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RESEARCH PAPER · Advanced Functional Materials · 2019

Single Crystal Perovskite Solar Cells: Development and Perspectives

Xiao Ling Cheng, Shuang Yang, Bingqiang Cao, Xutang Tao, Zhaolai Chen

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Single Crystal Perovskite Solar Cells: Development and PerspectivesOriginalDefect passivation strategies in perovskites for an enhanced photovoltaic performance463Perovskite CsPbBr 3 crystals: growth and applications169Seed crystal free growth of high-quality double cation – double halide perovskite single crystals for optoelectronic applications7Single-crystal perovskite detectors: development and perspectives88Recycling of FTO/TiO2 Substrates: Route toward Simultaneously High-Performance and Cost-Efficient Carbon-Based, All-Inorganic CsPbIBr2 Solar Cells64Low-Temperature Crystallization Enables 21.9% Efficient Single-Crystal MAPbI3 Inverted Perovskite Solar Cells284Zwitterion-Stabilizing Scalable Bladed α-Phase Cs0.1FA0.9PbI3 Films for Efficient Inverted Planar Perovskite Solar Cells41(1-C5H14N2Br)2MnBr4: A Lead-Free Zero-Dimensional Organic-Metal Halide With Intense Green Photoluminescence30Polymer-Controlled Growth and Wrapping of Perovskite Single Crystals Leading to Better Device Stability and Performance35The Effect of Extended Ball-Milling upon Three-Dimensional and Two-Dimensional Perovskite Crystals Properties21Ultrathin Perovskite Monocrystals Boost the Solar Cell Performance63The surface of halide perovskites from nano to bulk395Modulating MAPbI3 perovskite solar cells by amide molecules: Crystallographic regulation and surface passivation41Progress and perspective on CsPbX3 nanocrystals for light emitting diodes and solar cells31Shape Control of Metal Halide Perovskite Single Crystals: From Bulk to Nanoscale107Halide Perovskite Single Crystals: Optoelectronic Applications and Strategical Approaches29Numerical Analysis of rGO/Silver-Nanowire- Based Single-Crystal Perovskite Solar Cell11Passivation of defects in perovskite solar cell: From a chemistry point of view160Epitaxial lift-off for controllable single-crystalline perovskites22Epitaxial Metal Halide Perovskites by Inkjet‐Printing on Various Substrates31Enhanced Performance of Perovskite Single-Crystal Photodiodes by Epitaxial Hole Blocking Layer17Wide Band Gap Organic–Inorganic Hybrid (CH3NH3)2HgCl4 as Self‐Driven Ultraviolet Photodetector and Photoconductor62D Perovskite Single Crystals with Suppressed Ion Migration for High‐Performance Planar‐Type Photodetectors103Crystallization Kinetics in 2D Perovskite Solar Cells182Highly Conductive P-Type MAPbI3 Films and Crystals via Sodium Doping30Interface engineering, the trump-card for CsPbX3 (X˭I, Br) perovskite solar cells development28Recent advances of lead-free metal halide perovskite single crystals and nanocrystals: synthesis, crystal structure, optical properties, and their diverse applications74Charge Transport Properties of Methylammonium Lead Trihalide Hybrid Perovskite Bulk Single Crystals3Preparation of Cu-doped ZnO nanoparticles via layered double hydroxide and application for dye-sensitized solar cells58Is the strain responsible to instability of inorganic perovskites and their photovoltaic devices?31Sb2Se3 film with grain size over 10 µm toward X-ray detection10Perovskite Single Crystals: Synthesis, Optoelectronic Properties, and Application161A temperature-reduced method for the rapid growth of hybrid perovskite single crystals with primary alcohols15Effect of vacancy concentration on the lattice thermal conductivity of CH 3 NH 3 PbI 3 : a molecular dynamics study11Efficient and stable perovskite solar cells based on a quasi-point-contact and rear-reflection structure with 22.5% efficiency12Exploring the film growth in perovskite solar cells41Fabrication of single phase CsPbBr 3 films via in situ metal reaction4Inducing hybrid perovskite crystal growth on substrates for efficient, ambient stable optoelectronic devices0Insights into iodoplumbate complex evolution of precursor solutions for perovskite solar cells: from aging to degradation57Passivation and process engineering approaches of halide perovskite films for high efficiency and stability perovskite solar cells327The effect of dimensionality on the charge carrier mobility of halide perovskites108Evaporated Perovskite Thick Junctions for X-Ray Detection76Recent Progress in Growth of Single-Crystal Perovskites for Photovoltaic Applications51Perovskite single crystals: Synthesis, properties, and applications92Integrating n-type semiconductor for passivating the defects of electron transport layer in two-dimensional perovskite solar cells2Metal Halide Perovskites for X-ray Imaging Scintillators and Detectors891All‐Inorganic Lead‐Free Perovskite(‐Like) Single Crystals: Synthesis, Properties, and Applications108High-κ La2O3 as an anode modifier to reduce leakage current for efficient perovskite solar cells7Removal of residual compositions by powder engineering for high efficiency formamidinium-based perovskite solar cells with operation lifetime over 2000 h61Investigation on in-situ thermal treatment of room-temperature pulsed laser deposition technique: How to improve Cu2ZnSnS4 films for photoelectric application without sulfurization3Surface passivation using n-type organic semiconductor in two-dimensional perovskite solar cells1Tetraphenylporphyrin-modified perovskite nanocrystals enable ratiometric fluorescent determination of sulfide ion in water samples13Silicon‐Based Lithium Ion Battery Systems: State‐of‐the‐Art from Half and Full Cell Viewpoint180Advances in Lead-Free Perovskite Single Crystals: Fundamentals and Applications124Efficient Defect Passivation and Charge Extraction with Hexamethylenetetramine Interface Modification for Hole‐Transporting Layers‐Free CsPbBr3 Perovskite Solar Cells19Single-crystal halide perovskites: Opportunities and challenges100Perovskite crystals redissolution strategy for affordable, reproducible, efficient and stable perovskite photovoltaics74Oriented Halide Perovskite Nanostructures and Thin Films for Optoelectronics145Pulsed‐Laser Detectors Based on Metal Halide Perovskites11Antisolvent-fumigated grain growth of active layer for efficient perovskite solar cells22Surface Passivation Using N-Type Organic Semiconductor by One-Step Method in Two-Dimensional Perovskite Solar Cells8Fabrications of Halide Perovskite Single-Crystal Slices and Their Applications in Solar Cells, Photodetectors, and LEDs17NH3+-Functionalized PAMAM Dendrimers Enhancing Power Conversion Efficiency and Stability of Perovskite Solar Cells3Self‐Assembled Perovskite Nanoislands on CH 3 NH 3 PbI 3 Cuboid Single Crystals by Energetic Surface Engineering13Photo-induced defects in MAPbBr3 single crystals14Numerical Analysis of P0.6Na0.6O2.2Pb0.2 based Large Band Gap Perovskite Solar Cell3Quasi-Zero Dimensional Halide Perovskite Derivates: Synthesis, Status, and Opportunity17Monocrystalline Methylammonium Lead Halide Perovskite Materials for Photovoltaics38Lead-Free Perovskite Single Crystals: A Brief Review11Interfacial Defect Passivation and Charge Carrier Management for Efficient Perovskite Solar Cells via a Highly Crystalline Small Molecule108Efficient and stable perovskite solar cells doped by cesium acetate9Ethylamine Iodide Additive Enables Solid‐to‐Solid Transformed Highly Oriented Perovskite for Excellent Photodetectors49Dependence of the Heterogeneity of Grain Boundaries on Adjacent Grains in Perovskites and Its Impact on Photovoltage14Engineering the Hole Extraction Interface Enables Single‐Crystal MAPbI3 Perovskite Solar Cells with Efficiency Exceeding 22% and Superior Indoor Response160First‐Principles Calculation Design for 2D Perovskite to Suppress Ion Migration for High‐Performance X‐ray Detection118A Method for the Room Temperature Synthesis of High-Quality Single Phase Cspbbr3 Perovskite Single Crystals0Altering heating area assisted space confined method for growth of large scale and high quality MAPbBr 3 single crystal thin films29Combined Purification and Crystal Growth of CsPbBr3 by Modified Zone Refining4Electrode dependence in halide perovskite memories: resistive switching behaviours25Spray deposited polycrystalline MAPbBr 3 thick films for hole-transport-material free solar cells3Thermal degradation of lead halide perovskite surfaces28Transport tuning strategies in MOF film synthesis – a perspective16Development and Prospects of Halide Perovskite Single Crystal Films19Inch-Sized Thin Metal Halide Perovskite Single-Crystal Wafers for Sensitive X-Ray Detection23Recent Development of Optoelectronic Application Based on Metal Halide Perovskite Nanocrystals23Thin MAPb0.5Sn0.5I3 Perovskite Single Crystals for Sensitive Infrared Light Detection7A Universal Cosolvent Evaporation Strategy Enables Direct Printing of Perovskite Single Crystals for Optoelectronic Device Applications42Plasmonic–perovskite solar cells, light emitters, and sensors161Comprehensive Device Modeling and Performance Analysis of Quantum Dot-Perovskite Solar Cells9Growing MASnI3 perovskite single-crystal films by inverse temperature crystallization13Experimental and Theoretical Core Level and Valence Band Analysis of Clean Perovskite Single Crystal Surfaces14Sintesis Kristal Tunggal Perovskite MAPbBr3 Menggunakan Metode Inverse Temperature Crystallization untuk Aplikasi Fotodetektor Sinar-X0Cooperative effects of Dopant-Free Hole-Transporting materials and polycarbonate film for sustainable perovskite solar cells18UV and Visible Photodetectors of MAPbBr3 and MAPbCl3 Perovskite Single Crystals via Single Photocarrier Transport Design32Ag+/Bi3+ doping induced band structure and optoelectronic properties changes in CsPbBr3 crystals16Unveiling the Critical Role of Oxidants and Additives in Doped Spiro-OMeTAD toward Stable and Efficient Perovskite Solar Cells50Autonomous Reconstitution of Fractured Hybrid Perovskite Single Crystals42Highly efficient CsPbI3/Cs1-xDMAxPbI3 bulk heterojunction perovskite solar cell129In Situ Growth Mechanism for High‐Quality Hybrid Perovskite Single‐Crystal Thin Films with High Area to Thickness Ratio: Looking for the Sweet Spot42Engineering Surface Orientations for Efficient and Stable Hybrid Perovskite Single-Crystal Solar Cells67Halide Perovskite Crystallization Processes and Methods in Nanocrystals, Single Crystals, and Thin Films163Investigation on the Facet-Dependent Anisotropy in Halide Perovskite Single Crystals12Toward Efficient Perovskite Solar Cells: Progress, Strategies, and Perspectives169Bulk Defect Suppression of Micrometer-Thick Perovskite Single Crystals Enables Stable Photovoltaics40Raman spectroscopy in layered hybrid organic-inorganic metal halide perovskites38One-pot synthesis of multifunctional silicone elastomer: Ring-opening copolymerization of D4 and Dual-D4Vi9In Situ Green Preparation of Highly Stable CsPbBr3–Polyimide Films for Flexible Liquid Crystal Displays14Room-temperature cost-effective in-situ grown MAPbBr3 crystals and their characterization towards optoelectronic devices4Strain effects on electronic, optical properties and carriers mobility of Cs2SnI6 vacancy‐ordered double perovskite: A promising photovoltaic material17Probing the Surface and Bulk Electrical Response of MAPbBr3 Single Crystals6Surface-Passivated Single-Crystal Micro-Plates for Efficient Perovskite Solar Cells9Heterojunction engineering for improving perovskite solar cell performance3Low-cost planar organic small molecules as hole transport materials for high efficient perovskite solar cells13Single-Crystal Hybrid Lead Halide Perovskites: Growth, Properties, and Device Integration for Solar Cell Application19Chiral Rashba Ferroelectrics for Circularly Polarized Light Detection174Ultrafast Response of Centimeter Scale Thin CsPbBr 3 Single Crystal Film Photodetector for Optical Communication69Charge Carrier Recombination Dynamics in MAPb(Br1−yIy)3 Single Crystals7High performance perovskite solar cells synthesized by dissolving FAPbI3 single crystal2Anisotropy in Perovskite Single Crystals: From Fundamentals to Applications30Recent progress of crystal orientation engineering in halide perovskite photovoltaics74Progress of Metal Halide Perovskite Crystals From a Crystal Growth Point of View13Growth of single-crystalline MAPbI3 perovskite film by a modified space-confined inverse temperature crystallization method6Growth and Characterization of High-Quality Orthorhombic Phase CsPbBr3 Perovskite Single Crystals for Optoelectronic Applications25Spraying Perovskite Intermediate Enabling Inch‐Scale Microwire Film Fabrication for Integration Compatible Efficient‐Photodetectors Array12Recent progress in perovskite solar cells: material science169Mode-locking pulse generation based on lead-free halide perovskite CsCu 2 I 3 micro-rods with high stability294-Iodo-1 H -imidazole dramatically improves the open-circuit voltages of perovskite solar cells to 1.2 V4Challenges in the development of metal-halide perovskite single crystal solar cells18Synthetic approaches for perovskite thin films and single-crystals36Charge Carrier Recombination Dynamics in MAPb(BrxCl1–x)3 Single Crystals8Anisotropic Growth of Centimeter‐Size CsCu2I3 Single Crystals with Ultra‐Low Trap Density for Aspect‐Ratio‐Dependent Photodetectors61Regulating Radial Morphology in Hot-Casting Two-Dimensional Ruddlesden–Popper Perovskite Film Growth for High-Efficient Photovoltaics9Lead-free double perovskite Rb+, Sb3+-codoped Cs2NaInCl6 nanocrystals with highly efficient and tunable photoluminescence18Mitigating Surface Deficiencies of Perovskite Single Crystals Enables Efficient Solar Cells with Enhanced Moisture and Reverse‐Bias Stability88Single‐Crystal Nanowire Cesium Tin Triiodide Perovskite Solar Cell23Single-crystal perovskite for highly efficient and stable light-emitting diodes1Recent Progress on Synthesis, Intrinsic Properties and Optoelectronic Applications of Perovskite Single Crystals69Growth of Hybrid Perovskite Crystals from CH3NH3PbI3–xClx Solutions Subjected to Constant Solvent Evaporation Rates2In situ growth of perovskite single-crystal thin films with low trap density27Growth of New, Optically Active, Semi-Organic Single Crystals Glycine-Copper Sulphate Doped by Silver Nanoparticles6Single crystal Perovskite-Based solar Cells: Growth, Challenges, and potential strategies34Controllable preparation of high-quality MAPbCl3 perovskite single crystal sheets9Inorganic Lead Halide Perovskite Micro-/Nanostructures: From Self-Assembly to Applications4Perovskite single-crystal thin films: preparation, surface engineering, and application42Velocity field distribution control in antisolvent flow realizing highly stable and efficient perovskite nanocrystals3High-quality MAPbI3 film prepared by drip-pressing method in the air for perovskite solar cells5A self-power photodetector based on controlled growth of single crystal MAPbBr3/WO3 heterojunction2Growth of single crystal Sb2S3 semiconductor pillars by sol-gel method9Perovskite single crystals: physical properties and optoelectronic applications39Developments of Highly Efficient Perovskite Solar Cells121

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  5. Recycling of FTO/TiO2 Substrates: Route toward Simultaneously High-Performance and Cost-Efficient Carbon-Based, All-Inorganic CsPbIBr2 Solar Cells

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  10. The Effect of Extended Ball-Milling upon Three-Dimensional and Two-Dimensional Perovskite Crystals Properties

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  34. Effect of vacancy concentration on the lattice thermal conductivity of CH 3 NH 3 PbI 3 : a molecular dynamics study

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  38. Inducing hybrid perovskite crystal growth on substrates for efficient, ambient stable optoelectronic devices

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  39. Insights into iodoplumbate complex evolution of precursor solutions for perovskite solar cells: from aging to degradation

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  43. Recent Progress in Growth of Single-Crystal Perovskites for Photovoltaic Applications

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  47. All‐Inorganic Lead‐Free Perovskite(‐Like) Single Crystals: Synthesis, Properties, and Applications

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  48. High-κ La2O3 as an anode modifier to reduce leakage current for efficient perovskite solar cells

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  49. Removal of residual compositions by powder engineering for high efficiency formamidinium-based perovskite solar cells with operation lifetime over 2000 h

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