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RESEARCH PAPER · EcoMat · 2019

Internal electric field engineering for steering photogenerated charge separation and enhancing photoactivity

Yan Xia Guo, Wenxin Shi, Yongfa Zhu

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Internal electric field engineering for steering photogenerated charge separation and enhancing photoactivityOriginalFerroelectric polarization and thin-layered structure synergistically promoting CO 2 photoreduction of Bi 2 MoO 6164In situ construction of hydrazone-linked COF-based core–shell hetero-frameworks for enhanced photocatalytic hydrogen evolution159Boosting visible-light-driven hydrogen evolution from formic acid over AgPd/2D g-C3N4 nanosheets Mott-Schottky photocatalyst265Photocatalytic degradation of tetracycline antibiotics using three-dimensional network structure perylene diimide supramolecular organic photocatalyst under visible-light irradiation513Efficient and stable photocatalytic degradation of tetracycline wastewater by 3D Polyaniline/Perylene diimide organic heterojunction under visible light irradiation205Construction of ultrathin 2D/2D g-C3N4/In2Se3 heterojunctions with high-speed charge transfer nanochannels for promoting photocatalytic hydrogen production52Photocatalytic activity enhanced via surface hybridization125Perovskite Microcrystals with Intercalated Monolayer MoS2 Nanosheets as Advanced Photocatalyst for Solar-Powered Hydrogen Generation141Constructing Internal Electric Field in g-C3N4 Significantly Promotes the Photocatalytic Performance for H2O2 Generation27Durable Multimetal Oxychloride Intergrowths for Visible Light-Driven Water Splitting30A fluorine induced enhancement of the surface polarization and crystallization of g-C 3 N 4 for an efficient charge separation18An effective non-equivalent ion exchange method for building an advanced Z-scheme WO 3 /Bi 2 WO 6 photocatalyst7Core–Shell Materials for Photocatalytic CO2 Reduction0High carrier separation efficiency for a defective g-C 3 N 4 with polarization effect and defect engineering: mechanism, properties and prospects41Mechanism of surface and interface engineering under diverse dimensional combinations: the construction of efficient nanostructured MXene-based photocatalysts23Bi 3 O 4 Br nanoplates as an efficient piezo-photocatalyst for organic dye degradation11Effect of ferroelectric Ba0.8Sr0.2TiO3 on the charge carrier separation of BiOBr at different temperature21Tuning the strength of built-in electric field in 2D/2D g-C3N4/SnS2 and g-C3N4/ZrS2 S-scheme heterojunctions by nonmetal doping163Conjugated π Electrons of MOFs Drive Charge Separation at Heterostructures Interface for Enhanced Photoelectrochemical Water Oxidation57Recent Advances in Noncontact External-Field-Assisted Photocatalysis: From Fundamentals to Applications357Spatial separation of photo-induced charge carriers in a Na3VO2B6O11 polar material and its enhanced photocatalytic activity11Minimized external electric field on asymmetric monolayer maximizes charge separation for photocatalysis26Bismuth-based photocatalyst for photocatalytic oxidation of flue gas mercury removal: A review146In2O3/oxygen doped g-C3N4 towards photocatalytic BPA degradation: Balance of oxygen between metal oxides and doped g-C3N444Construction of dual-Z-scheme WS2-WO3·H2O/g-C3N4 catalyst for photocatalytic H2 evolution under visible light69Atomic interfacial structure and charge transfer mechanism on in-situ formed BiOI/Bi2O2SO4 p–n heterojunctions with highly promoted photocatalysis121Interfacial chemical bond and internal electric field modulated Z-scheme Sv-ZnIn2S4/MoSe2 photocatalyst for efficient hydrogen evolution1099A Full‐Spectrum Porphyrin–Fullerene D–A Supramolecular Photocatalyst with Giant Built‐In Electric Field for Efficient Hydrogen Production293Accurate guided alternating atomic layer enhance internal electric field to steering photogenerated charge separation for enhance photocatalytic activity53Schottky Barrier‐Induced Surface Electric Field Boosts Universal Reduction of NOx− in Water to Ammonia134Schottky Barrier‐Induced Surface Electric Field Boosts Universal Reduction of NOx− in Water to Ammonia14Durable Metal Heteroanionic Photocatalysts24Anion-exchange-mediated internal electric field for boosting photogenerated carrier separation and utilization136Piezo‐Photocatalysis over Metal–Organic Frameworks: Promoting Photocatalytic Activity by Piezoelectric Effect418BaTi4O9 Photocatalysts with Variously Loaded Ag Cocatalyst for Highly Selective Photocatalytic CO2 Reduction with Water11Internal Electric Field on Steering Charge Migration: Modulations, Determinations and Energy‐Related Applications274CuBi2O4 photocathode with integrated electric field for enhanced H2O2 production67Perovskite oxide for emerging photo(electro)catalysis in energy and environment99Photocatalytic degradation of xanthate in flotation plant tailings by TiO2/graphene nanocomposites218Local Spatial Polarization Induced Efficient Charge Separation of Squaraine‐Linked COF for Enhanced Photocatalytic Performance1732D/2D SnS2@Ti3C2 MXene heterojunction photocatalyst with a superior efficiency for tetracycline hydrochloride elimination14A lateral built-in field of the 2D/2D SnS 2 /SnSe 2 in-plane heterostructure with boosted interfacial charge transfer47Enhancing internal electric field by Zn 2+ doping for promoting bulk-charge separation and improving visible photocatalytic activity of Bi 2 YO 4 Cl12Enhancing the separation efficiency of photo-induced carriers in a Bi 2 S 3 /BiOCl heterostructure by cooperative influence of oxygen vacancies and the interfacial electric field18Highly Crystalline Linear Poly-Imine Photocatalyst with Giant Internal Electric Field for Visible-Light-Driven Water Disinfection0Multi-stepwise charge transfer via MOF@MOF/TiO 2 dual-heterojunction photocatalysts towards hydrogen evolution74Probing interfacial charge transfer in heterojunctions for photocatalysis28Recent advances in high-crystalline conjugated organic polymeric materials for photocatalytic CO 2 conversion31The asymmetrical-structure of supramolecular precursor to improve internal electric field for simultaneously enhancing contaminant degradation and H2O2 production performance32Enhanced photocatalytic O2 activation by the synergy of efficient oxygen adsorption and interfacial charge separation: A case of Bi3O4Br/rGO van der Waals heterojunction33Modulating Built‐In Electric Field via Variable Oxygen Affinity for Robust Hydrogen Evolution Reaction in Neutral Media59Modulating Built‐In Electric Field via Variable Oxygen Affinity for Robust Hydrogen Evolution Reaction in Neutral Media343Enhanced localized dipole of Pt-Au single-site catalyst for solar water splitting55In-situ-formed red phosphorus nanosheet on bulk red phosphorus for boosting charge separation in photocatalysis：The role of multiple interfacial effects29Efficient degradation of organic pollutants by enhanced interfacial internal electric field induced via various crystallinity carbon nitride homojunction93Perylenetetracarboxylic acid nanosheets with internal electric fields and anisotropic charge migration for photocatalytic hydrogen evolution284Unveiling the charge transfer dynamics steered by built-in electric fields in BiOBr photocatalysts336Catalytic radiosensitization: Insights from materials physicochemistry50Carbon nitride photocatalyst with internal electric field induced photogenerated carriers spatial enrichment for enhanced photocatalytic water splitting77Construction of internal electric field in imprinted poly (ionic liquid)-TiO2 composite nanoreactor for improving hole directional enrichment and selective photodegradation26Lewis acid Fe3+ in TiO2 ultra-thin nanosheet boosts oxygen species activation13TiO2/CsPbBr3 S-scheme heterojunctions with highly improved CO2 photoreduction activity through facet-induced Fermi level modulation61Regulating crystallinity in linear conjugated polymer to boost the internal electric field for remarkable visible-light-driven disinfection9Built-in electric field enabled in carbon-doped Bi3O4Br nanocrystals for excellent photodegradation of PAHs27Continuous Charge Transport in Carbon Nitride Modulated by Interfacial Chemical Bond and Homophase Junction to Boost Photocatalytic Hydrogen Production1Heterojunction structure for suppressing dark current toward high-performance ZnO microrod metal-semiconductor-metal ultraviolet photodetectors8Coupled internal electric field with hydrogen release kinetics for promoted photocatalytic hydrogen production through employing carbon coated transition metal as co-catalyst75Combined internal and external electric fields to promote photocarriers separation of TiO2 homogenous S-scheme composite for CIP photodegradation2Visible-light-driven g-C3N4 doped CuFe2O4 floating catalyst enhanced peroxymonosulfate activation for sulfamethazine removal via singlet oxygen and high-valent metal-oxo species69Photocatalytic and Photocurrent Responses to Visible Light of the Lone-Pair-Based Oxysulfide Sr6Cd2Sb6S10O728Bi-MOFs with two different morphologies promoting degradation of organic dye under simultaneous photo-irradiation and ultrasound vibration treatment107Boosting non-sacrificial H 2 O 2 production on a Bi 6 S 2 O 15 photocatalyst via creating a crystal surface-dependent internal electric field11Designing a Built-In Electric Field for Efficient Energy Electrocatalysis437Alkali Metal Cations as Charge‐Transfer Bridge for Polarization Promoted Solar‐to‐H2 Conversion42Advances in organic semiconductors for photocatalytic hydrogen evolution reaction92Building internal electric fields in porous ionic polymers for fast photocatalytic degradation of tetracycline hydrochloride6Exploration of the origin of the excellent charge-carrier dynamics in Ruddlesden–Popper oxysulfide perovskite Y 2 Ti 2 O 5 S 28Flake-Like Janus Tio2@Conjugated Polymer Photocatalysts with Enhanced Charge Carrier Separation Effect0Interfacial built-in electric-field for boosting energy conversion electrocatalysis125Metal-free photocatalysts for solar-driven water disinfection: recent progress and challenges7Photocatalytic Water Splitting and Co2 Reduction with Internal Electric Field Modulation1The effect of permanent electric dipoles on the stability and photoelectric properties of MAPbI 3 films4The mechanism insight for improved photocatalysis and interfacial charges transfer of surface-dispersed Ag0 modified layered graphite-phase carbon nitride nanosheets12Bi2S3‐Cu3BiS3 Mixed Phase Interlayer for High‐Performance Cu3BiS3‐Photocathode for 2.33% Unassisted Solar Water Splitting Efficiency39Local Electric Field Induced by Atomic‐Level Donor–Acceptor Couple of O Vacancies and Mn Atoms Enables Efficient Hybrid Capacitive Deionization71Internal electric field in carbon nitride-based heterojunctions for photocatalysis234Construction of charge transfer chain in Bi12TiO20-Bi4Ti3O12/α-Bi2O3 composites to accelerate photogenerated charge separation17Electron self-sufficient core-shell BiOCl@Fe-BiOCl nanosheets boosting Fe(III)/Fe(II) recycling and synergetic photocatalysis-Fenton for enhanced degradation of phenol125Room-temperature methane sensors based on ZnO with different exposed facets: A combined experimental and first-principle study14Efficient photosynthesis of H2O2 via two-electron oxygen reduction reaction by defective g-C3N4 with terminal cyano groups and nitrogen vacancies138T-mode adsorption and photoelectrocatalysis degradation for acyclovir on CuMn2O4@WO3/g-C3N4 electrode41Enhancing photocatalytic antibiotics mineralization and water oxidation via constructing interfacial electric field in plate-on-plate BiOCl/WO3 photocatalysts25Nanoclay‐Modulated Interfacial Chemical Bond and Internal Electric Field at the Co3O4/TiO2 p‐n Junction for Efficient Charge Separation22Accelerating the Gas–Solid Interactions for Conductometric Gas Sensors: Impacting Factors and Improvement Strategies23Bismuth‐Based Oxide Photocatalysts for Selective Oxidation Transformations of Organic Compounds43Internal Electric Field Induced by Superexchange Interaction on Mn4+‐O2−‐Ni2+ Unit Enables Highly Efficient Hybrid Capacitive Deionization17Pickering emulsion-based TiO2@PPy janus microspheres for efficient photocatalytic degradation of 5-methylbenzotriazole92D/2D SnS2/SnSe2 van der Waals heterostructure for highly sensitive room-temperature NO2 sensor: Key role of interface contact50Enhanced photocatalytic performance of Bi4O5Br2 with three-dimensionally ordered macroporous structure for phenol removal27Ultrathin ZnIn2S4/ZnSe heteronanosheets with modulated S-scheme enable high efficiency of visible-light-responsive photocatalytic hydrogen evolution109Study of the Electronic Interaction between NiO and Short Polythiophene Chains towards Solar Photon Harvesting0Unveiling the selective cleavage-bond mechanism during the photocatalytic degradation process with pH-mediated BiVO4/BiPO4 dipole controlled and changed glyphosate electron cloud distribution19Optical and Electrical Modulation Strategies of Photoelectrodes for Photoelectrochemical Water Splitting13Construction of an enhanced built-in electric field in S-doped g-C3N4/NiCo2O4 for boosting peroxymonosulfate activation48Theoretical DFT Investigation of Structure and Electronic Properties of η5-Cyclopentadienyl Half-Sandwich Organochalcogenide Complexes2Intramolecular built-in electric field enhanced polymerized nitrogen-carbon homojunction π*-electron delocalization enrichment promotes photocatalytic uranium (VI) reduction60Effect of external electric fields in the charge transfer rates of donor–acceptor dyads: A straightforward computational evaluation3High performance visible light response 0D/2D MoS2QDs/BiOCl photocatalyst with synergetic effects of up-conversion and direct Z-scheme heterojunction13Fabrication, structure, and application of sulfur-and sulfide-modified bismuth based photocatalysts: A review44Tuning of internal electric field and diffusion distance boosting the charge separation for photocatalytic electricity generation14A review on ZnO-based S-scheme heterojunction photocatalysts188Internal electric field enhanced photocatalytic transfer hydrogenation in heterojunction: modulations and applications12Optimization of photocatalytic degradation performance of organic dye using highly efficient bismuth MOFs: Preparation and parametric analysis15Effects of pH and ascorbic acid on the synthesis of Bi-modified bismuth oxyiodide composite catalysts5Dipole field in nitrogen-enriched carbon nitride with external forces to boost the artificial photosynthesis of hydrogen peroxide263Unveiling the dual charge modulation of built-in electric field in metal-free photocatalysts for efficient photo-Fenton-like reaction60Successive Gradient Internal Electric Field Strategy Toward Dendrite‐Free Zinc Metal Anode70Progress in wastewater treatment via organic supramolecular photocatalysts under sunlight irradiation20Towards the design of oxychalcogenide materials as candidates for solar water- splitting photocatalysis0Atomically dispersed Au confined by oxygen vacancies in Au-θ-Al2O3/Au/PCN hybrid for boosting photocatalytic CO2 reduction driven by multiple built-in electric fields33Intercalation- and Vacancy-Enhanced Internal Electric Fields in ZnIn2S4 for Highly Efficient Photocatalytic H2O2 Production26Low Carrier Effective Masses in Photoactive Sr2Sb2O2Q3 (Q = S, Se): The Role of the Lone Pair17Interface charge separation in Cu2CoSnS4/ZnIn2S4 heterojunction for boosting photocatalytic hydrogen production32Facial Construction of Hydroxyl Functional Modified Ultrafine BiPO4 with Variation of Dipole Moment Induced by –OH Group16Constructing Z-scheme WO 3 /C 3 N 4 heterojunctions with an enlarged internal electric field and accelerated water oxidation kinetics for robust CO 2 photoreduction22First-principles guidelines to select promising van der Waals materials for hybrid photovoltaic–triboelectric nanogenerators2Enhancing Photocatalyst Efficiency by Constructing a Flake-like Janus Structure for Efficient Degradation of Benzotriazole5Establishing Multiple‐Order Built‐In Electric Fields Within Heterojunctions to Achieve Photocarrier Spatial Separation103Facile solvothermal synthesis of CoO/BiOI flower-like nanocomposites for degradation of RhB under visible-light irradiation2Photocatalytic H2O splitting and CO2 reduction with internal electric field modulation23Custom‐Design of Strong Electron/Proton Extractor on COFs for Efficient Photocatalytic H2O2 Production206Custom‐Design of Strong Electron/Proton Extractor on COFs for Efficient Photocatalytic H2O2 Production23Dipole Field-Driven Organic–Inorganic Heterojunction for Highly Sensitive Ultraviolet Photodetector24Integration of bulk-surface charge polarization and active site manipulation for highly efficient photocatalytic aerobic oxidation of sulfides8Efficient selective aerobic oxidation of sulfides by molecular dipole modulation in methylphosphate-substituted perylene diimide supramolecular polarization photocatalyst14Regulating the crystal phase of bismuth-based semiconductors for promoted photocatalytic performance20Modulation of the Internal Electric Field in Te-Doped Bi2MoO6 Nanosheets: Implication for the Photocatalytic Degradation of Rhodamine B and Photooxidation of Benzylamine16Dual Function of Naphthalenediimide Supramolecular Photocatalyst with Giant Internal Electric Field for Efficient Hydrogen and Oxygen Evolution18Modulating interface internal electric field for efficient charge separation in Co3O4/M-TiO2 p-n junction8Built-in Electric Field Promotes Interfacial Adsorption and Activation of CO2 for C1 Products over a Wide Potential Window101A detailed investigation of the effect of graphene/Ag nanoparticles on the ion exchange properties of PVDF membrane for photocatalytic hydrogen evolution5A Dielectric MXene‐Induced Self‐Built Electric Field in Polymer Electrolyte Triggering Fast Lithium‐Ion Transport and High‐Voltage Cycling Stability2A Dielectric MXene‐Induced Self‐Built Electric Field in Polymer Electrolyte Triggering Fast Lithium‐Ion Transport and High‐Voltage Cycling Stability32MOF-templated tubular Ni1-xCoxS2-CdS heterojunction with intensified direct Z-scheme charge transmission for highly promoted visible-light photocatalysis21Enhancing internal electric field of 3D porous chitosan-PDI polymer with donor-acceptor structure for efficient photocatalytic advanced oxidation38Photocatalytic O2 activation carried out by organic aerosol: A case study of 1, 8-naphthalic anhydride15Reinforcing 2D Single‐Crystal Bi2O2CO3 with Additional Interlayer Carbonates by CO2‐Assisted Solid‐to‐Solid Phase Transition13Boosting photocatalytic nitrogen fixation over Ni/Fe co-doped BiOBr in pure water under the synergistic effect of enhanced internal electric field and oxygen vacancies37Magnetic Field Effect on Photocatalytic Dye Degradation: A Review4Boosting bulk photocharge separation and transfer in heterojunctions for antibiotics removal: Enhanced internal electric field and interfacial electric field8

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  33. Anion-exchange-mediated internal electric field for boosting photogenerated carrier separation and utilization

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  37. CuBi2O4 photocathode with integrated electric field for enhanced H2O2 production

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