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RESEARCH PAPER · Nature Catalysis · 2019

Control of metal-support interactions in heterogeneous catalysts to enhance activity and selectivity

Tom W. van Deelen, Carlos Hernández Mejía, Krijn P. de Jong

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Control of metal-support interactions in heterogeneous catalysts to enhance activity and selectivityOriginalHighly Active ZnO-ZrO2 Aerogels Integrated with H-ZSM-5 for Aromatics Synthesis from Carbon Dioxide361Hydrodeoxygenation of lignin-derived phenolics – a review on the active sites of supported metal catalysts276Nitrogen electroreduction performance of transition metal dimers embedded into N-doped graphene: a theoretical prediction160Strong Metal–Support Interactions between Pt Single Atoms and TiO 2585Boosting CO2 hydrogenation via size-dependent metal–support interactions in cobalt/ceria-based catalysts613Nanoconfinement-Mediated Water Treatment: From Fundamental to Application428Peroxymonosulfate activation of magnetic Co nanoparticles relative to an N-doped porous carbon under confinement: Boosting stability and performance160Tuning reactivity of Fischer–Tropsch synthesis by regulating TiOx overlayer over Ru/TiO2 nanocatalysts244Encapsulated Metal Nanoparticles for Catalysis855Metal-support interaction for heterogeneous catalysis: from nanoparticles to single atoms199Deep Understanding of Strong Metal Interface Confinement: A Journey of Pd/FeOx Catalysts151Raising the COx Methanation Activity of a Ru/γ‐Al2O3 Catalyst by Activated Modification of Metal–Support Interactions144Graphitic phosphorus coordinated single Fe atoms for hydrogenative transformations184Surface Coordination Chemistry of Atomically Dispersed Metal Catalysts596Supported Metal Clusters: Fabrication and Application in Heterogeneous Catalysis505Revealing the activity of different iron carbides for Fischer-Tropsch synthesis167Nontraditional Catalyst Supports in Surface Organometallic Chemistry141Metal@Zeolite Hybrid Materials for Catalysis293Recent progress on hybrid electrocatalysts for efficient electrochemical CO2 reduction138Interface Engineering of CoS/CoO@N-Doped Graphene Nanocomposite for High-Performance Rechargeable Zn–Air Batteries182Molecularly Engineered Strong Metal Oxide–Support Interaction Enables Highly Efficient and Stable CO2 Electroreduction150Propylene Epoxidation using Molecular Oxygen over Copper- and Silver-Based Catalysts: A Review154Catalyst design and tuning for oxidative dehydrogenation of propane – A review153Size-dependent strong metal-support interaction in TiO2 supported Au nanocatalysts347Enhancing the CO2 methanation activity of Ni/CeO2 via activation treatment-determined metal-support interaction154Nanoscale engineering of catalytic materials for sustainable technologies444Nanoporous Surface High‐Entropy Alloys as Highly Efficient Multisite Electrocatalysts for Nonacidic Hydrogen Evolution Reaction319Computational Methods in Heterogeneous Catalysis447Fully Exposed Cluster Catalyst (FECC): Toward Rich Surface Sites and Full Atom Utilization Efficiency305Nanoparticle Ex-solution for Supported Catalysts: Materials Design, Mechanism and Future Perspectives181Pd-Modified ZnO–Au Enabling Alkoxy Intermediates Formation and Dehydrogenation for Photocatalytic Conversion of Methane to Ethylene347Carbon-based catalysts for Fischer–Tropsch synthesis405Lanthanide electronic perturbation in Pt–Ln (La, Ce, Pr and Nd) alloys for enhanced methanol oxidation reaction activity159Propane dehydrogenation: catalyst development, new chemistry, and emerging technologies895Strategies to suppress hydrogen evolution for highly selective electrocatalytic nitrogen reduction: challenges and perspectives564Structural transformations of solid electrocatalysts and photocatalysts203Structure Sensitivity of Au‐TiO 2 Strong Metal–Support Interactions341Rare‐Earth Incorporated Alloy Catalysts: Synthesis, Properties, and Applications240Modulating electron density of vacancy site by single Au atom for effective CO2 photoreduction391Insights into the Interfacial Effects in Heterogeneous Metal Nanocatalysts toward Selective Hydrogenation258Pt Single Atoms Supported on N‐Doped Mesoporous Hollow Carbon Spheres with Enhanced Electrocatalytic H 2 ‐Evolution Activity585Switching of metal–oxygen hybridization for selective CO2 electrohydrogenation under mild temperature and pressure143Atomic Indium Catalysts for Switching CO2 Electroreduction Products from Formate to CO236Elucidation of Active Sites for CH 4 Catalytic Oxidation over Pd/CeO 2 Via Tailoring Metal–Support Interactions251Pt–CeO2-based composites in environmental catalysis: A review175Enhancing Thermocatalytic Activities by Upshifting the d‐Band Center of Exsolved Co‐Ni‐Fe Ternary Alloy Nanoparticles for the Dry Reforming of Methane140Strong metal–support interactions on gold nanoparticle catalysts achieved through Le Chatelier’s principle327The role of Fe-Nx single-atom catalytic sites in peroxymonosulfate activation: Formation of surface-activated complex and non-radical pathways142On-board methanol catalytic reforming for hydrogen Production-A review145Zeolite Fixed Metal Nanoparticles: New Perspective in Catalysis256Electronic metal–support interaction modulates single-atom platinum catalysis for hydrogen evolution reaction887Flexible carbon nanofiber film with diatomic Fe-Co sites for efficient oxygen reduction and evolution reactions in wearable zinc-air batteries171Interface dynamics of Pd–CeO2 single-atom catalysts during CO oxidation587Photoinduced Strong Metal–Support Interaction for Enhanced Catalysis182Engineering Platinum–Cobalt Nano‐alloys in Porous Nitrogen‐Doped Carbon Nanotubes for Highly Efficient Electrocatalytic Hydrogen Evolution268Solvent-free microwave synthesis of ultra-small Ru-Mo2C@CNT with strong metal-support interaction for industrial hydrogen evolution313One-stone, two birds: Alloying effect and surface defects induced by Pt on Cu2−xSe nanowires to boost C-C bond cleavage for electrocatalytic ethanol oxidation142Facet‐Dependent Oxidative Strong Metal‐Support Interactions of Palladium–TiO 2 Determined by In Situ Transmission Electron Microscopy154Wood Carbon Based Single-Atom Catalyst for Rechargeable Zn–Air Batteries223Single-Atom (Iron-Based) Catalysts: Synthesis and Applications373Sabatier principle of metal-support interaction for design of ultrastable metal nanocatalysts820Strong metal-support interactions induced by an ultrafast laser181Advanced Support Materials and Interactions for Atomically Dispersed Noble‐Metal Catalysts: From Support Effects to Design Strategies216Striding the threshold of an atom era of organic synthesis by single-atom catalysis145Cooperative catalysis coupling photo-/photothermal effect to drive Sabatier reaction with unprecedented conversion and selectivity228Anion-exchange membrane water electrolyzers and fuel cells574Metal–Support Interactions in Metal/Oxide Catalysts and Oxide–Metal Interactions in Oxide/Metal Inverse Catalysts538A review on ethanol steam reforming for hydrogen production over Ni/Al2O3 and Ni/CeO2 based catalyst powders137Strong Metal–Support Interaction of Ru on TiO 2 Derived from the Co-Reduction Mechanism of Ru x Ti 1– x O 2 Interphase139Interfacial compatibility critically controls Ru/TiO2 metal-support interaction modes in CO2 hydrogenation370Superiority of Dual‐Atom Catalysts in Electrocatalysis: One Step Further Than Single‐Atom Catalysts510Induced activation of the commercial Cu/ZnO/Al2O3 catalyst for the steam reforming of methanol516Strong Metal–Support Interaction Boosts Activity, Selectivity, and Stability in Electrosynthesis of H 2 O 2241Regulating the Tip Effect on Single‐Atom and Cluster Catalysts: Forming Reversible Oxygen Species with High Efficiency in Chlorine Evolution Reaction148Overturned Loading of Inert CeO 2 to Active Co 3 O 4 for Unusually Improved Catalytic Activity in Fenton‐Like Reactions189Tuning Two‐Electron Oxygen‐Reduction Pathways for H2O2 Electrosynthesis via Engineering Atomically Dispersed Single Metal Site Catalysts235Distinct Crystal‐Facet‐Dependent Behaviors for Single‐Atom Palladium‐On‐Ceria Catalysts: Enhanced Stabilization and Catalytic Properties254Advances in Oxygen Evolution Electrocatalysts for Proton Exchange Membrane Water Electrolyzers297Coordination environment of active sites and their effect on catalytic performance of heterogeneous catalysts143Reversible dehydrogenation and rehydrogenation of cyclohexane and methylcyclohexane by single-site platinum catalyst181Dilute Alloys Based on Au, Ag, or Cu for Efficient Catalysis: From Synthesis to Active Sites144Overturning CO 2 Hydrogenation Selectivity with High Activity via Reaction-Induced Strong Metal–Support Interactions402Heterogeneous Trimetallic Nanoparticles as Catalysts192Bifunctional WC‐Supported RuO 2 Nanoparticles for Robust Water Splitting in Acidic Media214Constructing Cu−C Bonds in a Graphdiyne‐Regulated Cu Single‐Atom Electrocatalyst for CO 2 Reduction to CH 4222Corrosion Chemistry of Electrocatalysts145Electrocatalytic Hydrogen Oxidation in Alkaline Media: From Mechanistic Insights to Catalyst Design152Electronically Engineering Water Resistance in Methane Combustion with an Atomically Dispersed Tungsten on PdO Catalyst165Highly Selective Photocatalytic CO2 Methanation with Water Vapor on Single‐Atom Platinum‐Decorated Defective Carbon Nitride146Tuning the Electronic and Steric Interaction at the Atomic Interface for Enhanced Oxygen Evolution208Dynamic interplay between metal nanoparticles and oxide support under redox conditions390Highly efficient CeO2-supported noble-metal catalysts: From single atoms to nanoclusters173Solid-State Reaction Synthesis of Nanoscale Materials: Strategies and Applications228Amorphous metallic ultrathin nanostructures: A latent ultra-high-density atomic-level catalyst for electrochemical energy conversion161Maximizing noble metal utilization in solid catalysts by control of nanoparticle location242Strong Metal–Support Interaction in Heterogeneous Catalysts469Carbon-based catalyst supports for oxygen reduction in proton-exchange membrane fuel cells139Adsorption Energy in Oxygen Electrocatalysis299Facet Engineering of a Metal–Organic Framework Support Modulates the Microenvironment of Palladium Nanoparticles for Selective Hydrogenation161A Review on the Different Aspects and Challenges of the Dry Reforming of Methane (DRM) Reaction178Catalysis of Alloys: Classification, Principles, and Design for a Variety of Materials and Reactions413Multi-heterointerfaces for selective and efficient urea production152Science and engineering for non-noble-metal-based electrocatalysts to boost their ORR performance: A critical review209Long‐Range Interactions in Diatomic Catalysts Boosting Electrocatalysis270Engineering Heterogeneous Catalysis with Strong Metal–Support Interactions: Characterization, Theory and Manipulation303Selective Hydrodeoxygenation of Aromatics to Cyclohexanols over Ru Single Atoms Supported on CeO 2207Design of the Synergistic Rectifying Interfaces in Mott–Schottky Catalysts376Copper/alkaline earth metal oxide interfaces for electrochemical CO2-to-alcohol conversion by selective hydrogenation261Bimetallic‐Based Electrocatalysts for Oxygen Evolution Reaction156Metal–support interactions for heterogeneous catalysis: mechanisms, characterization techniques and applications163Synergistic Mechanism of Sub‐Nanometric Ru Clusters Anchored on Tungsten Oxide Nanowires for High‐Efficient Bifunctional Hydrogen Electrocatalysis154Locking Effect in Metal@MOF with Superior Stability for Highly Chemoselective Catalysis174Active Site Engineering on Plasmonic Nanostructures for Efficient Photocatalysis186Room-temperature photosynthesis of propane from CO2 with Cu single atoms on vacancy-rich TiO2354Self‐Accommodation Induced Electronic Metal–Support Interaction on Ruthenium Site for Alkaline Hydrogen Evolution Reaction178Interface synergism and engineering of Pd/Co@N-C for direct ethanol fuel cells188Oxygen Evolution/Reduction Reaction Catalysts: From In Situ Monitoring and Reaction Mechanisms to Rational Design800Design Strategies of Stable Catalysts for Propane Dehydrogenation to Propylene185Diversity of platinum-sites at platinum/fullerene interface accelerates alkaline hydrogen evolution165Stabilizing Copper by a Reconstruction-Resistant Atomic Cu–O–Si Interface for Electrochemical CO2 Reduction240Reverse oxygen spillover triggered by CO adsorption on Sn-doped Pt/TiO2 for low-temperature CO oxidation190Recent Advances of VOCs Catalytic Oxidation over Spinel Oxides: Catalyst Design and Reaction Mechanism210Size of cerium dioxide support nanocrystals dictates reactivity of highly dispersed palladium catalysts327Recent Advances on Heterogeneous Non-noble Metal Catalysts toward Selective Hydrogenation Reactions164Fluorination of Covalent Organic Framework Reinforcing the Confinement of Pd Nanoclusters Enhances Hydrogen Peroxide Photosynthesis206Nano-metal diborides-supported anode catalyst with strongly coupled TaOx/IrO2 catalytic layer for low-iridium-loading proton exchange membrane electrolyzer280The reformation of catalyst: From a trial-and-error synthesis to rational design299Recent advances in the applications of encapsulated transition-metal nanoparticles in advanced oxidation processes for degradation of organic pollutants: A critical review264Reinforcing the Efficiency of Photothermal Catalytic CO 2 Methanation through Integration of Ru Nanoparticles with Photothermal MnCo 2 O 4 Nanosheets171Dealuminated Beta zeolite reverses Ostwald ripening for durable copper nanoparticle catalysts256Highly Stable Pt/CeO 2 Catalyst with Embedding Structure toward Water–Gas Shift Reaction237Activating lattice oxygen by a defect-engineered Fe 2 O 3 –CeO 2 nano-heterojunction for efficient electrochemical water oxidation326Efficient overall water splitting of a suspended photocatalyst boosted by metal-support interaction159Metal–support interactions in metal oxide-supported atomic, cluster, and nanoparticle catalysis414Renaissance of Strong Metal–Support Interactions381Light-Induced Variation of Lithium Coordination Environment in g-C 3 N 4 Nanosheet for Highly Efficient Oxygen Reduction Reactions258Selectivity Control by Relay Catalysis in CO and CO 2 Hydrogenation to Multicarbon Compounds142Emerging Atomically Precise Metal Nanoclusters and Ultrasmall Nanoparticles for Efficient Electrochemical Energy Catalysis: Synthesis Strategies and Surface/Interface Engineering164Selectivity control in CO2 hydrogenation to one-carbon products142From Charge to Spin: An In‐Depth Exploration of Electron Transfer in Energy Electrocatalysis180Pt-Modified High Entropy Rare Earth Oxide for Efficient Hydrogen Evolution in pH-Universal Environments177Overcoming Electrostatic Interaction via Pulsed Electroreduction for Boosting the Electrocatalytic Urea Synthesis188Synergetic catalytic effects by strong metal–support interaction for efficient electrocatalysis167Heterostructured Catalytic Materials as Advanced Electrocatalysts: Classification, Synthesis, Characterization, and Application149Upcycling waste sewage sludge into superior single-atom Fenton-like catalyst for sustainable water purification201Rationally designed Ru catalysts supported on TiN for highly efficient and stable hydrogen evolution in alkaline conditions137Nature of metal-support interaction for metal catalysts on oxide supports417Earth-abundant electrocatalysts for acidic oxygen evolution238Interfacial Catalysis at Atomic Level159Interfacial compatibility critically controls Ru/TiO2 metal-support interaction modes in CO2 hydrogenation281

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