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RESEARCH PAPER · National Science Review · 2020

Unleash electron transfer in C–H functionalization by mesoporous carbon-supported palladium interstitial catalysts

Xiaorui Zhao, Yueqiang Cao, Linlin Duan, Ruoou Yang, Zheng Rong Jiang, Chao Tian, Shangjun Chen, Xuezhi Duan, De Chen, Ying Wan

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Unleash electron transfer in C–H functionalization by mesoporous carbon-supported palladium interstitial catalystsOriginalDirect (Hetero)arylation of Heteroarenes Catalyzed by Unsymmetrical Pd-PEPPSI-NHC Complexes under Mild Conditions42The self-assembly of gold nanoparticles in large-pore ordered mesoporous carbons1Recent Advances in the Marriage of Catalyst Nanoparticles and Mesoporous Supports28ZIF-derived metal/N-doped porous carbon nanocomposites: efficient catalysts for organic transformations47Palladium catalyzed radical relay for the oxidative cross-coupling of quinolines33Cooperation of Pt and TiOx in the Hydrogenation of Nitrobenzothiazole50Iron Nanoparticles Protected by Chainmail‐structured Graphene for Durable Electrocatalytic Nitrate Reduction to Nitrogen173Iron Nanoparticles Protected by Chainmail‐structured Graphene for Durable Electrocatalytic Nitrate Reduction to Nitrogen62Solid‐State Redox Mediators for Decoupled H 2 Production: Principle and Challenges58A strong metal–support interaction strategy for enhanced binder-free electrocatalytic nitrate reduction30Optimizing the p charge of S in p-block metal sulfides for sulfur reduction electrocatalysis300Glycerol cascade oxidation on nearby Pt1-Ptn sites stabilized by Cu-CuZrOx0Metal and Metal Oxide Supported on Ordered Mesoporous Carbon as Heterogeneous Catalysts129Moiré Superlattice Structure in Two‐Dimensional Catalysts: Synthesis, Property and Activity23Intermediate Confinement for Selective Ammonia Electrosynthesis from Nitrate on Robust Mesoporous Metal Catalysts71Counting d ‐Orbital Vacancies of Transition‐Metal Catalysts for the Sulfur Reduction Reaction39Counting d ‐Orbital Vacancies of Transition‐Metal Catalysts for the Sulfur Reduction Reaction3Mesostructures Engineering to Promote Selective Nitrate‐to‐Ammonia Electroreduction68Electrocatalytic nitrate reduction: Selectivity at the crossroads between ammonia and nitrogen80Atomic Cu Sites Engineering Enables Efficient CO2 Electroreduction to Methane with High CH4/C2H4 Ratio59Emerging Multiscale Porous Anodes toward Fast Charging Lithium-Ion Batteries107Engineering interfacial architectures toward nitrate electrocatalysis and nitrogen neutral cycle24Synthesis and catalytic oxidation performance of gold@mesoporous carbon core-shell and yolk-shell hollow nanomaterials2Curved plane increases the d vacancy population of Pd for green production of cyclohexanone11Monomicelle‐Directed Synthesis of Mesoporous Carbon Nanomaterials for Energy Storage and Conversion7Self‐Reconstruction Induced Electronic Metal‐Support Interaction for Modulated Cu+ Sites on TiO2 Nanofibers in Electrocatalytic Nitrate Conversion24Phenylcarbazole-stabilized palladium catalysts for efficient acetylene hydrochlorination3Persulfate-Based Advanced Oxidation Reforming of Polyethylene Terephthalate Fiber into Formate via Singlet Oxygen Activation25A d‐Electron Deficient Pd Trimer for Exceptional Pyridine Hydrogenation Activity and Selectivity0A d‐Electron Deficient Pd Trimer for Exceptional Pyridine Hydrogenation Activity and Selectivity5In-situ reconstruction of electrocatalysts for efficient energy and environmental electrocatalytic reactions17Construction of Asymmetric Anion Layer to Accelerate Carrier Reaction Kinetics and Thermodynamically Promote Photocatalytic CO2 Reduction29eg Electron Occupancy as a Descriptor for Designing Iron Single‐Atom Electrocatalysts23A d-Electron Deficient Ru Single-Atom Catalyst that Increases the Carbon Utilization of Lignin Derivatives for the Production of Green Cyclohexanol and Methanol15Adjacent double boron vacancies in boron nitride: Catalysts with high activity and low energy barriers for HCHO oxidation0High-dimensional strain unlocks fast polysulfide redox kinetics for lithium-sulfur batteries51Ultrasonic Synthesis of Fluorene-Modified Pd/SAC Catalysts for Ultra-Stable Acetylene Hydrochlorination2A fluorescent hyperbranched thermoresponsive polymer for highly efficient detection and separation with real-time and in-situ monitoring of nitroaromatic pollutants1Low-Spin State Single-Atom Ni Catalyst for Electrochemical Carbon Dioxide Reduction at Ampere-Level Current7Ligand exchange determines the catalytic activity of the sulfur reduction reaction in lithium-sulfur batteries0Spike‐Embedded Nanocatalysts via Metal‐Directed Carbonization for Highly Efficient and Robust Semi‐Hydrogenation0Regulated and controlled electronic band structure of borophene nanoribbons using phosphorus for various adsorbing configurations: A first-principles calculation0Palladium Black from Decomposition Is a Directly Reusable Catalyst0Density functional theory-guided construction of catalytic systems for the valorization of ultra-dilute carbon dioxide0

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  2. The self-assembly of gold nanoparticles in large-pore ordered mesoporous carbons

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  3. Recent Advances in the Marriage of Catalyst Nanoparticles and Mesoporous Supports

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  5. Palladium catalyzed radical relay for the oxidative cross-coupling of quinolines

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  6. Cooperation of Pt and TiOx in the Hydrogenation of Nitrobenzothiazole

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  7. Iron Nanoparticles Protected by Chainmail‐structured Graphene for Durable Electrocatalytic Nitrate Reduction to Nitrogen

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  8. Iron Nanoparticles Protected by Chainmail‐structured Graphene for Durable Electrocatalytic Nitrate Reduction to Nitrogen

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  9. Solid‐State Redox Mediators for Decoupled H 2 Production: Principle and Challenges

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  10. A strong metal–support interaction strategy for enhanced binder-free electrocatalytic nitrate reduction

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  12. Glycerol cascade oxidation on nearby Pt1-Ptn sites stabilized by Cu-CuZrOx

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  13. Metal and Metal Oxide Supported on Ordered Mesoporous Carbon as Heterogeneous Catalysts

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  14. Moiré Superlattice Structure in Two‐Dimensional Catalysts: Synthesis, Property and Activity

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  15. Intermediate Confinement for Selective Ammonia Electrosynthesis from Nitrate on Robust Mesoporous Metal Catalysts

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  16. Counting d ‐Orbital Vacancies of Transition‐Metal Catalysts for the Sulfur Reduction Reaction

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  18. Mesostructures Engineering to Promote Selective Nitrate‐to‐Ammonia Electroreduction

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  19. Electrocatalytic nitrate reduction: Selectivity at the crossroads between ammonia and nitrogen

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  20. Atomic Cu Sites Engineering Enables Efficient CO2 Electroreduction to Methane with High CH4/C2H4 Ratio

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  21. Emerging Multiscale Porous Anodes toward Fast Charging Lithium-Ion Batteries

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  22. Engineering interfacial architectures toward nitrate electrocatalysis and nitrogen neutral cycle

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