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RESEARCH PAPER · ACS Energy Letters · 2021

Large-Grain Double Cation Perovskites with 18 μs Lifetime and High Luminescence Yield for Efficient Inverted Perovskite Solar Cells

Emilio Gutierrez‐Partida, Hannes Hempel, Sebastián Caicedo‐Dávila, Meysam Raoufi, Francisco Peña‐Camargo, Max Grischek, René Gunder, Jonas Diekmann, Pietro Caprioglio, Kai Oliver Brinkmann, Hans Köbler, Steve Albrecht, Thomas Riedl, Antonio Abate, Daniel Abou‐Ras, Thomas Unold, Dieter Neher, Martin Stolterfoht

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Large-Grain Double Cation Perovskites with 18 μs Lifetime and High Luminescence Yield for Efficient Inverted Perovskite Solar CellsOriginalBi-functional interfaces by poly(ionic liquid) treatment in efficient pin and nip perovskite solar cells1192D/3D perovskite engineering eliminates interfacial recombination losses in hybrid perovskite solar cells214Ambient Air Temperature Assisted Crystallization for Inorganic CsPbI2Br Perovskite Solar Cells13Light‐Emitting Perovskite Solar Cells: A Tale of Two States4Apparent Defect Densities in Halide Perovskite Thin Films and Single Crystals198A low-cost polymerized hole-transporting material for high performance planar perovskite solar cells2Crystal growth, defect passivation and strain release via In-situ Self-polymerization strategy enables efficient and stable perovskite solar cells54Bismuth-based halide perovskite and perovskite-inspired light absorbing materials for photovoltaics59Semitransparent Perovskite Solar Cells for Building Integration and Tandem Photovoltaics: Design Strategies and Challenges82Reducing energy barrier of δ-to-α phase transition for printed formamidinium lead iodide photovoltaic devices35Surface-tension release in PTAA-based inverted perovskite solar cells43Monolithic Lead Halide Perovskite Photoelectrochemical Cell with 9.16% Applied Bias Photon-to-Current Efficiency57Perovskite Solar Cells Go Bifacial—Mutual Benefits for Efficiency and Durability98Monolithic All‐Perovskite Tandem Solar Cells with Minimized Optical and Energetic Losses91Accelerating research on novel photovoltaic materials10Effects of temperature-dependent burn-in decay on the performance of triple cation mixed halide perovskite solar cells21Mechano-optical Modulation of Excitons and Carrier Recombination in Self-Assembled Halide Perovskite Quantum Dots30Interface Regulation by an Ultrathin Wide-Bandgap Halide for Stable and Efficient Inverted Perovskite Solar Cells22Understanding Performance Limiting Interfacial Recombination in pin Perovskite Solar Cells296Predicting Solar Cell Performance from Terahertz and Microwave Spectroscopy81Subtle side chain modification of triphenylamine‐based polymer hole‐transport layer materials produces efficient and stable inverted perovskite solar cells67Stable α‐FAPbI 3 in Inverted Perovskite Solar Cells with Efficiency Exceeding 22% via a Self‐Passivation Strategy120Revealing the doping density in perovskite solar cells and its impact on device performance74PTAA as Efficient Hole Transport Materials in Perovskite Solar Cells: A Review276Bridging the Interfacial Contact for Improved Stability and Efficiency of Inverted Perovskite Solar Cells38Toward Efficient Perovskite Solar Cells: Progress, Strategies, and Perspectives169Critical Role of Perovskite Film Stoichiometry in Determining Solar Cell Operational Stability: a Study on the Effects of Volatile A-Cation Additives27KBF 4 Additive for Alleviating Microstrain, Improving Crystallinity, and Passivating Defects in Inverted Perovskite Solar Cells91Future Research Directions in Perovskite Solar Cells: Exquisite Photon Management and Thermodynamic Phase Stability40Perovskite-Surface-Confined Grain Growth for High-Performance Perovskite Solar Cells23Interfacial Engineering for High‐Performance PTAA‐Based Inverted 3D Perovskite Solar Cells22α-FAPbI3 phase stabilization using aprotic trimethylsulfonium cation for efficient perovskite solar cells22Quantifying the Energy Losses in CsPbI2Br Perovskite Solar Cells with an Open-Circuit Voltage of up to 1.45 V69Mitigation of Open‐Circuit Voltage Losses in Perovskite Solar Cells Processed over Micrometer‐Sized‐Textured Si Substrates24Efficient Inverted Perovskite Solar Cells via Improved Sequential Deposition83Alkali element (Li, Na, K, and Rb) doping of Cu 2 BaGe 1− x Sn x Se 4 films4Cetrimonium bromide and potassium thiocyanate assisted post-vapor treatment approach to enhance power conversion efficiency and stability of FAPbI 3 perovskite solar cells15Numerical Study on the Effect of Dual Electron Transport Layer in Improving the Performance of Perovskite–Perovskite Tandem Solar Cells30Ag Alloying in Cu2−yAgyBa(Ge,Sn)Se4Films and Photovoltaic Devices6Neglected acidity pitfall: boric acid-anchoring hole-selective contact for perovskite solar cells112Recent progress in the development of high-efficiency inverted perovskite solar cells341Buried interface defects passivation of perovskite film by choline halide for high performance inverted perovskite solar cells with efficiency exceeding 22%17Stabilization of α ‐phase FAPbI 3 via Buffering Interfacial Region for Efficient p–i–n Perovskite Solar Cells36Enhanced surface morphology and photovoltaic properties of a new class of material copper silver bismuth iodide solar cell15Transforming characterization data into information in the case of perovskite solar cells8Influence of A-Site Cation Composition on the Electronic Properties of Halide Tin Perovskites13Uncovering of Some Citrus Rootstocks to Salt Stress Tolerance In Vitro Screening3Improving Efficiency and Stability of p–i–n Perovskite Solar Cells by Capsaicin‐Based Antisolvent Additive Engineering6When JV Curves Conceal Material Improvements: The Relevance of Photoluminescence Measurements in the Optimization of Perovskite Solar Cells14Controlling Lead Halide Residue in Perovskite Solar Cells: A Method to Improve the Photostability and Hysteresis11Bandgap Engineering of Two‐Step Processed Perovskite Top Cells for Perovskite‐Based Tandem Photovoltaics19“Freezing” intermediate phases for efficient and stable FAPbI 3 perovskite solar cells50Development on inverted perovskite solar cells: A review58Using a perovskite oxide as interfacial layer for halide perovskite optoelectronics0Grain boundaries in polycrystalline materials for energy applications: First principles modeling and electron microscopy69Ester‐Functionalized Polythiophene Interlayers for Enhanced Performance and Stability of Perovskite Solar Cells14Reduced recombination via tunable surface fields in perovskite thin films70Metal halide perovskite solar cells0Molecular cation and low-dimensional perovskite surface passivation in perovskite solar cells301Vacuum-Deposited Bifacial Perovskite Solar Cells23The Promise and Challenges of Inverted Perovskite Solar Cells295Understanding Power‐Law Photoluminescence Decays and Bimolecular Recombination in Lead‐Halide Perovskites60Lead carbanion anchoring for surface passivation to boost efficiency of inverted perovskite solar cells to over 25%11Molecularly tailored bifunctional nano-overlayers for efficient and stable inverted perovskite solar cells4Effective Steady‐State Recombination Decay Times in Comparison to Time‐Resolved Photoluminescence Decay Times in Halide Perovskite Solar Cells6Light‐Emitting Perovskite Solar Cells: Genesis to Recent Drifts2(111) Facet-engineered SnO 2 as an electron transport layer for efficient and stable triple-cation perovskite solar cells6Polyanionic surfactant modulates the substrate surface energy to achieve crystallization control for efficient perovskite solar cells2Transfer dynamics of photo-generated carriers in catalysis192Reactive Plasma Deposition of ITO as an Efficient Buffer Layer for Inverted Perovskite Solar Cells16Versatile Two‐Step Process for Perovskite‐Based Tandem Photovoltaics6Photoluminescence Quantum Yield in Perovskite Solar Cells: Probing Interface Recombination and Efficiency Limits11Dual Defect Passivation Engineering of Perovskite Photodetectors toward Infrared Filter‐Free Full‐Color Imaging6Multifunctional polymer additives enable highly efficient, mechanically durable, and deployable flexible perovskite photovoltaics0Decoding Interfacial Charge‐Carrier Dynamics in Integrated Perovskite/Organic Solar Cells via Numerical Modeling8Development of hole-transport layers in inverted perovskite solar cells1Dual carrier-selective contact transition metal dichalcogenide solar cells1Rapid Parameter Prediction in Perovskite Solar Cells via AI-Assisted Performance Analysis1Bright Near-Infrared Emission in Molybdenum Ions Doped with Lead-Free Double Perovskites1Journey toward a Global Understanding of Recombination in Halide Perovskites for Photovoltaic Applications3Critical analysis of recent advancements in incorporating Cs in hybrid perovskite solar cell to boost its stability and efficiency0Ultralow Voltage Bias-Switchable Perovskite Photodetectors Enabled by Interfacial Deep-Trap Engineering0Volatile eutectics to tailor crystallization for perovskite optoelectronics0

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  2. 2D/3D perovskite engineering eliminates interfacial recombination losses in hybrid perovskite solar cells

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  3. Ambient Air Temperature Assisted Crystallization for Inorganic CsPbI2Br Perovskite Solar Cells

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  4. Light‐Emitting Perovskite Solar Cells: A Tale of Two States

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  5. Apparent Defect Densities in Halide Perovskite Thin Films and Single Crystals

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  6. A low-cost polymerized hole-transporting material for high performance planar perovskite solar cells

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  7. Crystal growth, defect passivation and strain release via In-situ Self-polymerization strategy enables efficient and stable perovskite solar cells

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  8. Bismuth-based halide perovskite and perovskite-inspired light absorbing materials for photovoltaics

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  9. Semitransparent Perovskite Solar Cells for Building Integration and Tandem Photovoltaics: Design Strategies and Challenges

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  10. Reducing energy barrier of δ-to-α phase transition for printed formamidinium lead iodide photovoltaic devices

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  12. Monolithic Lead Halide Perovskite Photoelectrochemical Cell with 9.16% Applied Bias Photon-to-Current Efficiency

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  16. Effects of temperature-dependent burn-in decay on the performance of triple cation mixed halide perovskite solar cells

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  17. Mechano-optical Modulation of Excitons and Carrier Recombination in Self-Assembled Halide Perovskite Quantum Dots

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  18. Interface Regulation by an Ultrathin Wide-Bandgap Halide for Stable and Efficient Inverted Perovskite Solar Cells

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  19. Understanding Performance Limiting Interfacial Recombination in pin Perovskite Solar Cells

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  21. Subtle side chain modification of triphenylamine‐based polymer hole‐transport layer materials produces efficient and stable inverted perovskite solar cells

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  22. Stable α‐FAPbI 3 in Inverted Perovskite Solar Cells with Efficiency Exceeding 22% via a Self‐Passivation Strategy

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  28. KBF 4 Additive for Alleviating Microstrain, Improving Crystallinity, and Passivating Defects in Inverted Perovskite Solar Cells

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  46. Influence of A-Site Cation Composition on the Electronic Properties of Halide Tin Perovskites

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  47. Uncovering of Some Citrus Rootstocks to Salt Stress Tolerance In Vitro Screening

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  48. Improving Efficiency and Stability of p–i–n Perovskite Solar Cells by Capsaicin‐Based Antisolvent Additive Engineering

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  49. When JV Curves Conceal Material Improvements: The Relevance of Photoluminescence Measurements in the Optimization of Perovskite Solar Cells

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  50. Controlling Lead Halide Residue in Perovskite Solar Cells: A Method to Improve the Photostability and Hysteresis

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