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RESEARCH PAPER · ACS Catalysis · 2020

Nontraditional Catalyst Supports in Surface Organometallic Chemistry

Ryan J. Witzke, Alon Chapovetsky, Matthew P. Conley, David M. Kaphan, Massimiliano Delferro

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Nontraditional Catalyst Supports in Surface Organometallic ChemistryOriginalImmobilization of molecular catalysts on solid supports via atomic layer deposition for chemical synthesis in sustainable solvents20In crystallo organometallic chemistry40Strain in Silica-Supported Ga(III) Sites: Neither Too Much nor Too Little for Propane Dehydrogenation Catalytic Activity31Lewis Acid Strength of Interfacial Metal Sites Drives CH 3 OH Selectivity and Formation Rates on Cu‐Based CO 2 Hydrogenation Catalysts81Lewis Acid Strength of Interfacial Metal Sites Drives CH3OH Selectivity and Formation Rates on Cu‐Based CO2 Hydrogenation Catalysts12Surface vs Homogeneous Organo-Hafnium Catalyst Ion-Pairing and Ligand Effects on Ethylene Homo- and Copolymerizations29Beyond the Active Site. Cp*ZrMe3/Sulfated Alumina‐Catalyzed Olefin Polymerization Tacticity via Catalyst⋅⋅⋅Surface Ion‐Pairing14Ethylene Polymerization Activity of (R3P)Ni(codH)+ (cod = 1,5-cylcooctadiene) Sites Supported on Sulfated Zirconium Oxide17Deciphering Metal–Oxide and Metal–Metal Interplay via Surface Organometallic Chemistry: A Case Study with CO 2 Hydrogenation to Methanol99Hydrogen‐Bonding‐Induced Heterogenization of Nickel and Palladium Catalysts for Copolymerization of Ethylene with Polar Monomers99Hydrogen‐Bonding‐Induced Heterogenization of Nickel and Palladium Catalysts for Copolymerization of Ethylene with Polar Monomers24Computational Investigation of the Role of Active Site Heterogeneity for a Supported Organovanadium(III) Hydrogenation Catalyst26Speciality Grand Challenges in Organometallic Catalysis4Challenges with atomically dispersed supported metal catalysts: Controlling performance, improving stability, and enhancing metal loading2Surface organometallic and coordination chemistry approach to formation of single site heterogeneous catalysts3Photoresponsive Palladium and Nickel Catalysts for Ethylene Polymerization and Copolymerization87Photoresponsive Palladium and Nickel Catalysts for Ethylene Polymerization and Copolymerization7Single sites in heterogeneous catalysts: separating myth from reality42Reduction of Amides to Amines with Pinacolborane Catalyzed by Heterogeneous Lanthanum Catalyst La(CH2C6H4NMe2-o)3@SBA-1516Molecular approaches to heterogeneous catalysis58Single-Molecule Kinetics of Styrene Hydrogenation on Silica-Supported Vanadium: The Role of Disorder for Single-Atom Catalysts14Enhanced Catalysis Based on the Surface Environment of the Silica-Supported Metal Complex83Separation Strategies in Organometallic Catalysis2Promoting Ethylene (co)Polymerization in Aliphatic Hydrocarbon Solvents Using tert ‐Butyl Substituted Nickel Catalysts50Organometallic Chemistry on Oxide Surfaces0The Control of the Coordination Chemistry for the Genesis of Heterogeneous Catalytically Active Sites in Oxidation Reactions0The coordination chemistry of oxide and nanocarbon materials10An Ionic Cluster Strategy for Performance Improvements and Product Morphology Control in Metal-Catalyzed Olefin–Polar Monomer Copolymerization105Surface science approach to the heterogeneous cycloaddition of CO2 to epoxides catalyzed by site-isolated metal complexes and single atoms: a review71A Heterogeneous Palladium Catalyst for the Polymerization of Olefins Prepared by Halide Abstraction Using Surface R 3 Si + Species19A Heterogeneous Palladium Catalyst for the Polymerization of Olefins Prepared by Halide Abstraction Using Surface R 3 Si + Species10Designing Sites in Heterogeneous Catalysis: Are We Reaching Selectivities Competitive With Those of Homogeneous Catalysts?424K-edge XANES Analysis for Catalytically Relevant Molecular and Supported Vanadium Complexes0A general strategy for heterogenizing olefin polymerization catalysts and the synthesis of polyolefins and composites144A Cocatalyst Strategy to Enhance Ruthenium‐Mediated Metathesis Reactivity towards Electron‐Deficient Substrates1A Cocatalyst Strategy to Enhance Ruthenium‐Mediated Metathesis Reactivity towards Electron‐Deficient Substrates28Lithium-Ion Battery Materials as Tunable, “Redox Non-Innocent” Catalyst Supports13Computational Aspects of Single-Molecule Kinetics for Coupled Catalytic Cycles: A Spectral Analysis4A Heterogeneous Iridium Catalyst for the Hydroboration of Pyridines14Integrated Experimental and Computational K-Edge X-ray Absorption Near-Edge Structure Analysis of Vanadium Catalysts32Prospective Evaluation of an Amide-Based Zinc Scaffold as an Anti-Alzheimer Agent: In Vitro, In Vivo, and Computational Studies6Influence of Silica-Supported Alkylaluminum on Heterogeneous Zwitterionic Anilinonaphthoquinone Nickel and Palladium-Catalyzed Ethylene Polymerization and Copolymerization with Polar Monomers28Pd/Cu 2 O/CuO as Active Sites on the Cyclometalated Pd(II)/Cu(II) Nanosheet: Active Centre Formation, Synergistic and Catalytic Mechanism5The Control of the Coordination Chemistry for the Genesis of Heterogeneous Catalytically Active Sites in Oxidation Reactions**1The Control of the Coordination Chemistry for the Genesis of Heterogeneous Catalytically Active Sites in Oxidation Reactions**15Formation of a Strong Heterogeneous Aluminum Lewis Acid on Silica28Formation of a Strong Heterogeneous Aluminum Lewis Acid on Silica0Grafting of Group‐10 Organometallic Complexes on Silicas: Differences and Similarities, Surprises and Rationale17Sulfated Zirconium Metal–Organic Frameworks as Well-Defined Supports for Enhancing Organometallic Catalysis37Single‐Site Heterogeneous Organometallic Ir Catalysts Embedded on Graphdiyne: Structural Manipulation Beyond the Carbon Support11Molecular Catalyst Synthesis Strategies to Prepare Atomically Dispersed Fe-N-C Heterogeneous Catalysts52Dual roles of trifluoroborate in nickel-catalyzed ethylene polymerization: Electronic perturbation and anchoring for heterogenization10Rapid atom-efficient polyolefin plastics hydrogenolysis mediated by a well-defined single-site electrophilic/cationic organo-zirconium catalyst82A Co-Anchoring Strategy for the Synthesis of Polar Bimodal Polyethylene2Ceria supported single-site catalysts prepared by surface organometallic chemistry for the reduction of nitrogen oxides by ammonia (NH3-SCR)0Assembled Organoruthenium(II) for Formaldehyde Decomposition and Hydrogen Production3Synthesis of platinum nanoparticles on strontium titanate nanocuboids via surface organometallic grafting for the catalytic hydrogenolysis of plastic waste45Effects of surface acidity on the structure of organometallics supported on oxide surfaces21Palladium-catalyzed synthesis of oil-based functionalized polyolefins12‘Catalyst + X’ strategies for transition metal-catalyzed olefin-polar monomer copolymerization74Effects of Synthesis Procedures on Pt–Sn Alloy Formation and Their Catalytic Activity for Propane Dehydrogenation9Mechanistic Insights into Molecular Crystalline Organometallic Heterogeneous Catalysis through Parahydrogen-Based Nuclear Magnetic Resonance Studies11Synthesis and Surface Attachment of Molecular Re(I) Complexes Supported by Functionalized Bipyridyl Ligands32High-Throughput Experimentation, Theoretical Modeling, and Human Intuition: Lessons Learned in Metal–Organic-Framework-Supported Catalyst Design25A Tungsten Oxo Alkylidene Supported on Sulfated Zirconium Oxide for Olefin Metathesis0Cationic Tantalum Hydrides Catalyze Hydrogenolysis and Alkane Metathesis Reactions of Paraffins and Polyethylene38Outer‐Shell Self‐Supported Nickel Catalysts for the Synthesis of Polyolefin Composites40Outer‐Shell Self‐Supported Nickel Catalysts for the Synthesis of Polyolefin Composites5Heterogenized Molecular Rhodium Phosphine Catalysts within Metal–Organic Frameworks for Alkene Hydroformylation61A co-anchoring strategy for the synthesis of polar bimodal polyethylene76Silica Supported Organometallic IrI Complexes Enable Efficient Catalytic Methane Borylation27Silica‐Supported 1st Row Transition Metal (Nano)Catalysts: Synthetic and Catalytic Insight24Dual-Site Polymeric Heterogeneous α-Diimine Ni Catalysts with Tailored Spatial Distribution for Ethylene Polymerization17How Solid Surfaces Control Stability and Interactions of Supported Cationic CuI(dppf) Complexes─A Solid-State NMR Study6Single‐Site Carbon‐Supported Metal‐Oxo Complexes in Heterogeneous Catalysis: Structure, Reactivity, and Mechanism1Single‐Site Carbon‐Supported Metal‐Oxo Complexes in Heterogeneous Catalysis: Structure, Reactivity, and Mechanism14Heterogenization Strategies for Nickel Catalyzed Synthesis of Polyolefins and Composites64Functionalization of Poly (1‐hexene) with Maleic Anhydride: The Effect of Reaction Parameters3MAO- and Borate-Free Activating Supports for Group 4 Metallocene and Post-Metallocene Catalysts of α-Olefin Polymerization and Oligomerization11Synthesis and Surface Attachment of Molecular Re(I) Hydride Species with Silatrane Functionalized Bipyridyl Ligands20Supported Electrophilic Organoruthenium Catalyst for the Hydrosilylation of Olefins12Samarium- and Ytterbium-Grafted Periodic Mesoporous Silica for Carbon Dioxide Capture and Conversion22Synthesis and Characterization of Metal Phthalocyanine Complex Using Substituted 4-Nitrophthalonitrile Ligand0A Supported Ziegler-Type Organohafnium Site Metabolizes Polypropylene8Aberration-Corrected STEM to Determine the Surface Coverage and Distribution of Immobilized Molecular Complexes1Oxidative Grafting for Catalyst Synthesis in Surface Organometallic Chemistry9Catalysts Prepared from Atomically Dispersed Ce(III) on MgO Rival Bulk Ceria for CO Oxidation10Aberration-Corrected STEM to Determine the Surface Coverage and Distribution of Immobilized Molecular Complexes0Rapid Polyolefin Plastic Hydrogenolysis Mediated by Single-Site Heterogeneous Electrophilic/Cationic Organo-group IV Catalysts19Biomass-derived substrate hydrogenation over rhodium nanoparticles supported on functionalized mesoporous silica4Introduction to single-atom catalysts1Lewis acid-induced homo- and heterogeneous nickel catalysts for ethylene polymerization and copolymerization with polar monomers6Recent advances in the design of high-performance cobalt-based catalysts for dry reforming of methane44Tailoring the Active Species Distribution of Heterogeneous Catalyst for Regulating the Chain Structure of Nascent Polyethylene3Exploiting Organometallic Chemistry to Functionalize Small Cuprous Oxide Colloidal Nanocrystals13Synthesis of Polar-functionalized Isotactic Polypropylenes Using Commercial Heterogeneous Ziegler–Natta Catalyst32Formation of Strong Boron Lewis Acid Sites on Silica13Photoelectrochemical CO 2 Reduction to CO Enabled by a Molecular Catalyst Attached to High-Surface-Area Porous Silicon38Recent Advances on Computational Modeling of Supported Single-Atom and Cluster Catalysts: Characterization, Catalyst–Support Interaction, and Active Site Heterogeneity23Positional heterogenization effect in salicylaldimine nickel catalyzed ethylene polymerization1Silicon Nitride Surface Enabled Propane Dehydrogenation Catalyzed by Supported Organozirconium14Supported Organochromium Ethylene Oligomerization Enabled by Surface Lithiation8Alkene Isomerization Using a Heterogeneous Nickel-Hydride Catalyst27Silica‐Grafted Isonicotinamide to Boost Catalytic Activity of Cobalt Nanoparticles in Hydrogenation and Reductive Amination Reactions4Demystifying group-4 polyolefin hydrogenolysis catalysis: Gaseous propane hydrogenolysis mechanism over the same catalysts5Intercalative Redox Tuning for Cu/Li x Mn 2 O 4 -Catalyzed Oxidative Alkyne Coupling5Highly robust iminopyridyl nickel catalysts for the synthesis of polyethylene wax17Highly Active Immobilized Catalyst for Ethylene Polymerization: Neutral Single Site Y(III) Complex Bearing Bulky Silylallyl Ligand1Integrated Ziegler–Natta/Brookhart‐Ni Catalysts for the Synthesis of Sutured Polar High‐Impact Polypropylenes3Integrated Ziegler–Natta/Brookhart‐Ni Catalysts for the Synthesis of Sutured Polar High‐Impact Polypropylenes9Electronic Interactions between Anchored Molecular Catalyst and Support3Statistical analysis of HAADF-STEM images to determine the surface coverage and distribution of immobilized molecular complexes14C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid8C−H Bond Activation by Sulfated Zirconium Oxide is Mediated by a Sulfur‐Centered Lewis Superacid2A picolinamide iridium catalyst immobilized on an aluminum-hydride anchor for the selective dehydrogenation of neat formic acid0Preparation of bimodal polyethylene with different branching densities by a co-anchoring strategy4Techno-economic and life cycle analyses of the synthesis of a platinum–strontium titanate catalyst15Well-defined Pt(0) heterogeneous hydrosilylation catalysts supported by a surface bound phosphenium ligand2Photoelectrocatalytic reduction of CO2 to formate using immobilized molecular manganese catalysts on oxidized porous silicon16An Adaptive Palladium Single-Atom Catalyst Enabling Reactivity Switching between Borylation and C–C Coupling49Introduction of [DABCO](SO3H)2CoCl4 as a new catalyst for the synthesis of quinoxaline, 2,4,5−triarylimidazole, N,N′−diarylformamidine, and benzazole derivatives2Supported Single‐Atom Manganese Catalysts for the Trimerization of Ethylene2Cobalt doping induced electronic effects boosts the hydrogenation of phenol to cyclohexanone5Ultra-Confined Environments May Restrict the Possible Configurations of Supported Metal Complexes1Ir-Promoted Cobalt-Based Catalysts for Dry Reforming of Methane4Cycloaddition of CO2 to epoxides catalyzed by homogeneous metalorganic complexes under ambient conditions: an update6Metal–organic frameworks: frontier of surface organometallic chemistry3Oligomeric α-diimine nickel catalysts for enhanced ethylene polymerization6Heterogeneous SHOP-Type Ni Catalyzed Ethylene Polymerization3An integrated techno-economic analysis and life cycle assessment of lube oil production from post-use polypropylene and comparison with conventional base oils0Facile C–N bond construction from a molecular model of iron on silica0Structure–Activity–Kinetics Relationship of Ruthenium Species in Transfer Hydrogenation of Biomass-derived Levulinic Acid to γ-Valerolactone0Heterogenized homogeneous catalysts for photoelectrochemical carbon dioxide reduction: a path toward ideal hybrid systems2Regioselective Hydrosilylation Catalysis with Supported Well-Defined Pt(0) Complexes: Effects of Surface Anions and Phosphenium Ligands0Group 4 Metallocenes Supported on Sulfated Zirconium Oxide Catalyze Benzene C–H Borylation0A New Metal‐Ester Bonding Motif for the Synthesis of Hybrid Molecular Catalysts on Metal Oxide Supports Leads to Tunable Reactivity0A New Metal‐Ester Bonding Motif for the Synthesis of Hybrid Molecular Catalysts on Metal Oxide Supports Leads to Tunable Reactivity0Rational design of heterogeneous single-site catalysts via surface organometallic chemistry0Surface Functionalities, Speciation, and Strength of Brønsted Acid Sites from a 31 P– 109 Ag NMR Tag1Ionic Cluster Catalyst Assembly Strategy for Ethylene Polymerization and Copolymerization0

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    Hong Liu, Haiyuan Zou, Mei Wang, Hongliang Dong, Dan Wang, Fan Li, Hao Dai, Tao Song, Shuting Wei, Yongfei Ji, Chenguang Wang, Lele Duan

    Read original paper ↗ ·
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