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RESEARCH PAPER · Advanced Optical Materials · 2021

Photoluminescence of Singlet/Triplet Self‐Trapped Excitons in Sb3+‐Based Metal Halides

Yuyu Jing, Ying Liu, Mingze Li, Zhiguo Xia

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Photoluminescence of Singlet/Triplet Self‐Trapped Excitons in Sb3+‐Based Metal HalidesOriginalA deep-red-emission antimony( iii ) chloride with dual-cations: extremely large Stokes shift due to high [SbCl 6 ] distortion31An ultraviolet excitation anti-counterfeiting material of Sb 3+ doped Cs 2 ZrCl 6 vacancy-ordered double perovskite55Broadband light emitting zero-dimensional antimony and bismuth-based hybrid halides with diverse structures43Bulk assembly of a 0D organic antimony chloride hybrid with highly efficient orange dual emission by self-trapped states85Self-trapped exciton to dopant energy transfer in Sb 3+ -doped Cs 2 ZrCl 6 perovskite variants45Zero-dimensional Sb3+ doped Rb7Bi3Cl16 metal halides with triplet self-trapped exciton emission4Acentric Organic–Inorganic Hybrid Halide [N(CH3)4]2HgBr2I2 Featuring an Isolated [HgBr2I2]2– Tetrahedron and Second-Order Nonlinearity18Structural Dimensionality Modulation toward Enhanced Photoluminescence Efficiencies of Hybrid Lead‐Free Antimony Halides164Light-Emitting 0D Hybrid Metal Halide (C3H12N2)2Sb2Cl10 with Antimony Dimers38Realization of non-rare earth doped blue-emitting phosphor Ba2Y5B5O17: Sb by selective site excitation, and its application in n-UV excited wLEDs3Sb 3+ ‐Doping in Cesium Zinc Halides Single Crystals Enabling High‐Efficiency Near‐Infrared Emission370Crystalline‐Phase‐Recognition‐Induced Domino Phase Transition and Luminescence Switching for Advanced Information Encryption108Crystalline‐Phase‐Recognition‐Induced Domino Phase Transition and Luminescence Switching for Advanced Information Encryption9Tuning the luminous properties and optical thermometry of Cs2SnCl6 phosphor microcrystals via Bi and Sb codoping30Photoluminescent ionic metal halides based on s2 typed ions and aprotic ionic liquid cations87Bright Triplet Self-Trapped Excitons to Dopant Energy Transfer in Halide Double-Perovskite Nanocrystals95Multiexcitonic Emission in Zero-Dimensional Cs2ZrCl6:Sb3+ Perovskite Crystals275Te4+-doped Cs2InCl5·H2O single crystals for remote optical thermometry88Cyan Emission in Two-Dimensional Colloidal Cs2CdCl4:Sb3+ Ruddlesden–Popper Phase Nanoplatelets67Selective Luminescence Response of a Zero-Dimensional Hybrid Antimony(III) Halide to Solvent Molecules: Size-Effect and Supramolecular Interactions72Bright luminescence of Sb doping in all-inorganic zinc halide perovskite variant24Guest-Induced Reversible Phase Transformation of Organic–Inorganic Phenylpiperazinium Antimony (III) Chlorides with Solvatochromic Photoluminescence24Efficient dual-mode emissions of high-concentration erbium ions doped lead-free halide double perovskite single crystals39Highly Efficient Light‐Emitting Diodes Based on an Organic Antimony(III) Halide Hybrid139Highly Efficient Light‐Emitting Diodes Based on an Organic Antimony(III) Halide Hybrid22Broadband multimodal emission in Sb-doped CaZnOS-layered semiconductors25Realizing Near-Unity Quantum Efficiency of Zero-Dimensional Antimony Halides through Metal Halide Structural Modulation81Water-Molecule-Induced Emission Transformation of Zero-Dimension Antimony-Based Metal Halide79Highly emissive zero-dimensional antimony halide for anti-counterfeiting and confidential information encryption-decryption164Antimony-doped enhanced photoluminescence quantum yield in zero-dimensional lead-free metal halide Rb 2 CsBiCl 6 crystals20Bright tunable luminescence of Sb 3+ doping in zero-dimensional lead-free halide Cs 3 ZnCl 5 perovskite crystals26Manipulating the inorganic motif by kinetic control of antimony halide organic–inorganic hybrid materials for larger Stokes shift and significantly enhanced quantum efficiency8Soft crystal lattice and large anharmonicity facilitate the self-trapped excitonic emission in ultrathin 2D nanoplates of RbPb 2 Br 530The photoluminescence of isolated and paired Bi 3+ ions in layered LnOCl crystals: a first-principles study7Thermal stable zinc-based hybrid halides with high external quantum efficiency as temperature detectors29Three-dimensional all-inorganic dual halogen emitter Cs 2 Cd 2 BrCl 5 exhibiting broadband white-light emission18Triplet–triplet energy transfer from Bi 3+ to Sb 3+ in zero-dimensional indium hybrids via a B-site co-doping strategy toward white-light emission34Component Engineering to Tailor the Structure and Optical Properties of Sb-Doped Indium-Based Halides86Ternary zero-dimensional hybrid metal halides with dual emission10(C16H28N)2SbCl5: A new lead-free zero-dimensional metal-halide hybrid with bright orange emission111Integrated Afterglow and Self‐Trapped Exciton Emissions in Hybrid Metal Halides for Anti‐Counterfeiting Applications201Corrugated 1D Hybrid Metal Halide [C6H7ClN]CdCl3 Exhibiting Broadband White-Light Emission46In Situ Fabrication of Cs3Cu2I5: Tl Nanocrystal Films for High-Resolution and Ultrastable X-ray Imaging92Self‐Trapped Exciton Emission with High Thermal Stability in Antimony‐Doped Hybrid Manganese Chloride84Carbon dots embedded in lead-free luminescent metal halide crystals toward single-component white emitters32Phase-Selective Solution Synthesis of Cd-Based Perovskite Derivatives and Their Structure/Emission Modulation52Zero‐Dimensional Organic Copper(I) Iodide Hybrid with High Anti‐Water Stability for Blue‐Light‐Excitable Solid‐State Lighting114Efficient Yellow Self-Trapped Exciton Emission in Sb3+-Doped RbCdCl3 Metal Halides72Regulating the Singlet and Triplet Emission of Sb3+ Ions to Achieve Single-Component White-Light Emitter with Record High Color-Rendering Index and Stability145Investigation on Ba2(Y1-x, Lux)5B5O17: y at.% Bi as a new type of N-UV excited high efficient blue phosphor for wLED6Circularly Polarized Luminescence based on 0D Lead‐Free Antimony (III) Halide Hybrids63Bright Green Emission from Self-Trapped Excitons Triggered by Sb3+ Doping in Rb4CdCl6145Efficient Self-Trapped Exciton Emission in Ruddlesden–Popper Sb-Doped Cs3Cd2Cl7 Perovskites49Tunable photoresponse in twisted lead iodide homostructures via exciton-phonon coupling13H2O–NH4+-Induced Emission Modulation in Sb3+-Doped (NH4)2InCl5·H2O33Tunable emission color of [(2-mb)tpp]2Cd1-xMnxCl4 (x = 0–1) solid solutions synthesized via mechanochemical method for anti-counterfeit luminescent paper and WLEDs29Highly Stable Lead‐Free Perovskite Single Crystals with NIR Emission Beyond 1100 nm56Tuning Self‐Trapped Exciton States via Trivalent‐Metal Alloying in Lead‐Free 2D Double‐Perovskites28Boosting the Self-Trapped Exciton Emission in Cs2NaYCl6 Double Perovskite Single Crystals and Nanocrystals81Synthetic-Method-Dependent Antimony Bromides and Their Photoluminescent Properties36Molecular dimensionality and photoluminescence of hybrid metal halides92Excitation expansion in the high‐energy UV region for Dy 3+ ‐doped medium‐temperature molten silicate glass phosphors2Ultrasensitive Optical Thermometry via Inhibiting the Energy Transfer in Zero-Dimensional Lead-Free Metal Halide Single Crystals28Realizing High-Efficiency Yellow Emission of Organic Antimony Halides via Rational Structural Design105[PPh 3 H] 2 [SbCl 5 ]: A Zero-Dimensional Hybrid Metal Halide with a Supramolecular Framework and Stable Dual-Band Emission54Sequential and Reversible Phase Transformations in Zero‐Dimensional Organic‐Inorganic Hybrid Sb‐based Halides towards Multiple Emissions161Sequential and Reversible Phase Transformations in Zero‐Dimensional Organic‐Inorganic Hybrid Sb‐based Halides towards Multiple Emissions19Luminescence in the solid state7Recent Progress of Bismuth Effect on All‐Inorganic Lead‐Free Metal Halide Derivatives: Crystals Structure, Luminescence Properties, and Applications70Excitation-Dependent Tunable White Light of ns 2 Ions Doped Rb 2 SnCl 6 Vacancy Ordered Double Perovskite32All-inorganic non-perovskite copper halides for light emission33Orange/cyan emissive sensors of Sb 3+ for probing water via reversible phase transformation in rare-earth-based perovskite crystals24Effects of Cl/Br substitution of antimony octahedra on photoluminescence and a new engineering strategy for performance optimization1Unraveling the Defect-Dominated Broadband Emission Mechanisms in (001)-Preferred Two-Dimensional Layered Antimony-Halide Perovskite Film9Sn( ii )-doped one-dimensional hybrid metal halide [C 5 H 14 NO]CdCl 3 single crystals with broadband greenish-yellow light emission17Turn‐on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s2 Metal Centers56Turn‐on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s2 Metal Centers12Antimony doped tin( iv ) hybrid metal halides with high-efficiency tunable emission, WLED and information encryption31Crystal-glass phase transition enabling reversible fluorescence switching in zero-dimensional antimony halides40Effect of Mn 2+ doping on exciton recombination and carrier trapping in the Cs 2 CdCl 4 metal halide24Efficient triplet energy transfer in a 0D metal halide hybrid with long persistence room temperature phosphorescence for time-resolved anti-counterfeiting25Highly efficient warm white light emission in Sb 3+ -doped (NH 4 ) 4 CdCl 6 metal halides through A-site Rb-alloying regulation26Intrinsic vs. extrinsic STE emission enhancement in ns 2 ion doped metal (Cd, In) halide hybrids21Metal halides RbCdCl 3 :Sb 3+ and Rb 4 CdCl 6 :Sb 3+ with yellow and cyan emissions obtained via a facile hydrothermal process7Recent advances in ultralong room-temperature phosphorescence materials based on metal–organic halides31Regulating multiple self-trapped exciton emissions in zero-dimensional antimony halides with pyramidal units16Water-stable halide coordination polymers with dual self-trapped exciton emissions for dual-mode Hg 2+ sensing6Zero-dimensional antimony halides with tunable photoluminescence via halogen ligand modulation16Rational Design of a Super-Alkali Compound with Reversible Photoluminescence2Moisture-Induced reversible structure conversion of Zero-Dimensional organic cuprous bromide hybrids for multiple photoluminescent anti-Counterfeiting, information encryption and rewritable luminescent paper110Lead-free double perovskite Rb+, Sb3+-codoped Cs2NaInCl6 nanocrystals with highly efficient and tunable photoluminescence18Chemical doping of lead-free metal-halide-perovskite related materials for efficient white-light photoluminescence61Stable Organic Antimony Halides with Near‐Unity Photoluminescence Quantum Yield for X‐Ray Imaging61Supramolecular structures of new tetranuclear hydroxypiperidine iodoantimonates(iii)4Efficient Yellow Emission and Near-Unified Photoluminescence Quantum Yield of Sb 3+ in a One-Dimensional Confinement Cadmium Chloride Lattice16Bulk assemblies of organic antimony chloride with multiple reversible photoluminescence switching for anti-counterfeiting and information encryption35Mn 2+ -Activated Zero-Dimensional Metal (Cd, Zn) Halide Hybrids with Near-Unity PLQY and Zero Thermal Quenching23First-Principles Investigation on the Stability, Electronic Structure, and Exciton Self-Trapping Mechanism of 0D and 1D Cs3Cu2Cl520Strong Dopant–Dopant Electronic Coupling in Emissive Codoped Two Dimensional Metal Halide Hybrid11Ultra wideband NIR emission in all-inorganic lead-free metal halides through Sb3+ doping19Perovskite‐Organic Coupling WLED: Progress and Perspective23Two Novel Two-Dimensional Organic–Inorganic Hybrid Lead Halides with Broadband Emission for White-Light-Emitting Diodes23Surface Coating of Lead-free Perovskites to Break the Luminescence Threshold for Fluorescent Information Recognition12A New Class of Donor‐π‐Acceptor Phosphonium Salt Exhibiting Intriguing Thermally Activated Delayed Fluorescence15Turning Self‐Trapped Exciton Emission to Near‐Infrared Region in Thermochromism Zero‐Dimensional Hybrid Metal Halides39Ultrahigh PLQY Lead‐Free Organic–Inorganic Hybrid Zirconium‐Based Perovskites in Anticounterfeiting Applications43Zero-Dimensional Halides with ns2 Electron (Sb3+) Activation to Generate Broad Photoluminescence33Integrating Achiral and Chiral Organic Ligands in Zero‐Dimensional Hybrid Metal Halides to Boost Circularly Polarized Luminescence81Integrating Achiral and Chiral Organic Ligands in Zero‐Dimensional Hybrid Metal Halides to Boost Circularly Polarized Luminescence8Toward first-principles approaches for mechanistic study of self-trapped exciton luminescence15Bismuth-Doped Cesium Zirconium Chloride Microcrystal Scintillators for X-ray Computed Tomography Imaging5Simultaneously Achieving Multicolor Emission of Down‐Shifting and Up‐Conversion in Yb3+, Er3+ ‐Codoped Cs2NaGdCl6 Double Perovskites88Transparent 0D Antimony Halides Glassy Wafer with Near‐Unity Photoluminescence Quantum Yield for High Spatial Resolution X‐Ray Imaging43Bulk Coassembly of Zero-Dimensional Heterometallic Halide Hybrids for Broadband White Light Emission and Optical Thermometry10A review of the relationship between the structure and nonlinear optical properties of organic-inorganic hybrid materials149Sb‐Doped Cs 3 TbCl 6 Nanocrystals for Highly Efficient Narrow‐Band Green Emission and X‐Ray Imaging90Solution-Obtained (NH4)3In0.95Sb0.05Cl6 with High External Photoluminescence Quantum Yield and Excellent Antiquenching Properties10Effects of H3PO4 on synthesis and luminescence of metal halide perovskites1Luminescent Behavior of Sb3+-Activated Luminescent Metal Halide26Recent advances in lead-free Cs2ZrCl6 metal halide perovskites and their derivatives: From fundamentals to advanced applications52How Does Local Strain Affect Stokes Shifts in Halide Double Perovskite Nanocrystals?14Structural diversity and photoluminescence enhancement of indium-based hybrid metal halides190D Pyramid‐intercalated 2D Bimetallic Halides with Tunable Electronic Structures and Enhanced Emission under Pressure180D Pyramid‐intercalated 2D Bimetallic Halides with Tunable Electronic Structures and Enhanced Emission under Pressure1Anti‐Counterfeiting Application of Persistent Luminescence Materials and Its Research Progress189Bi 3+ /Sb 3+ co-doped Cs 2 HfCl 6 vacancy-ordered double perovskites for multifunctional optoelectronic applications21Energy Transfer and Self-Trapping Exciton Luminescence in Sb3+-Doped Two-Dimensional Layered Dion–Jacobson Phase Cadmium-Based Perovskites16A Zero-Dimensional Perovskite with Multi-Exciton Emission and Transient Response for Advanced Information Encryption0Alkali metal salt-assisted crystal structure switch of hybrid indium halides with near-unity photoluminescence quantum yield9An organic–inorganic hybrid photoluminescent ferroelastic with high phase transition temperature10Competition mechanism of self-trapped excitons and Te 4+ ions emission in the Te 4+ doped vacancy-ordered double perovskite Rb 2 HfCl 6 and its excellent properties10High-efficiency tunable self-trapped exciton emission in one-dimensional β-Cs 3 Cu 2 Br 5 via Ag alloying for optoelectronic applications2Modulating organic functional groups in stimuli-responsive luminescent antimony chlorides7Modulation of the near-infrared-I and -II luminescence of thulium-incorporated lead-free double perovskites10Multi-stimuli-responsive luminescence enabled by crown ether anchored chiral antimony halide phosphors54Optical activity levels of metal centers controlling multi-mode emissions in low-dimensional hybrid metal halides for anti-counterfeiting and information encryption34Realizing efficient broadband near-infrared emission under blue light excitation in Sb 3+ -doped zero-dimensional organic tin( iv )-based metal halides via coordination structure modulation12Recent strategies for triplet-state emission regulation toward non-lead organic–inorganic metal halides17Sb 3+ –doped 0D Cs 3 GdCl 6 microcrystals with a near-unity photoluminescence quantum yield and high thermal quenching resistance for light-emitting application14Temperature-dependent self-trapped models regulating energy transfer in rare earth double perovskites via 5s 2 electron doping32Tunable luminescence based on structural regulation in organic antimony halides for X-ray scintillation16Long-Persistent High-Temperature Phosphorescence of Zero-Dimensional Metal Halide Hybrid for Temperature-Sensitive Anticounterfeiting12Precise Manipulation the Efficient Multi‐Exciton Emission with High Thermal Stability in Hybrid Manganese‐Antimony Chloride for Optical Thermometry, Anti‐Counterfeiting, and Information Encryption21Sb 3+ -Doped Indium-Based Metal Halide (Gua) 3 InCl 6 with Efficient Yellow Emission58Antimony Doped Hybrid Zinc Halide Crystals with Tunable Light Emission and Long‐Term Stability25Unraveling the Photoluminescent Properties of Sb-Doped Cd-Based Inorganic Halides: A First-Principles Study7Increasing the Structural Rigidity and Quantum Yield of Highly Emissive Hybrid Antimony Chlorides Using a Diverse Set of Solvent Guests24Multisite Fine‐Tuning in Hybrid Cadmium Halides Enables Wide Range Emissions for Anti‐Counterfeiting6Multisite Fine‐Tuning in Hybrid Cadmium Halides Enables Wide Range Emissions for Anti‐Counterfeiting92White light emission in 0D halide perovskite [(CH3)3S]2SnCl6·H2O crystals through variation of doping ns2 ions14

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  4. Bulk assembly of a 0D organic antimony chloride hybrid with highly efficient orange dual emission by self-trapped states

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  7. Acentric Organic–Inorganic Hybrid Halide [N(CH3)4]2HgBr2I2 Featuring an Isolated [HgBr2I2]2– Tetrahedron and Second-Order Nonlinearity

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  9. Light-Emitting 0D Hybrid Metal Halide (C3H12N2)2Sb2Cl10 with Antimony Dimers

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  10. Realization of non-rare earth doped blue-emitting phosphor Ba2Y5B5O17: Sb by selective site excitation, and its application in n-UV excited wLEDs

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  29. Highly emissive zero-dimensional antimony halide for anti-counterfeiting and confidential information encryption-decryption

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  30. Antimony-doped enhanced photoluminescence quantum yield in zero-dimensional lead-free metal halide Rb 2 CsBiCl 6 crystals

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  31. Bright tunable luminescence of Sb 3+ doping in zero-dimensional lead-free halide Cs 3 ZnCl 5 perovskite crystals

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  32. Manipulating the inorganic motif by kinetic control of antimony halide organic–inorganic hybrid materials for larger Stokes shift and significantly enhanced quantum efficiency

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  33. Soft crystal lattice and large anharmonicity facilitate the self-trapped excitonic emission in ultrathin 2D nanoplates of RbPb 2 Br 5

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  34. The photoluminescence of isolated and paired Bi 3+ ions in layered LnOCl crystals: a first-principles study

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  35. Thermal stable zinc-based hybrid halides with high external quantum efficiency as temperature detectors

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  36. Three-dimensional all-inorganic dual halogen emitter Cs 2 Cd 2 BrCl 5 exhibiting broadband white-light emission

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  37. Triplet–triplet energy transfer from Bi 3+ to Sb 3+ in zero-dimensional indium hybrids via a B-site co-doping strategy toward white-light emission

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  38. Component Engineering to Tailor the Structure and Optical Properties of Sb-Doped Indium-Based Halides

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  42. Corrugated 1D Hybrid Metal Halide [C6H7ClN]CdCl3 Exhibiting Broadband White-Light Emission

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  43. In Situ Fabrication of Cs3Cu2I5: Tl Nanocrystal Films for High-Resolution and Ultrastable X-ray Imaging

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  44. Self‐Trapped Exciton Emission with High Thermal Stability in Antimony‐Doped Hybrid Manganese Chloride

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  45. Carbon dots embedded in lead-free luminescent metal halide crystals toward single-component white emitters

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  46. Phase-Selective Solution Synthesis of Cd-Based Perovskite Derivatives and Their Structure/Emission Modulation

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  47. Zero‐Dimensional Organic Copper(I) Iodide Hybrid with High Anti‐Water Stability for Blue‐Light‐Excitable Solid‐State Lighting

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  48. Efficient Yellow Self-Trapped Exciton Emission in Sb3+-Doped RbCdCl3 Metal Halides

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  49. Regulating the Singlet and Triplet Emission of Sb3+ Ions to Achieve Single-Component White-Light Emitter with Record High Color-Rendering Index and Stability

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  50. Investigation on Ba2(Y1-x, Lux)5B5O17: y at.% Bi as a new type of N-UV excited high efficient blue phosphor for wLED

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