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RESEARCH PAPER · Angewandte Chemie International Edition · 2021

Synergistic Polarization Engineering on Bulk and Surface for Boosting CO 2 Photoreduction

Lizhen Liu, Hongwei Huang, Zhensheng Chen, Hongjian Yu, Hongjian Yu, Keyang Wang, Jindi Huang, Han Yu, Han Yu, Yihe Zhang

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Synergistic Polarization Engineering on Bulk and Surface for Boosting CO 2 PhotoreductionOriginalAll-in-one polarized Cd/CdS/halloysite ferroelectric hybrid for exceptional photocatalytic hydrogen evolution38Enhanced photocatalytic activity and easy recovery of visible light active MoSe 2 /BiVO 4 heterojunction immobilized on Luffa cylindrica – experimental and DFT study11Heterojunction and Ferroelectric Polarization Co-Promoting Photocatalytic Activity43In situ construction of Bi 5 O 7 I/Bi 4 Ti 3 O 12 heterostructure composites with plentiful phase interfaces for the boosted selective oxidation of benzylic alcohols under visible light7Linking the enhanced deep NO oxidation of a ferroelectric K 0.5 Bi 0.5 TiO 3 nanowire photocatalyst to its spontaneous polarization and oxygen vacancies12Sc/C codoping effect on the electronic and optical properties of the TiO 2 (101) surface: a first-principles study8Single Pd Atoms Synergistically Manipulating Charge Polarization and Active Sites for Simultaneously Photocatalytic Hydrogen Production and Oxidation of Benzylamine148Synergetic polarization effect of protonation and Fe-doping on g-C 3 N 4 with enhanced photocatalytic activity14One-step synthesis of porous BiOCl microflowers with oxygen vacancies for photoreduction of CO2 under visible light irradiation13Defect-triggered catalysis with multiple reactive species over bismuth oxyhalides in the dark14Polymeric carbon nitride with internal n-p homojunctions for efficient photocatalytic CO2 reduction coupled with cyclohexene oxidation66Novel S-scheme WO3/CeO2 heterojunction with enhanced photocatalytic degradation of sulfamerazine under visible light irradiation99Fe atom clusters embedded N-doped graphene decorated with ultrathin mesoporous carbon nitride nanosheets for high efficient photocatalytic performance8Rational design of n-Bi12TiO20@p-BiOI core–shell heterojunction for boosting photocatalytic NO removal33Defect engineering in metal sulfides for energy conversion and storage215Advances in structural modification of perovskite semiconductors for visible light assisted photocatalytic CO2 reduction to renewable solar fuels: A review92Preparation and photocatalytic properties of g-C3N4/BiOCl heterojunction56Z-scheme junction Bi2O2(NO3)(OH)/g-C3N4 for promoting CO2 photoreduction46Probe Binding Mode and Structure of the Photocatalytic Center: Hydrogen Generation by Quantum Dots and Nickel Ions11Controllable functionalization of g-C 3 N 4 mediated all-solid-state (ASS) Z-scheme photocatalysts towards sustainable energy and environmental applications18A Facile In Situ Hydrothermal Etching Method to CaTiO3/TiO2 Heterostructure for Efficient Photocatalytic N2 Reduction20Donor-Acceptor structural polymeric carbon nitride with in-plane electric field accelerating charge separation for efficient photocatalytic hydrogen evolution78Flower decorated rod-like Pd @ MnO2 nanocomposite: Focus on photocatalysis, Rietveld refinement analysis and electron density distribution analysis14Versatile Titanates: Classification, Property, Preparation, and Sustainable Energy Catalysis40Rational Design of Dot‐on‐Rod Nano‐Heterostructure for Photocatalytic CO2 Reduction: Pivotal Role of Hole Transfer and Utilization112Bismuth-doped g-C 3 N 4 /ZIF-8 heterojunction photocatalysts with enhanced photocatalytic performance under visible light illumination19Cd3(C3N3S3)2 Polymer/Sn Schottky Heterojunction for Broadband‐Solar Highly Selective Photocatalytic CO2 Reduction52Enhanced photocatalytic benzyl alcohol oxidation over Bi4Ti3O12 ultrathin nanosheets66Self-doped Br in Bi5O7Br ultrathin nanotubes: Efficient photocatalytic NO purification and mechanism investigation33Metal–Organic Framework-Derived Tubular In2O3–C/CdIn2S4 Heterojunction for Efficient Solar-Driven CO2 Conversion57Black phosphorus-based heterostructures for photocatalysis and photoelectrochemical water splitting107Photo-assisted self-assembly synthesis of all 2D-layered heterojunction photocatalysts with long-range spatial separation of charge-carriers toward photocatalytic redox reactions82Au/g-C3N4 heterostructure sensitized by black phosphorus for full solar spectrum waste-to-hydrogen conversion32Preparation of double-layered Co−Ci/NiFeOOH co-catalyst for highly meliorated PEC performance in water splitting107Crystal design of bismuth oxyiodide with highly exposed (110) facets on curved carbon nitride for the photocatalytic degradation of pollutants in wastewater14Ferroelectrics in Photocatalysis47Effect of the Defect Modulator and Ligand Length of Metal–Organic Frameworks on Carbon Dioxide Photoreduction53Unique Cd 0.5 Zn 0.5 S/WO 3− x direct Z -scheme heterojunction with S, O vacancies and twinning superlattices for efficient photocatalytic water-splitting13Spontaneous Atomic Sites Formation in Wurtzite CoO Nanorods for Robust CO2 Photoreduction28Construction of Z-scheme heterojunction of (BiO)2CO3/ZnFe-LDH for enhanced photocatalytic degradation of tetracycline36Cation vacancy activating surface neighboring sites for efficient CO 2 photoreduction on Bi 4 Ti 3 O 12 nanosheets35Cocatalyst engineering to weaken the charge screening effect over Au–Bi 4 Ti 3 O 12 for piezocatalytic pure water splitting34Enhanced Piezocatalytic Activity in Ion-Doped Sns2 Via Lattice Distortion Engineering for Bpa Degradation and Hydrogen Production131Enhanced Piezocatalytic Activity of Sns2 for Bisphenol a Degradation and Hydrogen Production Via Ion Size-Induced Lattice Strain Engineering0FeVO 4 nanowires for efficient photocatalytic CO 2 reduction25Flux synthesis of Bi2MO4Cl (M = Gd and Nd) nanosheets for high-efficiency photocatalytic oxygen evolution under visible light14Synthesis of a UiO-66/g-C 3 N 4 composite using terephthalic acid obtained from waste plastic for the photocatalytic degradation of the chemical warfare agent simulant, methyl paraoxon65Unveiling the charge transfer behavior within ZSM-5 and carbon nitride composites for enhanced photocatalytic degradation of methylene blue34Visible-Light Photocatalytic Chlorite Activation Mediated by Oxygen Vacancy for Efficient Chlorine Dioxide Generation and Pollutant Degradation0Facile synthesis of Pd-doped Bi2WO6 nanoplates used for enhanced visible-light-driven photocatalysis5Electric Field Coupling in the S-Scheme CdS/BiOCl Heterojunction for Boosted Charge Transport toward Photocatalytic CO2 Reduction55Enhanced H2S sensing performance of BiFeO3 based MEMS gas sensor with corona poling43In Situ Self-Assembled ZIF-67/MIL-125-Derived Co3O4/TiO2 p–n Heterojunctions for Enhanced Photocatalytic CO2 Reduction73Surfactant assisted hydrothermal synthesis of MgO/g-C3N4 heterojunction nanocomposite for enhanced solar photocatalysis and antimicrobial activities38Unraveling Charge‐Separation Mechanisms in Photocatalyst Particles by Spatially Resolved Surface Photovoltage Techniques43Unraveling Charge‐Separation Mechanisms in Photocatalyst Particles by Spatially Resolved Surface Photovoltage Techniques166Facial construction of Pd/BiPO4 toward efficient photocatalytic oxidation of formaldehyde under UV light irradiation10Unveiling the effect of interstitial dopants on CO2 activation over CsPbBr3 catalyst for efficient photothermal CO2 reduction79Ionic liquids assisted preparation of BiPO4 photocatalyst with enhanced photocatalytic activity for tetracycline and rhodamine B removal7Bandgap engineered g-C3N4 and its graphene composites for stable photoreduction of CO2 to methanol82Boosted Inner Surface Charge Transfer in Perovskite Nanodots@Mesoporous Titania Frameworks for Efficient and Selective Photocatalytic CO 2 Reduction to Methane12Boosted Inner Surface Charge Transfer in Perovskite Nanodots@Mesoporous Titania Frameworks for Efficient and Selective Photocatalytic CO 2 Reduction to Methane202Electronic Engineering of ABO3 Perovskite Metal Oxides Based on d0 Electronic‐Configuration Metallic Ions toward Photocatalytic Water Splitting under Visible Light44A novel CeO2 / MIL101 (Fe) heterojunction for enhanced photocatalytic degradation of tetracycline under visible‐light irradiation35Multi-field driven hybrid catalysts for CO2 reduction: Progress, mechanism and perspective39Engineering unsaturated coordination of conductive TiOx clusters derived from Metal–Organic–Framework incorporated into hollow semiconductor for highly selective CO2 photoreduction21Boosting the photogenerated hole separation and injection of Ti-Fe2O3 by co-modifying carbon quantum dots and NiFe layered double hydroxide17Engineering piezoelectricity and strain sensitivity in CdS to promote piezocatalytic hydrogen evolution151Multidimensional In2O3/In2S3 heterojunction with lattice distortion for CO2 photoconversion94Controllable fabrication of sulfur-vacancy-rich Bi2S3 nanorods with efficient near-infrared light photocatalytic for nitrogen fixation68Inorganic ligands-mediated hole attraction and surface structural reorganization in InP/ZnS QD photocatalysts studied via ultrafast visible and midinfrared spectroscopies17Synergy Effect between Facet and Zero-Valent Copper for Selectivity Photocatalytic Methane Formation from CO 2120Enhanced visible-light photocatalytic performance of ZIF-8-derived ZnO/TiO2 nano-burst-tube by solvothermal system adjustment19Excellent piezo-photocatalytic performance of Bi4Ti3O12 nanoplates synthesized by molten-salt method172Fabrication of a Covalent Organic Framework-Based Heterojunction via Coupling with ZnAgInS Nanosphere with High Photocatalytic Activity30Piezocatalytic and Photocatalytic Hydrogen Peroxide Evolution of Sulfide Solid Solution Nano‐Branches from Pure Water and Air112Supramolecule self-assembly approach to direct Z-scheme TiO2/g-C3N4 heterojunctions for efficient photocatalytic degradation of emerging phenolic pollutants43BiOBr with oxygen vacancies capture 0D black phosphorus quantum dots for high efficient photocatalytic ofloxacin degradation68CsPbBr3 perovskite based tandem device for CO2 photoreduction15Amorphous iron oxides anchored on BiOCl nanoplates as robust catalysts for high-performance photo-Fenton oxidation30ZnIn2S4‐Based Nanostructures in Artificial Photosynthesis: Insights into Photocatalytic Reduction toward Sustainable Energy Production61Ni–Co Bimetallic Hydroxide Nanosheet Arrays Anchored on Graphene for Adsorption‐Induced Enhanced Photocatalytic CO2 Reduction87Atomically Thin Bi2O2(OH)1+x(NO3)1–x Nanosheets with Regulated Surface Composition for Enhanced Photocatalytic CO2 Reduction14C-scheme electron transfer mechanism: An efficient ternary heterojunction photocatalyst carbon quantum dots/Bi/BiOBr with full ohmic contact64Photodeposition of earth-abundant cocatalysts in photocatalytic water splitting: Methods, functions, and mechanisms115Construction of Plasmonic Metal@Semiconductor Core–Shell Photocatalysts: From Epitaxial to Nonepitaxial Strategies30Controllable Synthesis of BiOCl with Z‐Scheme (001)/(110) Facet Homojunction and their Photocatalytic Killing Effect on HePG2 Cells in vitro2In Situ Hydrothermal Synthesis of Metallic Bi Self‐Deposited Bi2SiO5 with Enhanced Photocatalytic CO2 Reduction Performance13A simple terpyridine–cobalt(II) complex sensitized by connective mpg–C3N4 for improved CO2 photoreduction16An S-scheme photocatalyst constructed by modifying Ni-doped Sn3O4 micro-flowers on g-C3N4 nanosheets for enhanced visible-light-driven hydrogen evolution33A novel Sillén-structured Bi-based oxybromide: CdBiO 2 Br ultrathin nanosheets for enhanced photocatalytic activity2Ball-milling assisted fabrication of hierarchical Na4Ti5O12/Na2Ti6O13 for enhanced tetracyclines photodegradation16Modulating Ti t 2g Orbital Occupancy in a Cu/TiO 2 Composite for Selective Photocatalytic CO 2 Reduction to CO171Modulating Tit2gOrbital Occupancy in a Cu/TiO2Composite for Selective Photocatalytic CO2Reduction to CO8Promoted photocarriers separation in atomically thin BiOCl/Bi2WO6 heterostructure for solar-driven photocatalytic CO2 reduction502D/2D Interface Engineering Promotes Charge Separation of Mo2C/g-C3N4 Nanojunction Photocatalysts for Efficient Photocatalytic Hydrogen Evolution64Phosphorus Tailors thed‐Band Center of Copper Atomic Sites for Efficient CO2Photoreduction under Visible‐Light Irradiation23Phosphorus Tailors thed‐Band Center of Copper Atomic Sites for Efficient CO2Photoreduction under Visible‐Light Irradiation209Visible-Light Photocatalytic Chlorite Activation Mediated by Oxygen Vacancy Abundant Nd-Doped BiVO 4 for Efficient Chlorine Dioxide Generation and Pollutant Degradation44DFT-Assisted Design of D–A Conjugated Polymers for Photocatalytic Reduction of Carbon Dioxide19Metal-induced oxygen vacancies on Bi2WO6 for efficient CO2 photoreduction39Spatial Separation of Electrons and Holes among ZnO Polar {0001} and {1010} Facets for Enhanced Photocatalytic Performance38Creation of SnxNb1−xO2 solid solution through heavy Nb-doping in SnO2 to boost its photocatalytic CO2 reduction to C2+ products under simulated solar illumination41Facet-Engineering of Materials for Photocatalytic Application: Status and Future Prospects90C–Doping Induced Oxygen-Vacancy in WO3 Nanosheets for CO2 Activation and Photoreduction242Atomically Dispersed Indium‐Copper Dual‐Metal Active Sites Promoting C−C Coupling for CO 2 Photoreduction to Ethanol352Atomically Dispersed Indium‐Copper Dual‐Metal Active Sites Promoting C−C Coupling for CO2 Photoreduction to Ethanol51Synergies of Adjacent Sites in Atomically Dispersed Ruthenium toward Achieving Stable Hydrogen Evolution121Preparation of a Flower-Like BiOCl/K-C3N4 p-n Heterojunction and Photodegradation Formaldehyde and Dyes6Adsorbent-to-photocatalyst: Recycling heavy metal cadmium by natural clay mineral for visible-light-driven photocatalytic antibacterial22Tunable band structure of synthesized carbon dots modified graphitic carbon nitride/bismuth oxychlorobromide heterojunction for photocatalytic degradation of tetracycline in water71Metal Carbide‐Based Cocatalysts for Photocatalytic Solar‐to‐Fuel Conversion49Facile synthesis CQDs/SnO2-x/BiOI heterojunction photocatalyst to effectively degrade pollutants and antibacterial under LED light19Few-layered MoS2 anchored on 2D porous C3N4 nanosheets for Pt-free photocatalytic hydrogen evolution56Symmetry breaking for semiconductor photocatalysis46Design and application of g-C3N4-based materials for fuels photosynthesis from CO2 or H2O based on reaction pathway insights20Enhanced adsorption and photocatalytic Cr(VI) reduction and sterilization of defective MoS2/PVP32Chlorine tailored p-d blocks dual-metal atomic catalyst for efficient photocatalytic CO2 reduction42Unveiling S‐Scheme Charge Transfer Pathways in In2S3/Nb2O5 Hybrid Nanofiber Photocatalysts for Low‐Concentration CO2 Hydrogenation16Cooperation of congenital and acquisitus sulfur vacancy for excellent photocatalytic hydrogen peroxide evolution of CdS nanorods from air73Amorphous SnO2 decorated ZnSn(OH)6 promotes interfacial hydroxyl polarization for deep photocatalytic toluene mineralization40Enhancement of photoelectrochemical performance of BiFeO3 by Sm3+ doping29High‐Performance Photocatalytic Reduction of Nitrogen to Ammonia Driven by Oxygen Vacancy and Ferroelectric Polarization Field of SrBi 4 Ti 4 O 15 Nanosheets61Synergy‐Compensation Effect of Ferroelectric Polarization and Cationic Vacancy Collaboratively Promoting CO2 Photoreduction37Maneuvering cuprous oxide-based photocathodes for solar-to-fuel conversion37Rapid Ferroelectric-Photoexcited Bacteria-Killing of Bi4Ti3O12/Ti3C2Tx Nanofiber Membranes60Design and synthesis of an S-scheme TiO 2 homojunction with an adjusted, well-defined phase for directional carrier transfer in solar water splitting7Vacancy Pair-Induced Charge Rebalancing with Surface and Interfacial Dual Polarization for CO2 Photoreduction44Photodegradation of tetracycline antibiotic by ternary recyclable Z-scheme g-C3N4/Fe3O4/Bi2WO6/Bi2S3 photocatalyst with improved charge separation efficiency: Characterization and mechanism studies37Highly transparent Bi 4 Ti 3 O 12 thin-film electrodes for ferroelectric-enhanced photoelectrochemical processes6Single-atom catalysts for energy conversion59Highly efficient photocatalytic hydrogen production by platinum modified ferroelectric SrBi4Ti4O1522Breaking through the interfacial energy barrier limitations of type-I heterojunctions via ferroelectric polarization engineering: a case study of Bi 5 Ti 3 FeO 15 /BiOCl10Efficient photocatalytic NO oxidation over novel NiAl layered double hydroxide/Bi 4 Ti 3 O 12 Z-scheme heterojunctions with boosted charge separation and O 2 activation25Oxygen-deficient MoO 3− x evoked synergistic photo-thermal catalytic CO 2 reduction over g-C 3 N 429Photothermal Structural Dynamics of Au Nanofurnace-Functionalized ZnO Nanotube (AuNI-ZNT) for In Situ Enhancement in Desorption and Ionization0Recent advances of single-atom catalysts in CO 2 conversion297Synergistic coupling of interface ohmic contact and LSPR effects over Au/Bi 24 O 31 Br 10 nanosheets for visible-light-driven photocatalytic CO 2 reduction to CO38Interfacial engineering in two-dimensional heterojunction photocatalysts522D–1D-2D multi-interfacial-electron transfer scheme enhanced g-C3N4/MWNTs/rGO hybrid composite for accelerating CO2 photoreduction17Enabling Internal Electric Fields to Enhance Energy and Environmental Catalysis235Integrating 3D porous morphology with efficient plasmonic Au nanoparticles in photo-responsive g-C3N4/Au hybrid photocatalyst for the enhancement of CO2 reduction23Combination of covalent-organic framework and Bi2O2S by covalent bonds to form p-n heterojunction for enhanced photocatalytic CO2 conversion45Defective materials for CO2 photoreduction: From C1 to C2+ products67Spatially Separated Redox Cocatalysts on Ferroelectric Nanoplates for Improved Piezophotocatalytic CO2 Reduction and H2O Oxidation10Understanding oxygen vacant hollow structure CeO 2 @In 2 O 3 heterojunction to promote CO 2 reduction103High Efficiency Photocatalyst with Ultra‐Fine Pd NPs Constructed at Room Temperature for CO 2 Reduction2Utilizing Cationic Vacancies and Spontaneous Polarization on Cathode to Enhance Zinc‐Ion Storage and Inhibit Dendrite Growth in Zinc‐Ion Batteries60Utilizing Cationic Vacancies and Spontaneous Polarization on Cathode to Enhance Zinc‐Ion Storage and Inhibit Dendrite Growth in Zinc‐Ion Batteries0Regulating Spin Polarization through Cationic Vacancy Defects in Bi 4 Ti 3 O 12 for Enhanced Molecular Oxygen Activation90

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  37. Effect of the Defect Modulator and Ligand Length of Metal–Organic Frameworks on Carbon Dioxide Photoreduction

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  39. Spontaneous Atomic Sites Formation in Wurtzite CoO Nanorods for Robust CO2 Photoreduction

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  40. Construction of Z-scheme heterojunction of (BiO)2CO3/ZnFe-LDH for enhanced photocatalytic degradation of tetracycline

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  41. Cation vacancy activating surface neighboring sites for efficient CO 2 photoreduction on Bi 4 Ti 3 O 12 nanosheets

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  42. Cocatalyst engineering to weaken the charge screening effect over Au–Bi 4 Ti 3 O 12 for piezocatalytic pure water splitting

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  43. Enhanced Piezocatalytic Activity in Ion-Doped Sns2 Via Lattice Distortion Engineering for Bpa Degradation and Hydrogen Production

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  44. Enhanced Piezocatalytic Activity of Sns2 for Bisphenol a Degradation and Hydrogen Production Via Ion Size-Induced Lattice Strain Engineering

    SSRN Electronic Journal · 2022-01-01

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  45. FeVO 4 nanowires for efficient photocatalytic CO 2 reduction

    Catalysis Science & Technology · 2022-01-01

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  46. Flux synthesis of Bi2MO4Cl (M = Gd and Nd) nanosheets for high-efficiency photocatalytic oxygen evolution under visible light

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  47. Synthesis of a UiO-66/g-C 3 N 4 composite using terephthalic acid obtained from waste plastic for the photocatalytic degradation of the chemical warfare agent simulant, methyl paraoxon

    RSC Advances · 2022-01-01

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  48. Unveiling the charge transfer behavior within ZSM-5 and carbon nitride composites for enhanced photocatalytic degradation of methylene blue

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  49. Visible-Light Photocatalytic Chlorite Activation Mediated by Oxygen Vacancy for Efficient Chlorine Dioxide Generation and Pollutant Degradation

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  50. Facile synthesis of Pd-doped Bi2WO6 nanoplates used for enhanced visible-light-driven photocatalysis

    Inorganic and Nano-Metal Chemistry · 2022-01-07

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