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RESEARCH PAPER · Inorganic Chemistry · 2020

Nearly Identical but Not Isotypic: Influence of Lanthanide Contraction on Cs2NaLn(PS4)2 (Ln = La–Nd, Sm, and Gd–Ho)

Vladislav V. Klepov, Kristen A. Pace, Logan S. Breton, Vancho Kocevski, Theodore M. Besmann, Hans‐Conrad zur Loye

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Nearly Identical but Not Isotypic: Influence of Lanthanide Contraction on Cs2NaLn(PS4)2 (Ln = La–Nd, Sm, and Gd–Ho)OriginalScaling the existence state of hydrogen in metal binary oxides9Dimensional reduction upon calcium incorporation in Cs 0.3 (Ca 0.3 Ln 0.7 )PS 4 and Cs 0.5 (Ca 0.5 Ln 0.5 )PS 45A series of Rb 4 Ln 2 (P 2 S 6 )(PS 4 ) 2 (Ln = La, Ce, Pr, Nd, Sm, Gd) rare earth thiophosphates with two distinct thiophosphate units [P V S 4 ] 3− and [P IV 2 S 6 ] 4−16Trends in rare earth thiophosphate syntheses: Rb 3 Ln(PS 4 ) 2 (Ln = La, Ce, Pr), Rb 3−x Na x Ln(PS 4 ) 2 (Ln = Ce, Pr; x = 0.50, 0.55), and RbEuPS 4 obtained by molten flux crystal growth5Hydrothermal Synthesis of New Iodates Ln2(IO3)3(IO4) (Ln = La, Nd, Pr) Containing the Tetraoxoiodate(V) Anion: Creation of Luminescence Properties by Doping with Eu, Dy, and Tb5Li3La[PS4]2: The First Lithium Lanthanum Ortho‐Thiophosphate12Synthesis of Hydrated Ternary Lanthanide-Containing Chlorides Exhibiting X-ray Scintillation and Luminescence7Synthesis, crystal structure, optical bandgap, and electronic structure of Cs2FeP2S62Transuranium Sulfide via the Boron Chalcogen Mixture Method and Reversible Water Uptake in the NaCuTS3 Family21A review of structures and physical properties of rare earth chalcophosphates78KREP2Se6 (RE = Sm, Gd, Tb): The First Rare‐Earth Selenophosphates with Remarkable Nonlinear Optical Activities Realized by Synergistic Effect of RE‐ and P‐Based Motifs39Li4Ln[PS4]2Cl: Chloride-Containing Lithium Thiophosphates with Lanthanoid Participation (Ln = Pr, Nd and Sm)1NaREP 2 Se 6 (RE = Y, Sm, Gd–Dy): Quaternary Rare-Earth Selenophosphates with Unique 3D {[REP 2 Se 6 ] − } ∞ Framework Built by RESe 8 and P 2 Se 6 Motifs and Multiple Properties4RbEr2AsS7: A Rubidium-Containing Erbium Sulfide Thioarsenate(III) with (S2)2− Ligands According to RbEr2S(S2)[AsS2(S2)]3KREP 2 S 6 (RE = Sm, Gd, Tb, Dy): A Series of Polar Rare-Earth Thiophosphates with High Laser-Induced Damage Thresholds and Moderate Nonlinear-Optical Responses Synergistically Contributed by Isolated P 2 S 6 Units and {[RE 2 S 15 ] 24– } ∞ Layers8B@LGTs of Nd, Eu, Er, and Yb lanthanides with physicochemical interfacing for enhanced photocatalytic reduction of fluorescent dyes, transition metal ions, and quinonoid phenolphthalein1Synthesis of Mixed Anion Rare Earth Sulfate Fluorides LnSO4F·H2O (Ln = Nd, Tb, Dy, and Ho) and LnSO4F (Ln = Tb, Dy, and Ho)5Introduction of Diverse Divalent Main-Group Metal Cations to Tune the Physical Properties of Rare-Earth Thiophosphates7Centrosymmetric to noncentrosymmetric structure transition of the RbREP 2 Se 6 (RE = La–Nd, Sm, Ho–Yb) series: crystal growth, magnetic and optical properties4Rb2Dy[S2][AsS4]: Synthesis and characterization of a novel lanthanoid thioarsenate(V) containing outer-sphere disulfide dumbbells1A Surprising Continuation of the Nonisotypic Rb 3 Ln [AsS 4 ] 2 Series: The Diverse Crystal Structures of the End‐Members with Ln = Gd–Ho0Lanthanide Contraction Associated Coordination Regimes and Photocatalytic Performance of Polyoxometalate-Based Lanthanide Phosphonates0

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  1. Scaling the existence state of hydrogen in metal binary oxides

    Acta Materialia · 2020-11-06

    Bingyun Ao

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  2. Dimensional reduction upon calcium incorporation in Cs 0.3 (Ca 0.3 Ln 0.7 )PS 4 and Cs 0.5 (Ca 0.5 Ln 0.5 )PS 4

    CrystEngComm · 2020-12-09

    Vladislav V. Klepov, Vancho Kocevski, Theodore M. Besmann, Hans‐Conrad zur Loye

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  3. A series of Rb 4 Ln 2 (P 2 S 6 )(PS 4 ) 2 (Ln = La, Ce, Pr, Nd, Sm, Gd) rare earth thiophosphates with two distinct thiophosphate units [P V S 4 ] 3− and [P IV 2 S 6 ] 4−

    Dalton Transactions · 2021-01-01

    Ceren Kütahyalı Aslani, Logan S. Breton, Vladislav V. Klepov, Hans‐Conrad zur Loye

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  4. Trends in rare earth thiophosphate syntheses: Rb 3 Ln(PS 4 ) 2 (Ln = La, Ce, Pr), Rb 3−x Na x Ln(PS 4 ) 2 (Ln = Ce, Pr; x = 0.50, 0.55), and RbEuPS 4 obtained by molten flux crystal growth

    CrystEngComm · 2021-01-01

    Logan S. Breton, Mark D. Smith, Hans‐Conrad zur Loye

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  5. Hydrothermal Synthesis of New Iodates Ln2(IO3)3(IO4) (Ln = La, Nd, Pr) Containing the Tetraoxoiodate(V) Anion: Creation of Luminescence Properties by Doping with Eu, Dy, and Tb

    Crystal Growth & Design · 2021-07-15

    Ceren Kütahyalı Aslani, Vladislav V. Klepov, Mahmoud A. A. Aslani, Hans‐Conrad zur Loye

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  6. Li3La[PS4]2: The First Lithium Lanthanum Ortho‐Thiophosphate

    European Journal of Inorganic Chemistry · 2021-08-03

    Pia L. Lange, Thomas Schleid

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  7. Synthesis of Hydrated Ternary Lanthanide-Containing Chlorides Exhibiting X-ray Scintillation and Luminescence

    Inorganic Chemistry · 2021-10-07

    Gyanendra B. Ayer, Mark D. Smith, Luiz Gustavo Jacobsohn, Gregory W. Morrison, Hunter B. Tisdale, Logan S. Breton, Weiguo Zhang, P. Shiv Halasyamani, Hans‐Conrad zur Loye

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  8. Synthesis, crystal structure, optical bandgap, and electronic structure of Cs2FeP2S6

    Solid State Sciences · 2022-04-14

    Subhendu Jana, Gopabandhu Panigrahi, Sweta Yadav, Manish K. Niranjan, Jai Prakash

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  9. Transuranium Sulfide via the Boron Chalcogen Mixture Method and Reversible Water Uptake in the NaCuTS3 Family

    Journal of the American Chemical Society · 2022-07-21

    Anna A. Berseneva, Vladislav V. Klepov, Koushik Pal, Kelly Seeley, Daniel Koury, Joseph C. Schaeperkoetter, Joshua Wright, Scott T. Misture, Mercouri G. Kanatzidis, Chris M. Wolverton, Artem V. Gelis, Hans‐Conrad zur Loye

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  10. A review of structures and physical properties of rare earth chalcophosphates

    Coordination Chemistry Reviews · 2022-10-11

    Zi‐Xia Chen, Wenlong Liu, Sheng‐Ping Guo

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  11. KREP2Se6 (RE = Sm, Gd, Tb): The First Rare‐Earth Selenophosphates with Remarkable Nonlinear Optical Activities Realized by Synergistic Effect of RE‐ and P‐Based Motifs

    Small · 2022-12-11

    Zi‐Xia Chen, Chen‐Yi Zhao, Xiaohui Li, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  12. Li4Ln[PS4]2Cl: Chloride-Containing Lithium Thiophosphates with Lanthanoid Participation (Ln = Pr, Nd and Sm)

    Crystals · 2023-09-22

    Pia L. Lange, Sebastian Bette, Sabine Strobel, Robert E. Dinnebier, Thomas Schleid

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  13. NaREP 2 Se 6 (RE = Y, Sm, Gd–Dy): Quaternary Rare-Earth Selenophosphates with Unique 3D {[REP 2 Se 6 ] − } ∞ Framework Built by RESe 8 and P 2 Se 6 Motifs and Multiple Properties

    Inorganic Chemistry · 2023-11-30

    Chen‐Yi Zhao, Zi‐Xia Chen, Wen‐Dong Yao, Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

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  14. RbEr2AsS7: A Rubidium-Containing Erbium Sulfide Thioarsenate(III) with (S2)2− Ligands According to RbEr2S(S2)[AsS2(S2)]

    Inorganics · 2023-12-01

    Katja Engel, Thomas Schleid

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  15. KREP 2 S 6 (RE = Sm, Gd, Tb, Dy): A Series of Polar Rare-Earth Thiophosphates with High Laser-Induced Damage Thresholds and Moderate Nonlinear-Optical Responses Synergistically Contributed by Isolated P 2 S 6 Units and {[RE 2 S 15 ] 24– } ∞ Layers

    Inorganic Chemistry · 2024-02-17

    Chen‐Yi Zhao, Wen‐Dong Yao, Mingyang Li, Wenfeng Zhou, Wenlong Liu, Sheng‐Ping Guo

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  16. B@LGTs of Nd, Eu, Er, and Yb lanthanides with physicochemical interfacing for enhanced photocatalytic reduction of fluorescent dyes, transition metal ions, and quinonoid phenolphthalein

    RSC Advances · 2025-01-01

    Krishan Kumar, Man Singh

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  17. Synthesis of Mixed Anion Rare Earth Sulfate Fluorides LnSO4F·H2O (Ln = Nd, Tb, Dy, and Ho) and LnSO4F (Ln = Tb, Dy, and Ho)

    Crystal Growth & Design · 2025-03-27

    Lakshani W. Masachchi, Gregory W. Morrison, Hans‐Conrad zur Loye

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  18. Introduction of Diverse Divalent Main-Group Metal Cations to Tune the Physical Properties of Rare-Earth Thiophosphates

    Inorganic Chemistry · 2025-07-18

    Zi-Nan Chen, Hai-Ping Xu, Wen‐Dong Yao, Mingyang Li, Chen‐Yi Zhao, Wenlong Liu, Sheng‐Ping Guo

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  19. Centrosymmetric to noncentrosymmetric structure transition of the RbREP 2 Se 6 (RE = La–Nd, Sm, Ho–Yb) series: crystal growth, magnetic and optical properties

    Dalton Transactions · 2026-01-01

    Habiba Binte Kashem, Abdullah Al Muhit, Hope Eden Smith, Eric A. Gabilondo, P. Shiv Halasyamani, Hans‐Conrad zur Loye

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  20. Rb2Dy[S2][AsS4]: Synthesis and characterization of a novel lanthanoid thioarsenate(V) containing outer-sphere disulfide dumbbells

    Solid State Sciences · 2026-01-18

    Katja Engel, Thomas Schleid

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  21. A Surprising Continuation of the Nonisotypic Rb 3 Ln [AsS 4 ] 2 Series: The Diverse Crystal Structures of the End‐Members with Ln = Gd–Ho

    Zeitschrift für anorganische und allgemeine Chemie · 2026-07-15

    Katja Engel, Thomas Schleid

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  22. Lanthanide Contraction Associated Coordination Regimes and Photocatalytic Performance of Polyoxometalate-Based Lanthanide Phosphonates

    Inorganic Chemistry · 2026-10-01

    Linlin Wang, Hong-Li Jia, Jianjie Xu, Qi–Ming Qiu, Chuan-Bing Hou, Wei Li, Hongliang Han, Heng‐Yun Ye, Rui-Lin Yang, Qiong‐Hua Jin

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