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RESEARCH PAPER · Chemical Reviews · 2020

Promises and Challenges of Next-Generation “Beyond Li-ion” Batteries for Electric Vehicles and Grid Decarbonization

Yaosen Tian, Guobo Zeng, Ann Rutt, Tan Shi, Haegyeom Kim, Jingyang Wang, Julius Koettgen, Yingzhi Sun, Bin Ouyang, Tina Chen, Zhengyan Lun, Ziqin Rong, Kristin Aslaug Persson, Gerbrand Ceder

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Promises and Challenges of Next-Generation “Beyond Li-ion” Batteries for Electric Vehicles and Grid DecarbonizationOriginalDemystifying the Lattice Oxygen Redox in Layered Oxide Cathode Materials of Lithium-Ion Batteries144Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive1081Simultaneous Regulation on Solvation Shell and Electrode Interface for Dendrite‐Free Zn Ion Batteries Achieved by a Low‐Cost Glucose Additive219Life‐Cycle Assessment Considerations for Batteries and Battery Materials304Recent advances of metal phosphates-based electrodes for high-performance metal ion batteries112Manipulating free-standing, flexible and scalable microfiber carbon papers unlocking ultra-high initial Coulombic efficiency and storage sodium behavior98Recent progress of cathode materials for aqueous zinc-ion capacitors: Carbon-based materials and beyond137High Energy Density Solid State Lithium Metal Batteries Enabled by Sub‐5 µm Solid Polymer Electrolytes241Synthetic accessibility and stability rules of NASICONs121Robust Solid Electrolyte Interphases in Localized High Concentration Electrolytes Boosting Black Phosphorus Anode for Potassium-Ion Batteries87Graphene‐Supported Atomically Dispersed Metals as Bifunctional Catalysts for Next‐Generation Batteries Based on Conversion Reactions212A novel Fe-defect induced pure-phase Na4Fe2.91(PO4)2P2O7 cathode material with high capacity and ultra-long lifetime for low-cost sodium-ion batteries279Hierarchically Porous Silica Membrane as Separator for High‐Performance Lithium‐Ion Batteries192Recent advances in Mg-Li and Mg-Na hybrid batteries83Defect‐Selectivity and “Order‐in‐Disorder” Engineering in Carbon for Durable and Fast Potassium Storage310Dynamic interphase–mediated assembly for deep cycling metal batteries155Advances in studying interfacial reactions in rechargeable batteries by photoelectron spectroscopy81Hydrated eutectic electrolytes for high-performance Mg-ion batteries129Ion transport in composite polymer electrolytes137Aluminum-copper alloy anode materials for high-energy aqueous aluminum batteries209An Advanced High‐Entropy Fluorophosphate Cathode for Sodium‐Ion Batteries with Increased Working Voltage and Energy Density393Challenges, interface engineering, and processing strategies toward practical sulfide‐based all‐solid‐state lithium batteries272Solid-state lithium battery cathodes operating at low pressures175Manganese‐based materials as cathode for rechargeable aqueous zinc‐ion batteries102Long‐Life Zn Anode Enabled by Low Volume Concentration of a Benign Electrolyte Additive131Hydrophobization Engineering of the Air–Cathode Catalyst for Improved Oxygen Diffusion towards Efficient Zinc–Air Batteries205Highly reversible Mg metal anodes enabled by interfacial liquid metal engineering for high-energy Mg-S batteries101Hybridization of 2D Nanomaterials with 3D Graphene Architectures for Electrochemical Energy Storage and Conversion79Freestanding Metal–Organic Frameworks and Their Derivatives: An Emerging Platform for Electrochemical Energy Storage and Conversion390A Polymerized‐Ionic‐Liquid‐Based Polymer Electrolyte with High Oxidative Stability for 4 and 5 V Class Solid‐State Lithium Metal Batteries102Rationally Designed Sodium Chromium Vanadium Phosphate Cathodes with Multi‐Electron Reaction for Fast‐Charging Sodium‐Ion Batteries194Predominant intercalation of H+ enables ultrahigh rate capability of oxygen deficient MoO3 for aqueous Al-ion batteries86Research Development on Aqueous Ammonium‐Ion Batteries170Synergetic Effect of Alkali‐Site Substitution and Oxygen Vacancy Boosting Vanadate Cathode for Super‐Stable Potassium and Zinc Storage85Stable Solid Electrolyte Interphase In Situ Formed on Magnesium‐Metal Anode by using a Perfluorinated Alkoxide‐Based All‐Magnesium Salt Electrolyte120Surface-Alloyed Nanoporous Zinc as Reversible and Stable Anodes for High-Performance Aqueous Zinc-Ion Battery202Insights into Ti doping for stabilizing the Na2/3Fe1/3Mn2/3O2 cathode in sodium ion battery116State of charge, remaining useful life and knee point estimation based on artificial intelligence and Machine learning in lithium-ion EV batteries: A comprehensive review97MXenes for advanced separator in rechargeable batteries96Gallium‐based liquid metals for lithium‐ion batteries88Thio‐/LISICON and LGPS‐Type Solid Electrolytes for All‐Solid‐State Lithium‐Ion Batteries135Stabilization of Multicationic Redox Chemistry in Polyanionic Cathode by Increasing Entropy126Calcium-tin alloys as anodes for rechargeable non-aqueous calcium-ion batteries at room temperature102Carbon/Lithium Composite Anode for Advanced Lithium Metal Batteries: Design, Progress, In Situ Characterization, and Perspectives115Towards better Mg metal anodes in rechargeable Mg batteries: Challenges, strategies, and perspectives126Toward Optimization of the Chemical/Electrochemical Compatibility of Halide Solid Electrolytes in All-Solid-State Batteries95In Situ Catalytic Polymerization of a Highly Homogeneous PDOL Composite Electrolyte for Long‐Cycle High‐Voltage Solid‐State Lithium Batteries295A Review on Regulating Li+Solvation Structures in Carbonate Electrolytes for Lithium Metal Batteries298Nano self-assembly of fluorophosphate cathode induced by surface energy evolution towards high-rate and stable sodium-ion batteries104Polymer nanocomposites based on Graphite Nanoplatelets and amphiphilic graphene platelets83Self‐Healing of Prussian Blue Analogues with Electrochemically Driven Morphological Rejuvenation92Biomimetic Dendrite‐Free Multivalent Metal Batteries98Edge-oxidation-induced densification towards hybrid bulk carbon for low-voltage, reversible and fast potassium storage84Heterogeneous NASICON‐Type Composite as Low‐Cost, High‐Performance Cathode for Sodium‐Ion Batteries172Cosolvent‐Assisted Formation of Charged Ion‐Solvent Clusters and Solid Electrolyte Interphase for High‐Performance Magnesium Metal Batteries80Uniformly MXene‐Grafted Eutectic Aluminum‐Cerium Alloys as Flexible and Reversible Anode Materials for Rechargeable Aluminum‐Ion Battery108From anode to cell: synergistic protection strategies and perspectives for stabilized Zn metal in mild aqueous electrolytes125From lithium to emerging mono- and multivalent-cation-based rechargeable batteries: non-aqueous organic electrolyte and interphase perspectives137Recent advances in dispersion and alignment of fillers in PVDF-based composites for high-performance dielectric energy storage92Boosting zinc-ion storage in hydrated vanadium oxides via migration regulation116Lithium nitrate regulated carbonate electrolytes for practical Li-metal batteries: Mechanisms, principles and strategies92Metal–organic framework-derived advanced oxygen electrocatalysts as air-cathodes for Zn–air batteries: recent trends and future perspectives111High-entropy mechanism to boost ionic conductivity558Li+ migration and transformation at the interface: A review for stable Li metal anode86Solvent Molecule Design Enables Excellent Charge Transfer Kinetics for a Magnesium Metal Anode112Creating water-in-salt-like environment using coordinating anions in non-concentrated aqueous electrolytes for efficient Zn batteries109Halide solid-state electrolytes for all-solid-state batteries: structural design, synthesis, environmental stability, interface optimization and challenges133Interfacial Challenges and Strategies toward Practical Sulfide-Based Solid-State Lithium Batteries147On a high-capacity aluminium battery with a two-electron phenothiazine redox polymer as a positive electrode84Progress of transition metal sulfides used as lithium-ion battery anodes95Recent advances in the utilization of covalent organic frameworks (COFs) as electrode materials for supercapacitors142Surface-dominated potassium storage enabled by single-atomic sulfur for high-performance K-ion battery anodes94Strengths, weaknesses, opportunities, and threats (SWOT) analysis of supercapacitors: A review172Robust NASICON-type iron-based Na4Fe3(PO4)2(P2O7) cathode for high temperature sodium-ion batteries132Manipulation of π-aromatic conjugation in two-dimensional Sn-organic materials for efficient lithium storage96Discriminating Active BN Sites in Coralloidal B, N Dual‐Doped Carbon Nano‐Bundles for Boosted Zn‐Ion Storage Capability155Terminal Group‐Oriented Self‐Assembly to Controllably Synthesize a Layer‐by‐Layer SnSe2 and MXene Heterostructure for Ultrastable Lithium Storage82Rational Design of Electrode Materials for Advanced Supercapacitors: From Lab Research to Commercialization447Enabling Highly Reversible Zn Anode by Multifunctional Synergistic Effects of Hybrid Solute Additives182State of the art of lithium-ion battery material potentials: An analytical evaluations, issues and future research directions188High Entropy Enabling the Reversible Redox Reaction of V 4+ /V 5+ Couple in NASICON‐Type Sodium Ion Cathode172Designing All-Solid-State Batteries by Theoretical Computation: A Review122Dynamically Interfacial pH‐Buffering Effect Enabled by N ‐Methylimidazole Molecules as Spontaneous Proton Pumps toward Highly Reversible Zinc‐Metal Anodes171A Fluorinated Covalent Organic Framework with Accelerated Oxygen Transfer Nanochannels for High‐Performance Zinc–Air Batteries89A High‐Energy NASICON‐Type Na 3.2 MnTi 0.8 V 0.2 (PO 4 ) 3 Cathode Material with Reversible 3.2‐Electron Redox Reaction for Sodium‐Ion Batteries115Electron and Ion Transport in Lithium and Lithium-Ion Battery Negative and Positive Composite Electrodes386Multiple Accessible Redox-Active Sites in a Robust Covalent Organic Framework for High-Performance Potassium Storage196Recent advances of cathode materials for zinc-ion hybrid capacitors191Preferential Pyrolysis Construction of Carbon Anodes with 8400 h Lifespan for High‐Energy‐Density K‐ion Batteries96A dielectric electrolyte composite with high lithium-ion conductivity for high-voltage solid-state lithium metal batteries574The Influences of DMF Content in Composite Polymer Electrolytes on Li + ‐Conductivity and Interfacial Stability with Li‐Metal91Realizing High Capacity and Zero Strain in Layered Oxide Cathodes via Lithium Dual-Site Substitution for Sodium-Ion Batteries238Prussian Blue Analogues with Optimized Crystal Plane Orientation and Low Crystal Defects toward 450 Wh kg−1 Alkali‐Ion Batteries138Cathode Materials and Chemistries for Magnesium Batteries: Challenges and Opportunities120Advances in biomass-derived electrode materials for energy storage and circular carbon economy108Integrated solution for a stable and high-performance zinc-ion battery using an electrolyte additive81Multifunctional Electrolyte Additives for Better Metal Batteries129Separation performance and fouling analyses of nanofiltration membrane for lithium extraction from salt lake brine95Sodium-Ion Battery: Can It Compete with Li-Ion?89Synergistic Cooperation of Zn(002) Texture and Amorphous Zinc Phosphate for Dendrite-Free Zn Anodes174Robust iron-based cathode for ultralong-lasting Na-ion battery with a wide operation-temperature107Design of phosphorus-doped porous hard carbon/Si anode with enhanced Li-ion kinetics for high-energy and high-power Li-ion batteries102Reaction-passivation mechanism driven materials separation for recycling of spent lithium-ion batteries1012D‐Layer‐Structure Bi to Quasi‐1D‐Structure NiBi 3 : Structural Dimensionality Reduction to Superior Sodium and Potassium Ion Storage117Health monitoring by optical fiber sensing technology for rechargeable batteries82Advanced anode materials for potassium batteries: Sorting out opportunities and challenges by potassium storage mechanisms126Recent progress on MOF/MXene nanoarchitectures: A new era in coordination chemistry for energy storage and conversion90Design principles for NASICON super-ionic conductors146Hierarchical Architecture Engineering of Branch‐Leaf‐Shaped Cobalt Phosphosulfide Quantum Dots: Enabling Multi‐Dimensional Ion‐Transport Channels for High‐Efficiency Sodium Storage132Recent Advancements of Graphene‐Based Materials for Zinc‐Based Batteries: Beyond Lithium‐Ion Batteries103Revealing the origin of high-thermal-stability of single-crystal Ni-rich cathodes toward higher-safety batteries82A Deeper Understanding of Metal Nucleation and Growth in Rechargeable Metal Batteries Through Theory and Experiment106Li, Na, K, Mg, Zn, Al, and Ca Anode Interface Chemistries Developed by Solid‐State Electrolytes115Amorphous Materials for Lithium‐Ion and Post‐Lithium‐Ion Batteries92Manipulating Li2S2/Li2S mixed discharge products of all-solid-state lithium sulfur batteries for improved cycle life175Recent Progress on Phase Engineering of Nanomaterials185A weakly ion pairing electrolyte designed for high voltage magnesium batteries97Electrochemical Processes and Reactions In Rechargeable Battery Materials Revealed via In Situ Transmission Electron Microscopy131Achieving a high loading of cathode in PVDF-based solid-state battery81Electrolyte Additives for Stable Zn Anodes196Morphology evolution of CoNi‐LDHs synergistically engineered by precipitant and variable cobalt for asymmetric supercapacitor with superior cycling stability139Optimizing electronic synergy of atomically dispersed dual-metal Ni–N 4 and Fe–N 4 sites with adjacent Fe nanoclusters for high-efficiency oxygen electrocatalysis158Advances in inorganic, polymer and composite electrolytes: Mechanisms of Lithium-ion transport and pathways to enhanced performance135Li/Ni Intermixing: The Real Origin of Lattice Oxygen Stability in Co‐Free Ni‐Rich Cathode Materials86Roadmap for rechargeable batteries: present and beyond224Challenges, Solutions and Future Trends in EV-Technology: A Review148Zinc iso-plating/stripping: toward a practical Zn powder anode with ultra-long life over 5600 h102Regulation of Coordination Chemistry for Ultrastable Layered Oxide Cathode Materials of Sodium‐Ion Batteries204Opportunities and challenges in cathode development for non-lithium-ion batteries135Complementary probes for the electrochemical interface107Hard carbon anode for lithium-, sodium-, and potassium-ion batteries: Advancement and future perspective107Production of Renewable Hydrocarbon Biofuels with Lignocellulose and Its Derivatives over Heterogeneous Catalysts223Boosting Multielectron Reaction Stability of Sodium Vanadium Phosphate by High-Entropy Substitution128Monitoring thermal runaway of lithium-ion batteries by means of gas sensors99Navigating phase diagram complexity to guide robotic inorganic materials synthesis83A data-driven bifunctional oxygen electrocatalyst with a record-breaking ΔE = 0.57 V for ampere-hour-scale zinc-air batteries114High-efficiently doping nitrogen in kapok fiber-derived hard carbon used as anode materials for boosting rate performance of sodium-ion batteries128Single Atom Catalysts Based on Earth-Abundant Metals for Energy-Related Applications309Challenges and Progress in Rechargeable Magnesium‐Ion Batteries: Materials, Interfaces, and Devices90Prussian Blue Analogue-Templated Nanocomposites for Alkali-Ion Batteries: Progress and Perspective88Multiple Redox‐Active Centers in An Azatriangulenetrione‐Based Covalent Organic Framework for High‐Capacity, High‐Rate and Ultra‐Stable Sodium‐Ion Batteries85Solid-State lithium-ion battery electrolytes: Revolutionizing energy density and safety93Rechargeable Batteries for the Electrification of Society: Past, Present, and Future81Mechanically Robust Bismuth-Embedded Carbon Microspheres for Ultrafast Charging and Ultrastable Sodium-Ion Batteries176Porous Carbon Materials: from Traditional Synthesis, Machine Learning‐Assisted Design, to Their Applications in Advanced Energy Storage and Conversion92Prussian blue analogues for advanced non-aqueous sodium ion batteries: Redox mechanisms, key challenges and modification strategies93Reshaping Electrical Double Layer via Synergistic Dual Additives for Ah‐Level Zinc Battery109Battery technologies for grid-scale energy storage249Understanding solid-state battery electrolytes using atomistic modelling and machine learning105Poly( p -benzoquinono)diimidazole-Linked Covalent Organic Framework as An Efficient Anode Endues Sodium-Ion Batteries with High Performance and Wide Temperature Adaptability81

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  50. Graphene‐Supported Atomically Dispersed Metals as Bifunctional Catalysts for Next‐Generation Batteries Based on Conversion Reactions

    Advanced Materials · 2021-10-22

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