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RESEARCH PAPER · Accounts of Materials Research · 2021

Expanding the Toolbox of Inorganic Mechanoluminescence Materials

Bing Chen, Xin Zhang, Feng Wang

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Expanding the Toolbox of Inorganic Mechanoluminescence MaterialsOriginalSynergistic defect engineering and microstructure tuning in lithium tantalate for high-contrast mechanoluminescence of Bi 3+ : toward application for optical information display28Stimuli responsive lanthanide ions doped layered piezophotonic microcrystals for optical multifunctional sensing applications91High-security anti-counterfeiting through upconversion luminescence240Effective Repeatable Mechanoluminescence in Heterostructured Li1−xNaxNbO3: Pr3+81Mechanoluminescence spectrum tuning from zinc sulfide and all-inorganic perovskite quantum dots composite8Recent Advances in Mechanoluminescence of Doped Zinc Sulfides123New mode of stress sensing in multicolor (Ca1-Sr )8Mg3Al2Si7O28:Eu2+ solid-solution compounds27Organometallic Complexes for Optoelectronic Applications1Properties of Photoluminescence and mechanoluminescence of KxNa1–xNbO3:Pr3+ ferroelectric4Ternary-Host and Heterojunction Enabled Eye-Visible Elastic Mechanoluminescence from (Ca0.5Sr0.5)ZnOS/xZnS/Mn2+19Doubly Doped BaZnOS Microcrystals for Multicolor Luminescence Switching31Design of Ratiometric Dual‐Emitting Mechanoluminescence: Lanthanide/Transition‐Metal Combination Strategy63Molten Salt Shielded Synthesis of Monodisperse Layered CaZnOS‐Based Semiconductors for Piezophotonic and X‐Ray Detection Applications56Interface synergistic effects induced multi-mode luminescence43Mechanism of the Luminescence Enhancement of SrSi2N2O2:Eu2+ Phosphor via Manganese Addition6Sensitive mechanoluminescence from Eu2+, Tm3+ co-doped Sr3Al2O5Cl2 phosphors21Ultrasound-Activated Persistent Luminescence Imaging and Bacteria-Triggered Drug Release for Helicobacter pylori Infection Theranostics44Delayed stress memory by CaAl2O4:Eu2+ mechanoluminescent phosphor with defect engineering regulation57Recent advances in cellular optogenetics for photomedicine25Self‐Charging Persistent Mechanoluminescence with Mechanics Storage and Visualization Activities103Alkaline‐Earth‐Metal‐Ions Blending Enhanced Self‐Activated and Bi3+‐Activated Mechanoluminescence from Ca1‐xBaxZnOS45Soft Human–Machine Interface Sensing Displays: Materials and Devices62Palette of Rechargeable Mechanoluminescent Fluids Produced by a Biomineral-Inspired Suppressed Dissolution Approach84Recent Development in Sensitizers for Lanthanide-Doped Upconversion Luminescence215An interactive mouthguard based on mechanoluminescence-powered optical fibre sensors for bite-controlled device operation201From single molecule to molecular aggregation science105Ratiometric Mechanoluminescence of Double‐Activator Doped Phosphatic Phosphors: Color‐Resolved Visualization of Stress‐Sensing and Quantified Evaluation for Sensing Performance58Persistent Luminescence in Strontium Aluminate: A Roadmap to a Brighter Future172Mechanoluminescence ratiometric thermometry via MgF 2 :Tb 3+17Self-recoverable near-infrared mechanoluminescence from ZnS:Mn by controlling manganese clusterization17Mechanically excited thermometry in erbium ions14Unrevealing Temporal Mechanoluminescence Behaviors at High Frequency via Piezoelectric Actuation22Tunable and enhanced mechanoluminescence in LiYGeO 4 :Tb 3+ via Bi 3+ → Tb 3+ energy transfer33Alkaline-earth-metal-ion blending enhanced mechanoluminescence of lanthanide ions in MZnOS hosts for stress sensing and anticounterfeiting19Doping dependent dual-response mechanoluminescence in ZnGa 2 O 418Energy focusing reinforced narrowband ultraviolet-B mechanoluminescence for bright-field stress visualization21Light storage perovskites: Synthesis, mechanisms, and applications2Smart Semiconductor-Heterojunctions Mechanoluminescence for printable and wearable sports light sources47Strengthening the non-pre-irradiated near-infrared mechanoluminescence of CaZnOS:Nd 3+ by Mn 2+ coactivation for biomechanical imaging31Recoverable Dual-Modal Responsive Sensing Materials Based on Mechanoluminescence and Thermally Stimulated Luminescence toward Noncontact Tactile Sensors44Synchrotron X-ray powder diffraction under high pressures up to 33 MPa for mechanoresponsive materials7Mechanoluminescence Affected by Trap Types and Excitation State Positions in Mg3Ca3(PO4)4:Eu2+/Mn2+/Ce3+ for Multimode Anticounterfeiting14A flexible organic mechanoluminophore device46Stress‐Triggered Mechanoluminescence in ZnO‐Based Heterojunction for Flexible and Stretchable Mechano‐Optics70Mechano-luminescence Behavior of Lanthanide-Doped Fluoride Nanocrystals for Three-Dimensional Stress Imaging49Ultrasound‐Induced Luminescence from Cr3+‐Doped ZnGa2O4 Glass–Ceramic Composites9Mechanically induced photons from ultraviolet-C to near-infrared in Tm3+-doped MgF28A broadband near-infrared nanoemitter powered by mechanical action110Opportunities and Challenges in Applying Solid‐State NMR Spectroscopy in Organic Mechanochemistry38Distributed Strain Sensor Based on Self‐Powered, Stretchable Mechanoluminescent Optical Fiber43Flexible composite material for self-powered applications via triboelectricity and mechanoluminescence: PDMS/ZnS:Cu composites78Mechanical force induced luminescence ratiometric thermometry in CaZnOS:Dy 3+9Unraveling Mechanoluminescent Mechanisms in Doped CaZnOS Materials: Co‐Mediation of Trap‐Controlled and Non‐Trap‐Controlled Processes55Ultrasound-Chargeable Persistent Luminescence Nanoparticles to Generate Self-Propelled Motion and Photothermal/NO Therapy for Synergistic Tumor Treatment67Calcination-Induced Transformation of ZnS:Mn2+ Nanorods to Microparticles for Enhanced Mechanoluminescence35Design and integration of electronic display textiles16Beyond External Light: On-Spot Light Generation or Light Delivery for Highly Penetrated Photodynamic Therapy57Soft devices empowered by mechanoluminescent materials21SrAl2O4:Eu2+,Dy3+ Long Afterglow Phosphor and Its Flexible Film for Optomechanical Sensing Application31Luminescence properties of a green-emitting mechanoluminescent phosphor CaSrGa 4 O 8 : x Tb 3+ without pre-excitation12Mechanoluminescence for display devices1Mechanoluminescence for electronic skins and wearable devices1Mechanoluminescence in anticounterfeiting0Other emerging applications of mechanoluminescence and outlook1Spontaneous Symmetry Breaking of Achiral Molecules Leading to the Formation of Homochiral Superstructures that Exhibit Mechanoluminescence3Spontaneous Symmetry Breaking of Achiral Molecules Leading to the Formation of Homochiral Superstructures that Exhibit Mechanoluminescence29Self-Reinforced Piezoelectric Response of an Electroluminescent Film for the Dual-Channel Signal Monitoring of Damaged Areas7Bright Circularly Polarized Mechanoluminescence from 0D Hybrid Manganese Halides101Mechanoluminescent functional devices: Developments, applications and prospects92Focused Ultrasound‐Responsive Nanocomposite with Near‐Infrared II Mechanoluminescence for Spatiotemporally Selective Immune Activation in Lymph Nodes13All‐Lanthanide Mechanoluminescence from Transparent Ln‐doped MgF2@Elastomer for Flexible and Stretchable Lighting and Stress Sensing12Ultraviolet-C mechanoluminescence from NaYF4:Pr3+17The Impact of the Amorphous-to-Crystalline Transition on the Upconversion Luminescence in Er3+-Doped Ga2O3 Thin Films7A promising route for developing green phosphor with mechanoluminescence and long persistent luminescence in Sr2Ga2GeO7: Tb3+12Thermally recovered mechanoluminescence in Ca 6 BaP 4 O 17 :Eu 2+2Quantifying the interfacial triboelectricity in inorganic-organic composite mechanoluminescent materials116Theoretical understanding of defects-driven mechanoluminescence for Pr3+-doped NaNbO3/LiNbO3 heterojunctions15Self‐Recoverable, Highly Repeatable, and Thermally Stable Mechanoluminescence for Dual‐Mode Information Storage and Photonic Skin Applications71A Review of Mechanoluminescence Based on Quaternary Oxysulfides: Research Progress, Mechanism and Applications14Awakening dumb Mn2+ mechanoluminescence site to achieve force, temperature and time-domain induced color tuning via trap-assisted energy transfer14Efficient synthesis of quaternary piezo-photonic materials for pressure visualization and E-signature anti-counterfeiting14Crystal structure, theoretical calculations, mechanoluminescence feature and antimicrobial activity based on a double-armed Salamo-type ligand and its trinuclear Cu(Ⅱ) complex19Mechanoluminescence from CaCl2:Eu2+1Pushing Trap‐Controlled Persistent Luminescence Materials toward Multi‐Responsive Smart Platforms: Recent Advances, Mechanism, and Frontier Applications124Enabling Multimodal Luminescence in a Single Nanoparticle for X-ray Imaging Encryption and Anticounterfeiting49Mechanically Triggered Bright Chemiluminescence from Polymers by Exploiting a Synergy between Masked 2-Furylcarbinol Mechanophores and 1,2-Dioxetane Chemiluminophores35Unlocking the Potential of Organic‐Inorganic Hybrid Manganese Halides for Advanced Optoelectronic Applications171Scale-Bridging Mechanics Transfer Enables Ultrabright Mechanoluminescent Fiber Electronics8Broadband near-infrared mechanoluminescence in Cr3+ doped Mg3Ga2GeO839Design of Visualized Ratiometric Mechanoluminescent Materials for High‐Resolution Pressure Sensing35Simultaneous Triboelectric and Mechanoluminescence Sensing Toward Self‐Powered Applications14Deeply trapped electrons induced long-time sustainable mechanoluminescence of X-ray irradiated La2Ti2O7:Pr3+ for detection of stress burst6Exploring Mechanoluminescence of Zinc Alkaline Earth Metal Oxysulfides from Fundamentals to Advanced Applications26Piezoelectric-induced mechanoluminescence in centrosymmetric Lu3Al5O12: Properties of self-recoverable and tunable near-infrared luminescence19Interfacial dipole moment engineering in self-recoverable mechanoluminescent platform15Self‐Recoverable and NIR‐I to NIR‐II Tunable Broadband Mechanoluminescence of Cr 3+ ‐Doped Antimonate Double Perovskites52Analysis of wireless powering modes for nanotransducer-mediated neuromodulation2Synthesis of SrZnOSe Crystals with Low Phonon Energy for Enhancing Near‐Infrared Mechanoluminescence42Visualization of strain rate based on mechanoluminescence tailing10Towards White Light Emission Through Metal‐to‐Metal Charge Transfer (MMCT) Effect in Bi3+ Activated Ca2YTi2‐mZrmGa3O12 (0≤m≤2) Garnets8Luminescent Tactile Sensor System for Robots: Enhancing Human–Computer Interaction in Complex Dark Environments11Biphasic structure construction based on a piezoelectric semiconductor for enhancing mechanoluminescent performance4Correlation between persistent luminescence and mechano-luminescence of Sm 3+ -doped YPO 44Excitation-mode-selective emission through multiexcitonic states in a double perovskite single crystal83Flexible mechano-optical sensors from mechanoluminescence to mechanoplasmonics: designs, applications, and prospects15Intense and repeatable orange mechanoluminescence of Mn 2+ activated CaGa 4 O 7 for visualized mechanics sensing7Mechanoluminescent-energy harvesting bimodal sensors for self-powered communication sensors6Novel multi-stimulus responsive mechanoluminescent phosphor Ca 5 Ga 6 O 14 :Pr 3+ ,Yb 3+ ,Er 3+ for dynamic multi-mode anti-counterfeiting1Innovations in phosphate phosphors: Bridging structure-property gaps for enhanced luminescence27Stress Distributions and Luminescent Responses of Mechanoluminescent Cylinders with Various Sizes and Loading Paths2Mechanoluminescence from Organic–Inorganic Metal Halide Perovskite Derivative20Tuning mechanoluminescence colors from aromatic imides with dyes0A self-recoverable mechano-photonic phosphor for high-level anti-counterfeiting8Daylight-activated recoverable mechano-luminescence material SrGa12O19: Tb3+ for enhanced speed detection applications2Force‐Triggered Non‐Volatile Multilevel Mechano‐Optical Memory System for Logic Computation and Image Recognition15Self-recoverable Ca5Ga6O14:Eu³⁺-ZnS:Cu mechanoluminescent composite for visualized stress and temperature sensing3Conformation Dependent Room Temperature Phosphorescence in Organic Materials10Mechanoluminescence ZnS/CaZnOS:Mn2+/PVC composite film-based triboelectric nanogenerator for energy harvesting and intelligent sensing19Trap‐Assisted Mechanoluminescence in Mn 2+ ‐Doped Transparent Amorphous Glass for Potential Stress Sensing3Stimulus-responsive alternating current electroluminescent textiles for visual human-machine interface8High-Efficiency Organic Mechanophosphorescence from A Phenoselenazine Phosphor for Multiple Applications21Multimodal Stimuli‐Responsive Luminescence and Photochromism of Cr 3+ ‐Doped Gallate β‐Alumina38Mechano‐Chemiluminescent Hydrogel for Sustained Stress Visualization Under Mechanical Equilibrium9Ultrasound‐Stimulated Luminescence from Mn2+‐Activated Crystal‐Free Germanate Glasses Charged by Sunlight2Exploring stimuli‐responsive luminescence in metal halide perovskites for emerging applications17Multi-stimulated far-UVC luminescence for solar-blind imaging30Incorporation of triboluminescence in solid lubricating composite for surface texture monitoring0Aliovalent doping strategy toward band structure modulation and enhanced mechanoluminescence of CaZnOS: Mn2+4Bright Chromium‐Sensitized Lanthanide NIR‐II Mechanoluminescence in a Piezoelectric Oxide20Preparation of Y3Ga5O12: Eu3+ garnet phosphors and study of their mechanoluminescence properties3Interfacial Interaction Modulated Radiation Defects for Self‐Charging Persistent Mechanoluminescence10Mechanoluminescence of ZnS Under Easily Tailored Phase Transitions23Concurrently bright photoluminescence and mechanoluminescence in helical chain-like Eu(III) coordination polymers5Mechanoluminescence: Mechanisms, emerging applications, and future prospects26Self‐Charging Near‐Infrared Mechano‐Afterglow in Cr 3+ Activated Composites5Enhancing Mn‐Activated Mechanoluminescence via Pressure‐Regulated Local Structure in Centrosymmetric BaZnOS for Dynamic Response Applications3Controllable Synthesis of Gradient α/β-ZnS:Cu for Revealing the Mechanoluminescent Mechanisms6Visually encoded mechanoluminescence through hierarchical structuring with microscale patterns and nanoscale features7A Self‐Powered Tactile Sensor Resistant to Environmental Interference22Smart Semiconductors: An Overview of AZnOS (A= Ca, Sr, Ba) Based Phosphors, Multi‐Stimuli Responsive Luminescence, and Potential Application Prospects12Minimizing barriers to efficient mechanoluminescence via polymer matrix integration7Recent Progress in Mechanoluminescence for Multi‐Dimensional Stress Monitoring6Supramolecular Mechanoluminescence via Fluorine Interactions6Supramolecular Mechanoluminescence via Fluorine Interactions3Chromium-activated phosphors: from theory to applications23Mechanoluminescent Probing of Elastic Moduli in CaZnOS:Mn 2+ , Bi 3+ Composites: Effects of Matrix Modulus and Filler Loading0Bifunction two-armed salamo-type complexes of Cu(II) and Zn(II) with fluorescent and antibacterial properties1Mechanoluminescent materials: toward advanced optoelectronic sensing and biomedical applications0Enhanced mechanoluminescence in Pr3+-doped LiNbO3-LiTaO3 ferroelectric phosphors0A Review of Flexible Mechanics Mapping: The Sensing, Transmission, Computation, and Integration Paradigm11

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  4. Effective Repeatable Mechanoluminescence in Heterostructured Li1−xNaxNbO3: Pr3+

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  5. Mechanoluminescence spectrum tuning from zinc sulfide and all-inorganic perovskite quantum dots composite

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  34. Alkaline-earth-metal-ion blending enhanced mechanoluminescence of lanthanide ions in MZnOS hosts for stress sensing and anticounterfeiting

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  35. Doping dependent dual-response mechanoluminescence in ZnGa 2 O 4

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  36. Energy focusing reinforced narrowband ultraviolet-B mechanoluminescence for bright-field stress visualization

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  39. Strengthening the non-pre-irradiated near-infrared mechanoluminescence of CaZnOS:Nd 3+ by Mn 2+ coactivation for biomechanical imaging

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  42. Mechanoluminescence Affected by Trap Types and Excitation State Positions in Mg3Ca3(PO4)4:Eu2+/Mn2+/Ce3+ for Multimode Anticounterfeiting

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  43. A flexible organic mechanoluminophore device

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  45. Mechano-luminescence Behavior of Lanthanide-Doped Fluoride Nanocrystals for Three-Dimensional Stress Imaging

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  46. Ultrasound‐Induced Luminescence from Cr3+‐Doped ZnGa2O4 Glass–Ceramic Composites

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  47. Mechanically induced photons from ultraviolet-C to near-infrared in Tm3+-doped MgF2

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  48. A broadband near-infrared nanoemitter powered by mechanical action

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