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RESEARCH PAPER · Advanced Synthesis & Catalysis · 2020

Recent Advances in Asymmetric Organomulticatalysis

Xiao Xiao, Bingxuan Shao, Yin‐Jie Lu, Qian‐Qian Cao, Chun‐Nian Xia, Fen‐Er Chen

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Recent Advances in Asymmetric OrganomulticatalysisOriginalCatalytic asymmetric synthesis of monofluoroalkenes and gem -difluoroalkenes: advances and perspectives102Enantioselective synthesis of functionalized 1,4-dihydropyrazolo-[4′,3′:5,6]pyrano[2,3- b ]quinolines through ferrocenyl-phosphine-catalyzed annulation of modified MBH carbonates and pyrazolones22Recent applications of asymmetric organocatalytic annulation reactions in natural product synthesis56Umpolung coupling of pyridine-2-carboxaldehydes and propargylic carbonates via N-heterocyclic carbene/palladium synergetic catalysis15FT-IR, Molecular Structure and Nonlinear Optical Properties of 2-(pyranoquinolin-4-yl)malononitrile (PQMN): A DFT Approach5TfOH-Catalyzed [4 + 1] Annulation of p-Quinone Methides with α-Aryl Diazoacetates: Straightforward Access to Highly Functionalized 2,3-Dihydrobenzofurans34Stereodivergent Synthesis of Enantioenriched 2,3-Disubstituted Dihydrobenzofurans via a One-Pot C–H Functionalization/Oxa-Michael Addition Cascade129Construction of Enantioenriched 4,5,6,7‐Tetrahydrofuro[2,3‐ b ]pyridines through a Multicatalytic Sequence Merging Gold and Amine Catalysis27Asymmetric organocatalyzed synthesis of coumarin derivatives20Reduction of Oximes and Hydrazones: Asymmetric and Diastereoselective Approaches9Regiodivergent Organocatalytic Reactions52Iridium‐Catalyzed Enantioselective and Diastereoselective Hydrogenation of Racemic β’‐Keto‐β‐Amino Esters via Dynamic Kinetic Resolution14Pd‐catalyzed decarboxylative [3 + 2] cycloaddition: Assembly of highly functionalized spirooxindoles bearing two quaternary centers8Acceleration by Double Activation Catalysis and its Negation with Rising Temperature in Hydrolysis of Cellobiose with Phthalic and Hydrochloric Acids2Mechanochemical, Water‐Assisted Asymmetric Transfer Hydrogenation of Ketones Using Ruthenium Catalyst23Copper-Catalyzed Ullmann-Type Coupling and Decarboxylation Cascade of Arylhalides with Malonates to Access α-Aryl Esters41Conjugate addition of 1,3-dicarbonyl compounds to maleimides using bifunctional primary amine‒(thio)phosphoramide organocatalysts15A highly stereoselective and recyclable microgel-supported bifunctional sulfonamide organocatalyst for asymmetric alcoholysis of meso -cyclic anhydrides: a thermo-responsive “organic nanoreactor”8Atom- and step-economic 1,3-thiosulfonylation of activated allenes with thiosulfonates to access vinyl sulfones/sulfides28Highly diastereo- and enantioselective synthesis of multisubstituted allylic amino acid derivatives by allylic alkylation of a chiral glycine-based nickel complex and vinylethylene carbonates6Organocatalytic atroposelective N -alkylation: divergent synthesis of axially chiral sulfonamides and biaryl amino phenols15Robust, scalable construction of an electrophilic deuterated methylthiolating reagent: facile access to SCD 3 -containing scaffolds36Further developments of β,γ-unsaturated α-ketoesters as versatile synthons in asymmetric catalysis24Synergistic Pd/Cu Catalyzed Allylation of Cyclic Ketimine Esters with Vinylethylene Carbonates: Enantioselective Construction of Trisubstituted Allylic 2H‐Pyrrole Derivatives16Palladium-Catalyzed Asymmetric [3 + 2] Annulation of Vinylethylene Carbonates with Alkenes Installed on Cyclic N-Sulfonyl Imines: Highly Enantio- and Diastereoselective Construction of Chiral Tetrahydrofuran Scaffolds Bearing Three Vicinal and Quaternary Stereocenters17Synergistic Strategies in Aminocatalysis39Recent Advances in the Total Synthesis of Aspidosperma and Kopsia Alkaloids Using Tetracyclic Pyridocarbazoles as Versatile Building Blocks22Chiral Aziridine Phosphines as Highly Effective Promoters of Asymmetric Rauhut–Currier Reaction6β-Amino Acid Organocatalysts in the Asymmetric Michael Addition of Isobutyraldehyde to N-Substituted Maleimides4Construction of Non-Biaryl Atropisomeric Amide Scaffolds Bearing a C–N Axis via Enantioselective Catalysis35Organocatalyzed Synthesis of Tetrahydro‐α‐Carboline Derivatives Bearing N,O‐Acetals8Synergistic Organo‐Organocatalysis2Regio- and stereoselective syntheses of chiral α-quaternary ( Z )-trisubstituted allylic amino acids via synergistic Pd/Cu catalysis13Carbenes and Nitrenes0Mechanism of a Dually Catalyzed Enantioselective Oxa-Pictet–Spengler Reaction and the Development of a Stereodivergent Variant11β‐Arylation of Racemic Secondary Benzylic Alcohols to Access Enantioenriched β‐Arylated Alcohols12β‐Arylation of Racemic Secondary Benzylic Alcohols to Access Enantioenriched β‐Arylated Alcohols1Enamine/Iminium‐based Dual Organocatalytic Systems for Asymmetric Catalysis and Synthesis14Asymmetric construction of enantioenriched furo[2,3- b ]pyridines through sequential gold, palladium/phosphoric acid catalysis11Auto tandem triple cascade organocatalysis: access to bis-lactone and butenolide derivatives3Enantioselective cross-dehydrogenative coupling enabled by organocatalysis27Photochemical Synthesis of Chiral Heterocycles via Asymmetric Carbon‐Heteroatom Bond Formation8Is the E/Z Iminium Ratio a Good Enantioselectivity Predictor in Iminium Catalysis?1Asymmetric amino acid-based homogeneous catalysts0Deuterated methylselenylating reagents designed for diverse Se -methyl- d 3 scaffold construction15Dynamic kinetic resolution of tert -alcohols via combination of a lipase/Brønsted acid in a biphasic reaction medium4Enantioselective Preparation of Chiral Succinimide Derivatives by Mechanochemical Catalytic Michael Addition3Dynamic Hydrogen Bonding Tuned Enantioselectivity Control in Cobaloxime‐Chiral Amine Cooperative Catalysis0Dynamic Hydrogen Bonding Tuned Enantioselectivity Control in Cobaloxime‐Chiral Amine Cooperative Catalysis6Recent advances in the application of CuAAC for the covalent immobilization of homogeneous catalysts, a decade of progress2Mimicking Natural Catalytic Systems: Design Inspired Beyond the Traditional Paradigm0

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  1. Catalytic asymmetric synthesis of monofluoroalkenes and gem -difluoroalkenes: advances and perspectives

    Organic Chemistry Frontiers · 2021-01-01

    Xiaojuan Zhang, Yamin Cheng, Xiaowei Zhao, Zhong‐Yan Cao, Xiao Xiao, Ying Xu

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  2. Enantioselective synthesis of functionalized 1,4-dihydropyrazolo-[4′,3′:5,6]pyrano[2,3- b ]quinolines through ferrocenyl-phosphine-catalyzed annulation of modified MBH carbonates and pyrazolones

    Chemical Communications · 2021-01-01

    Xiao Xiao, Bingxuan Shao, Jingyi Li, Zehui Yang, Yin‐Jie Lu, Fei Ling, Weihui Zhong

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  3. Recent applications of asymmetric organocatalytic annulation reactions in natural product synthesis

    Chemical Society Reviews · 2021-01-01

    Nengzhong Wang, Zugen Wu, Junjie Wang, Nisar Ullah, Yixin Lü

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  4. Umpolung coupling of pyridine-2-carboxaldehydes and propargylic carbonates via N-heterocyclic carbene/palladium synergetic catalysis

    Chemical Communications · 2021-01-01

    Weiyang Bi, Yunhui Yang, Song Ye, Congyang Wang

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  5. FT-IR, Molecular Structure and Nonlinear Optical Properties of 2-(pyranoquinolin-4-yl)malononitrile (PQMN): A DFT Approach

    Biointerface Research in Applied Chemistry · 2021-02-15

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  6. TfOH-Catalyzed [4 + 1] Annulation of p-Quinone Methides with α-Aryl Diazoacetates: Straightforward Access to Highly Functionalized 2,3-Dihydrobenzofurans

    The Journal of Organic Chemistry · 2021-05-15

    Zuolin Lu, Qingchun Zhang, Miaolin Ke, Sha Hu, Xiao Xiao, Fen‐Er Chen

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  7. Stereodivergent Synthesis of Enantioenriched 2,3-Disubstituted Dihydrobenzofurans via a One-Pot C–H Functionalization/Oxa-Michael Addition Cascade

    Journal of the American Chemical Society · 2021-06-01

    Dong‐Xing Zhu, Jianguo Liu, Ming‐Hua Xu

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  8. Construction of Enantioenriched 4,5,6,7‐Tetrahydrofuro[2,3‐ b ]pyridines through a Multicatalytic Sequence Merging Gold and Amine Catalysis

    Advanced Synthesis & Catalysis · 2021-07-29

    Manon Genet, Abdelilah Takfaoui, Jérôme Marrot, Christine Greck, Xavier Moreau

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  9. Asymmetric organocatalyzed synthesis of coumarin derivatives

    Beilstein Journal of Organic Chemistry · 2021-08-03

    Natália M. Moreira, Lorena S. R. Martelli, Arlene Gonçalves Corrêa

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  10. Reduction of Oximes and Hydrazones: Asymmetric and Diastereoselective Approaches

    Current Organic Chemistry · 2021-08-15

    João Ribeiro, Cláudia Alves, Ana L. Cardoso, Susana M. M. Lopes, Teresa M. V. D. Pinho e Melo

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  11. Regiodivergent Organocatalytic Reactions

    Catalysts · 2021-08-22

    Mayavan Viji, Srinu Lanka, Jaeuk Sim, Chanhyun Jung, Heesoon Lee, Manjunatha Vishwanath, Jae‐Kyung Jung

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  12. Iridium‐Catalyzed Enantioselective and Diastereoselective Hydrogenation of Racemic β’‐Keto‐β‐Amino Esters via Dynamic Kinetic Resolution

    Advanced Synthesis & Catalysis · 2021-08-24

    Fei Ling, Yifan Wang, An Huang, Ze Wang, Shiliang Wang, Jiayin He, Xianghua Zhao, Weihui Zhong

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  13. Pd‐catalyzed decarboxylative [3 + 2] cycloaddition: Assembly of highly functionalized spirooxindoles bearing two quaternary centers

    Applied Organometallic Chemistry · 2021-12-02

    Tiantian Li, Xinju Zhu, Hui Jiang, Yanong Wang, Nan Zheng, Tian Peng, Rui Gao, Linlin Shi, Xin‐Qi Hao, Mao‐Ping Song

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  14. Acceleration by Double Activation Catalysis and its Negation with Rising Temperature in Hydrolysis of Cellobiose with Phthalic and Hydrochloric Acids

    ChemPhysChem · 2021-12-03

    Nikolay Tarabanko, Viktor Aleksandrovich Golubkov, Valentin Vladimirovich Sychev, Valery Evgenievich Tarabanko, Оxana P. Тaran

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  15. Mechanochemical, Water‐Assisted Asymmetric Transfer Hydrogenation of Ketones Using Ruthenium Catalyst

    ChemCatChem · 2021-12-07

    Vanessza Judit Kolcsár, György Szőllősi

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  16. Copper-Catalyzed Ullmann-Type Coupling and Decarboxylation Cascade of Arylhalides with Malonates to Access α-Aryl Esters

    Organic Letters · 2021-12-21

    Fei Cheng, Tao Chen, Yin-Qiu Huang, Jiawei Li, Chen Zhou, Xiao Xiao, Fen‐Er Chen

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  17. Conjugate addition of 1,3-dicarbonyl compounds to maleimides using bifunctional primary amine‒(thio)phosphoramide organocatalysts

    Molecular Catalysis · 2021-12-30

    Viktória Kozma, György Szőllősi

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  18. A highly stereoselective and recyclable microgel-supported bifunctional sulfonamide organocatalyst for asymmetric alcoholysis of meso -cyclic anhydrides: a thermo-responsive “organic nanoreactor”

    New Journal of Chemistry · 2022-01-01

    Fei Xiong, Chao Ma, Yi‐Ren Zhu, Chen Sun, Lu Chen, Yanjun Zhang, Yuanjie Zhu, Zhonghua Wang

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  19. Atom- and step-economic 1,3-thiosulfonylation of activated allenes with thiosulfonates to access vinyl sulfones/sulfides

    Chemical Communications · 2022-01-01

    Xiao Xiao, Hongyu Tian, Yin-Qiu Huang, Yin‐Jie Lu, Jingjie Fang, Gao-Jie Zhou, Fen‐Er Chen

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  20. Highly diastereo- and enantioselective synthesis of multisubstituted allylic amino acid derivatives by allylic alkylation of a chiral glycine-based nickel complex and vinylethylene carbonates

    Organic & Biomolecular Chemistry · 2022-01-01

    Chao Yu, Yuyan Yu, Longwu Sun, Xinzhi Li, Zhigang Liu, Miaolin Ke, Fen‐Er Chen

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  21. Organocatalytic atroposelective N -alkylation: divergent synthesis of axially chiral sulfonamides and biaryl amino phenols

    Organic Chemistry Frontiers · 2022-01-01

    Xiao Xiao, Yin‐Jie Lu, Hongyu Tian, Hai-Jie Zhou, Jiawei Li, Yi-Ping Yao, Miaolin Ke, Fen‐Er Chen

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  22. Robust, scalable construction of an electrophilic deuterated methylthiolating reagent: facile access to SCD 3 -containing scaffolds

    Chemical Communications · 2022-01-01

    Xiao Xiao, Yin-Qiu Huang, Hongyu Tian, Jun Bai, Fei Cheng, Xu Wang, Miaolin Ke, Fen‐Er Chen

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  23. Further developments of β,γ-unsaturated α-ketoesters as versatile synthons in asymmetric catalysis

    iScience · 2022-02-10

    Ruixian Deng, Tian‐Jiao Han, Xiang Gao, Yuan-Fu Yang, Guang‐Jian Mei

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  24. Synergistic Pd/Cu Catalyzed Allylation of Cyclic Ketimine Esters with Vinylethylene Carbonates: Enantioselective Construction of Trisubstituted Allylic 2H‐Pyrrole Derivatives

    Advanced Synthesis & Catalysis · 2022-03-23

    Miaolin Ke, Yuyan Yu, Ke Zhang, Sheng Zuo, Zhigang Liu, Xiao Xiao, Fen‐Er Chen

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  25. Palladium-Catalyzed Asymmetric [3 + 2] Annulation of Vinylethylene Carbonates with Alkenes Installed on Cyclic N-Sulfonyl Imines: Highly Enantio- and Diastereoselective Construction of Chiral Tetrahydrofuran Scaffolds Bearing Three Vicinal and Quaternary Stereocenters

    The Journal of Organic Chemistry · 2022-04-04

    Miaolin Ke, Bolin Qiao, Yuyan Yu, Xinzhi Li, Xiao Xiao, Shijun Li, Yu Lan, Fen‐Er Chen

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  26. Synergistic Strategies in Aminocatalysis

    Chemistry - A European Journal · 2022-06-06

    Antonio Del Vecchio, Arianna Sinibaldi, Valeria Nori, Giuliana Giorgianni, Graziano Di Carmine, Fabio Pesciaioli

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  27. Recent Advances in the Total Synthesis of Aspidosperma and Kopsia Alkaloids Using Tetracyclic Pyridocarbazoles as Versatile Building Blocks

    Advanced Synthesis & Catalysis · 2022-06-29

    Nengzhong Wang, Xiao Xiao, Cheng‐Xiong Liu, Hui Qin Yao, Nianyu Huang, Kun Zou

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  28. Chiral Aziridine Phosphines as Highly Effective Promoters of Asymmetric Rauhut–Currier Reaction

    Symmetry · 2022-08-08

    Aleksandra Buchcic-Szychowska, Stanisław Leśniak, Michał Rachwalski

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  29. β-Amino Acid Organocatalysts in the Asymmetric Michael Addition of Isobutyraldehyde to N-Substituted Maleimides

    Catalysts · 2022-09-02

    Viktória Kozma, Zsolt Szakonyi, György Szőllősi

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  30. Construction of Non-Biaryl Atropisomeric Amide Scaffolds Bearing a C–N Axis via Enantioselective Catalysis

    Molecules · 2022-10-04

    Xiao Xiao, Biao Chen, Yi-Ping Yao, Hai-Jie Zhou, Xu Wang, Nengzhong Wang, Fen‐Er Chen

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  31. Organocatalyzed Synthesis of Tetrahydro‐α‐Carboline Derivatives Bearing N,O‐Acetals

    European Journal of Organic Chemistry · 2022-10-20

    Manon Genet, Abdelilah Takfaoui, Jérôme Marrot, Christine Greck, Xavier Moreau

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  32. Synergistic Organo‐Organocatalysis

    Asymmetric Organocatalysis · 2022-11-18

    Fabio Pesciaioli, Valeria Nori, Arianna Sinibaldi, Armando Carlone

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  33. Regio- and stereoselective syntheses of chiral α-quaternary ( Z )-trisubstituted allylic amino acids via synergistic Pd/Cu catalysis

    Chemical Communications · 2023-01-01

    Miaolin Ke, Yuyan Yu, Longwu Sun, Xinzhi Li, Qianqian Cao, Xiao Xiao, Fen‐Er Chen

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  34. Carbenes and Nitrenes

    Organic Reaction Mechanisms/Organic reaction mechanisms · 2023-01-20

    Emmanuel Gras, Stefan Chassaing

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  35. Mechanism of a Dually Catalyzed Enantioselective Oxa-Pictet–Spengler Reaction and the Development of a Stereodivergent Variant

    ACS Catalysis · 2023-01-27

    Alafate Adili, John-Paul Webster, Chenfei Zhao, Sharath Chandra Mallojjala, Moises A. Romero-Reyes, Ion Ghiviriga, Khalil A. Abboud, Mathew J. Vetticatt, Daniel Seidel

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  36. β‐Arylation of Racemic Secondary Benzylic Alcohols to Access Enantioenriched β‐Arylated Alcohols

    Angewandte Chemie International Edition · 2023-05-30

    Miao Wang, Jinyu Zhang, Yanyan Yang, Weijun Tang, Dong Qian Xue, Jianliang Xiao, Huaming Sun, Chao Wang

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  37. β‐Arylation of Racemic Secondary Benzylic Alcohols to Access Enantioenriched β‐Arylated Alcohols

    Angewandte Chemie · 2023-05-30

    Miao Wang, Jinyu Zhang, Yanyan Yang, Weijun Tang, Dong Qian Xue, Jianliang Xiao, Huaming Sun, Chao Wang

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  38. Enamine/Iminium‐based Dual Organocatalytic Systems for Asymmetric Catalysis and Synthesis

    Chemistry - An Asian Journal · 2023-11-01

    Diksha Gambhir, Sanjay Singh, Ravi Pratap Singh

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  39. Asymmetric construction of enantioenriched furo[2,3- b ]pyridines through sequential gold, palladium/phosphoric acid catalysis

    Organic Chemistry Frontiers · 2024-01-01

    Ke Xie, Guo-Qing Zhang, Bao-Rui Kong, Zhi‐Jun Jia, Zhichao Chen, Gu Zhan, Wei Du, Ying‐Chun Chen

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  40. Auto tandem triple cascade organocatalysis: access to bis-lactone and butenolide derivatives

    Chemical Communications · 2024-01-01

    Stéphane Wittmann, Elodie Deschamps, Chloée Bournaud, Régis Guillot, Jean‐François Brière, Giang Vo‐Thanh, Martial Toffano

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  41. Enantioselective cross-dehydrogenative coupling enabled by organocatalysis

    Green Chemistry · 2024-01-01

    Quanbin Jiang, Jie Luo, Xiaodan Zhao

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  42. Photochemical Synthesis of Chiral Heterocycles via Asymmetric Carbon‐Heteroatom Bond Formation

    Advanced Synthesis & Catalysis · 2024-04-28

    Yogesh Brijwashi Sharma, Sanjukta Saha, Murali Mohan Guru

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  43. Is the E/Z Iminium Ratio a Good Enantioselectivity Predictor in Iminium Catalysis?

    Chemistry - A European Journal · 2024-06-17

    Matthijs A. Hellinghuizen, Pietro Franceschi, Jana Roithová

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  44. Asymmetric amino acid-based homogeneous catalysts

    Elsevier eBooks · 2025-01-01

    Diego Quiroga, Sergio Alejandro Torres‐Cortés, Ericsson David Coy-Barrera

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  45. Deuterated methylselenylating reagents designed for diverse Se -methyl- d 3 scaffold construction

    Green Chemistry · 2025-01-01

    Xiao Xiao, Hongyu Tian, Jiachen Sun, Jun Bai, Min Wang, Biao Chen, Yu-Xia Jin, Haibo Jiang, Dang Cheng, Fen-Er Chen

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  46. Dynamic kinetic resolution of tert -alcohols via combination of a lipase/Brønsted acid in a biphasic reaction medium

    Green Chemistry · 2025-01-01

    Takusho Kin, Satoshi Horino, Jihoon Moon, Momoka Tsuda, Harald Gröger, Shuji Akai, Kyohei Kanomata

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  47. Enantioselective Preparation of Chiral Succinimide Derivatives by Mechanochemical Catalytic Michael Addition

    ChemCatChem · 2025-02-25

    György Szőllősi, Kristóf András Kőszegi, Ákos Kukovecz, Márton Szabados

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  48. Dynamic Hydrogen Bonding Tuned Enantioselectivity Control in Cobaloxime‐Chiral Amine Cooperative Catalysis

    Angewandte Chemie · 2025-05-16

    Zhao Liu, Long Zhang, Sanzhong Luo, Xiaotian Qi

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  49. Dynamic Hydrogen Bonding Tuned Enantioselectivity Control in Cobaloxime‐Chiral Amine Cooperative Catalysis

    Angewandte Chemie International Edition · 2025-05-16

    Zhao Liu, Long Zhang, Sanzhong Luo, Xiaotian Qi

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  50. Recent advances in the application of CuAAC for the covalent immobilization of homogeneous catalysts, a decade of progress

    Tetrahedron · 2025-12-19

    Antony E. Fernandes, Olivier Riant, Alain Marie Jonas

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