion Batteries0

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