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RESEARCH PAPER · Journal of the American Chemical Society · 2021

Tunable Band Gaps in MUV-10(M): A Family of Photoredox-Active MOFs with Earth-Abundant Open Metal Sites

Kevin Fabrizio, Konstantinos A. Lazarou, Lillian I. Payne Torres, Liam Peter Twight, Stephen L. Golledge, Christopher H. Hendon, Carl K. Brozek

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Tunable Band Gaps in MUV-10(M): A Family of Photoredox-Active MOFs with Earth-Abundant Open Metal SitesOriginalOn the limit of proton-coupled electronic doping in a Ti( iv )-containing MOF25Cooperativity and Metal–Linker Dynamics in Spin Crossover Framework Fe(1,2,3-triazolate)233A High-Spintronic Helix Metal-Organic Chain as a High-Output Triboelectric Nanogenerator Material for Self-Powered Anticorrosion28Determining Optical Band Gaps of MOFs100Engineering of catalytically active sites in photoactive metal–organic frameworks58Application of MOFs and COFs for photocatalysis in CO2 reduction, H2 generation, and environmental treatment476Highly Strained Bi‐MOF on Bismuth Oxyhalide Support with Tailored Intermediate Adsorption/Desorption Capability for Robust CO2 Photoreduction11Highly Strained Bi‐MOF on Bismuth Oxyhalide Support with Tailored Intermediate Adsorption/Desorption Capability for Robust CO2 Photoreduction153A Double‐Helix Metal‐Chain Metal‐Organic Framework as a High‐Output Triboelectric Nanogenerator Material for Self‐Powered Anticorrosion6A Double‐Helix Metal‐Chain Metal‐Organic Framework as a High‐Output Triboelectric Nanogenerator Material for Self‐Powered Anticorrosion75Metal–Organic Frameworks and Their Composites for Environmental Applications96Photoredox-Active Colloids and Polymer Membranes of Titanium-Based MOF Nanoparticles1Metal–Organic Frameworks as Photocatalysts for Solar-Driven Overall Water Splitting537A supported pyridylimine–cobalt catalyst for N -formylation of amines using CO 215Chemical complexity for targeted function in heterometallic titanium–organic frameworks30Electrically conductive [Fe 4 S 4 ]-based organometallic polymers13Gram-scale synthesis of MIL-125 nanoparticles and their solution processability17Size-Dependent Thermal Shifts to MOF Nanocrystal Optical Gaps Induced by Dynamic Bonding22Photoinduced Ligand-to-Metal Charge Transfer of Cobaltocene: Radical Release and Catalytic Cyclotrimerization12Chemical Bonding of g-C 3 N 4 /UiO-66(Zr/Ce) from Zr and Ce Single Atoms for Efficient Photocatalytic Reduction of CO 2 under Visible Light170Enhanced CO2 capture in partially interpenetrated MOFs: Synergistic effects from functional group, pore size, and steric-hindrance41Isoreticular Expansion and Linker-Enabled Control of Interpenetration in Titanium–Organic Frameworks30Hollow-shell hybrids with regulatable microelectronic structures for boosting photocatalytic H2 evolution via water splitting and isopropanol oxidation under visible light6Selective Reduction of Nitro Compounds by Organosilanes Catalyzed by a Zirconium Metal‐Organic Framework Supported Salicylaldimine‐Cobalt(II) Complex8Vapor-Assisted Conversion of Heterobimetallic Titanium–Organic Framework Thin Films3Dynamic metal-linker bonds in metal–organic frameworks32Covalent synthesis of Ti-MOF for enhanced photocatalytic CO2 reduction14Translocation and Confinement of Tetraamines in Adaptable Microporous Cavities0Translocation and Confinement of Tetraamines in Adaptable Microporous Cavities3Flexible and Stretchable Thermoresponsive Display for Multifunctional Device Applications1Catalytic open metal sites in Ti-MOFs obtained through plasma treatment for oxidative desulfurization25Tuning redox activity in metal–organic frameworks: From structure to application62Integrating Compositional and Structural Diversity in Heterometallic Titanium Frameworks by Metal Exchange Methods1Size-Dependent Spin Crossover and Bond Flexibility in Metal–Organic Framework Nanoparticles13Influence of NH2 Substitution and Position on the Photocatalytic Activity of Ti-Based Metal–Organic Frameworks5Integrating Compositional and Structural Diversity in Heterometallic Titanium Frameworks by Metal Exchange Methods11MOF and MOF-derived composites for flexible energy storage devices42Reticular Materials for Photocatalysis77Regulating the Electronic Band Structure of the Ti-Based Metal–Organic Framework toward Boosting Light-Driven Hydrogen Evolution16Ba/Ti MOF: A Versatile Heterogeneous Photoredox Catalyst for Visible‐Light Metallaphotocatalysis32Fine-tuning electronic and semiconducting properties of Co-MOF-74 upon encapsulating aniline and its derivatives3Ultrafine Cu2O nanoparticles supported on MIL-125-NH2 as an efficient and stable 4‑nitrophenol reduction catalyst1Unlocking potential and challenges of MOFs and COFs based energy materials for CO2 reduction and H2 production51MOF‐Based Electrocatalysts for Water Electrolysis, Energy Storage, and Sensing: Progress and Insights10Titanium Cluster Nuclearity Controls the Potential of Ti(IV/III) Reduction by Transfer Hydrogenation1Metal Node Control of Coordinatively Unsaturated Sites in Heterobimetallic MOFs for Stable and High Ammonia Adsorption22Turn-On Conductivity with Proton-Coupled Electron Transport in Metal–Organic Frameworks8Crystallographic Evidence of Size-Dependent Bond Flexibility in Metal–Organic Framework Nanocrystals4Cooperative Metal Ion Combinations in Ti-Based Multivariate Metal–Organic Frameworks2Size-Dependent Optical Band Gaps in Metal–Organic Framework Nanoparticles11Oxygen Vacancies Stabilize Zr(III) in the Metal–Organic Framework UiO-661Inducing Reactivity by Cluster Strain in Titanium Frameworks2Engineering Design Strategies for Boosting Photocatalytic Activity: Theory-to-Data-Driven Perspective2Construction of molecular-level heterojunctions and long-range electron transport channels in the MOF framework for boosted photoredox activity1Cluster-enabled control of single-electron photoredox catalysis in reticular frameworks0Synthesis and application of MUV-10/graphene oxide composite fibers for headspace SPME-GC-MS determination of flavor compounds in Baijiu0Modulating Charge Transfer Dynamics in Titanium Metal–Organic Frameworks via Conjugated Linker Engineering for Enhanced Photocatalytic Hydrogen Evolution0Halogen-controlled multi-level oxidation in tetrathiafulvalene-based metal-organic frameworks0

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  1. On the limit of proton-coupled electronic doping in a Ti( iv )-containing MOF

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  2. Cooperativity and Metal–Linker Dynamics in Spin Crossover Framework Fe(1,2,3-triazolate)2

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  7. Highly Strained Bi‐MOF on Bismuth Oxyhalide Support with Tailored Intermediate Adsorption/Desorption Capability for Robust CO2 Photoreduction

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  8. Highly Strained Bi‐MOF on Bismuth Oxyhalide Support with Tailored Intermediate Adsorption/Desorption Capability for Robust CO2 Photoreduction

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  9. A Double‐Helix Metal‐Chain Metal‐Organic Framework as a High‐Output Triboelectric Nanogenerator Material for Self‐Powered Anticorrosion

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  11. Metal–Organic Frameworks and Their Composites for Environmental Applications

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  12. Photoredox-Active Colloids and Polymer Membranes of Titanium-Based MOF Nanoparticles

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  13. Metal–Organic Frameworks as Photocatalysts for Solar-Driven Overall Water Splitting

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  14. A supported pyridylimine–cobalt catalyst for N -formylation of amines using CO 2

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  15. Chemical complexity for targeted function in heterometallic titanium–organic frameworks

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  18. Size-Dependent Thermal Shifts to MOF Nanocrystal Optical Gaps Induced by Dynamic Bonding

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  19. Photoinduced Ligand-to-Metal Charge Transfer of Cobaltocene: Radical Release and Catalytic Cyclotrimerization

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  21. Enhanced CO2 capture in partially interpenetrated MOFs: Synergistic effects from functional group, pore size, and steric-hindrance

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