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RESEARCH PAPER · ACS Sustainable Chemistry & Engineering · 2021

A High Efficiency Trivalent Chromium-Doped Near-Infrared-Emitting Phosphor and Its NIR Spectroscopy Application

Yunpeng Zhou, Xinjuan Li, Takatoshi Seto, Yuhua Wang

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A High Efficiency Trivalent Chromium-Doped Near-Infrared-Emitting Phosphor and Its NIR Spectroscopy ApplicationOriginalA novel Cr 3+ -doped Lu 2 CaMg 2 Si 3 O 12 garnet phosphor with broadband emission for near-infrared applications136Cr 3+ -activated Na 3 X 2 Li 3 F 12 (X = Al, Ga, or In) garnet phosphors with broadband NIR emission and high luminescence efficiency for potential biomedical application124Design of highly efficient deep-red emission in the Mn 4+ doped new-type structure CaMgAl 10 O 17 for plant growth LED light22Abnormal Self-Reduction Phenomenon of Europium-Doped Borate and Its Luminescence Properties26A General Ammonium Salt Assisted Synthesis Strategy for Cr3+‐Doped Hexafluorides with Highly Efficient Near Infrared Emissions212A Highly Efficient Eu2+ Excited Phosphor with Luminescence Tunable in Visible Range and Its Applications for Plant Growth66Ultra-broadband NIR luminescence in chromium doped magnesium aluminosilicate glass as future light sources for spectroscopy applications25Design of efficient color-tunable long persistent luminescence phosphor BaGa 2 O 4 :Pr 3+ and its performance enhancement via a trap-induced strategy56A new broadband near-infrared emitting Mg 2 Al 4 Si 5 O 18 :Cr 3+ phosphor for night-vision imaging29Cr 3+ -Doped InTaO 4 phosphor for multi-mode temperature sensing with high sensitivity in a physiological temperature range78Efficient and thermally stable broadband near-infrared emission in a garnet Gd 3 In 2 Ga 3 O 12 :Cr 3+ phosphor44Energy-saving chromium-activated garnet-structured phosphor-converted near-infrared light-emitting diodes73Enhancing the luminescence performance of Ca 2− x Sr x BO 3 Cl:Eu 2+ ,Dy 3+ by substitution of Sr 2+ for Ca 2+9Investigation on the Luminescent Property and Application of In2BP3O12:Cr3+ Broadband Near-Infrared Phosphor※8The Near-Infrared Luminescence Properties and Applications of Ca3lu2ge3o12: Cr3+ Phosphor29Crystal structure and optical performance analysis of a new type of persistent luminescence material with multi-functional application prospects21Broadband NIR Garnet Phosphors with Improved Thermal Stability via Energy Transfer49Novel broadband near-infrared emitting phosphor LiGe2(PO4)3:Cr3+ with tuning and enhancement of NIR emission by codoping Sb5+49Photoluminescence Properties of AScSi 2 O 6 :Cr 3+ (A = Na and Li) Phosphors with High Efficiency and Thermal Stability for Near-Infrared Phosphor-Converted Light-Emitting Diode Light Sources175Crystal‐Field Engineering Control of an Ultraviolet–Visible‐Responsive Near‐Infrared‐Emitting Phosphor and Its Applications in Plant Growth, Night Vision, and NIR Spectroscopy Detection123Novel one-dimensional Ga2O3:Cr3+ nanofibers with broadband emission for near infrared LED sources13Chromium(III)-Doped Phosphors of High-Efficiency Two-Site Occupation Broadband Infrared Emission for Vessel Visualization Applications32Cr3+/Yb3+/Nd3+-doped Ba2LaGa11O20 broadband NIR phosphors for NIR pc-LED and c-Si solar cells10Rapid Nondestructive Detection Enabled by an Ultra‐Broadband NIR pc‐LED137Efficient and broadband near-infrared emission of Cr3+-doped glass-ceramics for near-infrared light sources applications26Pressure-triggered enormous redshift and enhanced emission in Ca2Gd8Si6O26:Ce3+ phosphors: Ultrasensitive, thermally-stable and ultrafast response pressure monitoring128Enhancement of Near‐Infrared Phosphor Luminescence Properties via Construction of Stable and Compact Energy Transfer Paths54Manipulating Upconversion Emission and Thermochromic Properties of Ho3+/Yb3+-Codoped Al2Mo3O12 Microparticles by Negative Lattice Expansion for Multimode Visual Optical Thermometry79Near-Infrared Broadband ZnTa2O6:Cr3+ Phosphor for pc-LEDs and Its Application to Nondestructive Testing64Spectral Regulation and Efficiency Optimization in Cr3+‐Doped Gadolinium Aluminum Gallium Garnet Near‐Infrared Ceramic Phosphors via Crystal‐Field Engineering29Broadband near-infrared luminescence in the NaAlP2O7:Cr3+ phosphor for spectroscopy applications19Thermally Robust Broadband Near-Infrared Luminescence in the NaGaP2O7:Cr3+ Phosphor23Highly Efficient Broadband Near-Infrared Luminescence with Zero-Thermal-Quenching in Garnet Y3In2Ga3O12:Cr3+ Phosphors185Multiple Coordination of Chromium Ion Luminescence: A Strategy for Designing Ultra-broadband NIR Long Persistent Luminescent Materials49Efficient and Thermally Robust Broadband Near‐Infrared Emission in a Garnet Ca 3 MgHfGe 3 O 12 :Cr 3+ Phosphor48Recent Advances in Chromium‐Doped Near‐Infrared Luminescent Materials: Fundamentals, Optimization Strategies, and Applications252Highly efficient and thermally stable broadband NIR phosphors by rationally bridging Cr 3+ –Yb 3+ in LiScGe 2 O 6 for optical bioimaging69Achieving Persistent Luminescence Performance Based on the Cation-Tunable Trap Distribution3An efficient and thermally stable Cr 3+ -activated Y 2 GdSc 2 Al 2 GaO 12 garnet phosphor for NIR spectroscopy applications14An efficient and thermally stable near-infrared phosphor derived from the Ln 3 ScInGa 3 O 12 :Cr 3+ (Ln = La, Gd, Y, and Lu) garnet family18Design of highly efficient energy transfer phosphor Sr 4 Al 14 O 25 :Eu 2+ ,Mn 4+ with deep-red emission and application potential in plant growth11Non-destructive food-quality analysis using near-infrared luminescence from Mg 3 Gd 2 Ge 3 O 12 :Cr 3+32Understanding the broadband near-infrared luminescence in a highly distorted garnet Ca 4 HfGe 3 O 12 :Cr 3+ phosphor36Preparation of novel KAlSiO4: Ce3+ broadband cyan-emitting phosphors via partial cation substitution for applications in white-light LEDs20La3Ga5SiO14:Cr3+: A broadband near-infrared phosphor induced by the two-site occupation of Cr3+43Enhanced and Broadened NIR Emission of CaZnGe2O6:Cr3+ by Yb3+ Codoping for NIR Applications11High-performance Gd3Al4GaO12:Cr3+ phosphors for next-generation far-red LEDs18Luminescence enhancement of Cr3+ doped garnet phosphor for high-performance LED towards smart NIR light source47The co-optimization of efficiency and emission bandwidth in GSAGG:Cr3+ NIR ceramic phosphors19LiGaP2O7:Cr3+, Yb3+ phosphors for broadband NIR LEDs toward multiple applications44Modification of the green CSS:Ce3+ phosphor by ion substitution for obtaining an orange phosphor for white LEDs4Continuous Ultra‐Broadband Near‐Infrared Sc2O3‐Based Nanophosphor Realized by Spectral Bridge of Cr3+‐Yb3+‐Cr4+ for Multiple Optical Applications44The Upconversion Luminescence of Ca3Sc2Si3O12:Yb3+,Er3+ and Its Application in Thermometry20Chromium Doped Glasses for Photonic Applications: A Brief Review and Prospects5Upconversion NIR luminescence negative thermal quenching and temperature sensing in LiYGeO4:Yb3+/Nd3+ phosphors21Achieving Broadband NIR-I to NIR-II Emission in an All-Inorganic Halide Double-Perovskite Cs2NaYCl6:Cr3+ Phosphor for Night Vision Imaging107Cr3+-activated NaInSi2O6: An efficient broadband near-infrared phosphor with its applications in LED22Selective enrichment strategy induces ultra-broadband NIR emission in Cr3+-doped multi-phase glass-ceramics for NIR spectroscopy applications10Multifunctional near-infrared Zn2TiO4:Cr3+ phosphors for luminescence, thermometry, and plant cultivation24Six‐ and five‐coordinated Cr 3+ in Ga 2 GeO 5 invokes tunable broadband near‐infrared emission toward night‐vision applications61How to Achieve Excellent Luminescence Properties of Cr Ion‐Doped Near‐Infrared Phosphors103A novel co-substitution strategy to enhance the luminescence performance of Zn2TiO4:Cr3+ phosphor5Crystal structure, morphology and enhancement of luminescence properties of Cr3+-doped KZnF3 phosphor by using a HF-free hydrothermal method with different chromium sources3Unveiling the Potential of Sunlight‐Driven Multifunctional Blue Long Persistent Luminescent Materials via Cutting‐Edge Trap Modulation Strategies24A novel broadband near-infrared phosphor Ca3MgTiGe3O12:Cr3+12Novel YAGG: Cr garnet phosphor ceramic with broadband near infrared (NIR) emission and luminescence thermal stability for plant growth27Sr2(Ga/Al)TaO6:Cr3+ phosphor with tunable near-infrared emitting for light-emitting diodes and optical thermometer32Cr 3+ ‐Cr 3+ Ion Pair Induced Fast Energy Migration in Cr 3+ Doped Na‐β‐Al 2 O 3 Ultra‐Wide Near‐Infrared Phosphors for NIR Spectroscopy Application72A novel broadband near‐infrared Ca 2 Y 3 Sb 3 O 14 : Cr 3+ rhombohedral pyrochlores phosphor and its application in pc‐LEDs12High external quantum yield in near-infrared phosphor Bi2Ga4O9:Cr3+ excited by near-ultraviolet or blue light9Achieving spectrally tunable and thermally stable near-infrared emission in Fe 3+ -activated spinel phosphors via the cation site modulation strategy34Broadband Ca 3 MgZrGe 3 O 12 :Cr 3+ garnet phosphor for high-performance NIR pc-LED application14Crystal-field regulation enables broadband-to-line emission switching in Cr 3+ -activated pyroxenes15Long wavelength near-infrared II emitting Na3YSi3O9:x Cr3+ silicate and spectral broadening by multi-site occupancy0Modulation of the near-infrared-I and -II luminescence of thulium-incorporated lead-free double perovskites10Tailoring Emission Characteristics of Na-Sc Co-Substituted Camgge2o6:Cr3+ Phosphors for Iris Acquisition0Remote Control and Noninvasive Detection Enabled by a High-performance NIR pc-LED20Multisite Fine‐Tuning in Hybrid Cadmium Halides Enables Wide Range Emissions for Anti‐Counterfeiting6Multisite Fine‐Tuning in Hybrid Cadmium Halides Enables Wide Range Emissions for Anti‐Counterfeiting92Comprehensive Review on Downconversion/Downshifting Silicate-Based Phosphors for Solar Cell Applications21Ce3+ and Cr3+ co-activated ultra-wide visible-NIR garnet phosphor for phosphor-converted light emitting diode9Developing the Na2CaZr2Ge3O12:Cr3+ Garnet Phosphor for Advanced NIR pc-LEDs in Night Vision and Bioimaging87Near‐Infrared Luminescent Materials Incorporating Rare Earth/Transition Metal Ions: From Materials to Applications173Highly thermally stable SrLaMgTaO6: Cr3+ double-perovskite phosphors for night-vision applications23Ultra-broadband near-infrared emission of Cr3+-containing oxy-fluoride glass-ceramics29High quantum efficiency broadband near-infrared LaTiSbO6:Cr3+ phosphors10Simultaneously strong NIR-II and NIR-III luminescence induced by Cr3+-Yb3+-Er3+ energy transfer in KScP2O7 for NIR thermometry, NIR pc-LED and night-vision applications14Unlocking Chlorine Oxide‐Based Ultra‐Wideband Near‐Infrared Phosphor and Advancing Spectral Performance via Lattice Engineering43Tailoring emission characteristics of Na+-Sc3+ co-substituted CaMgGe2O6:Cr3+ phosphors for iris acquisition7Highly thermal-stable broadband near-infrared emission of Cr3+ doped spinel CdGa2O4 phosphors17The highly efficient and stable near-infrared phosphor Ca3MgSnGe3O12: Cr3+ for multifunctional application10Achieving a Balance of Good Quantum Efficiency and Thermal Stability in the Y2CaScAl3GeO12:Cr3+ Broadband Phosphor for Multiple NIR Spectroscopy Applications17Full-Visible-Spectrum White LEDs Enabled by a Blue-Light-Excitable Cyan Phosphor136Efficient and Thermally Stable Cr3+‐Doped Phosphor Achieved by Cation Substitution: Plant Lighting Application37Investigation of preparation and photoluminescence properties of europium-doped calcium orthoborate (Ca3B2O6:Eu3+) red phosphor and red LED37Red-shifting and boosting the emission of NaScP2O7:Cr3+ via efficient energy transfer for information encryption and anti-counterfeiting5Tunable Broadband NIR-II Emission via Cr 4+ -Er 3+ Energy Transfer in CaMgGeO 4 :Cr 4+ ,Er 3+ Phosphors for Nondestructive Analysis16A Cr3+-triggered near-infrared tungstate phosphor for organic compound non-destructive detection14Efficient Near‐Infrared Luminescence in Cr 3+ Activated β ‐Alumina Structure Phosphor via Multiple‐Sites Occupancy17Synthesis of a novel broadband near-infrared fluoride phosphor with nearly 100% internal quantum efficiency using a cationic substitution strategy13Unique Spectral Broadening Induced by Exchange Coupling Between Cr 3+ Ions in LiAl 5 O 8 :Cr 3+ Phosphors for Versatile Optical Applications44A Novel Multifunctional and Broadband Near‐Infrared Phosphor, Lu 3 MgGa 3 GeO 12 :Cr 3+ , Yb 3+ , Nd 3+ Achieved through a Chemical Unit Substitution and Energy Transfer Strategy23Anti-thermal quenching upconversion luminescence of Cr 3+ in Sc 2 (WO 4 ) 3 :Yb/Cr7Ca2+/Si4+ Modification of the (Gd,Lu)AG Garnet for Enhanced Broadband Cr3+ Luminescence of High Thermal Stability13Achieving high-performance far-red emission in Cr 3+ -activated garnet phosphors via Ca 2+ /Zr 4+ doping toward plant lighting5Constructing Efficient and Thermally-Stable Far Red Emitting Phosphor with Excellent Responsive To Phytochrome Pfr For Indoor Agriculture0Far-red emitting phosphors for plant growth applications: fitted and enhanced via cation substitution of Gd 3+4Hierarchical Symbolic Regression Modeling and Physical Mechanism Study of Stokes Shift of Cr³⁺-Activated Double Perovskite Phosphors0Highly Efficient Broadband Nir Emission of Cr3+- Activated Znwo4 Phosphors and Their Application in Phosphor-Converted Leds0Oxygen Vacancy-Engineered Cr3+:Ca2lanbo6 Glass-Ceramics Via Controlled Crystallization: Dual Enhancement of Photoluminescence and Magnetism0A cationic substitution strategy was employed to synthesize phosphor K2NaIn1-xAlxF6: Cr3+, Mn4+ with enhanced optical properties and thermal stability18Dual-emissive Bi3+, Cr3+ Co-doped K2LiGaF6 phosphors: Achieving white and near-infrared light for innovative applications in food detection and bio-imaging10CaLu 2 Sc 2 Al 2 SiO 12 :Ce 3+ Green Phosphors for High-Quality White LEDs31Constructing Broadband Near‐Infrared Garnet Emitters CaGd 2 Ga 4 SiO 12 :Cr 3+ with Unity Quantum Efficiency and High Thermal Stability for Versatile Applications72Tunable NIR Emission of Cr3+-Activated Double-Perovskite Tantalates and Improvement of Luminescence Properties via Codoping Yb3+11Fe3+-activated BaZrO3 with broadband NIR-II phosphor for large-area Illumination, non-visual and biomedical imaging24Accessing energy-efficient broadband near-infrared luminescence in Cr3+-doped disordered garnet with near-zero thermal quenching and an EQE of 50.26 %9Efficient and thermally stable Cr3+-activated germanate phosphor for thermometry, plant cultivation, and near-infrared light-emitting diode applications19Preparation and luminescent properties of chromium ion doped aluminum borate near-infrared phosphor (Al18B4O33: Cr3+) and its application of broadband near-infrared LED17Broadband near-infrared long persistent luminescence in Cr3+-Doped CaY2Ga4GeO12 phosphors for advanced light source applications4Efficient Ba2NaNb5O15:Cr3+,Yb3+ nanocrystals embedded transparent glass-ceramics toward night-vision application7Near-unity quantum efficiency and remarkable anti-thermal quenching of Cr3+-activated Gd3AlGa4O12 garnet emitter for advanced broadband NIR light source5Oxygen vacancy-engineered Cr³ ⁺:Ca₂LaNbO₆ glass-ceramics via controlled crystallization: Dual enhancement of photoluminescence and magnetism2Achieving near-unity efficiency and exceptional stability luminescence in Ca3Sc2Ge3O12: Cr3+, Si4+ phosphor through ion exchange and flux doping strategies for NIR spectroscopy applications2High-efficiency NIR luminescence of SrGe4O9:Cr3+ induced by charge compensation with lithium-ions and demonstration of its potential application1Tunable NIR emission in Cr3+ activated (La,Gd)Sc3(BO3)4 based on host crystal engineering strategy6High-sensitivity optical thermometry via dual-emissive Tb3+-Eu3+ in Y2MgAl4SiO12 phosphor10Highly efficient wide-spectrum green Y2BaScAl3SiO12:Ce3+ phosphor for advanced white LEDs applications5In Situ Transformation of Electrum Nanoclusters Embedded in Polymer Matrices Exhibit Near‐Infrared Emission With Quantum Yield Exceeding 70%8Unlocking novel halogen germanate phosphors for full-spectrum lighting and ultra-sensitive temperature sensing7Inducing B-site distortion in Gd3Sc1.5In0.5Ga3O12 garnet to accommodate Cr3+ ions: achieving high quantum efficiency and thermally stable broadband NIR phosphors for NIR spectroscopy applications9Excitation enhanced and tuned in Cs2KGaF6: Cr3+, Mn4+ with significantly improved EQE applied for NIR pc-LEDs3Heterovalent Substitution of K2SrP2O7:Cr3+ to Achieve Anti-Thermal-Quenching Broadband Near-Infrared Luminescence9Highly-efficient near-infrared emission from Cr3+ activated LaMgAl11O19 phosphor toward optical thermometer and pc-LED applications8Cr3 + -Cr3+ ion pair and crystal field engineering in magnetoplum type NIR-emitting phosphor for spectroscopic applications3Broadband and High Efficiency Near‐Infrared Emission in Cr 3+ ‐Doped ZnWO 4 Phosphors for Spectroscopic Applications5Structure and luminescence of Gd3Ga3MgSiO12:Cr3+ garnet phosphor with highly efficient broadband near-infrared emitting toward pc-LED application7Synthesis, optical properties and warm white LED applications of dysprosium ion (Dy3+)- activated barium orthoborate yellow phosphors9Comparative Study of Cr 3+ -Activated Garnet Ca 2 YZnMGe 3 O 12 (M = Sc, In) Phosphors: Ultraefficient Near-Infrared Luminescence and Structure–Property Relationships1Effects of Al/Ga ratio and Ce3+/Cr3+ Co-doping on the structural and luminescent properties of Z(A,G)GO:Ce3+,Cr3+ phosphors1Constructing efficient and thermally-stable far red emitting phosphor with excellent response to phytochrome Pfr for indoor agriculture5Hierarchical symbolic regression modeling and physical mechanism study of Stokes shift of Cr3+-activated double perovskite phosphors4Simultaneous emission and thermal stability enhancement of long-wavelength NIR luminescence of Cr 3+ ions in spinel phosphors via pivot-polyhedron linkage engineering4Multi-functional NIR phosphors based on peak position and bandwidth modulation via Cr3+-Cr3+ ion pairs5Excitation-Dependent Photoluminescence of Undoped Bimetallic Halides with Dual Emitting Centers for Optical Anticounterfeiting Application7Efficient and thermal stable broadband near-infrared emitting Gd2CaAl3GaZrO12:Cr3+ garnet phosphor: structure, luminescence, and pc-LED application9Progress in gallium oxide phosphors: synthesis, characteristics, and versatile application1Synchronously broadening excitation range and enhancing NIR emission intensity of Er3+ in CaLaGaO4 via energy transfer from Cr4+ for popularization of Er3+ lasers30Achieving High-Efficiency Near-Infrared Luminescence in LiScSi2O6:Cr3+ through In3+/Yb3+ Co-Doping and Its Application Exploration0Achieving High-Efficiency Near-Infrared Luminescence in LiScSi2O6:Cr3+ through In3+/Yb3+ Co-Doping and Its Application Exploration0

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  2. Cr 3+ -activated Na 3 X 2 Li 3 F 12 (X = Al, Ga, or In) garnet phosphors with broadband NIR emission and high luminescence efficiency for potential biomedical application

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  3. Design of highly efficient deep-red emission in the Mn 4+ doped new-type structure CaMgAl 10 O 17 for plant growth LED light

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  4. Abnormal Self-Reduction Phenomenon of Europium-Doped Borate and Its Luminescence Properties

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  5. A General Ammonium Salt Assisted Synthesis Strategy for Cr3+‐Doped Hexafluorides with Highly Efficient Near Infrared Emissions

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  32. Thermally Robust Broadband Near-Infrared Luminescence in the NaGaP2O7:Cr3+ Phosphor

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  33. Highly Efficient Broadband Near-Infrared Luminescence with Zero-Thermal-Quenching in Garnet Y3In2Ga3O12:Cr3+ Phosphors

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  34. Multiple Coordination of Chromium Ion Luminescence: A Strategy for Designing Ultra-broadband NIR Long Persistent Luminescent Materials

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  35. Efficient and Thermally Robust Broadband Near‐Infrared Emission in a Garnet Ca 3 MgHfGe 3 O 12 :Cr 3+ Phosphor

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  36. Recent Advances in Chromium‐Doped Near‐Infrared Luminescent Materials: Fundamentals, Optimization Strategies, and Applications

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  37. Highly efficient and thermally stable broadband NIR phosphors by rationally bridging Cr 3+ –Yb 3+ in LiScGe 2 O 6 for optical bioimaging

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  38. Achieving Persistent Luminescence Performance Based on the Cation-Tunable Trap Distribution

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  39. An efficient and thermally stable Cr 3+ -activated Y 2 GdSc 2 Al 2 GaO 12 garnet phosphor for NIR spectroscopy applications

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  40. An efficient and thermally stable near-infrared phosphor derived from the Ln 3 ScInGa 3 O 12 :Cr 3+ (Ln = La, Gd, Y, and Lu) garnet family

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  41. Design of highly efficient energy transfer phosphor Sr 4 Al 14 O 25 :Eu 2+ ,Mn 4+ with deep-red emission and application potential in plant growth

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  42. Non-destructive food-quality analysis using near-infrared luminescence from Mg 3 Gd 2 Ge 3 O 12 :Cr 3+

    Dalton Transactions · 2023-01-01

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  43. Understanding the broadband near-infrared luminescence in a highly distorted garnet Ca 4 HfGe 3 O 12 :Cr 3+ phosphor

    Physical Chemistry Chemical Physics · 2023-01-01

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  44. Preparation of novel KAlSiO4: Ce3+ broadband cyan-emitting phosphors via partial cation substitution for applications in white-light LEDs

    Ceramics International · 2023-01-30

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  45. La3Ga5SiO14:Cr3+: A broadband near-infrared phosphor induced by the two-site occupation of Cr3+

    Ceramics International · 2023-02-13

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  46. Enhanced and Broadened NIR Emission of CaZnGe2O6:Cr3+ by Yb3+ Codoping for NIR Applications

    ACS Applied Optical Materials · 2023-03-13

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  47. High-performance Gd3Al4GaO12:Cr3+ phosphors for next-generation far-red LEDs

    Materials Research Bulletin · 2023-03-15

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  48. Luminescence enhancement of Cr3+ doped garnet phosphor for high-performance LED towards smart NIR light source

    Ceramics International · 2023-04-05

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  49. The co-optimization of efficiency and emission bandwidth in GSAGG:Cr3+ NIR ceramic phosphors

    Ceramics International · 2023-04-05

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  50. LiGaP2O7:Cr3+, Yb3+ phosphors for broadband NIR LEDs toward multiple applications

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