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RESEARCH PAPER · The Journal of Physical Chemistry Letters · 2021

Limits to Electrical Mobility in Lead-Halide Perovskite Semiconductors

Chelsea Q. Xia, Jiali Peng, Samuel Poncé, Jay B. Patel, Adam D. Wright, Timothy W. Crothers, Mathias Uller Rothmann, Juliane Borchert, Rebecca L. Milot, Hans Kraus, Qianqian Lin, Feliciano Giustino, Laura M. Herz, Michael B. Johnston

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Limits to Electrical Mobility in Lead-Halide Perovskite SemiconductorsOriginalExtracting in Situ Charge Carrier Diffusion Parameters in Perovskite Solar Cells with Light Modulated Techniques49Instrumentação para medidas de mobilidade eletrônica e concentração de portadores em amostras semicondutoras, pelo método de van der Pauw2Ultrafast photo-induced phonon hardening due to Pauli blocking in MAPbI 3 single-crystal and polycrystalline perovskites7Interplay of Structure, Charge‐Carrier Localization and Dynamics in Copper‐Silver‐Bismuth‐Halide Semiconductors45Optimizing the Proton Conductivity with the Isokinetic Temperature in Perovskite‐Type Proton Conductors According to Meyer–Neldel Rule31Enhanced room-temperature terahertz detection and imaging derived from anti-reflection 2D perovskite layer on MAPbI 3 single crystals18Intrinsic aging in mixed-cation lead halide perovskites14Thick-junction perovskite X-ray detectors: processing and optoelectronic considerations33Further Advancement of Perovskite Single Crystals19Assessment of Photon Recycling in Perovskite Solar Cells by Fully Coupled Optoelectronic Simulation18Predicting Solar Cell Performance from Terahertz and Microwave Spectroscopy80Hybrid Halide Perovskite‐Based Near‐Infrared Photodetectors and Imaging Arrays94Understanding the Impacts of Grain Size Variation, Distribution, and Recombination Losses in Halide Perovskites: A Generalized Semi‐Analytical Model from Thin‐Film to Photovoltaics4Halide Perovskite Crystallization Processes and Methods in Nanocrystals, Single Crystals, and Thin Films163Is There a Polaron Signature in Angle-Resolved Photoemission of CsPbBr 3 ?28Perovskite Single‐Crystal Solar Cells: Advances and Challenges48Solvent-Free Method for Defect Reduction and Improved Performance of p-i-n Vapor-Deposited Perovskite Solar Cells96Damping the phase segregation in mixed halide perovskites: Influence of X-site anion10An investigation on carrier transport behavior of tetragonal halide perovskite: First-principles calculation14Inclusion of infrared dielectric screening in the GW method from polaron energies to charge mobilities2Photoinduced large polaron transport and dynamics in organic–inorganic hybrid lead halide perovskite with terahertz probes86Review on Perovskite Semiconductor Field–Effect Transistors and Their Applications46Performance Analysis of Perovskite Solar Cell by Considering Temperature Effect on Physical Parameters of the Absorber Layer3Two-Dimensional Layered Simple Aliphatic Monoammonium Tin Perovskite Thin Films and Potential Applications in Field-Effect Transistors24Low-intensity low-temperature analysis of perovskite solar cells for deep space applications22Mechanistic insights into the key role of methylammonium iodide in the stability of perovskite materials4Mitigation of Temperature Effects and Performance Enhancement of Perovskite Solar Cells Using Nano-Pyramids Grating17Optimised Spintronic Emitters of Terahertz Radiation for Time-Domain Spectroscopy13Achieving High Responsivity and Detectivity in a Quantum-Dot-in-Perovskite Photodetector94Ab initio calculation of carrier mobility in semiconductors including ionized-impurity scattering48An Interlayer of Ultrasmall N-Rich Carbon Dots for Optimization of SnO2/CsFAPbI3 Interface6Tungstate‐mediated In‐situ Passivation of Grain Boundary Grooves in Perovskite Solar Cells45Tungstate‐mediated In‐situ Passivation of Grain Boundary Grooves in Perovskite Solar Cells0Rotatable Skeleton for the Alleviation of Thermally Accumulated Defects in Inorganic Perovskite Solar Cells19Accurate Prediction of Hall Mobilities in Two-Dimensional Materials through Gauge-Covariant Quadrupolar Contributions46Halide perovskites: Properties, synthesis, and applications1Orientation and Grain Size in MAPbI 3 Thin Films: Influence on Phase Transition, Disorder, and Defects22Aromatic Additives Boost the Terahertz Properties of Mixed Halide Perovskite Single Crystals4CsPbI 3- perovskite quantum dot solar cells: unlocking their potential through improved absorber layer characteristics and reduced defects64High-performance metal halide perovskite transistors160Resolving the Ultrafast Charge Carrier Dynamics of 2D and 3D Domains within a Mixed 2D/3D Lead‐Tin Perovskite19The Electrical Behaviors of Grain Boundaries in Polycrystalline Optoelectronic Materials66Contrasting Charge‐Carrier Dynamics across Key Metal‐Halide Perovskite Compositions through In Situ Simultaneous Probes20Correlated anharmonicity and dynamic disorder control carrier transport in halide perovskites21Coated Spintronic Emitters for Improved THz Time-domain Spectroscopy1Impact of Mobile Ions on Transient Capacitance Measurements of Perovskite Solar Cells18Characterization of Intrinsic Charge Carrier Dynamics in Lead Halide Perovskite Films Using Time-Resolved Terahertz Spectroscopy4Intrinsic Limits of Charge Carrier Mobilities in Layered Halide Perovskites13Advances in Perovskite Single Crystal Thin Films: Synthesis Methods and Applications in Photodetection17A Comprehensive Study on the Thermal Behavior of Perovskite Solar Cell10Temperature-Dependent Structural and Optoelectronic Properties of the Layered Perovskite 2-Thiophenemethylammonium Lead Iodide7Giant Enhancement of Hole Mobility for 4H-Silicon Carbide through Suppressing Interband Electron–Phonon Scattering16Dominant Scattering Mechanisms in Limiting the Electron Mobility of Scandium Nitride11Strong Dependence of Point Defect Properties in Metal Halide Perovskites on Description of van der Waals Interaction4Improvement of interfacial electron extraction efficiency by suppressing Auger recombination in an indium-doped mixed cationic perovskite heterostructure0Exciton Transport in Perovskite Materials46Inorganic M 3 ACl 3 (M = Ca, Sr, Ba, A = N, P, As) perovskite-derivatives for next-generation solar cells and optoelectronics: in-depth analysis of stability, optoelectronic features, and temperature-dependent carrier mobilities10Odd-even effects in lead-iodide-based Ruddlesden–Popper 2D perovskites15Solar Energy0Temperature‐Dependent Charge‐Carrier Dynamics in Lead‐Halide Perovskites: Indications for Dynamic Disorder Dominated Scattering Mechanism13Transient Photoluminescence Reveals the Dynamics of Injected Charge Carriers in Perovskite Light-Emitting Diodes4Role of Size and Shape in Photoluminescence and Ultra-Low-Frequency Raman of Methylammonium Lead Iodide Perovskite Quantum Dots6Aerosol-Assisted Crystallization Lowers Intrinsic Quantum Confinement and Improves Optoelectronic Performance in FAPbI 3 Films4Advances in theory and computational methods for next-generation thermoelectric materials9Novel Method for Measuring Carrier Diffusion Lengths in Metal‐Halide Perovskites2Vapour-deposited high-performance tin perovskite transistors38Computational analysis of perovskite solar cells for space applications13Unique Performance Considerations for Printable Organic Semiconductor and Perovskite Radiation Detectors: Toward Consensus on Best Practice Evaluation2Spin Noise of a Halide Perovskite7Exploring the Influence of Grain Boundaries on Carrier Transport and PEC Activity of Hematite Photoelectrodes7Conformal Charge Transport Layers for Perovskite Solar Cells and Tandem Devices20Engineering Strategies for 2D Layered Tin Halide Perovskite Field‐Effect Transistors12Short‐Term Bienenstock‐Cooper‐Munro Learning in Optoelectrically‐Driven Flexible Halide Perovskite Single Crystal Memristors7Recent advances in halide perovskite material classes for field-effect transistors3Spatiotemporal imaging of photogenerated charge carriers in optoelectronic materials0Impact of anharmonicity on the carrier mobility of the Pb-free CsSnBr 3 perovskite5Diverse Responses in Lattice Thermal Conductivity of n ‐Type/ p ‐Type Wurtzite Semiconductors Driven by Asymmetric Electron‐Phonon Interactions2Correlated Vibrational and Electronic Signatures of Surface Disorder in CsPbBr 3 Nanocrystals10Comprehensive advances in gas sensing: Mechanisms, material innovations, and applications in environmental and health monitoring8Cu-doped mesoporous TiO 2 interlayer for highly efficient and stable hybrid perovskite solar cells4Enhanced carrier extraction and photostability in perovskite solar cells via a band-engineered Sb 2 O x /TiO 2 bilayer heterojunction1Perovskite Photon-Counting Detectors: Narrowing the Field2Toward Reliable Metal Halide Perovskite FETs: From Electronic Structure and Device Physics to Stability and Performance Engineering1Perspectives on halide perovskite-based in-memory and neuromorphic computing devices2On the Effects of Chlorine Doping in CsPbBr3 Single Crystals0Suppressed electron–phonon coupling in Ag-doped CsPbBr3 for high-performance photodetectors1Ascertaining the Transient State Pivotal for Fast Carrier Migration in Halide Perovskites0Performance analysis and current matching optimization of KGeCl3 based tandem solar cell using SCAPS-1D with a machine learning approach0Enhanced Carrier Mobility and Diffusion Length in Formamidinium-Rich Hybrid Perovskites: Effects of Grain-Size and Electron–Phonon Coupling1From symmetry to stability: Structural and electronic transformation in Cs 2 KInI 60Chloride‐Substituted Perovskite Enables Thick Middle Cell for Perovskite/Perovskite/Silicon Triple‐Junction Solar Cells0How Polarization Switch Influences Both Charge Separation and Carrier Recombination in Hybrid Perovskites1Study on the feasibility of halide perovskite material based gas sensor for NO2 and NH3 detection in environmental monitoring applications0Perovskite Solar Cell Efficiency and Thermal-Stability Enhancement via Interfacial Engineering: A Numerical Analysis0Large Polaron Screening Delays Mobility Roll-Off in Halide Perovskites under High Injection0Reinforced 1D perovskite growth via molecular synergy for enhanced perovskite solar cells stability0Importance of nonlinear long-range electron-phonon interaction for the carrier mobility of anharmonic halide perovskites0Overcoming the Charge Confinement-Transport Trade-Off in Perovskite Light-Emitting Diodes0

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  4. Interplay of Structure, Charge‐Carrier Localization and Dynamics in Copper‐Silver‐Bismuth‐Halide Semiconductors

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  48. Intrinsic Limits of Charge Carrier Mobilities in Layered Halide Perovskites

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