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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2020

Exsolution of Catalytically Active Iridium Nanoparticles from Strontium Titanate

Eleonora Calì, Gwilherm Kerherve, Faris Naufal, Kalliopi Kousi, Dragos Neagu, Evangelos I. Papaioannou, Melonie P. Thomas, Beth S. Guiton, Ian S. Metcalfe, John T. S. Irvine, David J. Payne

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Exsolution of Catalytically Active Iridium Nanoparticles from Strontium TitanateOriginalEmergence and Future of Exsolved Materials214In Situ Exsolution of Noble-Metal Nanoparticles on Perovskites as Enhanced Peroxidase Mimics for Bioanalysis59Hydrothermal Synthesis of Iridium-Substituted NaTaO3 Perovskites6CO2-mediated oxidative dehydrogenation of light alkanes to olefins: Advances and perspectives in catalyst design and process improvement107A New in-situ Exsolution Supporting Framework for Metal Nanoparticle Growth0New Insights into Crystal Defects, Oxygen Vacancies, and Phase Transition of Ir-TiO220An efficient strategy to enhance the photocatalytic activity of Ir-doped SrTiO 3 : a hybrid DFT approach8A Robust Approach to In Situ Exsolve Highly Dispersed and Stable Electrocatalysts3Low‐Temperature Exsolution of Ni–Ru Bimetallic Nanoparticles from A‐Site Deficient Double Perovskites31The metal/oxide heterointerface delivered by solid-based exsolution strategy: A review53Exsolution of CoFe(Ru) nanoparticles in Ru-doped (La0.8Sr0.2)0.9Co0.1Fe0.8Ru0.1O3−δ for efficient oxygen evolution reaction57High-Temperature 2D Optical Relaxation Visualizes Enhanced Oxygen Exchange Kinetics at Metal-Mixed Conducting Oxide Interfaces3Interfacial electron transfer in heterojunction nanofibers for highly efficient oxygen evolution reaction13Exsolution on perovskite oxides: morphology and anchorage of nanoparticles55Transition Metal‐based Perovskite Oxides: Emerging Electrocatalysts for Oxygen Evolution Reaction82Real-time insight into the multistage mechanism of nanoparticle exsolution from a perovskite host surface62Roadmap on exsolution for energy applications71Methane Catalytic Combustion under Lean Conditions over Pristine and Ir-Loaded La1−xSrxMnO3 Perovskites: Efficiency, Hysteresis, and Time-on-Stream and Thermal Aging Stabilities5Direct Observation of Sample Dynamics in the Gaseous Environment: A Perspective on Current Trends and Future Directions of In Situ Gas Cell Transmission Electron Microscopy14Nonreducing Ambient Atmosphere: Pulsed Electric Current Treatment of Co/Ni Doped Perovskite Oxides to Achieve Exsolution Enhanced Electrochemical Performance8Enhanced Stability of Iridium Nanocatalysts via Exsolution for the CO2 Reforming of Methane7Architecting multi-active center on 3DOM La0.76Ce0.19Ag0.05Mn0.9Co0.1O3-δ perovskite for soot oxidation11Conductive origin and design principles of electrically controllable high conductivity La-doped perovskites4Reversible exsolution of iron from perovskites for highly selective syngas production via chemical looping dry reforming of methane22Local Structures of Ex-Solved Nanoparticles Identified by Machine-Learned Potentials9Metal–Perovskite Interfacial Engineering to Boost Activity in Heterogeneous Catalysis6Synergistic growth of nickel and platinum nanoparticles via exsolution and surface reaction34Dielectric Barrier Plasma Discharge Exsolution of Nanoparticles at Room Temperature and Atmospheric Pressure13Constructing active lattice oxygen in high covalent perovskites for boosting catalytic activity18Thermal stability and coalescence dynamics of exsolved metal nanoparticles at charged perovskite surfaces39Critical assessment of the exsolution process in Cu-doped SrTiO 3 by a combined spectroscopic approach11New opportunities for tailored nanoparticle catalysts through exsolution from inherently disordered defect fluorite-type oxides1Perovskite oxide crystallization and exsolution: Laser-treatment dual synchronous regulation mechanism1Ligation of Single-Site Ruthenium within Perovskite Oxides for Efficient Conversion of Thermodynamically Stable Molecules3Bimetallic Fe–Ni exsolution from A site deficient SrTiO 3 : insight into the reciprocal role of metal active centers4Competitive modulation of carrier dynamics by valence states in Rh- and Ir-doped SrTiO3 for solar hydrogen production0Synthesis of exsolved iridium nanoparticles on titanium oxide nanorods as an efficient catalyst for the oxygen evolution reaction in acidic media2

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  1. Emergence and Future of Exsolved Materials

    Small · 2021-03-31

    Kalliopi Kousi, Chenyang Tang, Ian S. Metcalfe, Dragos Neagu

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  2. In Situ Exsolution of Noble-Metal Nanoparticles on Perovskites as Enhanced Peroxidase Mimics for Bioanalysis

    Analytical Chemistry · 2021-04-02

    Xiaoqian Jiang, Xiaoyu Wang, Anqi Lin, Hui Wei

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  3. Hydrothermal Synthesis of Iridium-Substituted NaTaO3 Perovskites

    Nanomaterials · 2021-06-10

    David Burnett, Christopher D. Vincent, Jasmine A. Clayton, Reza J. Kashtiban, Richard I. Walton

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  4. CO2-mediated oxidative dehydrogenation of light alkanes to olefins: Advances and perspectives in catalyst design and process improvement

    Applied Catalysis A General · 2021-06-23

    Yahya Gambo, Sagir Adamu, Gazali Tanimu, Ibrahim Munkaila Abdullahi, Rahima A. Lucky, Mohammed S. Ba‐Shammakh, Mohammad Mozahar Hossain

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  5. A New in-situ Exsolution Supporting Framework for Metal Nanoparticle Growth

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  6. New Insights into Crystal Defects, Oxygen Vacancies, and Phase Transition of Ir-TiO2

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    Vignesh Kumaravel, Enrico Bianchetti, Snehamol Mathew, Steven John Hinder, John Bartlett, Cristiana Di Valentin, Suresh C. Pillai

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  7. An efficient strategy to enhance the photocatalytic activity of Ir-doped SrTiO 3 : a hybrid DFT approach

    New Journal of Chemistry · 2021-12-09

    Brindaban Modak

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  8. A Robust Approach to In Situ Exsolve Highly Dispersed and Stable Electrocatalysts

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    Mengchu Wang, Bike Zhang, Jiaqi Ding, Fanxing Zhang, Rui Tu, Matthew T. Bernards, Yi He, Pengfei Xie, Yao Shi

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  9. Low‐Temperature Exsolution of Ni–Ru Bimetallic Nanoparticles from A‐Site Deficient Double Perovskites

    Small · 2022-02-19

    Jia Hong Guo, Rongsheng Cai, Eleonora Calì, George E. Wilson, Gwilherm Kerherve, Sarah J. Haigh, Stephen J. Skinner

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  10. The metal/oxide heterointerface delivered by solid-based exsolution strategy: A review

    Chemical Engineering Journal · 2022-03-17

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  11. Exsolution of CoFe(Ru) nanoparticles in Ru-doped (La0.8Sr0.2)0.9Co0.1Fe0.8Ru0.1O3−δ for efficient oxygen evolution reaction

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  12. High-Temperature 2D Optical Relaxation Visualizes Enhanced Oxygen Exchange Kinetics at Metal-Mixed Conducting Oxide Interfaces

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    Emily J. Skiba, Nicola H. Perry

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  13. Interfacial electron transfer in heterojunction nanofibers for highly efficient oxygen evolution reaction

    Nanoscale · 2022-11-28

    Lei Fu, Jun Hong Zhou, Qinyuan Deng, Jiaming Yang, Qinghao Li, Zihe Zhu, Kai Wu

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  14. Exsolution on perovskite oxides: morphology and anchorage of nanoparticles

    Chemical Communications · 2023-01-01

    Thomas Ruh, Dominic Berkovec, Florian Schrenk, Christoph Rameshan

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  15. Transition Metal‐based Perovskite Oxides: Emerging Electrocatalysts for Oxygen Evolution Reaction

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    Deeksha Deeksha, Pawanpreet Kour, Imtiaz Ahmed, Sunny Sharma, S. K. Sharma, Kamlesh Yadav, Yogendra Kumar Mishra

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  16. Real-time insight into the multistage mechanism of nanoparticle exsolution from a perovskite host surface

    Nature Communications · 2023-03-29

    Eleonora Calì, Melonie P. Thomas, Rama Krishnan Vasudevan, Ji Wu, Oriol Gavalda‐Diaz, Katharina Tinka Marquardt, Eduardo Saiz, Dragos Neagu, Raymond R. Unocic, Stephen C. Parker, Beth S. Guiton, David J. Payne

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  17. Roadmap on exsolution for energy applications

    Journal of Physics Energy · 2023-04-28

    Dragos Neagu, John T. S. Irvine, Jiayue Wang, Bilge Yildiz, Alexander Karl Opitz, Jürgen Fleig, Yuhao Wang, Jiapeng Liu, Longyun Shen, Francesco Ciucci, Brian Ashley Rosen, Yongchun Xiao, Kui Xie, Guangming Yang, Zongping Shao, Yubo Zhang, Jakob Michael Reinke, Travis Anthony Schmauss, Scott Alexander Barnett, Roelf Maring, Vasileios Kyriakou, Usman Mushtaq, Mihalis N. Tsampas, Youdong Kim, Ryan O’Hayre, Alfonso J. Carrillo, Thomas Ruh, Lorenz Lindenthal, Florian Schrenk, Christoph Rameshan, Evangelos I. Papaioannou, Kalliopi Kousi, Ian S. Metcalfe, Xiaoxiang Xu, Gang Yu Liu

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  18. Methane Catalytic Combustion under Lean Conditions over Pristine and Ir-Loaded La1−xSrxMnO3 Perovskites: Efficiency, Hysteresis, and Time-on-Stream and Thermal Aging Stabilities

    Nanomaterials · 2023-08-07

    Catherine Drosou, Ersi Nikolaraki, Theodora Georgakopoulou, Sotiris Fanourgiakis, V.T. Zaspalis, Ioannis V. Yentekakis

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  19. Direct Observation of Sample Dynamics in the Gaseous Environment: A Perspective on Current Trends and Future Directions of In Situ Gas Cell Transmission Electron Microscopy

    The Journal of Physical Chemistry C · 2023-09-13

    Manisha De Alwis Goonatilleke, Melonie P. Thomas, Ahamed Ullah, Rose H. Pham, Beth S. Guiton

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  20. Nonreducing Ambient Atmosphere: Pulsed Electric Current Treatment of Co/Ni Doped Perovskite Oxides to Achieve Exsolution Enhanced Electrochemical Performance

    The Journal of Physical Chemistry Letters · 2023-10-24

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  21. Enhanced Stability of Iridium Nanocatalysts via Exsolution for the CO2 Reforming of Methane

    ACS Applied Nano Materials · 2023-12-01

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  22. Architecting multi-active center on 3DOM La0.76Ce0.19Ag0.05Mn0.9Co0.1O3-δ perovskite for soot oxidation

    Applied Surface Science · 2023-12-24

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  23. Conductive origin and design principles of electrically controllable high conductivity La-doped perovskites

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  24. Reversible exsolution of iron from perovskites for highly selective syngas production via chemical looping dry reforming of methane

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  25. Local Structures of Ex-Solved Nanoparticles Identified by Machine-Learned Potentials

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  27. Synergistic growth of nickel and platinum nanoparticles via exsolution and surface reaction

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  28. Dielectric Barrier Plasma Discharge Exsolution of Nanoparticles at Room Temperature and Atmospheric Pressure

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  29. Constructing active lattice oxygen in high covalent perovskites for boosting catalytic activity

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  31. Critical assessment of the exsolution process in Cu-doped SrTiO 3 by a combined spectroscopic approach

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  32. New opportunities for tailored nanoparticle catalysts through exsolution from inherently disordered defect fluorite-type oxides

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  35. Bimetallic Fe–Ni exsolution from A site deficient SrTiO 3 : insight into the reciprocal role of metal active centers

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