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RESEARCH PAPER · ACS Catalysis · 2020

Encapsulation Methods for Control of Catalyst Deactivation: A Review

Hope O. Otor, Joshua B. Steiner, Cristina García‐Sancho, Ana C. Alba‐Rubio

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Encapsulation Methods for Control of Catalyst Deactivation: A ReviewOriginalMetal@Zeolite Hybrid Materials for Catalysis293In Situ Anchoring Ultra Small Au Nanoparticles by Conformal Coating of Carbon Layer within the Micro-Environments of Mesoporous Silica for Highly Efficient Catalytic Reduction of 4-nitrophenol4In Situ-Grown Island-Shaped Hollow Graphene on TaON with Spatially Separated Active Sites Achieving Enhanced Visible-Light CO2 Reduction63Novel one-dimensional Cu@C nanofibers: direct solid-state synthesis and applications in electrocatalytic water splitting9Increasing the activity of the Cu/CuAl 2 O 4 /Al 2 O 3 catalyst for the RWGS through preserving the Cu 2+ ions35Molecular modeling of interfacial layer-by-layer assembly towards functionalized capsule materials1Overall Insights into Sustainable Utilization of Methane and Carbon Dioxide in Heterogeneous Catalysis1Photocatalytic hydroxylation of benzene to phenol over organosilane-functionalized FeVO 4 nanorods43Promoted activity of annealed Rh nanoclusters on thin films of Al 2 O 3 /NiAl(100) in the dehydrogenation of Methanol-d 44Colloidal Nanocrystals as Electrocatalysts with Tunable Activity and Selectivity81A Career in Catalysis: James A. Dumesic7Carbon-Supported Nitrogen-Doped Graphene-Wrapped Copper Nanoparticles: An Effective Catalyst for the Oxidative Carbonylation of Methanol25Hydrogenolysis of Lignin-Derived Aromatic Ethers over Heterogeneous Catalysts119Tandem In 2 O 3 -Pt/Al 2 O 3 catalyst for coupling of propane dehydrogenation to selective H 2 combustion309Subsurface-Regulated PtGa Nanoparticles Confined in Silicalite-1 for Propane Dehydrogenation83Improving Hydrothermal Stability of Supported Metal Catalysts for Biomass Conversions: A Review219Density Functional Theory Study of Small Au Nanoparticles Anchored on the Inner Surface of Mesoporous Co3O4 for the Catalytic Reduction of 4-Nitrophenol16Agglomeration of Pt nanoparticles on the g-C3N4 surface dominated by oriented attachment mechanism and way of inhibition6Titanosilicate zeolite supported Pt nanoparticles with electronic metal-support interactions for efficient methanol steam reforming26Precisely Engineered Supported Gold Clusters as a Stable Catalyst for Propylene Epoxidation78Precisely Engineered Supported Gold Clusters as a Stable Catalyst for Propylene Epoxidation18Recent advances in alkaline hydrogen oxidation reaction107Interfacial Bifunctional Effect Promoted Non-Noble Cu/Fe y MgO x Catalysts for Selective Hydrogenation of Acetylene49Heterogeneous Catalysis14Photoinduction of palladium single atoms supported on defect-containing γ-AlOOH nanoleaf for efficient trans-stilbene epoxidation9Semi-quantitative design of synergetic surficial/interfacial sites for the semi-continuous oxidation of glycerol6Separation Strategies in Organometallic Catalysis2Boosted Hydrodeoxygenation of Lignin-Derived Phenolics to Cycloalkanes with a Complex Copper Acid Catalyst20The Size‐Dependent Catalytic Performances of Supported Metal Nanoparticles and Single Atoms for the Upgrading of Biomass‐Derived 5‐Hydroxymethylfurfural, Furfural, and Levulinic acid20BTP‐Rh@g‐C3N4 as an efficient recyclable catalyst for dehydrogenation and borrowing hydrogen reactions10Excellent stability for catalytic oxidation of methane over core–shell Pd@silicalite-1 with complete zeolite shell in wet conditions5Nanomaterials25Stabilization of Exposed Metal Nanocrystals in High‐Temperature Heterogeneous Catalysis47Noble metal (Pd, Pt and Rh) incorporated LaFeO3 perovskite oxides for catalytic oxidative cracking of n-propane21Recent Progress and Prospects in Catalytic Water Treatment378Effect of the reductive treatment on the state and electrocatalytic behavior of Pt in catalysts supported on Ti0.8Mo0.2O2-C composite7Chromium Oxides as Structural Modulators of Rhodium Dispersion on Ceria to Generate Active Sites for NO Reduction16Au 3+ Species-Induced Interfacial Activation Enhances Metal–Support Interactions for Boosting Electrocatalytic CO 2 Reduction to CO98Surface second harmonic generation spectra of titania coated Au NPs4An All-in-One Zeolite@Ru-Al2o3 Nanoplatform Towards Highly Efficient, Anticoking, and Recyclable Hydrocarbon Cracking Catalysis1Efficient production of ethylene glycol from cellulose over Co@C catalysts combined with tungstic acid14Encapsulation of the Hoveyda–Grubbs 2nd generation catalyst in magnetically separable alginate/mesoporous carbon beads for olefin metathesis reactions in water11Metal@hollow carbon sphere nanoreactors for sustainable biomass and CO 2 valorization19Recent advances in biomass-derived platform chemicals to valeric acid synthesis40Stability improvement of a Pt/TiO 2 photocatalyst during photocatalytic pure water splitting41Supported Gold Clusters as a Stable Catalyst for Propylene Epoxidation0Understanding Synthesis and Structural Variation of Nanomaterials Through In Situ/Operando XAS and SAXS62Designing Sites in Heterogeneous Catalysis: Are We Reaching Selectivities Competitive With Those of Homogeneous Catalysts?424Fe3O4 nanoparticles encapsulated in boron nitride support via N-doped carbon layer as a peroxymonosulfate activator for pollutant degradation: Important role of metal boosted C–N sites16A review on the development of supported non-noble metal catalysts for the endothermic high temperature sulfuric acid decomposition step in the Iodine–Sulfur cycle for hydrogen production17Encapsulation of Metal Nanoparticles (MNPs) as Catalyst5Porous titania nanotube confined ultrafine platinum catalysts synthesized by atomic layer deposition with enhanced hydrolytic dehydrogenation performance47The Native Oxide Skin of Liquid Metal Ga Nanoparticles Prevents Their Rapid Coalescence during Electrocatalysis64Investigation of reusability and deactivation mechanism of supported platinum catalysts in the practical isomerization of allylic esters8Transesterification of Glycerol to Glycerol Carbonate over Mg-Zr Composite Oxide Prepared by Hydrothermal Process15Peroxymonosulfate activation on a chainmail catalyst via an electron shuttle mechanism for efficient organic pollutant removal87An all-in-one zeolite@Ru–Al2O3 nanoplatform toward highly efficient, anti-coking, and recyclable hydrocarbon cracking catalysis1Recent advances on the construction of encapsulated catalyst for catalytic applications23Inverse Oxide/Metal Catalysts for CO2 Hydrogenation to Methanol31Tuning Strong Metal–Support Interaction Kinetics on Pt-Loaded TiO 2 (110) by Choosing the Pressure: A Combined Ultrahigh Vacuum/Near-Ambient Pressure XPS Study41Tuning the Product Distribution of Acetylene Dimerization through Bimetallic Metal–Organic Framework-Supported Nanoporous Systems23Cellulose hydrogenolysis to alcohol and ketone products using Co@C catalysts in the phosphoric acid aqueous solution8Effective catalytic hydrodechlorination removal of chloroanisole odorants in water using palladium catalyst confined in zeolite Y7The use of sol–gel processes in the development of supported catalysts43Metal Nanocatalyst Sintering Interrogated at Complementary Length Scales9Excellent catalytic oxidation performance on toluene over Pt supported on CeaTiOx with hierarchical tubular-like structures: Effects of Ce addition in CeaTiOx on activity of Pt/CeaTiOx12Photocatalytic formation of a gas permeable layer selectively deposited on supported metal nanoparticles for sintering-resistant thermal catalysis4Subsurface Ru-Triggered Hydrogenation Capability of TiO2–x Overlayer for Poison-Resistant Reduction of N-Heteroarenes43A hollow void catalyst of Co@C(Z-d)@void@CeO 2 for enhancing the performance and stability of the Fischer–Tropsch synthesis25Precise control of the catalyst interface at the atomic level13Recent developments of core–shell structured catalysts for the selective catalytic reduction of NO x with ammonia27Review on supported metal catalysts with partial/porous overlayers for stabilization20The mathematical catalyst deactivation models: a mini review66The phenomenon of “dead” metal in heterogeneous catalysis: opportunities for increasing the efficiency of carbon-supported metal catalysts29Unveiling effect of iron on pyrolysis of bisphenol A epoxy by comparisons of product characteristics and reaction mechanisms10Redispersion and Stabilization of Cu/MFI Catalysts by the Encapsulation Method for Ethanol Dehydrogenation25Review and Perspectives of Enhancement in the Catalytic Stability for the Complete Combustion of CO, CH4, and Volatile Organic Compounds39Thermal Aging of Rh/ZrO2–CeO2 Three-Way Catalysts under Dynamic Lean/Rich Perturbation Accelerates Deactivation via an Encapsulation Mechanism18Engineering nanointerfaces of Cu-based catalysts for balancing activity and stability of reverse water-gas-shift reaction24Nanoreactor Engineering Can Unlock New Possibilities for CO2 Tandem Catalytic Conversion to CC Coupled Products9Unraveling alkali-tolerance role of zeolite coupling CeWOx catalyst for NO reduction25Selectivity Regulation of Au/Titanate by Biochar Modification for Selective Oxidation of Benzyl Alcohol6The Fast Formation of a Highly Active Homogeneous Catalytic System upon the Soft Leaching of Pd Species from a Heterogeneous Pd/C Precursor12A mini-review on carbon and silicon-based yolk-shell structured catalysts for CO2 conversion: Design, advantages, and challenges14Recent advances and prospects in high purity H2 production from sorption enhanced reforming of bio-ethanol and bio-glycerol as carbon negative processes: A review45Construction of Ptδ+–O(H)–Ti3+ Species for Efficient Catalytic Production of Hydrogen36Reductive Treatment of Pt Supported on Ti0.8Sn0.2O2-C Composite: A Route for Modulating the Sn–Pt Interactions5Synthesis, Types, and Applications of Zeolite Capsule Catalysts5Coke resistant NiCo/CeO2 catalysts for dry reforming of methane derived from core@shell Ni@Co nanoparticles115Intramolecular engineering of defective terminations within triazine-based conjugated polymers for augmented photocatalytic H2 production and Cr(VI) reduction13PolyVinyl alcohol and copper nickel co‐doped titania nanocomposite: Designing, characterization, optical properties, and catalytic application in the synthesis of aryl derivatives of benzothiazole and benzimidazole3Solar‐driven co‐evolution of H2 and H2O2 from pure water splitting over emerging photocatalysts: Detailed mechanism and future outlook2Enteromorpha prolifera valorization to acetol over supported Pd catalysts: Role of the support12Quenching method to prepare ultra-low loading high-entropy catalyst for furfural selectively hydrogenation at ambient temperature40Removal of organic pollutants through hydroxyl radical-based advanced oxidation processes276A critical review towards the causes of the iron-based catalysts deactivation mechanisms in the selective oxidation of hydrogen sulfide to elemental sulfur from biogas24Recent Advances in Metal−Zeolite Catalysts for Direct Propane Dehydrogenation31A generalized strategy for the ultrafast encapsulation of metal oxide nanoclusters into zeolites1Carbon encapsulated nanoparticles: materials science and energy applications60Cobalt nanoparticles confined in silica networks with 3D hierarchical porous features for Fischer–Tropsch synthesis3Photocatalysis on Selective Hydroxylation of Benzene to Phenol0Rational design of metal-based nanocomposite catalysts for enhancing their stability in solid acid catalysis6Revolutionizing targeting precision: microfluidics-enabled smart microcapsules for tailored delivery and controlled release21A Review on Metal–Organic Framework as a Promising Catalyst for Biodiesel Production50Hybrid oxide coatings generate stable Cu catalysts for CO2 electroreduction122The Use of Sol–Gel Technology to Produce Nanomaterials for Air and Water Purification5In-Flow Heterogeneous Triplet–Triplet Annihilation Upconversion9Alteration of Hydrodeoxygenation Pathways of Ni/TiO 2 -A Catalyst through Controlled Regulation of Strong Metal–Support Interactions and Surface Acidity38Diamine‐Assistant Synthesis of Cu@MFI Catalysts for Ethanol Dehydrogenation9Comment on "AI in Healthcare: A Revolutionary Ally or an Ethical Dilemma?"0Molybdenum oxide-based catalyst towards better hydrogen production: effects of isothermal carburization2Tuning the strong metal support interaction of the Fischer-Tropsch synthesis silica-coated cobalt-based nano-catalyst32Titania-crystal-phase-engineered strong metal-support interactions and catalysis in CO2 hydrogenation19Noble-Metal-Free Metal Oxides for Catalyzing Acidic Oxygen and Hydrogen Evolution Reactions: Recent Developments and Future Perspectives60Photothermal conversion of CO2 with high activity and stability over Ni-based composite nanochains2Hydrogen Sensing with Palladium‐Based Materials: Mechanisms, Challenges, and Opportunities38The configuration of Auδ+-ZrO2δ− species induced activation enhances electrocatalytic CO2 to formate conversion15Tuning Adsorbate‐Mediated Strong Metal‐Support Interaction by Oxygen Vacancy: A Case Study in Ru/TiO 264Tuning Adsorbate‐Mediated Strong Metal‐Support Interaction by Oxygen Vacancy: A Case Study in Ru/TiO216Study on the Deactivation Mechanism of Ru/C Catalysts3Close Intimacy between PtIn Clusters and Zeolite Channels for Ultrastability toward Propane Dehydrogenation22Confining of PtCo into MCM-41-C for selective hydrogenation of biomass-derived unsaturated aldehydes6In situ synthesis of Rh@NaX catalyst for 1-hexene hydroformylation14Insights into reverse oxygen spillover effect induced via CeO2 modulation to enhance the stability of CuCoOx catalysts in hydrodeoxygenation of biomass derivatives26Hydrogenation of Ethyl Levulinate to Gamma-Valerolactone with Formic Acid and a Palladium–Manganese Catalyst Immobilized on Dendritic Fibrous Nanosilica (DFNS)11Optimization of catalyst service cycle and start-up considering the reactor-distillation-HEN integration and climate2N‐Doped Carbon Modified (NixFe1‐x)Se Supported on Vertical Graphene toward Efficient and Stable OER Performance26Hydrothermal Valorization of Biosugars with Heterogeneous Catalysts: Advances, Catalyst Deactivation, Mitigation Strategies and Perspectives1Strong Metal‐Support Interaction Triggered by Molten Salts5Strong Metal‐Support Interaction Triggered by Molten Salts20Cu nanoparticles immobilized in mesopores generated in zeolite for high-performing CO2 hydrogenation to methanol20Stability enhancement of molybdenum modified rutile – carbon composite supported platinum electrocatalysts by reductive pretreatment: Surface characteristics and advanced electrocatalytic properties3Encapsulating Transition Metal Nanoparticles inside Carbon (TM@C) Chainmail Catalysts for Hydrogen Evolution Reactions: A Review3Identification of Deactivation Mechanisms by the Periodic Transient Kinetic Method5Photothermal Dry Reforming of Methane on Yolk‐Shell Co–Ni Alloy@SiO2 Catalyst13Understanding and Tuning the Effects of H2O on Catalytic CO and CO2 Hydrogenation78A General Approach for Metal Nanoparticle Encapsulation Within Porous Oxides16The role of nitrogen and sulfur doping in the peroxymonosulfate activation of cobalt-immobilized Polygonatum kingianum dregs biochar9Catalytic hydroprocessing of yellow dodolla oil using thermally stable and mesoporous AlPO4-18 supported β-Mo2C, Ni3C, and WC nanoparticles to produce bio-jet fuel2Development of a salicylic acid-encapsulated zeolite–seaweed biochar composite for sustainable agricultural applications0Electron transfer in catalysis: from fundamentals to strategies90Non-oxidative coupling of methane via selective passivized catalysis2Recent advances in heterogeneous catalysts for biocrude hydrodeoxygenation35Cutting-edge innovations in bio-alcohol reforming: Pioneering pathways to high-purity hydrogen: A review14Mesoporous Silica-Encapsulated Cu Nanoparticles with Enhanced Performance for Ethanol Dehydrogenation to Acetaldehyde16Chemistry for water treatment under nanoconfinement34Z-scheme ZnAl2O4/Bi2O3 nanocomposite for enhanced photodegradation of Rhodamine B and Tetracycline9Sustainable energy cycles based on liquid oxygenates as carbon-neutral hydrogen carriers: A holistic vision6Role of stable Ni nano catalysts for dry reforming of methane4Modeling the impact of structure and coverage on the reactivity of realistic heterogeneous catalysts39

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