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RESEARCH PAPER · Nature Communications · 2020

Highly efficient phosphor-glass composites by pressureless sintering

Dao Zhang, Wenge Xiao, Chang Long Liu, Xiaofeng Liu, Jinjun Ren, Beibei Xu, Jianrong Qiu

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Highly efficient phosphor-glass composites by pressureless sinteringOriginalEnhancing the red upconversion luminescence of hybrid porous microtubes via an in situ O -substituted reaction through heat treatment20High quantum efficiency Ce:(Lu,Y) 3 (Al,Sc) 2 Al 3 O 12 transparent ceramics with excellent thermal stability for high-power white LEDs/LDs40Highly efficient and thermally stable luminescence of Ca 3 Gd 2 Si 6 O 18 :Ce 3+ ,Tb 3+ phosphors based on efficient energy transfer38The influence mechanism of nano-alumina content in semi-solid ceramic precursor fluid on the forming performance via a light-cured 3D printing method10A next-generation wide color gamut WLED with improved spectral performance in phosphor composite functional solid9Broad-Band and Stable Phosphor-in-Glass Enabling Ultrahigh Color Rendering for All-Inorganic High-Power WLEDs43Heat Dissipation Enhancement of Phosphor-Converted White Laser Diodes by Thermally Self-Managing Phosphor-in-Glass38New insights into phosphorescence properties of LuAGG: Long afterglow phosphor-in-glass for optical data storage29Gd3Al3Ga2O12:Ce, Mg2+ transparent ceramic phosphors for high-power white LEDs/LDs16Constructing lattice‐mismatched upconversion luminescence heterojunctions via light welding in seconds11Exploring color tunable emission characteristics of Eu 3+ -doped La 2 (MoO 4 ) 3 phosphors in the glass–ceramic form24General Overview and Applications of Ceramic Matrix Composites (CMCs)20Highly efficient and thermally robust cyan-green phosphor-in-glass films for high-brightness laser lighting32Highly Efficient and Thermally Stable Far-Red-Emitting Phosphors for Plant-Growth Lighting44Surface Deposition of YAG Phosphor on Borosilicate glass using a CO2 Laser2High‐Power Broadband NIR LEDs Enabled by Highly Efficient Blue‐to‐NIR Conversion113Designed glass frames full color in white light-emitting diodes and laser diodes lighting79High Efficiency Green‐Emitting LuAG:Ce Ceramic Phosphors for Laser Diode Lighting90Revealing the multicolor mechanism in borotellurite glass phosphor: From individual emission of dual-modes to WLED applications22Broadband emission Gd3Sc2Al3O12:Ce3+ transparent ceramics with a high color rendering index for high-power white LEDs/LDs38Tunable YAG:Ce3+ ceramic phosphors for white laser-diode lighting in transmissive/reflective models34Glass crystallization making red phosphor for high-power warm white lighting236Robust YAG:Ce single crystal for ultra-high efficiency laser lighting102Manipulating Nonlinear Optical Response via Domain Control in Nanocrystal‐in‐Glass Composites31High color rendering index composite phosphor-in-glass for high-power white laser lighting49Enhanced Color Rendering and Color Uniformity of PiG Based WLEDs by Using Red Phosphor Lens6Mn-doped Ca14Al10(Zn,Mg)6O35: A deep-red oxide phosphor with high photoluminescence quantum yield and thermal stability15Emerging and perspectives in microlasers based on rare-earth ions activated micro-/nanomaterials50Effect of Ca2+ - Si4+ on Y3Al5O12:Ce ceramic phosphors for white laser-diodes lighting16Phosphor converters for laser driven light sources77Near‐Unity and Zero‐Thermal‐Quenching Far‐Red‐Emitting Composite Ceramics via Pressureless Glass Crystallization70Preparation and photoluminescence of Tm3+/Eu2+/Eu3+ tri-doped fluorosilicate glass ceramics for warm WLED12Multichannel emissions from 5DJ metastable levels of Eu3+ in miscible-phase phosphors2Research on Laser Illumination Based on Phosphor in Metal (PiM) by Utilizing the Boron Nitride-Coated Copper Foams34Fluorescence regulation derived from Eu 3+ in miscible-order fluoride-phosphate blocky phosphor7The excellent luminous efficiency and high thermal stability of phosphor-in-glass for high-power laser13Synthesis, gamma and neutron attenuation capacities of boron-tellurite glass system utilizing Phy-X/PSD database16Reidinger defects induced thermally stable green emission from Eu2+, Mn2+ co-doped Ba0.75Al11O17.25 transparent ceramics16Review on transparent polycrystalline ceramics29Rapid and efficient preparation of phosphor-in-glass converter by induction heating for high-power white LEDs/LDs18Research progress of full electroluminescent white light-emitting diodes based on a single emissive layer183High efficiency fluorescent perovskite quantum dots encapsulated in superhydrophobic silica aerogel for wide color gamut backlight displays40An Extra‐Broadband VIS‐NIR Emitting Phosphor toward Multifunctional LED Applications153Photo Curing and Pressureless Sintering of Orange-emitting Glass-ceramics1Preparation of Luminescent Glass Aggregates from Soda-Lime Waste Glass10Boosting Continuous‐Wave Laser‐Driven Nonlinear Photothermal White Light Generation by Nanoscale Porosity30Translucent red-emitting AlN: Mn phosphor ceramics with high luminescence thermal stability6High thermal stability AlN-YAG: Ce composite phosphor ceramics for high-power laser-driven lighting37A promising all-inorganic green-emitting YAGG:Ce phosphor-in-glass for laser lighting26Additive Manufacturing Fiber Preforms for Structured Silica Fibers with Bismuth and Erbium Dopants23Correlating doping with the stability and color rendition of red phosphors10Reducing the cyan-cavity: Lu 2 MAl 4 SiO 12 :Ce 3+ (M = Mg, Ca, Sr and Ba) phosphor-in-glass film towards full-spectrum laser-driven lighting24Y 2 O 3 -YAG:Ce composite phosphor ceramics with enhanced light extraction efficiency for solid-state laser lighting18Overview of 3D-Printed Silica Glass47An effective heat dissipation strategy improving efficiency and thermal stability of phosphor-in-glass for high-power WLEDs40Glass‐Crystallized Luminescence Translucent Ceramics toward High‐Performance Broadband NIR LEDs120Energy transfer from Bi3+ to Mn2+ doped in oxyfluoride glass and transparent glass-ceramics containing KMgF38Amplified Spontaneous Emission from Perovskite Quantum Dots Inside a Transparent Glass28Luminous Performances Characterization of YAG: Ce3+ Phosphor/Silicone Composites Using Both Reflective and Transmissive Laser Excitations11Tailoring the Luminescent Properties of SrS:Ce3+ by Sr-Deficiency and Na+ Doping15Metal Inorganic–Organic Complex Glass and Fiber for Photonic Applications39Evaluation of gamma and neutron shielding capacities of tellurite glass system with Phy-X simulation software12Rapid fabrication of YAG-Ce phosphor glass composites on borosilicate glass for white light LEDs1Luminous output improvement in chip scale packaged Ce3+:YAG-based ceramic phosphors-converted white LEDs via laser assistance for application in automobile headlights22Ultra‐Efficient GAGG:Cr 3+ Ceramic Phosphor‐Converted Laser Diode: A Promising High‐Power Compact Near‐Infrared Light Source Enabling Clear Imaging109Rapid Pressureless Sintering of Glasses47Highly Luminescent and Ultra‐Stable Perovskite Films with Excellent Self‐Healing Ability for Flexible Lighting and Wide Color Gamut Displays42High efficiency green-emitting phosphor-in-glass films for high-power solid-state laser lighting13Patterned glass ceramic design for high-brightness high-color-quality laser-driven lightings101Enhancing opto-thermal performances of white laser lighting by high reflective phosphor converter58Efficient, Stable, and Ultra‐Broadband Near‐Infrared Garnet Phosphors for Miniaturized Optical Applications89Superhigh-Luminance Ce:YAG Phosphor in Glass and Phosphor-in-Glass Film for Laser Lighting103Highly efficient Ce: Lu(Mg,Al)2(Si,Al)3O12 phosphor ceramics for high-power white LEDs/LDs15Nanocrystal-in-glass composite (NGC): A powerful pathway from nanocrystals to advanced optical materials61High-performance and heat-resistant Ce:YAG phosphor in glass for laser lighting46High-Quality White Laser Diode Fabricated by Laser-Driven Tricolor PiG Film-on-Sapphire10All‐Inorganic Functional Phosphor–Glass Composites by Light Curing Induced 3D Printing for Next‐Generation Modular Lighting Devices18Dual-emitting phosphor-glass composites by the melt-quenching method for high-quality laser lighting12Emerging techniques for customized fabrication of glass8A novel fabrication strategy for alloyed Cd–Zn–S quantum dots–embedded glass with efficient red emission1Highly reflective interface design for phosphor-in-glass converter enabling ultrahigh efficiency laser-driven white lighting49Phosphor‐in‐Silica‐Glass: Filling the Gap between Low‐ and High‐Brightness Solid‐State Lightings46A review on the vitrification of metal coordination compounds and their photonic applications22Printing adaptability and vitrification of UV photo-responsive silica nanocomposites17Unique sandwich design of high-efficiency heat-conducting phosphor-in-glass film for high-quality laser-driven white lighting98Al 2 O 3 -YAG:Ce/YAG composite ceramic phosphor in a transmissive configuration for high-brightness laser-driven lighting36Design of the YAG:Ce3+ phosphor in tellurite-germanate glass with high luminous efficiency for laser lighting21Carbon Nanostructure-based Glass Composites: A Review6Realizing High‐Power Laser Lighting: Artfully Importing Micrometer BN into Ce: GdYAG Phosphor‐in‐Glass Film43Vitrification and Luminescence Properties of Metal–Organic Complexes23Nitride phosphor-in-glass films enabling high-performance white light in transmissive and reflective laser lighting27Exploiting Desired Phosphor‐In‐Glass for All‐Inorganic Solid‐State White Illumination47Layered array Al2O3-LuAG: Ce composite ceramic phosphors for high-brightness display19A super-high brightness and excellent colour quality laser-driven white light source enables miniaturized endoscopy59High brightness and vibronic luminescent behavior of YAG:Mn 4+ /Ca 2+ red phosphor for preparing phosphor-in-glass in white LED12High color rendering and high-luminance laser lighting using all inorganic nitride phosphor films15High-power NIR-II LED of Nd 3+ doped glass ceramics towards portable imaging9Imaging/nonimaging microoptical elements and stereoscopic systems based on femtosecond laser direct writing24Metallic Slurry Preparation and Printability Assessment for Material Extrusion Additive Manufacturing0Research progress on surface modifications for phosphors used in light-emitting diodes (LEDs)27Ultra-high efficiency green-emitting LuAG: Ce phosphor-in-ceramic applied for high-power laser lighting35A comprehensive review on additive manufacturing of glass: Recent progress and future outlook83Composite phosphor of a self-organized silica mixed YAG:Ce1Ultrahigh Power Density LuAG:Ce Green Converters For High‐Luminance Laser‐Driven Solid State Lighting54Performance optimization of Ce:YAG sapphire films for high power density white laser-driven lighting applications17Vigorous high-efficiency YAGG:Ce phosphor-in-glass film for next-generation laser lighting applications21High‐Performance Phosphor‐in‐Glass Film on Thermoelectric Generator for Non‐Radiative Energy Recycling in Laser Lighting243D Printing of Luminescent Glass with Controlled Distribution of Emission Colors for Multi‐Dimensional Optical Anti‐Counterfeiting31Cost-effective way of improving the optical properties of phosphor-in-glass by adjusting the particle size of glass powder12Thermally Stable Red‐Emitting Oxide Ceramics for Laser Lighting153Energy transfer controlled color-tunable luminescence of Tm3+/Dy3+ co-doped aluminoborosilicate glass-ceramics12Barcode-structured YAG:Ce/YAG:Ce,Mn ceramic phosphors for variable CCT and high CRI LED/LD lighting26Recent progress on garnet phosphor ceramics for high power solid-state lighting104Exploring interfacial reactions and optical properties of ZBLAN-based phosphor-in-glass color converters via spark plasma sintering for laser-driven lighting13Cyan-green-emitting Ca 3 Sc 2 Si 3 O 12 :Ce 3+ transparent ceramics: A promising color converter for high-brightness laser lighting43Ultra-high melting point Ho3+, Yb3+ co-doped HfO2 single-crystal fibers for high-precision and robust ratiometric thermometry towards harsh environments9Inorganic remote glass film based on yellowish‐green (Y, Ba) 3 (Al, Si) 5 O 12 :Ce garnet phosphor for warm white LEDs0Enhancing thermal performance in laser-driven illumination with metal–micropillars array three-dimensional substrate13Tricolor Pattern Design: Ultrahigh Thermal Conductivity Phosphor-in-Glass Film for Laser Illumination27Fe 57 Mössbauer, optical and structural properties with ligand field effects of borosilicate glass doped with iron oxide10A Novel Cyan Phosphor (K,Rb) 3 GdSi 2 O 7 :Ce 3+ for Full‐Spectrum Lighting through Local Structure Tailoring48Lithium-aluminium-silicate glass: A novel high-quality glass for preparing LuAG: Ce colour converter for laser illumination12Highly crystalline Y3Al5O12:Ce3+ phosphor-in-silica glass ceramics for high-power solid-state lighting43Patterned phosphor-in-glass films with efficient thermal management for high-power laser projection displays80Effect of sintering condition on the attenuation of silica glasses fabricated by additive manufacturing16Highly efficient blue‐emitting phosphor via charge compensation strategy and its application for white LED lighting10Facile Synthesis of Efficient Copper Chlorine‐In‐Glass for White Light‐Emitting Diode and Anticounterfeiting1Distinctive spatially separated structure of dichromatic phosphor-in-glass film for high-quality laser lighting7Enhanced quantum efficiency and moisture-resistant red-emitting K3AlF6:Mn4+ phosphor for high color rendering index WLED4Laminated structural Al 2 O 3 /YAG:Ce composite ceramic phosphor with high front light emission for transmissive laser lighting17Efficient thermal and luminescent regulations of LuAG: Ce-PiG based remote LED/LD13Facile Fabrication of Silica Glass Embedded with NiO Nanoparticles by 3D Printing Technology and its Optical Nonlinearity12Red‐Emitting Cordierite Ceramic Enabling General Healthy Warm White Laser Lighting55Robust high-efficiency LuAG: Ce phosphor-in-silica glass (PiSG) for high-brightness laser lighting20Synthesis, properties and applications of glasses containing chalcogenide quantum dots0Laser-Driven White Light Source With High Luminescence Saturation Through Reflective Color Converter36Achieving high brightness and thermally stable far-red luminescence via ultrathin phosphor–glass composite engineering3Carbon carrier-based rapid Joule heating technology: a review on the preparation and applications of functional nanomaterials30Enhanced quantum efficiency and thermal stability by crystal-field engineering in a Y(Ga,Al) 3 (BO 3 ) 4 :Cr 3+ ,Yb 3+ phosphor for diverse short-wave infrared applications19Laminated composite of ceramic/glass films to realize high luminous efficiency and high color quality in laser-driven white lighting16Reduction of injection molded silica glass defects and enhancement of glass quality via water debinding11Unveiling the Effect of CE 3+ Doping Concentration in Yag:Ce Single Crystals Towards High Luminance Laser Lighting2Unveiling the Effect of CE 3+ Doping Concentration in Yag:Ce Single Crystals Towards High Luminance Laser Lighting1像差预补偿的铌酸锂晶体内部激光直写（特邀）4High-Quality Laser-Driven White Lighting Enabling by Collecting Backward Emission Light of Phosphor-in-Glass Film15High luminous efficiency and high saturation threshold in highly transparent LuAG:Ce phosphor ceramics for laser diodes lighting20Solvent-free blending of CsPbBr3 and commercial polymer: Interface-visualization, bandgap engineering and improved stability in 3D printing12Rapid synthesis of phosphor-glass composites in seconds based on particle self-stabilization117High‐Throughput Fabrication of Phosphor‐In‐Silica Glass via Injection Molding11Photopolymerized 3D Printing Materials for Optical Elements14

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