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RESEARCH PAPER · Chemical Reviews · 2021

The 2D Halide Perovskite Rulebook: How the Spacer Influences Everything from the Structure to Optoelectronic Device Efficiency

Xiaotong Li, Justin M. Hoffman, Mercouri G. Kanatzidis

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The 2D Halide Perovskite Rulebook: How the Spacer Influences Everything from the Structure to Optoelectronic Device EfficiencyOriginalInterfaces in metal halide perovskites probed by solid-state NMR spectroscopy59Multifunctional layered hybrid perovskites62Role of spacer cations and structural distortion in two-dimensional germanium halide perovskites69Two-dimensional halide perovskites: synthesis, optoelectronic properties, stability, and applications108Using steric hindrance to manipulate and stabilize metal halide perovskites for optoelectronics76Two-dimensional perovskites for photovoltaics67Progress and perspective in Dion-Jacobson phase 2D layered perovskite optoelectronic applications130Fluorinated Aromatic Formamidinium Spacers Boost Efficiency of Layered Ruddlesden–Popper Perovskite Solar Cells121Synthesis, Applications, and Prospects of Quantum‐Dot‐in‐Perovskite Solids80Germanium‐Based Halide Perovskites: Materials, Properties, and Applications174Spacer Cations Dictate Photoinduced Phase Segregation in 2D Mixed Halide Perovskites74On the Mechanism of Alkylammonium Ligands Binding to the Surface of CsPbBr3 Nanocrystals93Multiple-Noncovalent-Interaction-Stabilized Layered Dion–Jacobson Perovskite for Efficient Solar Cells92Shedding Light on the Stability and Structure–Property Relationships of Two-Dimensional Hybrid Lead Bromide Perovskites51Oriented Halide Perovskite Nanostructures and Thin Films for Optoelectronics145Architecture of p-i-n Sn-Based Perovskite Solar Cells: Characteristics, Advances, and Perspectives138Bismuth/Silver-Based Two-Dimensional Iodide Double and One-Dimensional Bi Perovskites: Interplay between Structural and Electronic Dimensions66Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes119m-Phenylenediammonium as a New Spacer for Dion–Jacobson Two-Dimensional Perovskites109Stability of Perovskite Solar Cells: Degradation Mechanisms and Remedies211Highly Stable Inorganic Lead Halide Perovskite toward Efficient Photovoltaics87Mechanics-coupled stability of metal-halide perovskites127In situ growth of ultra-thin perovskitoid layer to stabilize and passivate MAPbI3 for efficient and stable photovoltaics93Metal Halide Perovskites as Emerging Thermoelectric Materials96Highly Efficient and Stable Dion−Jacobson Perovskite Solar Cells Enabled by Extended π‐Conjugation of Organic Spacer186Advancing 2D Perovskites for Efficient and Stable Solar Cells: Challenges and Opportunities247Cyan Emission in Two-Dimensional Colloidal Cs2CdCl4:Sb3+ Ruddlesden–Popper Phase Nanoplatelets67Surface Reconstruction for Stable Monolithic All‐Inorganic Perovskite/Organic Tandem Solar Cells with over 21% Efficiency91Machine learning for high-throughput experimental exploration of metal halide perovskites117Efficient and stable mesoscopic perovskite solar cell in high humidity by localized Dion-Jacobson 2D‐3D heterostructures68Spacer Engineering of Diammonium‐Based 2D Perovskites toward Efficient and Stable 2D/3D Heterostructure Perovskite Solar Cells113Unusual ferroelectric-dependent birefringence in 2D trilayered perovskite-type ferroelectric exploited by dimensional tailoring63Colloidal Metal‐Halide Perovskite Nanoplatelets: Thickness‐Controlled Synthesis, Properties, and Application in Light‐Emitting Diodes273Size and Quality Enhancement of 2D Semiconducting Metal–Organic Chalcogenolates by Amine Addition58Diammonium Molecular Configuration‐Induced Regulation of Crystal Orientation and Carrier Dynamics for Highly Efficient and Stable 2D/3D Perovskite Solar Cells119Efficient Bulk Defect Suppression Strategy in FASnI3 Perovskite for Photovoltaic Performance Enhancement62Intercalating-Organic-Cation-Induced Stability Bowing in Quasi-2D Metal-Halide Perovskites50Oriented 2D Perovskite Wafers for Anisotropic X‐ray Detection through a Fast Tableting Strategy111Water-Molecule-Induced Emission Transformation of Zero-Dimension Antimony-Based Metal Halide79Near-Infrared Phosphorescent Hybrid Organic–Inorganic Perovskite with High-Contrast Dielectric and Third-Order Nonlinear Optical Switching Functionalities74Zero-Dimensional Lead-Free Halide with Indirect Optical Gap and Enhanced Photoluminescence by Sb Doping76[PbX 6 ] 4− modulation and organic spacer construction for stable perovskite solar cells66Colloidal FAPbBr 3 perovskite nanocrystals for light emission: what's going on?50Optimized carrier extraction at interfaces for 23.6% efficient tin–lead perovskite solar cells467Metastable Dion-Jacobson 2D structure enables efficient and stable perovskite solar cells466Advanced porous borocarbonitride nanoarchitectonics: Their structural designs and applications60Recent Advances in Organic and Organic–Inorganic Hybrid Materials for Piezoelectric Mechanical Energy Harvesting335Two-dimensional perovskites: Impacts of species, components, and properties of organic spacers on solar cells134Stabilization of Metastable Halide Perovskite Lattices in the 2D Limit64Dynamic Exciton Polaron in Two-Dimensional Lead Halide Perovskites and Implications for Optoelectronic Applications94Tailoring Interlayered Spacers of Two‐Dimensional Cesium‐Based Perovskite Ferroelectrics toward Exceptional Ferro‐Pyro‐Phototronic Effects50The Emerging Role of Halogen Bonding in Hybrid Perovskite Photovoltaics51Centimeter-Sized 2D Perovskitoid Single Crystals for Efficient X-ray Photoresponsivity58Multifunctional Chiral 2D Lead Halide Perovskites with Circularly Polarized Photoluminescence and Piezoelectric Energy Harvesting Properties112From Structural Design to Functional Construction: Amine Molecules in High‐Performance Formamidinium‐Based Perovskite Solar Cells143Direct Observation of Fast Carriers Transport along Out-of-Plane Direction in a Dion–Jacobson Layered Perovskite60Tolerance Factor for Stabilizing 3D Hybrid Halide Perovskitoids Using Linear Diammonium Cations98Crystal Growth Regulation of 2D/3D Perovskite Films for Solar Cells with Both High Efficiency and Stability195Small symmetry-breaking triggering large chiroptical responses of Ag70 nanoclusters70CsPbI3-Based Phase-Stable 2D Ruddlesden–Popper Perovskites for Efficient Solar Cells56Pseudohalide-Assisted Growth of Oriented Large Grains for High-Performance and Stable 2D Perovskite Solar Cells57Colossal barocaloric effects with ultralow hysteresis in two-dimensional metal–halide perovskites93Strategies for high‐performance perovskite solar cells from materials, film engineering to carrier dynamics and photon management56Polar Photovoltaic Effect in Chiral Alternating Cations Intercalation‐Type Perovskites Driving Self‐Powered Ultraviolet Circularly Polarized Light Detection55Perovskite-based tandem solar cells: Device architecture, stability, and economic perspectives56X-ray diffraction of photovoltaic perovskites: Principles and applications138Screening of Excitons by Organic Cations in Quasi-Two-Dimensional Organic–Inorganic Lead-Halide Perovskites58Engineering van der Waals Materials for Advanced Metaphotonics100Discovery of a 2D Hybrid Silver/Antimony‐Based Iodide Double Perovskite Photoferroelectric with Photostrictive Effect and Efficient X‐Ray Response77Regulation of Quantum Wells Width Distribution in 2D Perovskite Films for Photovoltaic Application79Exploring the Steric Hindrance of Alkylammonium Cations in the Structural Reconfiguration of Quasi‐2D Perovskite Materials Using a High‐throughput Experimental Platform542D Ruddlesden-Popper perovskite ferroelectric film for high-performance, self-powered and ultra-stable UV photodetector boosted by ferro-pyro-phototronic effect and surface passivation53Pressure-Driven Phase Transition in Two-Dimensional Perovskite MHy2PbBr469Low-dimensional Sn-based perovskites: Evolution and future prospects of solar cells68High Efficiency Quasi‐2D Ruddlesden–Popper Perovskite Solar Cells80Stability of 2D and quasi-2D perovskite materials and devices279Magnetic Properties of Layered Hybrid Organic‐Inorganic Metal‐Halide Perovskites: Transition Metal, Organic Cation and Perovskite Phase Effects59Structural Descriptors to Correlate Pb Ion Displacement and Broadband Emission in 2D Halide Perovskites121Oriented Low‐n Ruddlesden‐Popper Formamidinium‐Based Perovskite for Efficient and Air Stable Solar Cells59Near-room-temperature martensitic actuation profited from one-dimensional hybrid perovskite structure60Orbital Interactions between the Organic Semiconductor Spacer and the Inorganic Layer in Dion–Jacobson Perovskites Enable Efficient Solar Cells60Recent Advances on Mn2+‐Doping in Diverse Metal Halide Perovskites66Electron‐Phonon Coupling Suppression by Enhanced Lattice Rigidity in 2D Perovskite Single Crystals for High‐Performance X‐Ray Detection163Recent progress in perovskite solar cells: material science169Synthesis-on-substrate of quantum dot solids566Composition Engineering of Perovskite Single Crystals for High‐Performance Optoelectronics115Recent progress in layered metal halide perovskites for solar cells, photodetectors, and field-effect transistors53Rational Design of Non-Centrosymmetric Hybrid Halide Perovskites109Prominent Free Charges Tunneling Through Organic Interlayer of 2D Perovskites56Expanding the low-dimensional interface engineering toolbox for efficient perovskite solar cells134Roadmap on commercialization of metal halide perovskite photovoltaics64Revealing stability origin of Dion-Jacobson 2D perovskites with different-rigidity organic cations107Prospects for Tin-Containing Halide Perovskite Photovoltaics51Chirality-Dependent Structural Transformation in Chiral 2D Perovskites under High Pressure75Feature Selection in Machine Learning for Perovskite Materials Design and Discovery59Inhibition of Ion Migration for Highly Efficient and Stable Perovskite Solar Cells152Exciton Formation Dynamics and Band‐Like Free Charge‐Carrier Transport in 2D Metal Halide Perovskite Semiconductors79Phase-pure two-dimensional layered perovskite thin films199Additive Engineering for Stable and Efficient Dion–Jacobson Phase Perovskite Solar Cells56Mixed perovskites (2D/3D)-based solar cells: a review on crystallization and surface modification for enhanced efficiency and stability57Carriers, Quasi-particles, and Collective Excitations in Halide Perovskites110How to GIWAXS: Grazing Incidence Wide Angle X‐Ray Scattering Applied to Metal Halide Perovskite Thin Films230Design Rules for Obtaining Narrow Luminescence from Semiconductors Made in Solution87Quantum Confinement Breaking: Orbital Coupling in 2D Ruddlesden–Popper Perovskites Enables Efficient Solar Cells72Mixed Ruddlesden–Popper and Dion–Jacobson Phase Perovskites for Stable and Efficient Blue Perovskite LEDs53Mixed-Halide Perovskites with Halogen Bond Induced Interlayer Locking Structure for Stable Pure-Red PeLEDs52Synergy of 3D and 2D Perovskites for Durable, Efficient Solar Cells and Beyond249Inverted Wide-Bandgap 2D/3D Perovskite Solar Cells with >22% Efficiency and Low Voltage Loss87Giant Polarization Sensitivity via the Anomalous Photovoltaic Effect in a Two-Dimensional Perovskite Ferroelectric69Synthesis of Layered Lead-Free Perovskite Nanocrystals with Precise Size and Shape Control and Their Photocatalytic Activity74Highly Stable and Efficient Formamidinium‐Based 2D Ruddlesden–Popper Perovskite Solar Cells via Lattice Manipulation56A Self‐Powered UV Photodetector With Ultrahigh Responsivity Based on 2D Perovskite Ferroelectric Films With Mixed Spacer Cations64Emerging Two-Dimensional Organic Semiconductor-Incorporated Perovskites─A Fascinating Family of Hybrid Electronic Materials101Tailoring Interlayer Charge Transfer Dynamics in 2D Perovskites with Electroactive Spacer Molecules79Spin Quantum Dot Light‐Emitting Diodes Enabled by 2D Chiral Perovskite with Spin‐Dependent Carrier Transport83Strategies for improving the stability of perovskite for photocatalysis: A review of recent progress54Synthesis of 2D perovskite crystals via progressive transformation of quantum well thickness75Nucleation and Crystallization in 2D Ruddlesden‐Popper Perovskites using Formamidinium‐based Organic Semiconductor Spacers for Efficient Solar Cells55Hydrogen bonding in perovskite solar cells142Advances in Optical Imaging and Optical Communications Based on High‐Quality Halide Perovskite Photodetectors95Reinforcing built-in electric field to enable efficient carrier extraction for high-performance perovskite solar cells52Tuning Structure and Excitonic Properties of 2D Ruddlesden–Popper Germanium, Tin, and Lead Iodide Perovskites via Interplay between Cations60Bilayer 2D-3D Perovskite Heterostructures for Efficient and Stable Solar Cells77Regulating the crystallization of mixed-halide perovskites by cation alloying for perovskite–organic tandem solar cells52Revealing degradation mechanisms in 3D/2D perovskite solar cells under photothermal accelerated ageing56Ultra-large dipole moment organic cations derived 3D/2D p–n heterojunction for high-efficiency carbon-based perovskite solar cells81Modulating the Dipole Moment of Secondary Ammonium Spacers for Efficient 2D Ruddlesden‐Popper Perovskite Solar Cells61Universal machine learning aided synthesis approach of two-dimensional perovskites in a typical laboratory86Single-Crystal-Assisted In Situ Phase Reconstruction Enables Efficient and Stable 2D/3D Perovskite Solar Cells51Ramifications of Ion Migration in 2D Lead Halide Perovskites84Phase Transitions and Dynamics in Mixed Three- and Low-Dimensional Lead Halide Perovskites134Narrow Bandgap Metal Halide Perovskites for All-Perovskite Tandem Photovoltaics209Phase-Stable Wide-Bandgap Perovskites with 2D/3D Structure for All-Perovskite Tandem Solar Cells61Arising 2D Perovskites for Ionizing Radiation Detection93Exciton engineering of 2D Ruddlesden–Popper perovskites by synergistically tuning the intra and interlayer structures113Key Roles of Interfaces in Inverted Metal-Halide Perovskite Solar Cells52Toward Self-Driven Autonomous Material and Device Acceleration Platforms (AMADAP) for Emerging Photovoltaics Technologies54What Matters for the Charge Transport of 2D Perovskites?93Molecular cation and low-dimensional perovskite surface passivation in perovskite solar cells302Two-dimensional perovskitoids enhance stability in perovskite solar cells282Ultrastable and efficient slight-interlayer-displacement 2D Dion-Jacobson perovskite solar cells65Advanced Organic–Inorganic Hybrid Materials for Optoelectronic Applications222Reliable and Robust Two-Dimensional Perovskite Memristors for Flexible-Resistive Random-Access Memory Array60Linearly programmable two-dimensional halide perovskite memristor arrays for neuromorphic computing156A-Site Cation Chemistry in Halide Perovskites123Boosting Carrier Transport in Quasi‐2D/3D Perovskite Heterojunction for High‐Performance Perovskite/Organic Tandems66Two-Dimensional Organic–Inorganic van der Waals Hybrids58Synergistic Integration of Halide Perovskite and Rare‐Earth Ions toward Photonics55Perovskite Solar Cells and Light Emitting Diodes: Materials Chemistry, Device Physics and Relationship72Diverse Perovskite Solar Cells: Progress, Challenges, and Perspectives74

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    Federico Locardi, Margarita Samoli, A. Martinelli, Onur Erdem, Débora Vale Magalhães, Sara Bals, Zeger Hens

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  48. Surface Reconstruction for Stable Monolithic All‐Inorganic Perovskite/Organic Tandem Solar Cells with over 21% Efficiency

    Advanced Functional Materials · 2021-10-20

    Weijie Chen, Dong Li, Xu Chen, Haiyang Chen, Shuo Liu, Haidi Yang, Xinqi Li, Yunxiu Shen, Xuemei Ou, Yang Yang, Lin Jiang, Yaowen Li, Yaowen Li, Yongfang Li, Yongfang Li

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  49. Structure‐Property Relationships and Idiosyncrasies of Bulk, 2D Hybrid Lead Bromide Perovskites

    Israel Journal of Chemistry · 2021-10-22

    Eugenia S. Vasileiadou, Mercouri G. Kanatzidis

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  50. Machine learning for high-throughput experimental exploration of metal halide perovskites

    Joule · 2021-10-25

    Mahshid Ahmadi, Maxim A Ziatdinov, Yuanyuan Zhou, Eric Andrew Lass, Sergei V. Kalinin

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