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RESEARCH PAPER · Journal of the Physical Society of Japan · 2020

Hydrogen-Bonded Small-Molecular Crystals Yielding Strong Ferroelectric and Antiferroelectric Polarizations

Sachio Horiuchi, Shoji Ishibashi

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Hydrogen-Bonded Small-Molecular Crystals Yielding Strong Ferroelectric and Antiferroelectric PolarizationsOriginalMetaelectric multiphase transitions in a highly polarizable molecular crystal11One-dimensional DABCO hydrogen-bonding chain in a hexagonal channel of magnetic [Ni(dmit) 2 ]6Birefringent Field-Modulation Imaging of Transparent Ferroelectrics17Observation of the Three-Dimensional Polarization Vector in Films of Organic Molecular Ferroelectrics Using Terahertz Radiation Emission5Competing hydrogen-bonding interactions in a high- T c organic molecular-ionic crystal with evident nonlinear optical response2Ferroelectricity and switching polarization on the C–H⋯π bond in a pure organic molecular crystal – 1,3,5-trimethylnitrobenzene3Monofluorine substitution achieved high- T c dielectric transition in a one-dimensional lead bromide hybrid photoluminescent perovskite semiconductor21Room-temperature dielectric switching in a host–guest crown ether inclusion complex27Single-component organic molecular ferroelectrics based on disk- or wheel-like rotation6Plastic/ferroelectric molecular crystals: Ferroelectric performance in bulk polycrystalline forms57Experimental evidence for the existence of a second partially-ordered phase of ice VI59Mechanisms of Molecular Ferroelectrics Made Simple5Various Stacking Patterns of Two‐Dimensional Molecular Assemblies in Hydrogen‐Bonded Cocrystals: Insight into Competitive Intermolecular Interactions and Control of Stacking Patterns28Various Stacking Patterns of Two‐Dimensional Molecular Assemblies in Hydrogen‐Bonded Cocrystals: Insight into Competitive Intermolecular Interactions and Control of Stacking Patterns1Ferroic alternation in methylammonium lead triiodide perovskite21A Metal-Free Molecular Antiferroelectric Material Showing High Phase Transition Temperatures and Large Electrocaloric Effects54An electric field cell for performing in situ single-crystal synchrotron X-ray diffraction8Hydrogen-bonded single-component organic ferroelectrics revisited by van der Waals density-functional theory calculations10Structural Properties and Dielectric Hysteresis of Molecular Organic Ferroelectric Grown from Different Solvents15AFM Visualization of Ferroelastic and Ferroelectric Domains in 2-Methylbenzimidazole С8H8N2 Crystals3Raman scattering and luminescence in single crystals of the amino acid glycine C2H5NO2 with an admixture of croconic acid C5H2O51Glycine: The Gift that Keeps on Giving31A room-temperature antiferroelectric in hybrid perovskite enables highly efficient energy storage at low electric fields32Chemical design of a new displacive-type ferroelectric20Competing ferroelectric polarization: hydroxyl flip-flop versus proton-transfer mechanisms10Ferroelectricity in organic materials: from materials characteristics to de novo design39Hydrogen-bonded organic molecular ferroelectrics/antiferroelectrics7Above-room-temperature ferroelectricity and piezoelectric activity of dimethylglycinium-dimethylglycine chloride14Photoinduced Persistent Polarization Change in a Spin Transition Crystal35Photoinduced Persistent Polarization Change in a Spin Transition Crystal2Ultrafast opto-protonics in a hydrogen-bonded π-molecular ferroelectric crystal6Ab Initio Study of H‐Bond Dynamics in Three‐Component Crystals Comprising (DABCOH+)n Polycationic Chains1Emission of Terahertz Electromagnetic Waves: A New Spectroscopic Method to Investigate Physical Properties of Solids8Ferroelectric Ionic Molecular Crystals with Significant Plasticity and a Low Melting Point: High Performance in Hot‐Pressed Polycrystalline Plates and Melt‐Grown Crystalline Sheets32Ferroelectric Ionic Molecular Crystals with Significant Plasticity and a Low Melting Point: High Performance in Hot‐Pressed Polycrystalline Plates and Melt‐Grown Crystalline Sheets0Origin of high piezoelectricity of a bismuth-based organic–inorganic hybrid crystal14Dielectric magnetochiral anisotropy in triglycine sulfate4Competition of polar and antipolar states hidden behind a variety of polarization switching modes in hydrogen-bonded molecular chains6Control of electronic polarization via charge ordering and electron transfer: electronic ferroelectrics and electronic pyroelectrics32Observation of proton-transfer-coupled spin transition by single-crystal neutron-diffraction measurement4Ultrafast variation of the polarized state in proton-π electron coupled ferroelectric cocrystal Phz-H 2 ca2Intersecting multiaxial domain walls in plastic ferroelectric crystal films2A straightforward method using the sign of the piezoelectric coefficient to identify the ferroelectric switching mechanism3Development of an Iron(II) Complex Exhibiting Thermal- and Photoinduced Double Proton-Transfer-Coupled Spin Transition in a Short Hydrogen Bond12Ferroelectric Crystals of Globular Molecules: Cambridge Structural Database Mining and Computational Assessment12Phase Transition and Point Defects in the Ferroelectric Molecular Perovskite (MDABCO)(NH4)I35Designing multifunctional organic thermochromic ferroelectric materials: remarkable melt-cool large thermal hysteresis of reversible single crystal to single crystal transformation3General Introduction0Various Stacking Patterns of Two-Dimensional Molecular Assemblies in Hydrogen-Bonded Cocrystals: Insight into Competitive Intermolecular Interactions and Control of Stacking Patterns0Development of an FeII Complex Exhibiting Intermolecular Proton Shifting Coupled Spin Transition0Development of an FeII Complex Exhibiting Intermolecular Proton Shifting Coupled Spin Transition6Solid Solutions of Plastic/Ferroelectric Crystals: Toward Tailor-Made Functional Materials20Visible‐Photo‐Assisted Phase Switching of Antiferroelectric‐to‐Ferroelectric Orders in an I3−‐Intercalated 2D Perovskite0Visible‐Photo‐Assisted Phase Switching of Antiferroelectric‐to‐Ferroelectric Orders in an I3−‐Intercalated 2D Perovskite6Exploration and development of molecule-based printed electronics materials: an integrated approach using experimental, computational, and data sciences6Mise en forme et caractérisation des propriétés diélectriques et calorimétriques de matériaux moléculaires ferroélectriques en vue d'applications en énergie électrique0Barkhausen noise in the organic ferroelectric copolymer P(VDF:TrFE)1Correlation between ferroelectricity and torsional motion of acetyl groups in tris(4-acetylphenyl)amine observed by muon spin relaxation1Correlations between the constituent molecules, crystal structures, and dielectric constants in organic crystals2Dimethylglycinium hydrogen maleate‒maleic acid, a new all-organic ferroelectric with an incommensurate phase0Field-Effect Crystal Engineering in Proton–π-Electron Correlated Systems1Kite-quadrilateral lattice and unique domain-wall pattern formation in plastic/ferroelectric films of [ MDABCO ] [ PF 6 ]0Quantum paraelectricity in the H-bonded ferroelectrics KH2PO4 and KD2PO4 under pressure02,5-Dihydroxy-1,4-benzoquinones Appended with −P(═O)(OR) 2 (R = Me or Et) Groups and Their Ammonium and Lithium Salts: Structural, Spectroscopic, and Electrochemical Properties0Ultrafast Polarization Control by Proton Vibrational Excitation Investigated by Terahertz Radiation Spectroscopy0Engineering Small-Molecule Proton-Transfer Ferroelectrics by Crystal Structure Prediction: Design Limits at the Salt–Cocrystal Boundary0Growth, Structural Characterization, and Nonlinear Optical Properties of L-Lysinium Hydrogen Adipate Single Crystals: An Integrated Experimental and DFT Study0

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  1. Metaelectric multiphase transitions in a highly polarizable molecular crystal

    Chemical Science · 2020-01-01

    Sachio Horiuchi, Shoji Ishibashi, Rie Haruki, Reiji Kumai, Satoshi Inada, Shigenobu Aoyagi

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  2. One-dimensional DABCO hydrogen-bonding chain in a hexagonal channel of magnetic [Ni(dmit) 2 ]

    Dalton Transactions · 2020-01-01

    Simin Li, Kiyonori Takahashi, Ichiro Hisaki, Kenta Kokado, Takayoshi Nakamura

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  3. Birefringent Field-Modulation Imaging of Transparent Ferroelectrics

    Physical Review Applied · 2020-08-21

    Yohei Uemura, Satoshi Matsuoka, Jun’ya Tsutsumi, Sachio Horiuchi, Shunto Arai, Tatsuo Hasegawa

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  4. Observation of the Three-Dimensional Polarization Vector in Films of Organic Molecular Ferroelectrics Using Terahertz Radiation Emission

    Physical Review Applied · 2020-11-02

    Yuto Kinoshita, Masato Sotome, Tatsuya Miyamoto, Yohei Uemura, Shunto Arai, Sachio Horiuchi, Tatsuo Hasegawa, Hiroshi Okamoto, N. Kida

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  5. Competing hydrogen-bonding interactions in a high- T c organic molecular-ionic crystal with evident nonlinear optical response

    CrystEngComm · 2021-01-01

    Wentao Xu, Jun‐Chao Liu, Yu‐Ling Zeng, Hua Zhang, Zhong‐Xia Wang

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  6. Ferroelectricity and switching polarization on the C–H⋯π bond in a pure organic molecular crystal – 1,3,5-trimethylnitrobenzene

    CrystEngComm · 2021-01-01

    Przemysław Szklarz, Vasyl Kinzhybalo, G. Bator

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  7. Monofluorine substitution achieved high- T c dielectric transition in a one-dimensional lead bromide hybrid photoluminescent perovskite semiconductor

    Materials Chemistry Frontiers · 2021-01-01

    Fang‐Fang Di, Hang Peng, Hua Zhang, Xue-Qin Huang, Wu-Jia Chen, Yu-Ling Liu, Yuan‐Yuan Tang

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  8. Room-temperature dielectric switching in a host–guest crown ether inclusion complex

    Inorganic Chemistry Frontiers · 2021-01-01

    Fang‐Fang Di, Lin Zhou, Wu-Jia Chen, Jun‐Chao Liu, Hang Peng, Shuyu Tang, Hang Yu, Wei‐Qiang Liao, Zhong‐Xia Wang

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  9. Single-component organic molecular ferroelectrics based on disk- or wheel-like rotation

    Journal of Materials Chemistry C · 2021-01-01

    Sachio Horiuchi, Reiji Kumai, Shoji Ishibashi

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  10. Plastic/ferroelectric molecular crystals: Ferroelectric performance in bulk polycrystalline forms

    APL Materials · 2021-02-01

    Jun Harada

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  11. Experimental evidence for the existence of a second partially-ordered phase of ice VI

    Nature Communications · 2021-02-18

    Ryo Yamane, Kazuki Komatsu, Jun Gouchi, Yoshiya Uwatoko, Shinichi Machida, Takanori Hattori, Hayate Ito, Hiroyuki Kagi

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  12. Mechanisms of Molecular Ferroelectrics Made Simple

    The Journal of Physical Chemistry C · 2021-06-02

    Xiaoqing Zhu, Wenbin Fan, Wei Li Ren, Yongle Li

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  13. Various Stacking Patterns of Two‐Dimensional Molecular Assemblies in Hydrogen‐Bonded Cocrystals: Insight into Competitive Intermolecular Interactions and Control of Stacking Patterns

    Angewandte Chemie International Edition · 2021-08-10

    Masaki Donoshita, Yukihiro Yoshida, Mikihiro Hayashi, Ryuichi Ikeda, Susumu Tanaka, Yasuhisa Yamamura, Kazuya Saito, Shogo Kawaguchi, Kunihisa Sugimoto, Hiroshi Kitagawa

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  14. Various Stacking Patterns of Two‐Dimensional Molecular Assemblies in Hydrogen‐Bonded Cocrystals: Insight into Competitive Intermolecular Interactions and Control of Stacking Patterns

    Angewandte Chemie · 2021-08-10

    Masaki Donoshita, Yukihiro Yoshida, Mikihiro Hayashi, Ryuichi Ikeda, Susumu Tanaka, Yasuhisa Yamamura, Kazuya Saito, Shogo Kawaguchi, Kunihisa Sugimoto, Hiroshi Kitagawa

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  15. Ferroic alternation in methylammonium lead triiodide perovskite

    EcoMat · 2021-08-11

    Shengjian Qin, Shenghui Yi, Yanqing Xu, Mi Zhou, Jinjin Zhao, Xiaobao Tian, Huajun Guo, Yinan Jiao, Guanglei Zhang, Jian Lü

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  16. A Metal-Free Molecular Antiferroelectric Material Showing High Phase Transition Temperatures and Large Electrocaloric Effects

    Journal of the American Chemical Society · 2021-08-30

    Haojie Xu, Wuqian Guo, Jiaqi Wang, Yu Ma, Shiguo Han, Yi Liu, Lei Lu, Xiong Pan, Junhua Luo, Zhihua Sun

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  17. An electric field cell for performing in situ single-crystal synchrotron X-ray diffraction

    Journal of Applied Crystallography · 2021-09-04

    Lucy K. Saunders, Hamish H.‐M. Yeung, Mark R. Warren, Peter Smith, Stuart Gurney, Stephen F. Dodsworth, Íñigo J. Vitórica‐Yrezábal, Adrian Wilcox, Paul V. Hathaway, G. Preece, P. S. Roberts, Sarah A. Barnett, David R. Allan

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  18. Hydrogen-bonded single-component organic ferroelectrics revisited by van der Waals density-functional theory calculations

    Physical Review Materials · 2021-09-22

    Shoji Ishibashi, Sachio Horiuchi, Reiji Kumai

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  19. Structural Properties and Dielectric Hysteresis of Molecular Organic Ferroelectric Grown from Different Solvents

    Crystals · 2021-10-21

    Е. В. Балашова, А. А. Левин, Alexander V. Fokin, Alexey V. Redkov, Boris B. Krichevtsov

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  20. AFM Visualization of Ferroelastic and Ferroelectric Domains in 2-Methylbenzimidazole С8H8N2 Crystals

    Journal of Surface Investigation X-ray Synchrotron and Neutron Techniques · 2021-11-01

    Е. В. Балашова, Boris B. Krichevtsov, Tatyana S. Kunkel, A. V. Ankudinov

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  21. Raman scattering and luminescence in single crystals of the amino acid glycine C2H5NO2 with an admixture of croconic acid C5H2O5

    Journal of Physics Conference Series · 2021-11-01

    Е. В. Балашова, Alexander N. Smirnov, Yu V Davydov, Boris B. Krichevtsov, A. N. Starukhin

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  22. Glycine: The Gift that Keeps on Giving

    Israel Journal of Chemistry · 2021-11-02

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  23. A room-temperature antiferroelectric in hybrid perovskite enables highly efficient energy storage at low electric fields

    Chemical Science · 2022-01-01

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  24. Chemical design of a new displacive-type ferroelectric

    Dalton Transactions · 2022-01-01

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  25. Competing ferroelectric polarization: hydroxyl flip-flop versus proton-transfer mechanisms

    Journal of Materials Chemistry C · 2022-01-01

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  26. Ferroelectricity in organic materials: from materials characteristics to de novo design

    Journal of Materials Chemistry C · 2022-01-01

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  27. Hydrogen-bonded organic molecular ferroelectrics/antiferroelectrics

    Elsevier eBooks · 2022-01-01

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  28. Above-room-temperature ferroelectricity and piezoelectric activity of dimethylglycinium-dimethylglycine chloride

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  29. Photoinduced Persistent Polarization Change in a Spin Transition Crystal

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  30. Photoinduced Persistent Polarization Change in a Spin Transition Crystal

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  31. Ultrafast opto-protonics in a hydrogen-bonded π-molecular ferroelectric crystal

    APL Materials · 2022-09-01

    Y. Okimoto, Peiyu Xia, Jiro Itatani, Haruka Matsushima, T. Ishikawa, Shin‐ya Koshihara, Sachio Horiuchi

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  32. Ab Initio Study of H‐Bond Dynamics in Three‐Component Crystals Comprising (DABCOH+)n Polycationic Chains

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  33. Emission of Terahertz Electromagnetic Waves: A New Spectroscopic Method to Investigate Physical Properties of Solids

    Journal of the Physical Society of Japan · 2022-10-18

    N. Kida, Tatsuya Miyamoto, Hiroshi Okamoto

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  34. Ferroelectric Ionic Molecular Crystals with Significant Plasticity and a Low Melting Point: High Performance in Hot‐Pressed Polycrystalline Plates and Melt‐Grown Crystalline Sheets

    Angewandte Chemie International Edition · 2022-11-21

    Jun Harada, Haruka Takahashi, Rin Notsuka, Mika Takehisa, Yukihiro Takahashi, Tomoyasu Usui, Hiroki Taniguchi

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  35. Ferroelectric Ionic Molecular Crystals with Significant Plasticity and a Low Melting Point: High Performance in Hot‐Pressed Polycrystalline Plates and Melt‐Grown Crystalline Sheets

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  36. Origin of high piezoelectricity of a bismuth-based organic–inorganic hybrid crystal

    Journal of Materials Chemistry C · 2022-12-13

    Zongyi Zhang, Yifan Zhang, Yue Zhao, Minglei Zhao, Ruyue Zhang, Jun-Yi Guo, Fuhao An, Xuan Sun

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  37. Dielectric magnetochiral anisotropy in triglycine sulfate

    Physical review. B./Physical review. B · 2022-12-15

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  38. Competition of polar and antipolar states hidden behind a variety of polarization switching modes in hydrogen-bonded molecular chains

    Materials Horizons · 2023-01-01

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  39. Control of electronic polarization via charge ordering and electron transfer: electronic ferroelectrics and electronic pyroelectrics

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  40. Observation of proton-transfer-coupled spin transition by single-crystal neutron-diffraction measurement

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  41. Ultrafast variation of the polarized state in proton-π electron coupled ferroelectric cocrystal Phz-H 2 ca

    Materials Advances · 2023-01-01

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  42. Intersecting multiaxial domain walls in plastic ferroelectric crystal films

    Physical Review Materials · 2023-03-02

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  43. A straightforward method using the sign of the piezoelectric coefficient to identify the ferroelectric switching mechanism

    Scientific Reports · 2023-05-31

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  44. Development of an Iron(II) Complex Exhibiting Thermal- and Photoinduced Double Proton-Transfer-Coupled Spin Transition in a Short Hydrogen Bond

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  45. Ferroelectric Crystals of Globular Molecules: Cambridge Structural Database Mining and Computational Assessment

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  46. Phase Transition and Point Defects in the Ferroelectric Molecular Perovskite (MDABCO)(NH4)I3

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  47. Designing multifunctional organic thermochromic ferroelectric materials: remarkable melt-cool large thermal hysteresis of reversible single crystal to single crystal transformation

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  48. General Introduction

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  49. Various Stacking Patterns of Two-Dimensional Molecular Assemblies in Hydrogen-Bonded Cocrystals: Insight into Competitive Intermolecular Interactions and Control of Stacking Patterns

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  50. Development of an FeII Complex Exhibiting Intermolecular Proton Shifting Coupled Spin Transition

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