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RESEARCH PAPER · Chemical Reviews · 2020

New Concepts in Electrolytes

Matthew Li, Chunsheng Wang, Zhongwei Chen, Kang Xu, Jun Biao Lu

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New Concepts in ElectrolytesOriginalA review on energy chemistry of fast-charging anodes662Basic knowledge in battery research bridging the gap between academia and industry143Emerging interfacial chemistry of graphite anodes in lithium-ion batteries145Liquefied gas electrolytes for wide-temperature lithium metal batteries209Revitalising sodium–sulfur batteries for non-high-temperature operation: a crucial review327The Current State of Aqueous Zn-Based Rechargeable Batteries390Design Principles of Artificial Solid Electrolyte Interphases for Lithium-Metal Anodes280Hydrated Eutectic Electrolytes with Ligand-Oriented Solvation Shells for Long-Cycling Zinc-Organic Batteries771Perspective on High‐Energy Carbon‐Based Supercapacitors216Eutectic Electrolytes as a Promising Platform for Next-Generation Electrochemical Energy Storage279A Liquid Electrolyte with De-Solvated Lithium Ions for Lithium-Metal Battery265Anion Solvation Reconfiguration Enables High‐Voltage Carbonate Electrolytes for Stable Zn/Graphite Cells104Nanoarchitectured Design of Vertical‐Standing Arrays for Supercapacitors: Progress, Challenges, and Perspectives204Homogeneous and Fast Ion Conduction of PEO‐Based Solid‐State Electrolyte at Low Temperature549The Features and Progress of Electrolyte for Potassium Ion Batteries154Regulating Interfacial Chemistry in Lithium‐Ion Batteries by a Weakly Solvating Electrolyte**855Regulating Interfacial Chemistry in Lithium‐Ion Batteries by a Weakly Solvating Electrolyte**119Fast Charging Li-Ion Batteries for a New Era of Electric Vehicles136Recent Progress on Flexible Zn-Air Batteries247Recent Progress on High‐Performance Cathode Materials for Zinc‐Ion Batteries117Polyimide separators for rechargeable batteries169Thermal runaway of Lithium-ion batteries employing LiN(SO2F)2-based concentrated electrolytes326Rationally designed nanostructured metal chalcogenides for advanced sodium-ion batteries119Structure Code for Advanced Polymer Electrolyte in Lithium‐Ion Batteries161Lithium Metal Anodes with Nonaqueous Electrolytes730The Mystery of Electrolyte Concentration: From Superhigh to Ultralow227Solid Electrolytes for High‐Temperature Stable Batteries and Supercapacitors168Manipulating Electrode/Electrolyte Interphases of Sodium-Ion Batteries: Strategies and Perspectives195Insights into the Nanostructure, Solvation, and Dynamics of Liquid Electrolytes through Small‐Angle X‐Ray Scattering108Review—Localized High-Concentration Electrolytes for Lithium Batteries591Constructing nitrided interfaces for stabilizing Li metal electrodes in liquid electrolytes120Determinants of lithium-ion battery technology cost decline149Emerging trends in anion storage materials for the capacitive and hybrid energy storage and beyond168High-voltage liquid electrolytes for Li batteries: progress and perspectives980Controlling electrochemical growth of metallic zinc electrodes: Toward affordable rechargeable energy storage systems407Electrolytes and Interphases in Potassium Ion Batteries379Diluted High Concentration Electrolyte with Dual Effects for Practical Lithium-Sulfur Batteries116Mechanism for Zincophilic Sites on Zinc‐Metal Anode Hosts in Aqueous Batteries395Comprehensive Insights into Electrolytes and Solid Electrolyte Interfaces in Potassium-Ion Batteries129Effects of fluorinated solvents on electrolyte solvation structures and electrode/electrolyte interphases for lithium metal batteries327High‐Energy Aqueous Sodium‐Ion Batteries232Simultaneous Stabilization of the Solid/Cathode Electrolyte Interface in Lithium Metal Batteries by a New Weakly Solvating Electrolyte128Review—recent advances in non-aqueous liquid electrolytes containing fluorinated compounds for high energy density lithium-ion batteries126Sustainable Lithium‐Metal Battery Achieved by a Safe Electrolyte Based on Recyclable and Low‐Cost Molecular Sieve106Water-in-Salt LiTFSI Aqueous Electrolytes. 1. Liquid Structure from Combined Molecular Dynamics Simulation and Experimental Studies132Nitrate Additives Coordinated with Crown Ether Stabilize Lithium Metal Anodes in Carbonate Electrolyte102Electrolyte Structure of Lithium Polysulfides with Anti‐Reductive Solvent Shells for Practical Lithium–Sulfur Batteries190Unlocking the self-supported thermal runaway of high-energy lithium-ion batteries221Manipulating anion intercalation enables a high-voltage aqueous dual ion battery196Covalent Organic Frameworks for Batteries318Interphase Engineering by Electrolyte Additives for Lithium-Rich Layered Oxides: Advances and Perspectives180Characterising lithium-ion electrolytes via operando Raman microspectroscopy123Advanced High‐Voltage All‐Solid‐State Li‐Ion Batteries Enabled by a Dual‐Halogen Solid Electrolyte190Electrolyte Design for Lithium Metal Anode‐Based Batteries Toward Extreme Temperature Application220Advanced Electrolyte Design for High‐Energy‐Density Li‐Metal Batteries under Practical Conditions173Stable Anion‐Derived Solid Electrolyte Interphase in Lithium Metal Batteries301Issues and rational design of aqueous electrolyte for Zn‐ion batteries128Water or Anion? Uncovering the Zn2+ Solvation Environment in Mixed Zn(TFSI)2 and LiTFSI Water-in-Salt Electrolytes101Design strategies and research progress for Water-in-Salt electrolytes104A synergistic exploitation to produce high-voltage quasi-solid-state lithium metal batteries198Wide Voltage Aqueous Asymmetric Supercapacitors: Advances, Strategies, and Challenges289On the crystallography and reversibility of lithium electrodeposits at ultrahigh capacity181A Dynamic and Self‐Adapting Interface Coating for Stable Zn‐Metal Anodes358Fast Li-ion Conductor of Li 3 HoBr 6 for Stable All-Solid-State Lithium–Sulfur Battery108Small‐Dipole‐Molecule‐Containing Electrolytes for High‐Voltage Aqueous Rechargeable Batteries134Steric Effect Tuned Ion Solvation Enabling Stable Cycling of High-Voltage Lithium Metal Battery605Advances and Prospects of Dual‐Ion Batteries143Hydrogen-bond network manipulation of aqueous electrolytes with high-donor solvent additives for Al-air batteries106Non‐Electrode Components for Rechargeable Aqueous Zinc Batteries: Electrolytes, Solid‐Electrolyte‐Interphase, Current Collectors, Binders, and Separators162Eutectic Electrolytes in Advanced Metal-Ion Batteries222Upgrading Carbonate Electrolytes for Ultra‐stable Practical Lithium Metal Batteries114Challenges and advances in wide-temperature rechargeable lithium batteries517Eco-friendly electrolytes via a robust bond design for high-energy Li metal batteries236Ether-based electrolytes for sodium ion batteries597Historical development and novel concepts on electrolytes for aqueous rechargeable batteries308Ultrafast, long-life, high-loading, and wide-temperature zinc ion supercapacitors129Asymmetric donor-acceptor molecule-regulated core-shell-solvation electrolyte for high-voltage aqueous batteries143Insight on Organic Molecules in Aqueous Zn‐Ion Batteries with an Emphasis on the Zn Anode Regulation478A Self-Supporting Covalent Organic Framework Separator with Desolvation Effect for High Energy Density Lithium Metal Batteries177Challenges, interface engineering, and processing strategies toward practical sulfide‐based all‐solid‐state lithium batteries273Practical High‐Voltage Lithium Metal Batteries Enabled by Tuning the Solvation Structure in Weakly Solvating Electrolyte164Hydrogen bonds enhanced composite polymer electrolyte for high-voltage cathode of solid-state lithium battery121Biopolymer-based hydrogel electrolytes for advanced energy storage/conversion devices: Properties, applications, and perspectives430Eutectic Electrolytes Chemistry for Rechargeable Zn Batteries114Rigid and Flexible SEI Layer Formed Over a Cross‐Linked Polymer for Enhanced Ultrathin Li Metal Anode Performance102A stable quasi-solid electrolyte improves the safe operation of highly efficient lithium-metal pouch cells in harsh environments234Structural regulation chemistry of lithium ion solvation for lithium batteries106Promoting favorable interfacial properties in lithium-based batteries using chlorine-rich sulfide inorganic solid-state electrolytes259Dual ions intercalation drives high-performance aqueous Zn-ion storage on birnessite-type manganese oxides cathode127Tailoring the Solvation Sheath of Cations by Constructing Electrode Front‐Faces for Rechargeable Batteries176Progress in Gel Polymer Electrolytes for Sodium‐Ion Batteries173Regulating Solvation Structure in Nonflammable Amide‐Based Electrolytes for Long‐Cycling and Safe Lithium Metal Batteries128Atomic‐Scale Design of Anode Materials for Alkali Metal (Li/Na/K)‐Ion Batteries: Progress and Perspectives150Eutectic Electrolyte with Unique Solvation Structure for High‐Performance Zinc‐Ion Batteries320Li−N Interaction Induced Deep Eutectic Gel Polymer Electrolyte for High Performance Lithium‐Metal Batteries148Electrolyte Solvation Structure Design for Sodium Ion Batteries671Modification of Cu current collectors for lithium metal batteries – A review217Weak Cation–Solvent Interactions in Ether‐Based Electrolytes Stabilizing Potassium‐ion Batteries143Are Polymer‐Based Electrolytes Ready for High‐Voltage Lithium Battery Applications? An Overview of Degradation Mechanisms and Battery Performance233Tailoring Electrolyte Dehydrogenation with Trace Additives: Stabilizing the LiCoO 2 Cathode beyond 4.6 V132Enabling High‐Voltage “Superconcentrated Ionogel‐in‐Ceramic” Hybrid Electrolyte with Ultrahigh Ionic Conductivity and Single Li + ‐Ion Transference Number157Phase-locked constructing dynamic supramolecular ionic conductive elastomers with superior toughness, autonomous self-healing and recyclability325Rechargeable Batteries for Grid Scale Energy Storage1769Rejuvenating Propylene Carbonate‐based Electrolyte Through Nonsolvating Interactions for Wide‐Temperature Li‐ions Batteries137Locking Active Li Metal through Localized Redistribution of Fluoride Enabling Stable Li‐Metal Batteries111Deciphering and modulating energetics of solvation structure enables aggressive high-voltage chemistry of Li metal batteries282Mechanism, quantitative characterization, and inhibition of corrosion in lithium batteries105Mitigating Electron Leakage of Solid Electrolyte Interface for Stable Sodium‐Ion Batteries114Non-nucleophilic electrolyte with non-fluorinated hybrid solvents for long-life magnesium metal batteries113Designing better electrolytes751Materials design and preparation for high energy density and high power density electrochemical supercapacitors319A tailored electrolyte for safe and durable potassium ion batteries219Emerging electrolytes with fluorinated solvents for rechargeable lithium-based batteries390Interfaces and interphases in batteries161Challenges of polymer electrolyte with wide electrochemical window for high energy solid‐state lithium batteries256Anode-free sodium metal batteries as rising stars for lithium-ion alternatives116A non-academic perspective on the future of lithium-based batteries820Electrolytes in Organic Batteries303Challenges and Opportunities to Mitigate the Catastrophic Thermal Runaway of High‐Energy Batteries252A monofluoride ether-based electrolyte solution for fast-charging and low-temperature non-aqueous lithium metal batteries352High-Performance Supercapacitors: A Comprehensive Review on Paradigm Shift of Conventional Energy Storage Devices316An overview of deep eutectic solvents: Alternative for organic electrolytes, aqueous systems & ionic liquids for electrochemical energy storage144Tuning the Li + Solvation Structure by a “Bulky Coordinating” Strategy Enables Nonflammable Electrolyte for Ultrahigh Voltage Lithium Metal Batteries139Inhibiting gas generation to achieve ultralong-lifespan lithium-ion batteries at low temperatures12940 Years of Low‐Temperature Electrolytes for Rechargeable Lithium Batteries180Ten concerns of Zn metal anode for rechargeable aqueous zinc batteries912Multifunctional Electrolyte Additives for Better Metal Batteries130Unleashing recent electrolyte materials for next-generation supercapacitor applications: A comprehensive review111Gel Polymer Electrolyte toward Large‐Scale Application of Aqueous Zinc Batteries140Reconstructing Hydrogen Bond Network Enables High Voltage Aqueous Zinc‐Ion Supercapacitors109A reflection on polymer electrolytes for solid-state lithium metal batteries422Nonaqueous Liquid Electrolytes for Sodium‐Ion Batteries: Fundamentals, Progress and Perspectives201Electrolyte Interphases in Aqueous Batteries105Green Ether Electrolytes for Sustainable High‐voltage Potassium Ion Batteries117Trend of Developing Aqueous Liquid and Gel Electrolytes for Sustainable, Safe, and High-Performance Li-Ion Batteries118Rejuvenating propylene carbonate-based electrolytes by regulating the coordinated structure toward all-climate potassium-ion batteries113A Critical Review on Room‐Temperature Sodium‐Sulfur Batteries: From Research Advances to Practical Perspectives137Graphic, Quantitation, Visualization, Standardization, Digitization, and Intelligence of Electrolyte and Electrolyte‐Electrode Interface102Designing Advanced Electrolytes for High-Safety and Long-Lifetime Sodium-Ion Batteries via Anion–Cation Interaction Modulation152Molecular-docking electrolytes enable high-voltage lithium battery chemistries210Supercapacitors: Overcoming current limitations and charting the course for next-generation energy storage310Electrolyte additives for Li-ion batteries: classification by elements127High-entropy electrolyte toward battery working under extreme conditions116Supercapacitors for energy storage applications: Materials, devices and future directions: A comprehensive review179Anode-free sodium metal batteries: optimisation of electrolytes and interphases109Polysulfide chemistry in metal–sulfur batteries113Reviving ether-based electrolytes for sodium-ion batteries103Dissolution, solvation and diffusion in low-temperature zinc electrolyte design196From Present Innovations to Future Potential: The Promising Journey of Lithium-Ion Batteries108Two-Stage Solvation of Lithium Polysulfides in Working Lithium–Sulfur Batteries121

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